In this article, we present a numerical study of the optical properties of a metal nanowire interacting with a localized cavity in a two dimensional photonic crystal. The nature of the modes, their wavelength and width are investigated as a function of the particle radius. It is shown in particular that a particle with diameter about the lattice constant presents very narrow resonances corresponding to hybrid photonic-plasmonic modes, where increased lifetime is attributed to the decrease of the radiative losses by interaction with the photonic crystal. These results open interesting applications in areas where narrow plasmonic resonances are required, as in LSP-resonance based biosensing.
We discuss three formally different formulas for normalization of quasinormal modes currently in use for modeling optical cavities and plasmonic resonators and show that they are complementary and provide the same result. Regardless of the formula used for normalization, one can use the norm to define an effective mode volume for use in Purcell factor calculations.
Hybrid photonic-plasmonic cavities have emerged as a new platform to increase light-matter interaction capable to enhance the Purcell factor in a singular way not attainable with either photonic or plasmonic cavities separately. In the hybrid cavities proposed so far, mainly consisting of metallic bow-tie antennas, the plasmonic gap sizes defined by lithography in a repeatable way are limited to minimum values \approx 10 nm. Nanoparticle-on-a-mirror (NPoM) cavities are far superior to achieve the smallest possible mode volumes, as gaps smaller than 1 nm can be created. Here, we design a hybrid…
We found that very strong negative optical pressure can be induced in plasmonic cavities by LC resonance. This interesting effect could be described qualitatively by a Lagrangian model which shows that the negative optical pressure is driven by the internal inductance and the kinetic energy of the conduction electrons. If the metal is replaced by perfect conductors, the optical pressure becomes much smaller and positive.
We design a polarization-sensitive resonator for use in midinfrared photodetectors, utilizing a photonic crystal cavity and a single or double-metal plasmonic waveguide to achieve enhanced detector efficiency due to superior optical confinement within the active region. As the cavity is highly frequency and polarization-sensitive, this resonator structure could be used in chip-based infrared spectrometers and cameras that can distinguish among different materials and temperatures to a high degree of precision.
Spin defects in hexagonal boron nitride, and specifically the negatively charged boron vacancy (VB) centres, are emerging candidates for quantum sensing. However, the VB defects suffer from low quantum efficiency and as a result exhibit weak photoluminescence. In this work, we demonstrate a scalable approach to dramatically enhance the VB- emission by coupling to a plasmonic gap cavity. The plasmonic cavity is composed of a flat gold surface and a silver cube, with few-layer hBN flakes positioned in between. Employing these plasmonic cavities, we extracted two orders of magnitude in photolumin…
We report systematic studies of plasmonic and photonic guiding modes in large-area chemical-vapor-deposition-grown graphene on nanostructured silicon substrates. Light interaction in graphene with substrate photonic crystals can be classified into four distinct regimes depending on the photonic crystal lattice constant and the various modal wavelengths (i.e. plasmonic, photonic and free-space). By optimizing the design of the substrate, these resonant modes can magnify the graphene absorption in infrared wavelength, for efficient modulators, filters, sensors and photodetectors on silicon photo…
Molecular vibrations and their dynamics are of outstanding importance for electronic and thermal transport in nanoscale devices as well as for molecular catalysis. The vibrational dynamics of <100 molecules are studied through three-colour time-resolved coherent anti-Stokes Raman spectroscopy (trCARS) using plasmonic nanoantennas. This isolates molecular signals from four-wave mixing (FWM), while using exceptionally low nanowatt powers to avoid molecular damage via single-photon lock-in detection. FWM is found to be strongly suppressed in nm-wide plasmonic gaps compared to plasmonic nanopartic…
We demonstrate that the surface second-harmonic generation can lead to the formation of nonlinear plasmonic whispering-gallery modes (WGMs) in microcavities made of metallic nanowires. Since these WGMs are excited by induced surface nonlinear dipoles, they can be generated even when they are not coupled to the radiation continuum. Consequently, the quality factor of these nonlinear modes can be as large as the theoretical limit imposed by the optical losses in the metal. Remarkably, our theoretical analysis shows that nonlinear plasmonic WGMs are characterized by fractional azimuthal modal num…
The concept of cross density of states characterizes the intrinsic spatial coherence of complex photonic or plasmonic systems, independently on the illumination conditions. Using this tool and the associated intrinsic coherence length, we demonstrate unambiguously the spatial squeezing of eigenmodes on disordered fractal metallic films, thus clarifying a basic issue in plasmonics.
