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arXiv 1602.04162cond-mat.mes-hall
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斜向磁场作用下GaAs(1-x)N(x)合金中的自旋相关复合

Spin-dependent recombination in GaAs(1-x)N(x) alloys at oblique magnetic field

E. L. Ivchenko, L. A. Bakaleinikov, M. M. Afanasiev, V. K. Kalevich

摘要:

本文从实验和理论上研究了磁场中的光学取向和自旋相关的Shockley-Read-Hall复合。实验是在室温下进行的GaAsN合金深顺磁中心负责自旋相关的复合。所观察到的光致发光的圆偏振r(B)和强度J(B)的磁场依赖性可以近似地描述为两个洛伦兹轮廓(正向和反向)的叠加,其半宽度相差一个数量级。正常的(窄)洛伦兹轮廓是与退极化的横向(到字段)组件的自旋极化的本地化的电子,而反转(宽)洛伦兹是由于抑制超精细相互作用的本地化的电子与缺陷核。一个洛伦兹线的高度和另一个洛伦兹线的深度之间的比率由场倾斜角决定。与浅施主束缚电子与大量晶格核的超精细相互作用相反,在所研究的电子-核系统的光学取向中,在斜场中没有出现额外的窄峰。这一结果表明,在GaAsN合金中,即使在室温下,局域电子与顺磁中心的单核的超精细相互作用仍然很强。对于实验的理论描述,我们已经扩展了通过深顺磁中心的自旋相关的复合理论与核角动量I = 1/2以前开发的特定情况下的纵向场。计算曲线r(B),J(B)与实验依赖性的近似描述一致,近似描述为两个Lorentzian之和。

英文摘要:

We have studied experimentally and theoretically the optical orientation and spin-dependent Shockley-Read-Hall recombination in a semiconductor in a magnetic field at an arbitrary angle between the field and circularly polarized exciting beam. The experiments are performed at room temperature in GaAsN alloys where deep paramagnetic centers are responsible for the spin-dependent recombination. The observed magnetic-field dependences of the circular polarization r(B) and intensity J(B) of photoluminescence can be approximately described as a superposition of two Lorentzian contours, normal and inverted, with their half-widths differing by an order of magnitude. The normal (narrow) Lorentzian contour is associated with depolarization of the transverse (to the field) component of spin polarization of the localized electrons, whereas the inverted (broad) Lorentzian is due to suppression of the hyperfine interaction of the localized electron with the defect nucleus. The ratio between the height of one Lorentzian and depth of the other is governed by the field tilt angle. In contrast to the hyperfine interaction of a shallow-donor-bound electron with a large number of nuclei of the crystal lattice, in the optical orientation of the electron-nuclear system under study no additional narrow peak appears in the oblique field. This result demonstrates that in the GaAsN alloys the hyperfine interaction of the localized electron with the single nucleus of the paramagnetic center remains strong even at room temperature. For a theoretical description of the experiment, we have extended the theory of spin-dependent recombination via deep paramagnetic centers with the nuclear angular momentum I = 1/2 developed previously for the particular case of the longitudinal field. The calculated curves r(B), J(B) agree with the approximate description of the experimental dependences as a sum of two Lorentzians.

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