We report on a comprehensive study of CePd$_{1-x}$Rh$_x$ $(0.6 \leq x \leq 0.95)$ poly- and single crystals close to the ferromagnetic instability by means of low-temperature ac susceptibility, magnetization and volume thermal expansion. The signature of ferromagnetism in this heavy-fermion system can be traced from 6.6 K in CePd down to 25 mK for $x=0.87$. Despite pronounced non-Fermi-liquid (NFL) effects in both, specific heat and thermal expansion, the Grüneisen ratio {\it does not} diverge as $T\to 0$, providing evidence for the absence of a quantum critical point. Instead, a peculiar "Kondo-cluster-glass" state is found for $x\geq 0.65$, and the NFL effects in the specific heat, ac susceptibility and magnetization are compatible with the quantum Griffiths phase scenario.
We investigate the one-dimensional Kondo lattice model (1D KLM) for ferromagnetic Kondo couplings, by using the bosonization method. The ferromagnet ic 2-leg spin ladder and the S=1 antiferromagnet occur as new one-dimensional Kondo insulators, for a half-filled band. First,a very small hole-doping makes the charge sector massless and it can produce, either an incommensurate RKKY interaction or a S=1 ferromagnet according to the strength of the ferromagnetic Kondo coupling. Second, we investigate, the effects of a weak and quenched disorder on these two Kondo insulators, by applying renormaliz…
We report the coexistence of the Kondo effect and spin glass behavior in Fe-doped NbS$_2$ single crystals. The Fe$_x$NbS$_2$ shows the resistance minimum and negative magnetoresistance due to the Kondo effect, and exhibits no superconducting behavior at low temperatures. The resistance curve follows a numerical renormalization-group theory using the Kondo temperature $T_K =12.3$~K for $x=0.01$ as evidence of Kondo effect. Scanning tunneling microscope/spectroscopy (STM/STS) revealed the presence of Fe atoms near sulfur atoms and asymmetric spectra. The magnetic susceptibility exhibits a featur…
In our recent study, Phys. Rev. Lett. 108 086402 (2012), we have revealed the intriguing properties of the ferromagnetic state in the Kondo lattice model with antiferromagnetic coupling in infinite dimensions: within the ferromagnetic metallic phase, the minority conduction electrons form a gap at the Fermi energy and do not participate in transport irrespective of interaction strength and filling. This half-metallic state is referred to as a spin-selective Kondo insulator. We here show that the spin-selective Kondo insulator can also be realized in the one-dimensional Kondo lattice model by s…
Dynamical spin susceptibility is calculated for the generalized ferromagnetic Kondo model which describes itinerant $e_{g}$ electrons interacting with localized $t_{2g}$ electrons with antiferromagnetic coupling. The calculations done in the mean field approximation show that the spin-wave spectrum of the system in ferromagnetic state has two branches, acoustic and optic ones. Self-energy corrections to the spectrum are considered and the acoustic spin-wave damping is evaluated.
Motivated by recent experiments, we study a quasi-one dimensional model of a Kondo lattice with Ferromagnetic coupling between the spins. Using bosonization and dynamical large-N techniques we establish the presence of a Fermi liquid and a magnetic phase separated by a local quantum critical point, governed by the Kondo breakdown picture. Thermodynamic properties are studied and a gapless charged mode at the quantum critical point is highlighted.
