Collinear phase-matched optical rectification is studied in ZnGeP$_{2}$ pumped with near-infrared light. The pump-intensity dependence is presented for three crystal lengths (0.3, 1.0 and 3.0 mm) to determine the effects of linear optical absorption, nonlinear optical absorption and terahertz free-carrier absorption on the generation. Critical parameters such as the coherence length (for velocity matching), dispersion length (for linear pulse broadening) and nonlinear length (for self-phase modulation) are determined for this material. These parameters provide insight into the upper limit of pulse intensity and crystal length required to generate intense terahertz pulse without detriment to the pulse shape. It is found that for 1-mm thick ZnGeP$_{2}$(012), pumped at 1.28 micron with intensity of ~15 GW/cm2 will produce intense undistorted pulses, whereas longer crystals or larger intensities modify the pulse shape to varying degrees. Moreover, phase-matching dispersion maps are presented for the terahertz generation over a large tuning range (1.1-2.4 micron) in longer (3 mm) crystal, demonstrating the phase-matching bandwidth and phase mismatch that leads to fringing associated with multi-pulse interference. All observed results are simulated numerically showing good qualitative agreement.
We experimentally demonstrate intensity and phase modulation of terahertz radiation using actively controlled large-area planar metamaterial (metafilm) hybridized with a 12 um thick layer of a liquid crystal. Active control was introduced through in-plane electrical switching of the liquid crystal, which enabled us to achieve a reversible single-pass absolute transmission change of 20 % and a phase change of 40 deg at only 20 V.
The two-color strong-field mixing in gas medium is a widely-used approach to generate bright broadband terahertz (THz) radiation. Here, we present a new and counterintuitive method to promote THz performance in two-color scheme. Beyond our knowledge that the maximum THz generation occurs with two-color foci overlapped, we found that, when the foci of two-color beams are noticeably separated along the propagation axis resulting in cascading plasmas, the THz conversion efficiency is surged by one order of magnitude and the bandwidth is stretched by more than 2 times, achieving $10^{-3}$ conversi…
We report on the first direct measurement of the emission character of quantum cascade laser based frequency combs, using intensity autocorrelation. The correlation technique is based on fast electro-optic sampling, with a bandwidth optimized to match the emission spectra of the comb laser, centered around 2.5~THz. We find the output light to be amplitude and frequency modulated at the same time, with intensity modulation depth as high as 90\%, occuring on timescales as short as few picoseconds. We compare these findings with intensity autocorrelation measurements of pulsed Terahertz light ori…
It is shown that optical synthesis of terahertz and millimeter-wave frequencies can be achieved using two-mode and mode-locked discrete mode diode lasers. These edge-emitting devices incorporate a spatially varying refractive index profile which is designed according to the spectral output desired of the laser. We first demonstrate a device which supports two primary modes simultaneously with high spectral purity. In this case sinusoidal modulation of the optical intensity at terahertz frequencies can be obtained. Cross saturation of the material gain in quantum well lasers prevents simultaneo…
Although Gigahertz-scale free-carrier modulators have been previously demonstrated in silicon, intensity modulators operating at Terahertz speeds have not been reported because of silicon's weak ultrafast optical nonlinearity. We have demonstrated intensity modulation of light with light in a silicon-polymer integrated waveguide device, based on the all-optical Kerr effect - the same ultrafast effect used in four-wave mixing. Direct measurements of time-domain intensity modulation are made at speeds of 10 GHz. We showed experimentally that the ultrafast mechanism of this modulation functions a…
A tilted-pulse-front pumped terahertz pulse source is proposed for the generation of extremely high field single-cycle terahertz pulses. The very simple and compact source consists of a single crystal slab having a blazed reflection grating grooved in its back surface. Its further important advantages are the energy scalability and the symmetric THz beam profile. Generation of 50 MV/cm focused field with 5.6 mJ terahertz pulse energy is predicted for a 5 cm diameter LiNbO$_3$ crystal, if the pump pulse is of 450 mJ energy, 1030 nm central wavelength and 1 ps pulse duration. Such sources can ba…
Ultrashort electron bunches are useful for applications like ultrafast imaging and coherent radiation production. Currently, however, the shortest achievable bunches, at attosecond time scales, have only been realized in the single or very few electron regime, limited by Coulomb repulsion and electron energy spread. Using ab initio simulations and theoretical analysis, we show that highly-charged bunches are achievable by subjecting relativistic (few MeV-scale) electrons to a superposition of terahertz and optical pulses. Using realistic electron bunches and laser pulse parameters which are wi…
