We introduce a solution for producing ultrashort ($\sim$fs) high charge ($\sim$pC) from ultra-compact guns utilizing single-cycle THz pulses. We show that the readily available THz pulses with energies as low as 20 ?J are sufficient to generate multi-10 keV electron bunches. Moreover, It is demonstrated that THz energies of 2mJ are sufficient to generate relativistic electron bunches with higher than 2 MeV energy. The high acceleration gradients possible in the structures provide 30 fs electron bunches at 30 keV energy and 45 fs bunches at 2 MeV energy. These structures will underpin future devices for strong field THz physics in general and miniaturized electron guns, in which the high fields combined with the short pulse duration enable electron beams with ultrahigh brightness.
Femtosecond electron bunches with keV energies and eV energy spread are needed by condensed matter physicists to resolve state transitions in carbon nanotubes, molecular structures, organic salts, and charge density wave materials. These semirelativistic electron sources are not only of interest for ultrafast electron diffraction, but also for electron energy-loss spectroscopy and as a seed for x-ray FELs. Thus far, the output energy spread (hence pulse duration) of ultrafast electron guns has been limited by the achievable electric field at the surface of the emitter, which is 10 MV/m for DC …
A comparison of the two most prominent electron sources of high average current high brightness electron beams, DC and superconducting RF photoemission guns, is carried out using a large-scale multivariate genetic optimizer interfaced with space charge simulation codes. The gun geometry for each case is varied concurrently with laser pulse shape and parameters of the downstream beamline elements of the photoinjector to obtain minimum emittance as a function of bunch charge. Realistic constraints are imposed on maximum field values for the two gun types. The SRF and DC gun emittances and beam e…
Megaelectronvolt ultrafast electron diffraction (UED) is a promising detection tool for ultrafast processes. The quality of diffraction image is determined by the transverse evolution of the probe bunch. In this paper, we study the contributing terms of the emittance and space charge effects to the bunch evolution in MeV UED scheme, employing a mean-field model with an ellipsoidal distribution as well as particle tracking simulation. Small transverse dimension of the drive laser is found critical to improve the reciprocal resolution, exploiting both smaller emittance and larger transverse bunc…
We present the design of a high repetition rate MeV energy ultrafast electron diffraction instrument based on a DC photoelectron gun and an SRF linac with multiple independently controlled accelerating and bunching cavities. The design is based on the existing Cornell photoinjector, which can readily be applied to the presented findings. Using particle tracking simulations in conjunction with multiobjective genetic algorithm optimization, we explore the smallest bunch lengths, emittance, and probe spot sizes achievable. We present results for both stroboscopic conditions (with single electrons…
High-repetition-rate sources of bright electron bunches have a wide range of applications. They can directly be employed as probes in electron-scattering setups, or serve as a backbone for the generation of radiation over a broad range of the electromagnetic spectrum. This paper describes the development of a compact sub-Mega-electronvolt (sub-MeV) electron-source setup capable of operating at MHz repetition rates and forming sub-picosecond electron bunches with transverse emittance below 20~nm. The setup relies on a conduction-cooled superconducting single-cell resonator with its geometry alt…
We present the results of transverse emittance and longitudinal current profile measurements of high bunch charge (greater than or equal to 100 pC) beams produced in the DC gun-based Cornell Energy Recovery Linac Photoinjector. In particular, we show that the cathode thermal and core beam emittances dominate the final 95% and core emittance measured at 9-9.5 MeV. Additionally, we demonstrate excellent agreement between optimized 3D space charge simulations and measurement, and show that the quality of the transverse laser distribution limits the optimal simulated and measured emittances. These…
Free Electron Lasers driven by Super-Conducting Linacs require the generation, acceleration and transport of trains of bunches with high charge, high repetition rate and low emittance. A numerical model already developed for the modeling of beam dynamics in SC Linacs has been now extended to treat RF guns with proper description of the photocathode bunch generation. The model algorithm is based on a coupled integration of Newton and Maxwell equations under a slowly varying envelope approximation for the time evolution of mode amplitudes in the accelerating structure and an envelope equation de…