Magnetic impurities bridging nanocontacts and break junctions of nearly magnetic metals may lead to permanent moments, analogous to the giant moments well known in the bulk case. A numerical renormalization group (NRG) study shows that, contrary to mean field based expectations, a permanent moment never arises within an Anderson model, which invariably leads to strong Kondo screening. By including in the model an additional ferromagnetic exchange coupling between leads and impurity, the NRG may instead stabilize a permanent moment through a ferromagnetic Kondo effect. The resulting state is a …
Motivated by the recent discovery of ferromagnetic quantum criticality in the heavy fermion compound CeRh$_6$Ge$_4$, we develop a numerical algorithm of infinite projected entangled pair states for the anisotropic ferromagnetic Kondo-Heisenberg model in two dimensions and study the ferromagnetic quantum phase transitions with varying magnetic and hopping anisotropy. Our calculations reveal a continuous ferromagnetic quantum phase transition in the large anisotropic region and first-order quantum phase transitions for smaller anisotropy. Our results highlight the importance of magnetic anisotro…
We study the Kondo effect of a two-orbital vertical quantum dot (QD) coupled to two ferromagnetic leads by employing an equation of motion method. When the ferromagnetic leads are coupled with parallel spin polarization, we find three peaks in the single-particle excitation spectra. The middle one is the Kondo resonance caused by the orbital degrees of freedom. In magnetic fields, the Kondo effect vanishes. However, at a certain magnetic field new two-fold degenerate states arise and the Kondo effect emerges there. In contrast, when the ferromagnetic leads are coupled with antiparallel spin po…
Based on a simple approximation scheme we have computed the local density of states (LDOS) of the antiferromagnetic and ferromagnetic Kondo models for the full range of band occupations and coupling strengths. For both models the LDOS with its full energy dependence has not been calculated before. Arguments are given for the results to be qualitatively trustworthy despite the simplicity of the approximation scheme.
The Kondo-lattice model, which couples a lattice of localized magnetic moments to conduction electrons, is often used to describe heavy-fermion systems. Because of the interplay between Kondo physics and magnetic order it displays very complex behavior and is notoriously hard to solve. The ferromagnetic Kondo-lattice model, with a ferromagnetic coupling between the local moments, describes a phase transition from a paramagnetic phase to a ferromagnetic one as a function of either temperature or the ferromagnetic local-moment coupling. At zero temperature, this is a quantum phase transition tha…
The magnetic properties of the ferromagnetic Kondo-lattice model (FKLM) are investigated. Starting from an analysis of the magnon spectrum in the spin-wave regime, we examine the ferromagnetic stability as a function of the occupation of the conduction band $n$ and the strength $J$ of the coupling between the localised moments and the conduction electrons. From the properties of the spin-wave stiffness $D$ the ferromagnetic phase at zero temperature is derived. Using an approximate formula the critical temperature $T_c$ is calculated as a function of $J$ and $n$.
We present an new approach for the ferromagnetic, three-dimensional, translational-symmetric Kondo lattice model which allows us to derive both magnon energies and linewidths (lifetimes) and to study the properties of the ferromagnetic phase at finite temperatures. Both "anomalous softening" and "anomalous damping" are obtained and discussed. Our method consists of mapping the Kondo lattice model onto an effective Heisenberg model by means of the "modified RKKY interaction" and the "interpolating self-energy approach". The Heisenberg model is approximatively solved by applying the Dyson-Maleev…
We present low-temperature heat and charge transport as well as caloric properties of a ThAsSe single crystal. An extra -AT1/2 term in the electrical resistivity, independent of magnetic fields as high as 14 T, provides evidence for an unusual scattering of conduction electrons. Additionally, both the thermal conductivity and specific heat show a glass-type temperature dependence which signifies the presence of tunneling states. These observations apparently point to an experimantal realization of a two-channel Kondo effect derived from structural two-level systems.