The gain recovery time of a heterogeneous active region terahertz quantum cascade laser is studied by terahertz-pump,i terahertz-probe spectroscopy. The investigated active region, which is based on a bound-to-continuum optical transition with an optical phonon assisted extraction, exhibits a gain recovery time in the range of 34$\,$-$\,$50$\,$ps dependent on the operation condition of the laser. The recovery time gets shorter for stronger pumping of the laser while the recovery dynamics slows down with increasing operation temperature. These results indicate the important role of the intracav…
Driving a double-quantum-well excitonic intersubband resonance with a terahertz (THz) electric field of frequency ω_{THz} generated terahertz optical sidebands ω=ω_{THz}+ω_{NIR} on a weak NIR probe. At high THz intensities, the intersubband dipole energy which coupled two excitons was comparable to the THz photon energy. In this strong-field regime the sideband intensity displayed a non-monotonic dependence on the THz field strength. The oscillating refractive index which gives rise to the sidebands may be understood by the formation of Floquet states, which oscillate with the same periodicity…
The Terahertz frequency range bears intriguing opportunities, beyond very advanced applications in spectroscopy and matter control. Peculiar quantum phenomena are predicted to lead to light emission by non-trivial mechanisms. Typically, such emission mechanisms are unraveled by temporal correlation measurements of photon arrival times, as demonstrated in their pioneering work by Hanbury Brown and Twiss. So far, the Terahertz range misses an experimental implementation of such technique with very good temporal properties and high sensitivity. In this paper, we propose a room-temperature scheme …
We report an integrated all-optical radio frequency spectrum analyzer based on a ~ 4cm long doped silica glass waveguide, with a bandwidth greater than 2.5 THz. We use this device to characterize the intensity power spectrum of ultrahigh repetition rate mode-locked lasers at repetition rates up to 400 GHz, and observe dynamic noise related behavior not observable with other techniques.
Nonlinear frequency conversion provides an elegant method to detect photons in a spectral range which differs from the pump wavelength, making it highly attractive for photons with inherently low energy. Aside from the intensity of the light, represented by the number of photons, their phase provides important information and enables a plethora of applications. We present a phase-sensitive measurement method in the terahertz spectral range by only detecting visible light. Using the optical interference of frequency-converted photons and leftover pump photons of the involved ultrashort pulses, …
We propose the use of a silicon-core optical fiber for terahertz (THz) waveguide applications. Finite-difference time-domain simulations have been performed based on a cylindrical waveguide with a silicon core and silica cladding. High-resistivity silicon has a flat dispersion over a 0.1 - 3 THz range, making it viable for propagation of tunable narrowband CW THz and possibly broadband picosecond pules of THz radiation. Simulations show the propagation dynamics and the integrated intensity, from which transverse mode profiles and absorption lengths are extraced. It is found that for 140 - 250 …
Scattering-assisted synthesis of broadband optical pulses is recognized to have a cross-disciplinary funda-mental and application importance. Achieving full-waveform synthesis generally requires means for assessing the instantaneous electric field, i.e. the absolute electromagnetic phase. These are generally not accessible to established methodologies for scattering-assisted pulse envelope and phase shaping. The lack of field sensitivity also results in complex indirect approaches to evaluate the scattering space-time properties. The terahertz frequency domain potentially offers some distincti…
We report here on terahertz (THz) digital holography on a biological specimen. A continuous-wave (CW) THz in-line holographic setup was built based on a 2.52 THz CO2 pumped THz laser and a pyroelectric array detector. We introduced novel statistical method of obtaining true intensity values for the pyroelectric array detector's pixels. Absorption and phase-shifting images of a dragonfly's hind wing were reconstructed simultaneously from single in-line hologram. Furthermore, we applied phase retrieval routines to eliminate twin image and enhanced the resolution of the reconstructions by hologra…
Metallic structures with periodic array of slits are well-known to lead to extraordinary power transmission, when slits have dimensions much less than the wavelength of incident optical wave. Excellent power transmission originates from surface waves excited by incident transverse magnetic wave. Here we show that metallic structure with array of stepped-slits can transmit power of incident wave into the substrate at desired optical frequency entirely and simultaneously in terahertz frequency band by 70%, for In0.53Ga0.47As substrate. Transmitted power of the proposed structure is studied both …