Self consistent analytic and numeric design for a set of electron guns with a high beams quality to be used in high power Ka-band klystrons are presented in this paper. The set of electron guns can be used in the high power Ka-band klystrons in order to feed linear accelerating structures at 36 GHz with an estimated 20 MW input power by achieving an effective accelerating electric field in the (100-150) MV/m range. In the framework of the Compact Light XLS project, a short Ka-band linearizer by working at 36 GHz able for providing an integrated voltage of at least 15 MV is proposed for bunch-p…
For the purpose of laser wakefield acceleration, it turned out that also the injection of electron bunches longer than a plasma wavelength can generate accelerated femtosecond bunches with relatively low energy spread. This is of high interest because such injecting bunches can be provided, e.g., by state-of-the-art photo cathode RF guns. Here we point out that when an e-bunch is injected in the wakefield it is important to take into account the ponderomotive scattering of the injecting bunch by the laser pulse in the vacuum region located in front of the plasma. At low energies of the injecte…
The temporal resolution of sub-relativistic ultrafast electron diffraction (UED) is generally limited by radio frequency (RF) phase and amplitude jitter of the RF lenses that are used to compress the electron pulses. We theoretically show how to circumvent this limitation by using a combination of several RF compression cavities. We show that if powered by the same RF source and with a proper choice of RF field strengths, RF phases and distances between the cavities, the combined arrival time jitter due to RF phase jitter of the cavities is cancelled at the compression point. We also show that…
Ultrashort electron beams with narrow energy spread, high charge, and low jitter are essential for resolving phase transitions in metals, semiconductors, and molecular crystals. These semirelativistic beams, produced by phototriggered electron guns, are also injected into accelerators for x-ray light sources. The achievable resolution of these time-resolved electron diffraction or x-ray experiments has been hindered by surface field and timing jitter limitations in conventional RF guns, which thus far are <200 MV/m and >96 fs, respectively. A gun driven by optically-generated single-cycle THz …
Visualizing ultrafast dynamics at the atomic scale requires time-resolved pump-probe characterization with femtosecond temporal resolution. For single-shot ultrafast electron diffraction (UED) with fully relativistic electron bunch probes, existing techniques are limited by the achievable electron probe bunch length, charge, and timing jitter. We present the first experimental demonstration of pump-probe UED with THz-driven compression and time-stamping that enable UED probes with unprecedented temporal resolution. This technique utilizes two counter-propagating quasi-single-cycle THz pulses g…
Ultrashort electron bunches are useful for applications like ultrafast imaging and coherent radiation production. Currently, however, the shortest achievable bunches, at attosecond time scales, have only been realized in the single or very few electron regime, limited by Coulomb repulsion and electron energy spread. Using ab initio simulations and theoretical analysis, we show that highly-charged bunches are achievable by subjecting relativistic (few MeV-scale) electrons to a superposition of terahertz and optical pulses. Using realistic electron bunches and laser pulse parameters which are wi…
In this paper, we use an envelope equation-based approach to obtain analytical scaling laws for the shortest pulse length achievable using radiofrequency (RF) based bunch compression. The derived formulas elucidate the dependencies on the electron beam energy and beam charge and reveal how to obtain bunches containing 1 million electrons with single-digit fs pulse lengths; relativistic energies are strongly desirable. The effect of the non-linearities associated with the RF curvature and the beam propagation in a drift is shown to strongly limit the attainability of extreme compression ratios.…
We present the first demonstration of THz-driven bunch compression and timing stabilization of a few-fC relativistic electron beam with kinetic energy of 2.5 MeV using quasi-single-cycle strong field THz radiation in a shorted parallel-plate structure. Compression by nearly a factor of 3 produced a 39 fs rms bunch length and a reduction in timing jitter by more than a factor of 2, to 31 fs rms, offering a significant improvement to beam performance for applications like ultrafast electron diffraction. This THz-driven technique provides a critical step towards unprecedented timing resolution in…
Ultrafast electron experiments usually work with low-emittance few-electron pulsed beams. The structures are usually much larger than the (average) electron pulse size posing challenges to the resolution of simulations. We present the tracking code FemtoTrack, which allows tackling these multi-scale challenges in a simple manner. The computationally most heavy interpolation of the fields is treated either by a moving window or by a supplemental grid, leading to a significant speedup. Space charge is treated by direct particle-particle interaction within each bunch, where however many bunches c…
