这项工作提出了准确的{ \it ab initio}调查的各种光谱性质的几个锂离子在德拜屏蔽电位内的等离子体环境的存在。在相对论框架下用耦合团簇理论计算了类锂C $^{3+}$、N $^{4+}$和O $^{5+}$离子的电离势、激发能、电偶极振子强度和电四极跃迁几率.为了提高计算的准确性，采用了非延迟Breit相互作用。研究了等离子体环境中离子密度和温度对电离势、激发能、电偶极振子强度和电四极跃迁几率的影响。结果表明，随着屏蔽强度的增加，等离子体屏蔽导致电离势急剧下降。随着强度的增加，与2个$s ^{2}S_{1/2}$ $\rightarrow2 p ^{2}P_{1/2, 3/2}$跃迁相关的振子强度增加，而与3个$d ^2D_{3/2, 5/2}$ $\rightarrow2 s ^2S_{1/2}$跃迁相关的跃迁概率减小。
英文摘要：
This work presents accurate {\it ab initio} investigations of various spectroscopic properties of a few Li-like ions in presence of a plasma environment within the Debye screening potential. The coupled-cluster theory in the relativistic framework has been employed to compute ionization potentials, excitation energies, electric dipole oscillator strengths, and electric quadrupole transition probabilities of Li-like C$^{3+}$, N$^{4+}$, and O$^{5+}$ ions. The unretarded Breit interaction has been implemented to increase the accuracy of the calculations. The effects of ion density and temperature on the ionization potentials, excitation energies, electric dipole oscillator strengths, and electric quadrupole transition probabilities have been investigated in the plasma environment. It is found that the plasma screening leads to a sharp decrease in the ionization potential as the screening strength increases. With increasing strength, the oscillator strengths associated with 2$s ^{2}S_{1/2}$$\rightarrow2 p ^{2}P_{1/2, 3/2}$ transitions increase, whereas the transition probabilities associated with 3$d ^2D_{3/2, 5/2}$$\rightarrow2 s ^2S_{1/2}$ transitions decrease.
We report an investigation of the self-energy screening effects for the $g$ factor of the ground state of Li-like ions. The leading screening contribution of the relative order $1/Z$ is calculated to all orders in the binding nuclear strength parameter $Zα$ (where $Z$ is the nuclear charge number and $α$ is the fine-structure constant). We also extend the known results for the $Zα$ expansion of the QED screening correction by deriving the leading logarithmic contribution of order $α^5\lnα$ and obtaining approximate results for the $α^5$ and $α^6$ contributions. The comparison of the two approa…
Spectroscopic properties of the molecular ions BeX^+ (X=Na, K, Rb): Forming cold molecular ions from an ion-atom mixture by stimulated Raman adiabatic process
Atomic properties of $n=3$ states of the W$^{56+}$ $-$ W$^{61+}$ ions are systematically investigated through two state-of-the-art methods, namely, the second-order many-body perturbation theory, and the multi-configuration Dirac-Hartree-Fock method combined with the relativistic configuration interaction approach. The contributions of valence-valence and core-valence electron correlations, the Breit interaction, the higher-order retardation correction beyond the Breit interaction through the transverse photon interaction, and the quantum electrodynamical corrections to the excitation energies…
We present high-accuracy spectroscopy data of line strengths, transition probabilities and oscillator strengths for the allowed transitions among the $nS_{1/2}$, $nP_{1/2,3/2}$ and $n'D_{3/2,5/2}$ states with $n=5$ to $10$ and $n'=4$ to $10$ of the Rb-isoelectronic Zr (Zr IV) and Nb (Nb V) ions. %\textcolor{red}{except for a few transitions that seem to be unreliable.} They can serve to analyse various astrophysical phenomena undergoing inside the heavenly bodies containing Zr and Nb elements. Since there is a lack of precise observational and calculated data for the spectroscopic properties i…
Using the multiconfiguration Dirac-Hartree-Fock and the relativistic configuration interaction methods, a consistent set of transition energies and radiative transition data for the main states of the $2s^2 2p^4$, $2s 2p^5$, $2p^6$, $2s^2 2p^3 3s$, $2s^2 2p^3 3p$, $2s^2 2p^3 3d$, $2s 2p^4 3s$, $2s 2p^4 3p$, and $2s 2p^4 3d$ configurations in O-like Ions between Ar XI ($Z = 18$) and Cr XVII ($Z = 24$) is provided. Our data set is compared with the NIST compiled values and previous calculations. The data are accurate enough for identification and deblending of new emission lines from hot astroph…
Recent advances in quantum technologies have enabled the precise control of single trapped molecules on the quantum level. Exploring the scope of these new technologies, we studied theoretically the implementation of qubits and clock transitions in the spin, rotational, and vibrational degrees of freedom of molecular nitrogen ions including the effects of magnetic fields. The relevant spectroscopic transitions span six orders of magnitude in frequency illustrating the versatility of the molecular spectrum for encoding quantum information. We identified two types of magnetically insensitive qub…
Extended relativistic configuration interaction and many-body perturbation calculations of spectroscopic data for the $n \leq 6$ configurationsin ne-like ions between Cr XV and Kr XXVII