We investigate the generation of broadband terahertz (THz) pulses with phase singularity from air plasmas created by fundamental and second harmonic laser pulses. We show that when the second harmonic beam carries a vortex charge, the THz beam acquires a vortex structure as well. A generic feature of such THz vortex is that the intensity is modulated along the azimuthal angle, which can be attributed to the spatially varying relative phase difference between the two pump harmonics. Fully space and time resolved numerical simulations reveal that transverse instabilities of the pump further affe…
We demonstrate a compact source of energetic and phase-locked multi-terahertz pulses at a repetition rate of 190 kHz. Difference frequency mixing of the fundamental output of an Yb:KGW amplifier with the idler of an optical parametric amplifier in GaSe and LiGaS2 crystals yields a passively phase-locked train of waveforms tunable between 12 and 42 THz. The shortest multi-terahertz pulses contain 1.8 oscillation cycles within the intensity FWHM. Pulse energies of up to 0.16 μJ and peak electric fields of 13 MV/cm are achieved. Electro-optic sampling reveals a phase stability better than 0.1 $π$…
Hyperspectral imaging is a technique that allows for the creation of multi-color images. At terahertz wavelengths, it has emerged as a prominent tool for a number of applications, ranging from non-ionizing cancer diagnosis and pharmaceutical characterization to non-destructive artifact testing. Contemporary terahertz imaging systems typically rely on non-linear optical down-conversion of a fiber-based near-infrared femtosecond laser, requiring complex optical systems. Here, we demonstrate hyperspectral imaging with chip-scale frequency combs based on terahertz quantum cascade lasers. The dual …
A highly superlinear in radiation intensity photoconductance induced by terahertz laser radiation with moderate intensities has been observed in quantum point contacts made of GaAs quantum wells operating in the deep tunneling regime. For very low values of the normalized dark conductance $G_{\rm dark}/ G_0 \approx 10^{-6}$, with the conductance quantum $G_0=2e^2/h$, the photoconductance scales exponentially with the radiation intensity, so that already at $ 100 \text{ mW}/\text{cm}^2$ it increases by almost four orders of magnitude. This effect is observed for a radiation electric field orien…
We report on a waveguide engineering technique that enables the generation of a bandwidth up to 1 THz and record ultra-short pulse length of 2.5 ps in injection seeded terahertz quantum cascade lasers. The reported technique is able to control and fully suppress higher order lateral modes in broadband terahertz quantum cascade lasers by introducing side-absorbers to metal-metal waveguides. The side-absorbers consist of a top metalization set-back with respect to the laser ridge and an additional lossy metal layer. In continuous wave operation the side-absorbers lead to octave spanning laser em…
We report enhanced broadband Terahertz (THz) generation and detailed characterization from the interaction of femtosecond two colour laser pulses with thin transparent dielectric tape target in ambient air. The proposed source is easy to implement, exhibits excellent scalability with laser energy. Spectral characterization using Fourier transform spectrometer reveals yield enhancement of more than 150 % in the THz region of 0.1 - 10 THz with respect to conventional two-colour laser plasma source in ambient air. Further, the source spectrum extends up to 40 THz with an enhancement of flux > 30 …
We systematically investigate the influence of annealing effect on terahertz (THz) generation from CoFeB based magnetic nanofilms driven by femtosecond laser pulses. Three times enhancement of THz yields are achieved in W/CoFeB through annealing effect, and double boosting is obtained in Pt/CoFeB. The mechanism of annealing effect originates from the increase of hot electron mean free path induced by crystallization, which is experimentally corroborated by THz transmission measurement on time-domain spectroscopy. Comparison studies of the thickness dependent THz efficiency after annealing are …
We propose a method to generate isolated relativistic terahertz (THz) pulses using a high-power laser irradiating a mirco-plasma-waveguide (MPW). When the laser pulse enters the MPW, high-charge electron bunches are produced and accelerated to ~ 100 MeV by the transverse magnetic modes. A substantial part of the electron energy is transferred to THz emission through coherent diffraction radiation as the electron bunches exit the MPW. We demonstrate this process with three-dimensional particle-in-cell simulations. The frequency of the radiation is determined by the incident laser duration, and …
Free-space super-strong terahertz (THz) electromagnetic fields offer multifaceted capabilities for reaching extreme nonlinear THz optics, accelerating and manipulating charged particles, and realizing other fascinating applications. However, the lack of powerful solid-state THz sources with single pulse energy >1 mJ is impeding the proliferation of extreme THz applications. The fundamental challenge lies in hard to achieve high efficiency due to high intensity pumping caused crystal damage, linear absorption and nonlinear distortion induced short effective interaction length, and so on. Here, …