Temporally-shaped electron bunches at ultrafast time scales are foreseen to support an array of applications including the development of small-footprint accelerator-based coherent light sources or as probes for, e.g., ultrafast electron-diffraction. We demonstrate a method where a transversely-segmented electron bunch produced via photoemission from a transversely-patterned laser distribution is transformed into an electron bunch with modulated temporal distribution. In essence, the presented transformation enables the mapping of the transverse laser distribution on a photocathode surface to …
We present a method for producing sub-100 fs electron bunches that are suitable for single-shot ultrafast electron diffraction experiments in the 100 keV energy range. A combination of analytical results and state-of-the-art numerical simulations show that it is possible to create 100 keV, 0.1 pC, 20 fs electron bunches with a spotsize smaller than 500 micron and a transverse coherence length of 3 nm, using established technologies in a table-top set-up. The system operates in the space-charge dominated regime to produce energy-correlated bunches that are recompressed by established radio-freq…
Dielectric laser acceleration is a versatile scheme to accelerate and control electrons with the help of femtosecond laser pulses in nanophotonic structures. We demonstrate here the generation of a train of electron pulses with individual pulse durations as short as $270\pm80$ attoseconds(FWHM), measured in an indirect fashion, based on two subsequent dielectric laser interaction regions connected by a free-space electron drift section, all on a single photonic chip. In the first interaction region (the modulator), an energy modulation is imprinted on the electron pulse. During free propagatio…
Acceleration and manipulation of ultrashort electron bunches are the basis behind electron and X-ray devices used for ultrafast, atomic-scale imaging and spectroscopy. Using laser-generated THz drivers enables intrinsic synchronization as well as dramatic gains in field strengths, field gradients and component compactness, leading to shorter electron bunches, higher spatio-temporal resolution and smaller infrastructures. We present a segmented THz electron accelerator and manipulator (STEAM) with extended interaction lengths capable of performing multiple high-field operations on the energy an…
In this paper we describe a measurement technique capable of resolving femtosecond X-ray pulses from XFEL facilities. Since these ultrashort pulses are themselves the shortest event available, our measurement strategy is to let the X-ray pulse sample itself. Our method relies on the application of a "fresh" bunch technique, which allows for the production of a seeded X-ray pulse with a variable delay between seed and electron bunch. The shot-to-shot averaged energy per pulse is recorded. It turns out that one actually measures the autocorrelation function of the X-ray pulse, which is related i…
We propose and demonstrate a novel scheme to produce ultrashort and ultrastable MeV electron beam. In this scheme, the electron beam produced in a photocathode radio-frequency (rf) gun first expands under its own Coulomb force with which a positive energy chirp is imprinted in the beam longitudinal phase space. The beam is then sent through a double bend achromat with positive longitudinal dispersion where electrons at the bunch tail with lower energies follow shorter paths and thus catch up with the bunch head, leading to longitudinal bunch compression. We show that with optimized parameter s…
Coulomb interaction between charged particles is a well-known phenomenon in many areas of researches. In general the Coulomb repulsion force broadens the pulse width of an electron bunch and limits the temporal resolution of many scientific facilities such as ultrafast electron diffraction and x-ray free-electron lasers. Here we demonstrate a scheme that actually makes use of Coulomb force to compress a relativistic electron beam. Furthermore, we show that the Coulomb-driven bunch compression process does not introduce additional timing jitter, which is in sharp contrast to the conventional ra…
Ultralow emittance ($\leq20$ nm, normalized) electron beams with $10^5$ electrons per bunch are obtained by tightly focusing an ultrafast ($\sim$ 100 fs) laser pulse on the cathode of a 1.6 cell radiofrequency photoinjector. Taking advantage of the small initial longitudinal emittance, a downstream velocity bunching cavity is used to compress the beam to $<10$ fs rms bunch length. The measurement is performed using a thick high voltage deflecting cavity which is shown to be well-suited to measure ultrashort durations of bunching beams, provided that the beam reaches a ballistic longitudinal fo…
In recent and future synchrotron radiation facilities, relativistic electron bunches with increasingly high charge density are needed for producing brilliant light at various wavelengths, from X-rays to terahertz. In such conditions, interaction of electrons bunches with their own emitted electromagnetic fields leads to instabilities and spontaneous formation of complex spatial structures. Understanding these instabilities is therefore key in most electron accelerators. However, investigations suffer from the lack of non-destructive recording tools for electron bunch shapes. In storage rings, …