A novel type of a plasmonic waveguide has been proposed featuring an "open" design that is easy to manufacture, simple to excite and that offers a convenient access to a plasmonic mode. Optical properties of photonic bandgap (PBG) plasmonic waveguides are investigated experimentally by leakage radiation microscopy and numerically using the finite element method confirming photonic bandgap guidance in a broad spectral range. Propagation and localization characteristics of a PBG plasmonic waveguide have been discussed as a function of the wavelength of operation, waveguide core size and the numb…
We propose and demonstrate a hybrid photonic-plasmonic nanolaser that combines the light harvesting features of a dielectric photonic crystal cavity with the extraordinary confining properties of an optical nano-antenna. In that purpose, we developed a novel fabrication method based on multi-step electron-beam lithography. We show that it enables the robust and reproducible production of hybrid structures, using fully top down approach to accurately position the antenna. Coherent coupling of the photonic and plasmonic modes is highlighted and opens up a broad range of new hybrid nanophotonic d…
Orbital angular momentum of light is a core feature in photonics. Its confinement to surfaces using plasmonics has unlocked many phenomena and potential applications. Here we introduce the reflection from structural boundaries as a new degree of freedom to generate and control plasmonic orbital angular momentum. We experimentally demonstrate plasmonic vortex cavities, generating a succession of vortex pulses with increasing topological charge as a function of time. We track the spatio-temporal dynamics of these angularly decelerating plasmon pulse train within the cavities for over 300 femtose…
We theoretically analyse photonic-plasmonic coupling between a high Q whispering gallery mode (WGM) resonator and a core-shell nanoparticle. Blue and red shifts of WGM resonances are shown to arise from crossing of the photonic and plasmonic modes. Level repulsion in the hybrid system is further seen to enable sensitivity enhancements in WGM sensors: maximal when the two resonators are detuned by half the plasmon linewidth. Approximate bounds are given to quantify possible enhancements. Criteria for reactive vs. resistive coupling are also established.
We report an approach of realization and characterization of a novel plasmonic-photonic hybrid nanodevice. The device comprises a plasmonic nano-antenna (NA) and a defect mode based PC cavity, and were fabricated based on a multi-step electron-beam lithography. The laser emission of the devices was demonstrated and the coupling conditions between the NA and PC cavity were investigated in near-field level.
We report an approach to achieve this goal via build a plasmonic-dielectric photonic hybrid system. We induce a defect mode based photonic crystal (PC) cavity to work as a intermedium storage as well as a near-field light source to excite a plasmonic nanoantenna (NA). In this way, a plasmonic-photonic nano-laser source is created in present experiment. The coupling condition between the two elements is investigated in far-field and near-field level. We found that the NA reduces the Q-factor of the PC-cavity. Meanwhile, the NA concentrates and enhances the laser emission of the PC-cavity. This …
We demonstrate second harmonic generation at telecommunications wavelengths in L3 photonic crystal cavities in (111)-oriented GaAs. The second harmonic power from photonic crystal cavities fabricated in (111)-oriented GaAs is significantly increased compared to those fabricated in conventional (001)-oriented GaAs.
