Photoluminescence from silicon dioxide photonic crystal cavities with embedded silicon nanocrystals

Plasmonic Enhancement of Emission from Si-nanocrystals

Plasmonic gratings of different periodicities are fabricated on top of Silicon nanocrystals embedded in Silicon Dioxide. Purcell enhancements of up to 2 were observed, which matches the value from simulations. Plasmonic enhancements are observed for the first three orders of the plasmonic modes, with the peak enhancement wavelength varying with the periodicity. Biharmonic gratings are also fabricated to extract the enhanced emission from the first order plasmonic mode, resulting in enhancements with quality factors of up to 16.

Spontaneous emission enhancement from polymer-embedded colloidal PbS nanocrystals into Si-based photonics at telecom wavelengths

We experimentally demonstrate the coupling of optically excited PbS nanocrystal (NC) photoluminescence (PL) into Si-based ring resonators and waveguides at 300K. The PbS NCs are dissolved into Novolak polymer at various concentrations and applied by drop-casting. The coupling mechanism and the spontaneous emission enhancement are experimentally investigated and compared to theoretical predictions. Quality (Q) factors of 2500 were obtained in emission and transmission for wavelengths centered around 1.45μm. PL intensity shows a linear dependence on the excitation power and no degradation of the…

Local field corrections to the spontaneous emission in arrays of Si nanocrystals

We present a theory of the local field corrections to the spontaneous emission rate for the array of silicon nanocrystals in silicon dioxide. An analytical result for the Purcell factor is obtained. We demonstrate that the local-field corrections are sensitive to the volume fill factor of the nanocrystals in the sample and are suppressed for large values of the fill factor. The local-field corrections and the photonic density of states are shown to be described by two different effective permittivities: the harmonic mean between the nanocrystal and the matrix permittivities and the Maxwell-Gar…

Whispering-gallery modes and light emission from a Si-nanocrystal-based single microdisk resonator

We report on visible light emission from Si-nanocrystal based optically active microdisk resonators. The room temperature photoluminescence (PL) from single microdisks shows the characteristic modal structure of whispering-gallery modes. The emission is both TE and TM-polarized in 300 nm thick microdisks, while thinner ones (135 nm) support only TE-like modes. Thinner disks have the advantage to filter out higher order radial mode families, allowing for measuring only the most intense first order modal structure. We reveal subnanometer linewidths and corresponding quality factors as high as 28…

Determination of the Surface Plasmons Polaritons extraction efficiency from a self-assembled plasmonic crystal

We experimentally measure and analytically describe the fluorescence enhancement obtained by depositing CdSe/CdS nanocrystals onto a gold plasmonic crystal, a two-dimensional grating of macroscopic size obtained by gold deposition on a self-assembled opal. We show evidences of nanocrystals near-field coupling to the gold Surface Plasmons Polaritons (SPP) followed by grating-induced SPP re-emission to far-field. We develop a theoretical framework and an original method in order to evaluate, from photoluminescence experiments, the SPP extraction efficiency of a grating.

Refractive index mediated plasmon hybridization in an array of aluminium nanoparticles

The arrangement of plasmonic nanoparticles in a non-symmetrical environment can feature the far-field and/or near-field interactions depending on the distance between the objects. In this work, we study the hybridization of three intrinsic plasmonic modes (dipolar, quadrupolar and hexapolar modes) sustained by one elliptical aluminium nanocylinder, as well as behavior of the hybridized modes when the nanoparticles are organized in array or when the refractive index of the surrounding medium is changed. The position and the intensity of these hybridized modes were shown to be affected by the ne…

25-nm diamond crystals hosting single NV color centers sorted by photon-correlation near-field microscopy

Diamond nanocrystals containing highly photoluminescent color centers are attractive non-classical and near-field light sources. For near-field applications the size of the nanocrystal is crucial since it defines the optical resolution. NV (Nitrogen-Vacancy) color centers are efficiently created by proton irradiation and annealing of a nanodiamond powder. Using near-field microscopy and photon statistics measurements, we show that nanodiamond with size down to 25 nm can hold a single NV color center with bright and stable photoluminescence.

MaPBI3 and 2D hybrid organic inorganic perovskite based microcavities employing periodic, aperiodic and disordered photonic structures and with the possibility of light-induced tuning

Inorganic-organic perovskites semiconductors are becoming increasingly interesting due to their remarkable optical properties, such as a high photoluminescence quantum yield and the possibility to show optical gain in a broad range of wavelengths. We have here simulated microcavities that embed MaPBI3 and 2D hybrid organic inorganic perovskite semiconductors by sandwiching such active layers between periodic, aperiodic and disordered photonic structures. We have carefully considered the refractive index dispersion of all the materials employed, such silicon dioxide, titanium dioxide and the pe…

Visible luminescence from hydrogenated amorphous silicon modified by femtosecond laser radiation

Visible luminescence is observed from the composite of SiO2 with embedded silicon nanocrystallites produced by femtosecond laser irradiation of hydrogenated amorphous silicon (a-Si:H) film in air. The photoluminescence originates from the defect states at the interface between silicon crystallites and SiO2 matrix. The method could be used for fabrication of luminescent layers to increase energy conversion of a-Si:H solar cells.

回音壁模式介导的量子点球形超粒子中光致发光的角分布模式

Angular Patterns of Photoluminescence in Quantum Dot Spherical Superparticles Mediated by Whispering-Gallery Modes

本文通过数值模拟研究CdS量子点超粒子的光致发光角分布，发现其发射具有后向不对称性，且回音壁模式激发可增强发射并降低不对称性，二氧化硅包覆可提高场谐振激发概率。

Influence of the magnetron power on the Er-related photoluminescence of AlN:Er films prepared by magnetron sputtering

The effect of magnetron power on the room temperature 1.54 $μ$m infra-red photoluminescence intensity of erbium doped AlN films grown by r. f. magnetron sputtering, has been studied. The AlN:Er thin films were deposited on (001) Silicon substrates. The study presents relative photoluminescence intensities of nanocrystallized samples prepared with identical sputtering parameters for two erbium doping levels (0.5 and 1.5 atomic %). The structural evolution of the crystallites as a function of the power is followed by transmission electron microscopy. Copyright line will be provided by the publis…

Transfer-printed quantum-dot nanolasers on a silicon photonic circuit

Quantum-dot (QD) nanolasers integrated on a silicon photonic circuit are demonstrated for the first time. QD nanolasers based on one-dimensional photonic crystal nanocavities containing InAs/GaAs QDs are integrated on CMOS-processed silicon waveguides cladded by silicon dioxide. We employed transfer-printing, whereby the three-dimensional stack of photonic nanostructures is assembled in a simple pick-and-place manner. Lasing operation and waveguide-coupling of an assembled single nanolaser are confirmed through micro-photoluminescence spectroscopy. Furthermore, by repetitive transfer-printing,…

Fabrication and characterization of high quality factor silicon nitride nanobeam cavities

Si3N4 is an excellent material for applications of nanophotonics at visible wavelengths due to its wide bandgap and moderately large refractive index (n $\approx$ 2.0). We present the fabrication and characterization of Si3N4 photonic crystal nanobeam cavities for coupling to diamond nanocrystals and Nitrogen-Vacancy centers in a cavity QED system. Confocal micro-photoluminescence analysis of the nanobeam cavities demonstrates quality factors up to Q ~ 55,000, which is limited by the resolution of our spectrometer. We also demonstrate coarse tuning of cavity resonances across the 600-700nm ran…