Highly efficient terahertz (THz) wave sources based on difference frequency generation (DFG) process in nonlinear optical crystals play an important role for the applications of THz wave. In order to find more novel nonlinear crystals, here we theoretically investigate the generation of THz wave using the isomorphs of periodically poled $\mathrm{KTiOPO_4}$ (PPKTP), including periodically poled RTP, KTA, RTA and CTA. By solving the cascaded difference frequency coupled wave equations, it is found that the intensities of the THz wave generated from the cascaded difference frequency processes are…
We report a plasma-based strong THz source generated by using intense femtosecond laser pulses to irradiate solid targets at relativistic intensity >10^18W/cm2. Energies up to 50 microJ/sr per THz pulse is observed in the specular direction when the laser pulses are incident onto a copper foil at 67.5 degree. The source appears to be linearly polarized. The temporal, spectral properties of the THz are measured by a single shot, electro-optic sampling method with a chirped laser pulse. The THz radiation is attributed to the self-organized transient fast electron currents formed along the target…
In recent years, a range of reconfigurable metamaterials controlled with thermal, electric, magnetic and optical signals have been developed for dynamically manipulating the intensity, phase and wave-front of electromagnetic radiation across the broad electromagnetic spectrum ranging from microwave to optics. Here for the first time, we demonstrate a reconfigurable metasurface performing exclusive OR (XOR) logical operation using two independent control electrical inputs and an optical read-out in the form of far-field Fano intensity states at terahertz wavelengths. At the same time, the near …
All-photonic W-band terahertz receiver based on THz-to-optical carrier conversion with soliton microcomb dual carriers for high-speed OOK wireless transmission
Graduate School of Sciences and Technology for Innovation, Tokushima University（德岛大学科学技术研究生院）；Institute of Post-LED Photonics (pLED), Tokushima University（德岛大学后LED光子学研究所）；Institute of Photonics and Human Health Frontier (IPHF), Tokushima University（德岛大学光子学与人类健康前沿研究所）；Center for Higher Education and Digital Transformation, University of Yamanashi（山梨大学高等教育与数字化转型中心）；National Institute of Information and Communications Technology（信息通信技术研究所）；Department of Electrical, Electronic and Computer Engineering, Gifu University（岐阜大学电气电子计算机工程系）；Department of Electrical and Mechanical Engineering, Nagoya Institute of Technology（名古屋工业大学电气机械工程系）
We report on an asymmetric high energy dual optical parametric amplifier (OPA) which is capable of having either the idlers, signals, or depleted pumps, relatively phase locked at commensurate or incommensurate wavelengths. Idlers and signals can be locked on the order of 200 mrad rms or better, corresponding to a 212 as jitter at $λ$=2$μ$m. The high energy arm of the OPA outputs a combined 3.5 mJ of signal and idler, while the low energy arm outputs 1.5 mJ, with the entire system being pumped with a 1 kHz, 18 mJ Ti:Sapphire laser. Both arms are independently tunable from 1080 nm-2600 nm. The …
We report on a reflective wave-plate system utilizing phase-shifting mirrors (PSM) for a continuous variation of elliptical polarization without changing the beam position and direction. The scalability of multilayer optics to large apertures and the suitability for high-intensity broad-bandwidth laser beams make reflective wave-plates an ideal tool for experiments on relativistic laser-plasma interaction. Our measurements confirm the preservation of the pulse duration and spectrum when a 30-fs Ti:Sapphire laser beam passes the system.
The conventional lens's tunability drawback always restricts their application compared to the metasurface lens (metalens). On the other side, reconfigurable metalenses offer the benefits of ultrathin thickness and capable of tunability. Therefore achieving reconfigurable functionalities in a single metasurface has attracted significant research interest for potential terahertz (THz) applications. In this paper, an adjustable metasurface is presented using Vanadium dioxide (VO2) to manipulate the electromagnetic waves and provide the full reflection phase. The phase-change metasurface is compo…
Spintronic terahertz (THz) emitter provides the advantages such as apparently broader spectrum, significantly lower cost, and more flexibility in compared with the commercial THz emitters, and thus attracts great interests recently. In past few years, efforts have been made in optimizing the material composition and structure geometry, and the conversion efficiency has been improved close to that of ZnTe crystal. One of the drawbacks of the current designs is the rather limited laser absorption - more than 50% energy is wasted and the conversion efficiency is thus limited. Here, we theoretical…