The geometric phase and topological property for one-dimensional hybrid plasmonic-photonic crystals consisting of a simple lattice of graphene sheets are investigated systematically. For transverse magnetic waves, both plasmonic and photonic modes exist in the momentum space. The accidental degeneracy point of these two kinds of modes is identified to be a diabolic point accompanied with a topological phase transition. For a closed loop around this degeneracy point, the Berry phase is Pi as a consequence of the discontinuous jump of the geometric Zak phase. The wave impedance is calculated ana…
We demonstrate a simple and rapid epoxy-based method for transferring photonic crystal cavities to the facets of optical fibers. Passive Si cavities were measured via fiber taper coupling as well as direct transmission from the fiber facet. Active quantum dot containing GaAs cavities showed photoluminescence that was collected both in free space and back through the original fiber. Cavities maintain a high quality factor (2000-4000) in both material systems. This new design architecture provides a practical mechanically stable platform for the integration of photonic crystal cavities with macr…
A bound state in the continuum (BIC) is a localized state of an open structure with access to radiation channels, yet it remains highly confined with, in theory, infinite lifetime and quality factor. There have been many realizations of such exceptional states in dielectric systems without loss. However, realizing BICs in systems with losses such as plasmonics remains a challenge. In this Letter, we explore the possibility of realizing BICs in a hybrid plasmonic-photonic structure consisting of a plasmonic grating coupled to a dielectric optical waveguide. The plasmonic-photonic system support…
We demonstrate high optical quality factors in aluminum nitride (AlN) photonic crystal nanobeam cavities. Suspended AlN photonic crystal nanobeams are fabricated in sputter-deposited AlN-on-insulator substrates using a self-protecting release process. Employing one-dimensional photonic crystal cavities coupled to integrated optical circuits we measure quality factors up to 146,000. By varying the waveguide-cavity coupling gap, extinction ratios in excess of 15 dB are obtained. Our results open the door for integrated photonic bandgap structures made from a low loss, wide-transparency, nonlinea…
We propose and analyze a new type of a resonant high-Q cavity for lasing, sensing or filtering applications, which is based on a surface states of a finite photonic crystal. We demonstrate that such the cavity can have a Q factor comparable with that one of conventional photonic band-gap defect mode cavities. At the same time, the distinguished feature of the surface mode cavity is that it is situated directly at the surface of the photonic crystal. This might open up new possibilities for design of novel photonic devices and integration of photonic circuits.
One dimensional nano-beam photonic crystal cavities fabricated in silicon dioxide are considered in both simulation and experiment. Quality factors of over 10^4 are found via simulation, while quality factors of over 5*10^3 are found in experiment, for cavities with mode volumes of 2.0 cubic wavelengths (in oxide) and in the visible wavelength range (600-716nm). The dependences of the cavity quality factor and mode volume for different design parameters are also considered.
We demonstrate fast (up to 20 GHz), low power (5 $μW$) modulation of photonic crystal (PC) cavities in GaAs containing InAs quantum dots. Rapid modulation through blue-shifting of the cavity resonance is achieved via free carrier injection by an above-band picosecond laser pulse. Slow tuning by several linewidths due to laser-induced heating is also demonstrated.
We theoretically study the interactions between plasmonic and photonic modes within a structure that is composed of two thin corrugated metallic plates, embedded in air. We show that the interactions depend upon the symmetry of the interacting modes. This observation is explained by the phase difference between the Fourier components of the two gratings. The phase can be controlled by laterally shifting one grating with respect to the other. Therefore, this relative shift provides an efficient "knob" that allows to control the interaction between the various modes, resulting in an efficient mo…
In this paper we study thermo-optical effects in gallium phosphite photonic crystal cavities in the visible. By measuring the shift of narrow resonances we derive the temperature dependency of the local refractive index of gallium phosphide in attoliter volumina over a temperature range between 5 K and 300 K at a wavelength of about 605 nm. Additionally, the potential of photonic crystal cavities for thermo-optical switching of visible light is investigated. As an example we demonstrate thermo-optical switching with 13 dB contrast.
We report on the first experimental demonstration that the microstructure based on a dielectric cuboid combined to a thin metal film can act as an efficient plasmonic lens allowing focusing surface plasmons in a subwavelength scale. By means of numerical simulation of surface plasmon-polariton (SPP) field intensity distributions in the microstructure, we observe a low divergence of plasmonic photonic jet (PPJ) and high intensity subwavelength spots at the communication wavelength of 1530 nm. Then we fabricate an experimental sample of the microstructure and study the SSP field intensity distri…
We demonstrate an approach, based on plasmonic apertures and gratings, to enhance the radiative decay rate of single NV centers in diamond, while simultaneously improving their collection efficiency. Our structures are based on metallic resonators formed by surrounding sub-wavelength diamond nanoposts with a silver film, which can enhance the spontaneous emission rate of an embedded NV center. However, the collection efficiency of emitted photons remains low due to losses to surface plasmons and reflections at the diamond-air interface. In this work, we mitigate photon losses into these channe…
Owing to their ability to concentrate light on nanometer scales, plasmonic surface structures are ideally suited for on-chip functionalization with nonlinear or gain materials. However, achieving a high effective quantum yield across a surface not only requires strong light localization but also control over losses. Here, we report on a particular class of tunable low-loss metasurfaces featuring dense arrangements of nanometer sized focal points on a photonic chip with an underlying waveguide channel. Guided within the plane, the photonic wave evanescently couples to the nano-gaps, concentrati…
We investigate the design, fabrication and experimental characterization of high Quality factor photonic crystal nanobeam cavities in silicon. Using a five-hole tapered 1D photonic crystal mirror and precise control of the cavity length, we designed cavities with theoretical Quality factors as high as 14 million. By detecting the cross-polarized resonantly scattered light from a normally incident laser beam, we measure a Quality factor of nearly 750,000. The effect of cavity size on mode frequency and Quality factor was simulated and then verified experimentally.