Electron Spin Resonance (ESR) measurements of the ferromagnetic Kondo lattice system CeRuPO show a well defined ESR signal which is related to the magnetic properties of the Ce3+ moment. In contrast, no ESR signal could be observed in the antiferromagnetic homologue CeOsPO. Additionally, we detect an ESR signal in a further ferromagnetic Yb compound, YbRh, while it was absent in a number of Ce or Yb intermetallic compounds with dominant antiferromagnetic exchange, independently of the presence of a strong Kondo interaction or the proximity to a (quantum) critical point. Thus, the observation o…
We investigate the one-dimensional Kondo lattice model (1D KLM) for ferromagnetic Kondo couplings. The so-called ferromagnetic 2-leg spin ladder and the S=1 antiferromagnet occur as new one-dimensional Kondo insulators. Both exhibit a spin gap. But, in contrast to the strong coupling limit, the Haldane state which characterizes the 2-leg spin ladder Kondo insulator cannot fight against very weak exterior perturbations. First, by using standard bosonization techniques, we prove that an antiferromagnetic ground state occurs by doping with few holes; it is characterized by a form factor of the sp…
Carrier-induced ferromagnetism is investigated in a diluted ferromagnetic Kondo lattice model for several ordered impurity arrangements on square and cubic lattices, allowing for quantitative comparison with different theoretical pictures. The spin stiffness is found to be optimized with respect to hole doping concentration, exchange interaction strength, as well as spin dilution due to a competition involving magnitude of carrier spin polarization and its oscillation length scale. The ferromagnetic transition temperature determined within the spin-fluctuation theory is in good agreement with …
The 2D ferromagnetic Kondo model with classical corespins is studied for a hole doping up to x = 0.125 via unbiased Monte Carlo (MC) simulations. A canonical algorithm for finite temperatures is developed. We show that with realistic parameters for the manganites and at low temperatures, the double-exchange mechanism does not lead to phase separation on a two-dimensional lattice but rather stabilizes individual ferromagnetic polarons. A detailed analysis of unbiased MC results reveals that the polarons can be treated as independent particles. It is found that a simple polaron model perfectly d…
We study the low temperature behavior of a boundary magnetic impurity S'=1/2 in an open ferromagnetic Takhatajian-Babujian spin-S chain. For antiferromagnetic Kondo coupling, it is show via Bethe ansatz solution that the impurity spin is always locked into the critical behavior the bulk. At low temperature, a local composite of spin S-1/2 forms near the impurity site and its contribution to specific heat is of simple power law T^{1/2}. The absence of overscreened Kondo effect is due to the large correlation length of host spins which is divergent near the quantum critical point.
We present a high temperature series expansion for the ferromagnetic Kondo lattice model in the large coupling limit, which is used to model CMR perovskites. Our results show the expected cross-over to Curie-Weiß behavior at a temperature related to the bandwidth. Estimates for the magnetic transition temperatures are in the experimentally observed range. The compressibility shows that the high temperature charge excitations can be modeled by spinless fermions. The CMR effect itself, however, warrants the inclusion of dynamic effects and cannot be explained by a static calculation.
The Kondo effect in a Luttinger liquid is studied using the renormalization group method. By renormalizing the boson fields, scaling equations to the second order for an arbitrary Luttinger interaction are obtained. For the ferromagnetic Kondo coupling, a spin bound state(triplet) can be realized without invoking a nearest neighbor spin interaction in agreement with the recent Bethe ansatz calculation. The scaling theory in the presence of the scalar potential shows that there is no interplay between the magnetic and non-magnetic interaction. Also a study on the crossover behavior of the Kondo…
Kondo effect originates from antiferromagnetic (AFM) s-d coupling between magnetic impurity and the conduction electron, while it will be totally quenched in ferromagnetic (FM) regime due to malfunction of spin-flip. We investigate the possibility of switching on/off Kondo effect by transition of AFM/FM s-d coupling using 3d-metal phthalocyanine molecule (MPc) on Au(111) as a model system. A Hamiltonian model is constructed based on the feature of MPc molecule to show the condition for AFM/FM s-d coupling. The AFM s-d coupling could transform to FM s-d coupling if the spin state of the lowest …
We establish the low-temperature phase diagrams of the spin-1/2 and spin-1 Kondo lattice models as a function of the conduction-band filling n and the exchange coupling strength J in the regime of ferromagnetic effective exchange interactions (n ~< 0.5). We show that both models have several distinct ferromagnetic phases separated by continuous Lifshitz transitions of the Fermi-pocket vanishing or emergence type: one of the phases has a true gap in the minority band (half metal), the others only a pseudogap. They can be experimentally distinguished by their magnetization curves; only the gappe…
The spin dynamics of the ferromagnetic Kondo lattice CeRuPO is investigated by Electron Spin Resonance (ESR) at microwave frequencies of 1, 9.4, and 34~GHz. The measured resonance can be ascribed to a rarely observed bulk Ce3+ resonance in a metallic Ce compound and can be followed below the ferromagnetic transition temperature Tc=14 K. At T>Tc the interplay between the RKKY-exchange interaction and the crystal electric field anisotropy determines the ESR parameters. Near Tc the spin relaxation rate is influenced by the critical fluctuations of the order parameter.
