We report enhanced broadband Terahertz (THz) generation and detailed characterization from the interaction of femtosecond two colour laser pulses with thin transparent dielectric tape target in ambient air. The proposed source is easy to implement, exhibits excellent scalability with laser energy. Spectral characterization using Fourier transform spectrometer reveals yield enhancement of more than 150 % in the THz region of 0.1 - 10 THz with respect to conventional two-colour laser plasma source in ambient air. Further, the source spectrum extends up to 40 THz with an enhancement of flux > 30 %. Experimental results, well supported with two-dimensional particle-in-cell simulations establishes that the transient photo-current produced by the asymmetric laser pulse interaction with air plasma as well as near solid density plasma formed on the tape surface is responsible for the enhanced terahertz generation. The source will be useful for the multidisciplinary activities and ongoing applications of the laboratory-based terahertz sources.
A novel terahertz hybrid waveguide chip consisting of silicon photonic crystals sandwiched in parallel gold plates is developed. Both simulation and experimental results demonstrate that the hybrid waveguide offers a wide single-mode transmission window with low group velocity dispersion and low loss. This compact, substrate-free terahertz chip would play a significant role in broadband, dense-integrated, multi-functional terahertz systems.
Flexible manipulation of terahertz-wave polarization during the generation process is very important for terahertz applications, especially for the next-generation on-chip functional terahertz sources. However, current terahertz emitters could not satisfy such demand, hence calling for new mechanism and conceptually new terahertz source. Here we demonstrate a magnetic-field-controlled, highly-efficient, cost-effective, and broadband terahertz source with flexible switch of terahertz polarization states in ferromagnetic heterostructures driven by femtosecond laser pulses. We verify that the chi…
The nonlinear metamaterials have been shown to provide nonlinear properties with high nonlinear conversion efficiency and in a myriad of light manipulation. Here we study terahertz generation from nonlinear metasurface consisting of single layer nanoscale split-ring resonator array. The terahertz generation due to optical rectification by the second-order nonlinearity of the split-ring resonator is investigated by a time-domain implementation of the hydrodynamic model for electron dynamics in metal. The results show that the nonlinear metasurface enables us to generate broadband terahertz radi…
We introduce a general technique to generate compressed broadband terahertz pulses based on difference frequency generation of optical pump radiation using aperiodically poled structures. The pump pulse format and poling of the crystals conceived are such that the emergent terahertz pulse is compressed. The approach circumvents pump pulse distortions that result from non-collinear approaches and the need for external compression. It is particularly efficient for the generation of pulses of intermediate durations of few to tens of cycles. For instance, conversion efficiencies in the few percent…
We investigate terahertz emission from two-color fs-laser-induced microplasmas. Under strongest focusing conditions, microplasmas are shown to act as point-sources for broadband terahertz-to-far-infrared radiation, where the emission bandwidth is determined by the plasma density. Semi-analytical modeling allows us to identify scaling laws with respect to important laser parameters. In particular, we find that the optical-to-THz conversion efficiency crucially depends on the focusing conditions. We use this insight to demonstrate by means of Maxwell-consistent 3D simulations, that for only 10-$…
High absorption in a wide frequency band has attracted considerable interest since their potential applications in frequency spectrum imaging systems and anti-radar cloaking. In this paper, a polarization-independent, ultra-broadband and omnidirectional terahertz absorber is proposed, fabricated and evaluated. It is experimentally demonstrated that an over 95% absorption can be obtained in the frequency range of 0.75~2.41 THz. Attributing to the multi-frequency destructive interference between the layers and the impedance-matching condition of the grating, five successive absorption peaks at 0…
We present a monolithic solution to extract efficiently light from terahertz quantum cascade lasers with metal-metal waveguides suitable for broadband frequency comb applications. The design is optimized for a bandwidth of 500 GHz around a center frequency of 2.6 THz. A five-fold increase in total output power is observed compared to standard metal-metal waveguides. The extractor features a single-lobed far-field pattern and increases the frequency comb dynamical range to cover more than 50 % of the laser dynamic range. Frequency comb operation up to a spectral bandwidth of 670 GHz is achieved…
The intense terahertz (THz) pulses facilitate the observation of various nonlinear optical effects and manipulation of material properties. In this work, we report a convenient approach that can produce strong broadband terahertz pulses with center frequency tunable between 2-4 THz. The coherent THz light source with pulse energy of 1.2 microjoule can be generated from a low-cost crystalline quartz pumped by an ultrashort tilted wave-front pulse. Thanks to the wide transparent spectral window and high damage threshold, our theoretical analysis and experiment show that the optical rectification…
A novel broadband technique to effectively launch plasmons along a single graphene layer at terahertz (THz) frequencies is proposed. To this end, the coupling of the electromagnetic wave from a readily available plasmonic waveguide established by a periodically corrugated metallic surface to the graphene sheet is proposed. As will be shown, this technique can significantly surmount the need for efficient excitation of plasmons in graphene. For this purpose, an analytical technique based on transmission line theory is employed to calculate the scattering parameters of the connection of the plas…
We report a simple single-pixel imaging system with a low mean squared error in the entire terahertz frequency region (3-13 THz) that employs a thin metallic ring with a series of directly perforated random masks and a subpixel mask digitization technique. This imaging system produces high pixel resolution reconstructed images, up to 1200 x 1200 pixels, and imaging area of 32 mm x 32 mm. It can be extended to develop advanced imaging systems in the near-ultraviolet to terahertz region.