We present diffraction patterns from micron-sized areas of mono-crystalline graphite obtained with an ultracold and ultrafast electron source. We show that high spatial coherence is manifest in the visibility of the patterns even for picosecond bunches of appreciable charge, enabled by the extremely low source temperature (~ 10 K). For a larger, ~ 100 um spot size on the sample, spatial coherence lengths > 10 nm result, sufficient to resolve diffraction patterns of complex protein crystals. This makes the source ideal for ultrafast electron diffraction of complex macromolecular structures such…
We present experimental measurements of the femtosecond time-scale generation of strong magnetic-field fluctuations during the interaction of ultrashort, moderately relativistic laser pulses with solid targets. These fields were probed using low-emittance, highly relativistic electron bunches from a laser wakefield accelerator, and a line-integrated $B$-field of $2.70 \pm 0.39\,\rm kT\,μm$ was measured. Three-dimensional, fully relativistic particle-in-cell simulations indicate that such fluctuations originate from a Weibel-type current filamentation instability developing at submicron scales …
We propose and demonstrate a novel method to reduce the pulse width and timing jitter of a relativistic electron beam through THz-driven beam compression. In this method the longitudinal phase space of a relativistic electron beam is manipulated by a linearly polarized THz pulse in a dielectric tube such that the bunch tail has a higher velocity than the bunch head, which allows simultaneous reduction of both pulse width and timing jitter after passing through a drift. In this experiment, the beam is compressed by more than a factor of four from 130 fs to 28 fs with the arrival time jitter als…
Due to their ultra-short duration and peak currents in the kA range, laser-wakefield accelerated electron bunches are promising drivers for ultrafast X-ray generation in compact free-electron-lasers (FELs), Thomson-scattering or betatron sources. Here we present the first single-shot, high-resolution measurements of the longitudinal bunch profile obtained without prior assumptions about the bunch shape. Our method allows complex features, such as multi-bunch structures, to be detected. Varying the length of the gas target, and thus the acceleration length, enables an assessment of the bunch pr…
In this paper, we describe a harmonic kicker system used in the beam exchange scheme for the Circulator Cooling Ring (CCR) of the Jefferson Lab Electron Ion Collider(JLEIC). By delivering an ultra-fast deflecting kick, a kicker directs electron bunches selectively in/out of the CCR without degrading the beam dynamics of the CCR optimized for ion beam cooling. We will discuss the design principle of the kicker system and demonstrate its performance with various numerical simulations. In particular, the degrading effects of realistic harmonic kicks on the beam dynamics, such as 3D kick field pro…
In this paper we propose a new method for measurements of the longitudinal profile of 100 femtosecond electron bunches for X-ray Free Electron Lasers (XFELs). The method is simply the combination of two well-known techniques, which where not previously combined to our knowledge. We use seed 10-ps 1047 nm quantum laser to produce exact optical replica of ultrafast electron bunches. The replica is generated in apparatus which consists of an input undulator (energy modulator), and the short output undulator (radiator) separated by a dispersion section. The radiation in the output undulator is exc…
The heating of the electronic distribution of a copper photocathode due to an intense drive laser pulse is calculated under the two-temperature model using fluences and pulse lengths typical in RF photoinjector operation. Using the finite temperature-extended relations for the photocathode intrinsic emittance and quantum efficiency, the time-dependent emittance growth due to the same photoemission laser pulse is calculated. This laser heating is seen to limit the intrinsic emittance achievable for photoinjectors using short laser pulses and low quantum efficiency metal photocathodes. A pump-pr…
We present the results of multi-objective genetic algorithm optimizations of a potential single shot ultra fast electron diffraction beamline utilizing a 225 kV dc gun with a novel cryocooled photocathode system and buncher cavity. Optimizations of the transverse projected emittance as a function of bunch charge are presented and discussed in terms of the scaling laws derived in the charge saturation limit. Additionally, optimization of the transverse coherence length as a function of final rms bunch length at sample location have been performed for three different sample radii: 50, 100, 200 m…