We investigate the two- and three-dimensional ferromagnetic Kondo lattice model by unbiased Monte Carlo simulations. A phase diagram for the two-dimensional model is presented, in which the stability of magnetic order and ferromagnetic polarons is examined with respect to the antiferromagnetic superexchange J' and temperature. The Monte Carlo simulations reveal that J' > 0.02 strengthens individual polarons while small J' < 0.02 favors larger clusters and phase separation except for small doping. Lowering the temperature stabilizes ferromagnetic polarons for realistic J' > 0.01, while phase se…
Ferromagnetic Kondo lattice compounds are far less common than their antiferromagnetic analogs. In this work, we report the discovery of a new ferromagnetic Kondo lattice compound, YbIr3Ge7. Like almost all ferromagnetic Kondo lattice systems, YbIr3Ge7 shows magnetic order with moments aligned orthogonal to the crystal electric field (CEF) easy axis. YbIr3Ge7 is unique in that it is the only member of this class of compounds that crystallizes in a rhombohedral structure with a trigonal point symmetry of the magnetic site, and it lacks broken inversion symmetry at the local moment site. AC magn…
The transport properties of the ferromagnetic Kondo lattice model in one dimension are studied via bosonization methods. The antiferromagnetic fluctuations, which normally appear because of the RKKY interactions, are explicitly taken into account as a direct exchange between the ``core'' spins. It is shown that in the paramagnetic regime with the local antiferromagnetic fluctuations, the resistivity decays exponentially as the temperature increases while in the ferromagnetic regime the system is an almost perfect conductor. %A non-perturbative description of localized spin polarons %in the par…
Inelastic neutron scattering investigation on ferromagnetic Kondo lattice compounds belonging to CeSi_{2-x}Ga_{x}, x = 0.7, 1.0 and 1.3, system is reported. The thermal evolution of the quasielastic response shows that the Kondo interactions dominate over the RKKY interactions with increase in Ga concentration from 0.7 to 1.3. This is related to the increase in k-f hybridization with increasing Ga concentration. The high energy response indicates the ground state to be split by crystal field in all three compounds. Using the experimental results we have calculated the crystal field parameters …
The experimental existence and stability of the quantum criticality point of the two-channel Kondo (2CK) effect displaying exotic non-Fermi liquid physics has been buried in persistent confusion despite the intensive theoretical and experimental efforts in past three decades. Here we report an experimental realization of the two-level system scattering-induced orbital 2CK effect in a ferromagnetic L10-MnGa film, which is signified by a magnetic field-independent resistivity upturn that has a logarithmic and square-root temperature dependence beyond and below the Kondo temperature of ~14.5 K, r…
The ferromagnetic Kondo model with classical corespins is studied via unbiased Monte-Carlo simulations. We show that with realistic parameters for the manganites and at low temperatures, the double-exchange mechanism does not lead to phase separation in one-dimensional chains but rather stabilizes individual ferromagnetic polarons. Within the ferromagnetic polaron picture, the pseudogap in the one-particle spectral function A_k(ω) can easily be explained. Ferromagnetic polarons also clear up a seeming failure of the double-exchange mechanism in explaining the comparable bandwidths in the ferro…
We carefully consider the interplay between ferromagnetism and the Kondo screening effect in the conventional Kondo lattice systems at finite temperatures. Within an effective mean-field theory for small conduction electron densities, a complete phase diagram has been determined. In the ferromagnetic ordered phase, there is a characteristic temperature scale to indicate the presence of the Kondo screening effect. We further find two distinct ferromagnetic long-range ordered phases coexisting with the Kondo screening effect: spin fully polarized and partially polarized states. A continuous phas…
We study numerically the one-dimensional ferromagnetic Kondo lattice. This model is widely used to describe nickel and manganese perovskites. Due to the competition between double and super-exchange, we find a region where the formation of magnetic polarons induces a charge-ordered state. This ordering is present even in the absence of any inter-site Coulomb repulsion. There is an insulating gap associated to the charge structure formation. We also study the insulator-metal transition induced by a magnetic field which removes simultaneously both charge and spin ordering.