A nearly omni-directional THz absorber for both transverse electric (TE) and transverse magnetic (TM) polarizations is proposed. Through the excitation of magnetic polariton in a metal-dielectric layer, the incident light is perfectly absorbed in a thin thickness which is about 25 times smaller than the resonance wavelength. By simply stacking several such structural layers with different geometrical dimensions, the bandwidth of this strong absorption can be effectively enhanced due to the hybridization of magnetic polaritons in different layers.
We report on a giant Faraday effect in an electron plasma in n-InSb probed via polarization-resolved terahertz (THz) time-domain spectroscopy. Polarization rotation angles and ellipticities reach as large as π/2 and 1, respectively, over a wide frequency range (0.3-2.5 THz) at magnetic fields of a few Tesla. The experimental results together with theoretical simulations show its promising ability to construct broadband and tunable THz polarization optics, such as a circular polarizer, half-wave plate, and polarization modulators.
We present an antipodal Vivaldi antenna for broadband double metal waveguide terahertz quantum cascade lasers and frequency combs. Its exponentially curved flare profile results in an adiabatic in-plane mode expansion, producing an improved far-field with a single-lobed beam of (23°x19°) full width half maximum with an octave-spanning bandwidth. The antenna also acts as a wave retarder, rotating the polarization from vertical toward horizontal polarization by a frequency-dependent angle. The laser's emission spectrum and current-voltage characteristics are not affected, as well as frequency co…
A hybrid metal-graphene metamaterial (MM) is reported to achieve the active control of the broadband plasmon-induced transparency (PIT) in THz region. The unit cell consists of one cut wire (CW), four U-shape resonators (USRs) and monolayer graphene sheets under the USRs. Via near-field coupling, broadband PIT can be produced through the interference between different modes. Based on different arrangements of graphene positions, not only can we achieve electrically switching the amplitude of broadband PIT, but also can realize modulating the bandwidth of the transparent window. Simultaneously,…
Metals have been studied as terahertz sources for decades. Recent research has shown the potential of metals in generating extremely high THz pulse energy excited by intense laser pulses. To avoid the metal surface debris caused by laser pulses, here, we report the results of the broadband terahertz wave emission from a flowing liquid metal line excited by sub-picosecond laser pulses. The THz signal emitted from the liquid gallium line shows stronger field with broader bandwidth comparing with the signal from water under the identical optical excitation conditions. Our preliminary study sugges…
We report the coherent generation and detection of terahertz (THz) pulses covering the bandwidth of 0.1-9 THz in a high repetition rate, low pulse energy laser system. In this work we demonstrate the application and evaluation of solid-state biased coherent detection in combination with a spintronic emitter. This combination was used to generate and detect THz pulses in a time-domain spectroscopy (TDS) setup and tested on bulk nonlinear crystals. These results establish a new promising candidate to extend the possibilities for compact, broadband THz TDS systems driven by high repetition rate l…
The surface plasmon-polaritons (SPPs) switch is the key element of the integrated devices in optical computation and terahertz (THz) communications. In this paper, we propose a novel design of THz SPPs switch based on quantum engineering. Due to the robustness of coherent quantum control technique, our switch is very robust against with perturbations of geometrical parameters and presents a good performance at on-state (and off-state) from 0.5 THz to 0.7 THz. The on-state and off-state of our device can be controlled by the external voltage. We believe this finding will be the great improvemen…
We demonstrate the broadband operation of a switchable terahertz quarter-wave plate achieved with an active metasurface employing vanadium dioxide. For this purpose, we utilize anisotropically deformed checkerboard structures, which present broadband characteristics compatible with deep modulation. Moreover, the metasurface is integrated with a current injection circuit to achieve state switching; this injection circuit can also be employed to monitor the electric state of vanadium dioxide. We estimate the Stokes parameters derived from the experimental transmission spectra of the fabricated m…