We measured a change in the current transport of an antenna-coupled, multi-gate, GaAs/AlGaAs field-effect transistor when terahertz electromagnetic waves irradiated the transistor and attribute the change to bolometric heating of the electrons in the two-dimensional electron channel. The observed terahertz absorption spectrum indicates coherence between plasmons excited under adjacent biased device gates. The experimental results agree quantitatively with a theoretical model we developed that is based on a generalized plasmonic transmission line formalism and describes an evolution of the plas…
We investigate optical parametric oscillations through four-wave mixing in resonant cavities and photonic crystals. The theoretical analysis underlines the relevant features of the phenomenon and the role of the density of states. Using fully vectorial 3D time-domain simulations, including both dispersion and nonlinear polarization, for the first time we address this process in a face centered cubic lattice and in a photonic crystal slab. The results lead the way to the development of novel parametric sources in isotropic media.
Over the last few years, optical nanoantennas are continuously attracting interest owing to their ability to efficiently confine, localize resonance, and significantly enhanced electromagnetic fields at subwavelength scale. However, such strong confinement can be further enhanced by using an appropriate combination of optical nanoantenna and Slanted Bound states in the continuum cavities. Here, we propose to synergistically bridge the plasmonic nanoantenna and high optical quality-factor cavities to numerically demonstrate three orders of magnitude local intensity enhancement. The proposed hyb…
We experimentally demonstrate high Quality factor dual-polarized TE-TM photonic crystal nanobeam cavities. The free-standing nanobeams are fabricated in a 500 nm thick silicon layer, and are probed using both tapered optical fiber and free-space resonant scattering set-ups. We measure Q-factors greater than 10^4 for both TM and TE modes, and observe large fiber transmission drops (0.3 -- 0.4) at the TM mode resonances.
We refute all claims of the "Comment on "Normalization of quasinormal modes in leaky optical cavities and plasmonic resonators" " by E. A. Muljarov and W. Langbein (arXiv:1602.07278v1). Based entirely on information already contained in our original article (P. T. Kristensen, R.-C. Ge and S. Hughes, Physical Review A 92, 053810 (2015)), we dismiss every point of criticism as being completely unjustified and point out how important parts of our argumentation appear to have been overlooked by the Comment Authors. In addition, we provide additional calculations showing directly the link between t…
We present the integrated chip-scale tuning of multiple photonic crystal cavities. The optimized implementation allows effective and precise tuning of multiple cavity resonances (up to ~1.60 nm/mW) and inter-cavity phase (~ 0.038 pi/mW) by direct local temperature tuning on silicon nanomembranes. Through designing the serpentine metal electrodes and careful electron-beam alignment to avoid cavity mode overlap, the coupled photonic crystal L3 cavities preserve their high quality factors. The deterministic resonance and phase control enables switching between the all-optical analogue of electrom…
One dimensional nanobeam photonic crystal cavities are fabricated in silicon dioxide with silicon nanocrystals. Quality factors of over 9 x 10^3 are found in experiment, matching theoretical predictions, with mode volumes of 1.5(lambda/n)^3 . Photoluminescence from the cavity modes is observed in the visible wavelength range 600-820 nm. Studies of the lossy characteristics of the cavities are conducted at varying temperatures and pump powers. Free carrier absorption effects are found to be significant at pump powers as low as a few hundred nanowatts.
