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arXiv 1502.05155cond-mat.str-el
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U(Co $_{1-x}$ Fe $_x$)Al($0 \leq x \leq 0.02$)铁磁临界行为的$^{59}$ Co核四极共振研究

Ferromagnetic Critical Behavior in U(Co$_{1-x}$Fe$_x$)Al ($0 \leq x \leq 0.02$) Studied by $^{59}$Co Nuclear Quadrupole Resonance Measurement

Kosuke Karube, Taisuke Hattori, Kenji Ishida, Noriaki Kimura

摘要:

为了研究巡游电子变磁化合物UCoAl中铁磁(FM)量子跃迁点和三临界点附近的物理性质,我们对Fe取代的U(Co $_{1-x}$ Fe $_x$)Al($x$ = 0,0.5,1,2%)在零外磁场下进行了$^{59}$ Co核四极共振(NQR)测量.低温下$^{59}$ Co-NQR谱的Fe浓度依赖性表明,至少在$x$ = 1%以上发生一阶FM跃迁。由核自旋-自旋弛豫速率$1/T_2$探测到的沿$c$轴的磁涨落在$T_\mathrm{max}$ $\sim$ 20 K时表现出异常,并随着$x$的增加而增强。这些结果是在良好的协议与理论预测,并表明在TCP在该系统中存在突出的临界波动。

英文摘要:

In order to investigate physical properties around a ferromagnetic (FM) quantum transition point and a tricritical point (TCP) in the itinerant-electron metamagnetic compound UCoAl, we have performed the $^{59}$Co nuclear quadrupole resonance (NQR) measurement for the Fe-substituted U(Co$_{1-x}$Fe$_x$)Al ($x$ = 0, 0.5, 1, and 2%) in zero external magnetic field. The Fe concentration dependence of $^{59}$Co-NQR spectra at low temperatures indicates that the first-order FM transition occurs at least above $x$ = 1%. The magnetic fluctuations along the $c$ axis detected by the nuclear spin-spin relaxation rate $1/T_2$ exhibit an anomaly at $T_\mathrm{max}$ $\sim$ 20 K and enhance with increasing $x$. These results are in good agreement with theoretical predictions and indicate the presence of prominent critical fluctuations at the TCP in this system.

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