We propose that a simple device of three laterally-coupled quantum dots, the central one contacted by metal leads, can realize the ferromagnetic Kondo model, which is characterized by interesting properties like a non-analytic inverted zero-bias anomaly and an extreme sensitivity to a magnetic field. Furthermore, by tuning the gate voltages of the lateral dots, this device may allow to study the transition from ferromagnetic to antiferromagnetic Kondo effect, a simple case of a Berezinskii-Kosterlitz-Thouless transition. We model the device by three coupled Anderson impurities that we study by…
We report the temperature-pressure-magnetic field phase diagram made from electrical resistivity measurements for the ferromagnetic (FM) Kondo lattice CeRuPO. The ground state at zero field changes from the FM state to another state, which is suggested to be an antiferromagnetic (AFM) state, above ~0.7 GPa, and the magnetically ordered state is completely suppressed at ~2.8 GPa. In addition to the collapse of the AFM state under pressure and a magnetic field, a metamagnetic (MM) transition from a paramagnetic state to a polarized paramagnetic state appears. CeRuPO will give us a rich playgroun…
A purely fermionic representation is introduced for the ferromagnetic Kondo lattice model which allows conventional diagrammatic tools to be employed to study correlation effects. Quantum 1/S corrections to magnon excitations are investigated using a systematic inverse-degeneracy expansion scheme which incorporates correlation effects in the form of self-energy and vertex corrections, while explicitly preserving the continuous spin-rotation symmetry. Magnon self-energy is studied in the full range of interaction strength, and shown to result in strong magnon damping and anomalous softening for…
The magnetic ground state phase diagram of the ferromagnetic Kondo-lattice model is constructed by calculating internal energies of all possible bipartite magnetic configurations of the simple cubic lattice explicitly. This is done in one dimension (1D), 2D and 3D for a local moment of S = 3/2. By assuming saturation in the local moment system we are able to treat all appearing higher local correlation functions within an equation of motion approach exactly. A simple explanation for the obtained phase diagram in terms of bandwidth reduction is given. Regions of phase separation are determined …
We present an extensive numerical study of a new type of frustrated itinerant magnetism on the pyrochlore lattice. In this theory, the pyrochlore magnet can be viewed as a cross-linking network of Kondo or double-exchange chains. Contrary to models based on Mott insulators, this itinerant magnetism approach provides a natural explanation for several spin and orbital superstructures observed on the pyrochlore lattice. Through extensive Monte Carlo simulations, we obtain the phase diagrams at two representative electron filling fractions $n = 1/2$ and 2/3. In particular, we show that an intrigui…
We introduce a two-band Kondo-lattice model to describe ferromagnetic half-metals with local magnetic moments. In a model study, the electronic and magnetic properties are presented by temperature dependent magnetization curves, band-structures, spin polarizations and plasma frequencies. These are obtained from numerically evaluated equations, based on the single-electron Green functions. We show that the mutual influence between the itinerant electrons and the local magnetic moments is responsible for several phase transitions of the half-metals, namely first and second order magnetic phase t…