In the Phase 2 of the AWAKE first experimental run (from May to November 2018), an electron beam was used to probe and test proton-driven wakefield acceleration in a rubidium plasma column. In this work, we analyze the overall charge capture and shot-to-shot reproducibility of the proton-driven plasma wakefield accelerator with various electron bunch injection parameters. The witness electron bunches were produced using an RF-gun equipped with a Cs2Te photocathode illuminated by a tailorable ultrafast deep ultraviolet (UV) laser pulse. The construction of the UV beam optical system enabled app…
We propose a new concept of an electron source for ultrafast electron diffraction with sub-10~fs temporal resolution. Electrons are generated in a laser-plasma accelerator, able to deliver femtosecond electron bunches at 5 MeV energy with kHz repetition rate. The possibility of producing this electron source is demonstrated using Particle-In-Cell simulations. We then use particle tracking simulations to show that this electron beam can be transported and manipulated in a realistic beamline, in order to reach parameters suitable for electron diffraction. The beamline consists of realistic stati…
High quality electron beams with flat distributions in both energy and current are critical for many accelerator-based scientific facilities such as free-electron lasers and MeV ultrafast electron diffraction and microscopes. In this Letter we report on using corrugated structures to compensate for the beam nonlinear energy chirp imprinted by the curvature of the radio-frequency field, leading to a significant reduction in beam energy spread. By using a pair of corrugated structures with orthogonal orientations, we show that the quadrupole wake fields which otherwise increase beam emittance ca…
Ultrafast electron diffraction (UED) is a technique in which short-pulse electron beams can probe the femtosecond-scale evolution of atomic structure in matter driven far from equilibrium. As an accelerator physics challenge, UED imposes stringent constraints on the brightness of the probe electron beam. The low normalized emittance employed in UED, often at the 10 nm scale and below, is particularly sensitive to both applied field aberrations and space charge effects. The role of aberrations is increasingly important in small probe systems that often feature multiple orders of magnitude varia…
We propose and demonstrate a novel method to produce few-femtosecond electron beam with relatively low timing jitter. In this method a relativistic electron beam is compressed from about 150 fs (rms) to about 7 fs (rms, upper limit) with the wakefield at THz frequency produced by a leading drive beam in a dielectric tube. By imprinting the energy chirp in a passive way, we demonstrate through laser-driven THz streaking technique that no additional timing jitter with respect to an external laser is introduced in this bunch compression process, a prominent advantage over the conventional method …
We present measurements of the pulse length of ultracold electron bunches generated by near-threshold two-photon photoionization of a laser-cooled gas. The pulse length has been measured using a resonant $3$ GHz deflecting cavity in TM$_{110}$ mode. We have measured the pulse length in three ionization regimes. The first is direct two-photon photoionization using only a $480$ nm femtosecond laser pulse, which results in short ($\sim 15$ ps) but hot ($\sim 10^{4}$ K) electron bunches. The second regime is just-above-threshold femtosecond photoionization employing the combination of a continuous…
We present the results of multi-objective genetic algorithm optimizations of a potential single shot ultra fast electron diffraction beamline utilizing a 100 MV/m 1.6 cell normal conducting rf (NCRF) gun, as well as a 9 cell 2pi/3 bunching cavity placed between two solenoids. Optimizations of the transverse projected emittance as a function of bunch charge are presented and discussed in terms of the scaling laws derived in the charge saturation limit. Additionally, optimization of the transverse coherence length as a function of final rms bunch length at the sample location have been performed…
Dielectric structures driven by laser-generated terahertz (THz) pulses may hold the key to overcoming the technological limitations of conventional particle accelerators and with recent experimental demonstrations of acceleration, compression and streaking of low-energy (sub-100 keV) electron beams, operation at relativistic beam energies is now essential to realize the full potential of THz-driven structures. We present the first THz-driven linear acceleration of relativistic 35 MeV electron bunches, exploiting the collinear excitation of a dielectric-lined waveguide driven by the longitudina…
High resolution single-shot non-relativistic ultrafast electron microscopy(UEM) relies on adaptive optics to compress high intensity bunches using Radio Frequency (RF) cavities. We present a comprehensive discussion of the analytic approaches available to characterize bunch dynamics as an electron bunch goes through a longitudinal focal point after an RF cavity where space charge effects can be large. Methods drawn from the Coulomb explosion literature, the accelerator physics literature and the analytic Gaussian model developed for UEM are compared, utilized and extended in some cases. In par…