In this paper we study the influence of electron screening on the Bohr-Weisskopf (BW) effect in many-electron atoms. The BW effect gives the finite-nucleus magnetization contribution to the hyperfine structure. Relativistic atomic many-body calculations are performed for s and p_1/2 states of several systems of interest for studies of atomic parity violation and time-reversal-violating electric dipole moments -- Rb, Cs, Fr, Ba+, Ra+, and Tl. For s states, electron screening effects are small, and the relative BW correction for hydrogenlike ions and neutral atoms is approximately the same. We r…
Hyperfine-structures of highly charged ions (HCIs) are favourable spectroscopic targets for exploring fundamental physics as well as nuclear properties. Recent proposals of HCI atomic clocks highlight their importance, especially for many-electron HCIs, and they have been theoretically investigated by refining atomic-structure calculations. Nonetheless, no established spectroscopic method is currently available to verify these theoretical calculations. Here, we demonstrate hyperfine-structure-resolved laser spectroscopy of HCIs in an electron beam ion trap plasma, employing the magnetic-dipole…
Radiative and interelectronic-interaction corrections to the hyperfine splitting in highly charged B-like ions
The ground-state hyperfine splitting values of high-Z boronlike ions are calculated. Calculation of the interelectronic-interaction contribution is based on a combination of the 1/Z perturbation theory and the large-scale configuration-interaction Dirac-Fock-Sturm method. The screened QED corrections are evaluated utilizing an effective screening potential approach. Total hyperfine splitting energies are presented for several B-like ions of particular interest: {}^{45}Sc{}^{16+}, {}^{57}Fe{}^{21+}, {}^{207}Pb{}^{77+}, and {}^{209}Bi{}^{78+}. For lead and bismuth the experimental values of the …
X-ray emission K-spectra of highly charged He- and Li-like argon ions recorded with high spectral, spatial, and temporal resolution at the TEXTOR tokamak were employed to develop a self-consistent approach (SCA) for deriving information on plasma parameters and the verification (estimation of accuracy) of both atomic data, needed for spectra interpretation, and methods of their calculation. The approach is based on solving the spectral inverse problem for these spectra in the framework of the semi-empirical ``spectroscopic model'' (SM) by means of two complimentary inversion methods. The SCA w…
$g$ factor of the $2p_j$ excited states in lithium-like ions
St. Petersburg State University（圣彼得堡国立大学）；ITMO University（伊托莫大学）；Petersburg Nuclear Physics Institute named by B. P. Konstantinov of National Research Centre “Kurchatov Institute”（库尔恰托夫国家研究中心鲍·波·康斯坦丁诺夫彼得堡核物理研究所）
Plasma environment effects on K lines of astrophysical interest. II. Ionization potentials, K thresholds, radiative rates and Auger widths in Ne- through He-like iron ions (Fe xvii - Fe xxv)
目的。在黑洞周围的吸积盘的背景下，我们估计等离子体环境的原子参数的影响与高电荷铁离子，即Fe xvii - Fe xxv的K-空位状态的衰变。方法.在相对论多组态Dirac-Fock（MCDF）框架下，电子-核和电子-电子等离子体屏蔽近似为时间平均Debye-Huckel势。结果本文报道了电子温度和密度分别在1 E5 - 1 E7 K和1 E18 - 1 E22 cm-3范围内的天体物理等离子体的修正电离势、K阈值、波长、辐射发射率和俄歇宽度。结论.我们的结论是，高分辨率的微量热仪机载未来的X射线任务，如XRISM和ATHENA预计将是敏感的铁K边缘的降低，由于极端的等离子体条件下发生在紧凑的物体周围的吸积盘。
A recently proposed classical-trajectory dynamical screening model for the description of multiple ionization and capture during ion-water molecule collisions is extended to incorporate dynamical screening on both the multi-center target potential and the projectile ion. Comparison with available experimental data for He$^{2+}$ + H$_2$O collisions at intermediate energies (10-150 keV/u) and Li$^{3+}$ + H$_2$O at higher energies (100-850 keV/u) demonstrates the importance of both screening mechanisms. The question of how to deal with the repartitioning of the capture flux into allowed capture c…
We present precise radiative data of line strengths, transition probabilities and oscillator strengths for the allowed transitions among the $nS_{1/2}$, $nP_{1/2,3/2}$, $n'D_{3/2,5/2}$ and $n'F_{5/2,7/2}$ states with $n=4$ to $6$ and $n'=4,5$ of the Cu-isoelectronic As, Se and Br ions. Due to unavailability of precise observations of these spectroscopic data, their accurate estimations are of great interest and useful in analyzing various astrophysical phenomena undergoing inside the heavenly bodies that contain As, Se and Br elements. An all-order perturbative many-body method in the relativi…
The Gamma Factory (GF) initiative aims at the construction of a unique experimental tool exploiting resonant interaction of light with ultra-relativistic partially stripped ions (PSI) stored in circular accelerators at CERN. Resonant excitation of high-energy electronic transitions in the ions is achieved through Doppler-boosting (by twice the Lorentz factor; from hundred to several thousand times) of light energy. In order to efficiently excite the ions, and hence generate intense beams of scattered/fluorescent photons, a detailed knowledge of the ions' electronic energy structure and the dyn…