Hybrid photonic-plasmonic cavities can be tailored to display high Q-factors and extremely small mode volumes simultaneously, which results in large values of the Purcell factor, FP. Amongst the different hybrid configurations, those based on a nanoparticle-on-a-mirror (NPoM) plasmonic cavity provide one of the lowest mode volumes, though so far their operation has been constrained to wavelengths below 1 μm. Here, we propose a hybrid configuration consisting of a silicon photonic crystal cavity with a slot at its center in which a gold nanoparticle is introduced. This hybrid system operates at…
We present design guidelines for realizing side-coupled photonic crystal nanobeam (PCN) cavities with efficient coupling to low order resonances through adjusting the overlap of the PCN cavity mode and a feeding bus waveguide in both physical and k-space. We show that optimal side-coupled configurations function at a non-zero k-vector offset between the bus waveguide and PCN cavity modes. The straightforward design of side-coupled PCNs with high contrast resonances opens the door to their practical implementation in multiplexed, on-chip photonic devices.
We present a simple one-pot co-assembly method for the synthesis of hierarchically structured pigment particles consisting of silica inverse-opal bricks that are doped with plasmonic absorbers. We study the interplay between the plasmonic and photonic resonances and their effect on the visual appearance of macroscopic collections of photonic bricks that are distributed in randomized orientations. Manipulating the pore geometry tunes the wavelength- and angle-dependence of the scattering profile, which can be engineered to produce angle-dependent Bragg resonances that can either enhance or cont…
Microcavity and whispering gallery mode (WGM) biosensors derive their sensitivity from monitoring frequency shifts induced by protein binding at sites of highly confined field intensities, where field strengths can be further amplified by excitation of plasmon resonances in nanoparticle layers. Here, we propose a mechanism based on optical trapping of a protein at the site of plasmonic field enhancements for achieving ultra sensitive detection in only microliter-scale sample volumes, and in real-time. We demonstrate femto-Molar sensitivity corresponding to a few 1000s of macromolecules. Simula…
We report the observation of optical bistability in Si-based photonic crystal cavities operating around 4.5 \mum. Time domain measurements indicate that the source of this optical bistability is thermal, with a time constant on the order of 5 \mus. Quality (Q) factor improvement is shown by the use of surface treatments (wet processes and annealing), resulting in an increase of Q-factor from 11,500 to 29,300 at 4.48 \mum. After annealing in a N2 environment, optical bistability is no longer seen in our cavities.
The loss of surface plasmon polaritons has long been considered as a fatal shortcoming in information transport. Here we propose a plasmonic absorber utilizing this "shortcoming" to absorb the stray light in photonic integrated circuits (PICs). Based on adiabatic mode evolution, its performance is insensitive to incident wavelength with bandwidth larger than 300nm, and robust against surrounding environment and temperature. Besides, the use of metal enables it to be very compact and beneficial to thermal dissipation. With this 40um-long absorber, the absorption efficiency can be over 99.8% at …
We demonstrate second harmonic generation in photonic crystal cavities in (001) and (111)B oriented GaAs. The fundamental resonance is at 1800 nm, leading to second harmonic below the GaAs bandgap. Below-bandgap operation minimizes absorption of the second harmonic and two photon absorption of the pump. Photonic crystal cavities were fabricated in both orientations at various in-plane rotations of the GaAs substrate. The rotation dependence and farfield patterns of the second harmonic match simulation. We observe similar maximum efficiencies of 1.2 %/W in (001) and (111)B oriented GaAs.
We demonstrate an add-drop filter based on a dual photonic crystal nanobeam cavity system that emulates the operation of a traveling-wave resonator and drops light on resonance to a single output port. Realized on an advanced SOI CMOS (IBM 45nm SOI) chip without any foundry process modifications, the device shows 16dB extinction in through port and 1dB loss in drop port with a 3dB bandwidth of 64GHz. To the best of our knowledge, this is the first implementation of a four-port add-drop filter based on photonic crystal nanobeam cavities.
We report temporal and spectral domain observation of regenerative oscillation in monolithic silicon heterostructured photonic crystals cavities with high quality factor to mode volume ratios (Q/V). The results are interpreted by nonlinear coupled mode theory (CMT) tracking the dynamics of photon, free carrier population and temperature variations. We experimentally demonstrate effective tuning of the radio frequency (RF) tones by laser-cavity detuning and laser power levels, confirmed by the CMT simulations with sensitive input parameters.