Spin dynamics is calculated in the ferromagnetic (FM) state of the generalized Kondo lattice model taking into account strong on-site correlations between e_g electrons and antiferromagnetic (AFM) exchange among t_{2g} spins. Our study suggests that competing FM double-exchange and AFM super-exchange interaction lead to a rather nontrivial spin-wave spectrum. While spin excitations have a conventional Dq^2 spectrum in the long-wavelength limit, there is a strong deviation from the spin-wave spectrum of the isotropic Heisenberg model close to the zone boundary. The relevance of our results to t…
Enhanced Anomalous Nernst Effect in the Ferromagnetic Kondo Lattice CeCo2As2
International Center for Quantum Materials, School of Physics, Peking University（北京大学物理学院量子材料国际中心）；State Key Laboratory of Quantum Functional Materials, Department of Physics, and Guangdong Basic Research Center of Excellence for Quantum Science, Southern University of Science and Technology（南方科技大学物理学院量子功能材料国家重点实验室及广东省量子科学基础研究中心）；Department of Chemistry, Michigan State University（密歇根州立大学化学系）
We report the first experimental realization of orbital two-channel Kondo (2CK) effect from two-level systems (TLSs) in epitaxial L10-MnAl films with giant perpendicular magnetic anisotropy. The resistivity exhibits a low-temperature (T) upturn with a clear transition from a lnT-dependence to T1/2-dependence and deviation from it in three distinct T regimes, which are independent of applied magnetic fields. The magnitudes of Kondo temperature and energy splitting of the TLSs are greatly enhanced in comparison to those in other systems exhibiting orbital 2CK, suggesting strong coupling between …
The magnetic phase diagram of the ferromagnetic Kondo lattice model is determined at T=0 in 1D, 2D, and 3D for various magnitudes of the quantum mechanical localized spins ranging from S=1/2 to classical spins. We consider the ferromagnetic phase, the paramagnetic phase, and the ferromagnetic/antiferromagnetic phase separated regime. There is no significant influence of the spin quantum number on the phase boundaries except for the case S=1/2, where the model exhibits an instability of the ferromagnetic phase with respect to spin disorder. Our results give support, at least as far as the low t…
Magnon self energy due to spin-charge coupling is calculated for the correlated ferromagnetic Kondo lattice model using a diagrammatic expansion scheme. Systematically incorporating correlation effects in the form of self-energy and vertex corrections, the expansion scheme explicitly preserves the continuous spin rotation symmetry and hence the Goldstone mode. Due to a near cancellation of the correlation-induced quantum correction terms at intermediate coupling and optimal band filling relevant for ferromagnetic manganites, the renormalized magnon energies for the correlated FKLM are nearly i…
We study numerically the one dimensional ferromagnetic Kondo lattice, a model widely used to describe nickel and manganese perovskites. By including a nearest neighbor Coulomb interaction (V) and a superexchange interaction between the localized moments (K), we obtain the phase diagram in parameter space for several dopings at T=0. Due to the competition between double and superexchange, we find a region where the formation of magnetic polarons induces a charge ordered (CO) state which survives also for V=0. This mechanism should be taken into account in theories of charge ordering involving s…
We use the Popov-Fedotov representation of spin operators to construct an effective action for a Kondo lattice model with quenched disorder at finite temperatures. We study the competition between the Kondo effect and frozen spin order in Ising-like spin glass. We present the derivation of new mean-field equations for the spin-glass order parameter and analyze the effects of screening of localized spins by conduction electrons on the spin-glass phase transition.