Photonic crystal point-defect cavities were fabricated in a GaN free-standing photonic crystal slab. The cavities are based on the popular L3 design, which was optimized using an automated process based on a genetic algorithm, in order to maximize the quality factor. Optical characterization of several individual cavity replicas resulted in an average unloaded quality factor Q = 16,900 at the resonant wavelength λ $\sim 1.3$ μm, with a maximal measured Q value of 22,500. The statistics of both the quality factor and the resonant wavelength are well explained by first-principles simulations inc…
We demonstrate a new photo-induced oxidation technique for tuning GaAs photonic crystal cavities using a $390~\mathrm{nm}$ pulsed laser with an average power of $10~\mathrm{μW}$. The laser oxidizes a small $\left(\sim 500~\mathrm{nm}\right)$ diameter spot, reducing the local index of refraction and blueshifting the cavity. The tuning progress can be actively monitored in real time. We also demonstrate tuning an individual cavity within a pair of proximity-coupled cavities, showing that this method can be used to correct undesired frequency shifts caused by fabrication imperfections in cavity a…
We have demonstrated what we believe to be the first waveguide photonic crystal cavity operating in the mid-infrared. The devices were fabricated from Ge23Sb7S70 chalcogenide glass on CaF2 substrates by combing photolithographic patterning and focus ion beam milling. The waveguide-coupled cavities were characterized using a fiber end fire coupling method at 5.2 μm wavelength, and a loaded quality factor of ~ 2,000 was measured near the critical coupling regime.
We propose a novel method to generate vector beams in planar photonic crystal cavities with multiple missing-hole defects. Simulating the resonant modes in the cavities, we observe that the optical fields in each defect have different phase and polarization state distributions, which promise the compositions of vector beams by the scattered light from the defects. The far-field radiation patterns of the cavity modes calculated via the Sommerfeld diffraction theory present vector beams possessing hollow intensity profiles and polarization singularities. In addition, the extraction efficiencies …
Crystal-symmetry-protected photonic topological edge states (PTESs) based on air rods in conventional dielectric materials are designed as photonic topological waveguides (PTWs) coupled with side optical cavities. We demonstrate that the cavity coupled with the PTW can change the reflection-free transport of the PTESs, where the cavities with single mode and twofold degenerate modes are taken as examples. The single-mode cavities are able to perfectly reflect the PTESs at their resonant frequencies, forming a dip in the transmission spectra. The dip full width at half depth depends on the coup…
We present the design of mid-infrared and THz quantum cascade laser cavities formed from planar photonic crystals with a complete in-plane photonic bandgap. The design is based on a honeycomb lattice, and achieves a full in-plane photonic gap for transverse-magnetic polarized light while preserving a connected pattern for efficient electrical injection. Candidate defects modes for lasing are identified. This lattice is then used as a model system to demonstrate a novel effect: under certain conditions - that are typically satisfied in the THz range - a complete photonic gap can be obtained by …
By modifying the density of optical states at the location of an emitter, weak cavity-emitter coupling can enable a host of potential applications in quantum optics, from the development of low- threshold lasers to brighter single-photon sources for quantum cryptography. Although some of the first demonstrations of spontaneous emission modification occurred in metallic structures, it was only after the recent demonstration of cavity quantum electrodynamics effects in dielectric optical cavities that metal-based optical cavities were considered for quantum optics applications. Advantages of met…
Recently, Kristensen, Ge and Hughes have compared [Phys. Rev. A 92, 053810 (2015)] three different methods for normalization of quasinormal modes in open optical systems, and concluded that they all provide the same result. We show here that this conclusion is incorrect and illustrate that the normalization of [Opt. Lett. 37, 1649 (2012)] is divergent for any optical mode having a finite quality factor, and that the Silver-Mueller radiation condition is not fulfilled for quasinormal modes.
Plasmon polaritons in van der Waals (vdW) materials hold promise for next-generation photonics. The ability to deterministically imprint spatial patterns of high carrier density in cavities and circuitry with nanoscale features underlies future progress in nonlinear nanophotonics and strong light-matter interactions. Here, we demonstrate a general strategy to atomically imprint low-loss graphene plasmonic structures using oxidation-activated charge transfer (OCT). We cover graphene with a monolayer of WSe$_2$, which is subsequently oxidized into high work-function WOx to activate charge transf…