Some well-established examples of itinerant-electron ferromagnetism in one dimension occur in a Mott-insulating phase. We examine the consequences of doping a ferromagnetic insulator and cou- pling magnons to gapless charge fluctuations. Using a bosonization scheme for strongly interacting electrons, we derive an effective field theory for the magnon-holon interaction. When the magnon momentum matches the Fermi momentum of the holons, the backscattering of the magnon at low energies gives rise to a Kondo effect of a pseudospin defined from the chirality degree of freedom (right- or left-moving…
$^{51}$V nuclear magnetic resonance (NMR) and magnetization studies on CeTi$_{1-x}$V$_x$Ge$_3$ have been performed to explore the evolution from the ferromagnetic ($x = 0.113$) to the antiferromagnetic Kondo lattice state ($x = 1$), with focus on the emergence of a possible ferromagnetic quantum critical point (FMQCP) at $x_c \approx 0.4$. From the temperature dependence of the nuclear spin-lattice relaxation rate, $1/T_1T$, and the Knight shift, \textit{K}, for $x=0.113$ and $x=1$ a considerable competition between ferro- and antiferromagnetic correlations is found. Around the critical concen…
We report measurements of inelastic neutron scattering, magnetic susceptibility, magnetization, and the magnetic field dependence of the specific heat for the heavy Fermion compounds Ce$_3$In and Ce$_3$Sn. The neutron scattering results show that the excited crystal field levels have energies $E_1$ = 13.2 meV, $E_2$ = 44.8 meV for Ce$_3$In and $E_1$ = 18.5 meV, $E_2$ = 36.1 meV for Ce$_3$Sn. The Kondo temperature deduced from the quasielastic linewidth is 17 K for Ce$_3$In and 40 K for Ce$_3$Sn. The low temperature behavior of the specific heat, magnetization, and susceptibility can not be wel…
A new ``Dynamical Mean-field theory'' based approach for the Kondo lattice model with quantum spins is introduced. The inspection of exactly solvable limiting cases and several known approximation methods, namely the second-order perturbation theory, the self-consistent CPA and finally a moment-conserving decoupling of the equations of motion help in evaluating the new approach. This comprehensive investigation gives some certainty to our results: Whereas our method is somewhat limited in the investigation of the J<0-model, the results for J>0 reveal important aspects of the physics of the mod…
Motivated by recent scanning tunneling microscope (STM) experiments on cobalt clusters adsorbed on single wall metallic nanotubes [Odom {\em et al.}, Science {\bf 290}, 1549 (2000)], we study theoretically the size dependence of STM spectra and spin-flip scattering of electrons from finite size ferromagnetic clusters adsorbed on metallic surfaces. We study two models of nanometer size ferromagnets: (i) An itinerant model with delocalized s, p and d electrons and (ii) a local moment model with both localized d-level spins and delocalized cluster electrons. The effective exchange coupling betwee…
The Kondo-Spin Glass competition is studied in a theoretical model of a Kondo lattice with an intra-site Kondo type exchange interaction treated within the mean field approximation, an inter-site quantum Ising exchange interaction with random couplings among localized spins and an additional transverse field in the x direction, which represents a simple quantum mechanism of spin flipping. We obtain two second order transition lines from the spin-glass state to the paramagnetic one and then to the Kondo state. For a reasonable set of the different parameters, the two second order transition lin…
The physics of disordered alloys, such as typically the well known case of CeNi1-xCux alloys, showing an interplay among the Kondo effect, the spin glass state and a magnetic order, has been studied firstly within an average description like in the Sherrington-Kirkpatrick model. Recently, a theoretical model (PRB 74, 014427 (2006)) involving a more local description of the intersite interaction has been proposed to describe the phase diagram of CeNi1-xCux. This alloy is an example of the complex interplay between Kondo effect and frustration in which there is in particular the onset of a clust…
We present a many-body approach to the electronic and magnetic properties of the (multiband) Kondo-lattice model with ferromagnetic interband exchange. The coupling between itinerant conduction electrons and localized magnetic moments leads, on the one hand, to a distinct temperature-dependence of the electronic quasiparticle spectrum and, on the other hand, to magnetic properties, as e.~g.the Curie temperature T_C or the magnon dispersion, which are strongly influenced by the band electron selfenergy and therewith in particular by the carrier density. We present results for the single-band Ko…
We determine the boundary of the fully polarized ferromagnetic ground state in the one dimensional Kondo lattice model at partial conduction electron band filling by using a newly developed infinite size DMRG method which conserves the total spin quantum number. The obtained paramagnetic to ferromagnetic phase boundary is below $J \approx 3.5$ for the whole range of band filling. By this we solve the controversy in the phase diagram over the extent of the ferromagnetic region close to half filling.
The optical conductivity of the double exchange and the orbital degenerate Kondo lattice Hamiltonian (orbital t-J model) are invetigated by means of finite temperature diagonalization for different doping concentrations. The temperature dependence of sum rules, kinetic energy and Drude weight are studied. In particular it is shown that the double exchange model cannot explain the anomalous absorption in the uniform ferromagnetic phase of manganites discovered Okimoto et al. [Phys. Rev. Lett. 75, 109 (1995)]. The orbital t-J model explains the increase of the anomalous absorption with decreasin…
We present an extensive numerical study of the ferromagnetic Kondo lattice model with quantum mechanical S=3/2 core spins. We treat one orbital per site in one dimension using the density matrix renormalization group and include on-site Coulomb repulsion between the electrons. We examine parameters relevant to manganites, treating the range of low to intermediate doping, 0<x<0.5. In particular, we investigate whether quantum fluctuations favor phase separation over the ferromagnetic polarons observed in a model with classical core spins. We obtain very good agreement of the quantum model with …
We report on the low-temperature physical properties of a novel compound Ce$_{11}$Pd$_4$In$_9$ that crystallizes with the orthorhombic Nd$_{11}$Pd$_4$In$_9$-type crystal structure (space group $Cmmm$). The compound exhibits ferromagnetic ordering at $T_{\rm {C}}$ = 18.6 K and an order-order transition at $T_{\rm {t}}$ $\sim$~1.6 K, as inferred from the low-temperature magnetic susceptibility, heat capacity and electrical resistivity data. In the paramagnetic region, the electrical transport in Ce$_{11}$Pd$_4$In$_9$ is dominated by Kondo effect. Below $T_{\rm {C}}$, a distinct contribution due …
We report on the physical properties of the series Ce_(1-x)La_xIr_2B_2 (x D 0-0.9), obtained by means of magnetization, heat capacity and electrical resistivity measurements as a function of temperature (down to 0.7 K for the latter two measurements). The Curie temperature of CeIr2B2 (?5 K) is lowered due to La substitution, as expected. However, no quantum critical point or 'non-Fermi liquid' behavior was observed even in the dilute limit of x D 0:9. Interestingly, ferromagnetic ordering persists even for Ce0:1La0:9Ir2B2, below 0.8 K. Among the Ce systems, CeIr2B2 is one of the compounds in w…
A theory is proposed to describe the competition among antiferromagnetism (AF), spin glass (SG) and Kondo effect. The model describes two Kondo sublattices with an intrasite Kondo interaction strength $J_{K}$ and a random Gaussian interlattice interaction in the presence of a transverse field $Γ$. The $Γ$ field is introduced as a quantum mechanism to produce spin flipping and the random coupling has average $-2J_0/N$ and variance $32 J^{2}/N$. The path integral formalism with Grassmann fields is used to study this fermionic problem, in which the disorder is treated within the framework of the …
Neutron diffraction experiments on TmTe at pressures up to 7 GPa are reported. The semiconductor-to-metal transition occurring at 2 GPa in this compound is accompanied by the appearance of strong ferromagnetic exchange interactions producing a Curie temperature as high as 14 K. This behavior is characteristic for the incipient mixed-valence regime just above the transition pressure and traced back to the release of a small concentration of free charge carriers in the material. The steep decrease of both the Curie temperature and ordered magnetic moment occurring at higher pressures emphasizes …