Dynamically switchable half-/quarter-wave plates have recently been the focus in the terahertz regime. Conventional design philosophy leads to multilayer metamaterials or narrowband metasurfaces. Here we propose a novel design philosophy and a VO2-metal hybrid metasurface for achieving broadband dynamically switchable half-/quarter-wave plate (HWP/QWP) based on the transition from the overdamped to the underdamped resonance. Results show that, by varying the VO2 conductivity by three orders of magnitude, the proposed metasurface's function can be switched between an HWP with polarization conve…
We are reporting on terahertz generation from organic crystal BNA using a 1.15 to 1.55 um near infrared pump. We observed a very large emission spectrum extending up to 7 THz, compared to 2.5 THz from Ti:Sa pump in previous reports. The maximum optical-to-THz conversion efficiency in our experiment was 0.8% at 1 kHz repetition rate and without saturation leading to a peak electric field of 1 GV/m. Our results show pronounced phase matching privilege for intense terahertz generation using a pump in the 1.15 to 1.25 um range where high energy near infrared pump sources operate.
Broadband dual-comb spectroscopy has attracted increasing interests due to its unique advantages in high spectral resolution, fast detection, and so on. Although the dual-comb technique is relatively mature in the infrared wavelengths, it is, currently, not commercially capable of practical applications in the terahertz regime due to the lack of high performance broadband terahertz dual-comb sources. In the terahertz frequency range, the electrically pumped quantum cascade laser (QCL) is a suitable candidate for the dual-comb operation. However, free running terahertz QCL dual-comb sources nor…
We report on a waveguide engineering technique that enables the generation of a bandwidth up to 1 THz and record ultra-short pulse length of 2.5 ps in injection seeded terahertz quantum cascade lasers. The reported technique is able to control and fully suppress higher order lateral modes in broadband terahertz quantum cascade lasers by introducing side-absorbers to metal-metal waveguides. The side-absorbers consist of a top metalization set-back with respect to the laser ridge and an additional lossy metal layer. In continuous wave operation the side-absorbers lead to octave spanning laser em…
Spintronic terahertz emitters are novel, broadband and efficient sources of terahertz radiation, which emerged at the intersection of ultrafast spintronics and terahertz photonics. They are based on efficient spin-current generation, spin-to-charge-current and current-to-field conversion at terahertz rates. In this review, we address the recent developments and applications, the current understanding of the physical processes as well as the future challenges and perspectives of broadband spintronic terahertz emitters.
We present optically tunable magnetic 3D metamaterials at terahertz (THz) frequencies which exhibit a tuning range of ~30% of the resonance frequency. This is accomplished by fabricating 3D array structures consisting of double-split-ring resonators (DSRRs) on silicon-on-sapphire, fabricated using multilayer electroplating. Photoexcitation of free carriers in the silicon within the capacitive region of the DSRR results in a red-shift of the resonant frequency from 1.74 THz to 1.16 THz. The observed frequency shift leads to a transition from a magnetic-to-bianisotropic response as verified thro…
Carbon nanomaterials such as carbon nanotubes and graphene have proved to be efficient building blocks for active optoelectronic devices. Especially, the exotic properties of crystalline graphene, such as a linear/gapless energy dispersion, offer a generic route to the development of active photonic modulator at the infrared (IR) and terahertz (THz) regime with large modulation depth. Here, we show that graphene oxide (GO), an oxygenated derivative of graphene with randomly distributed molecular defects (e.g., adsorbed water molecules and punched holes), can provide a different way to effectiv…
Spintronic emitters are a unique class of terahertz (THz) sources due to their quasi-two-dimensional geometry and thereby their capability to couple to resonator near fields. Global excitation of the emitters often obstructs the intricate details of the coupling mechanisms between local THz dipoles and the individual modes of resonator structures. Here, we demonstrate the spatial mapping of the coupling strength between a local terahertz source on a spintronic emitter and far-field light mediated by a structured metallic environment. For a bow-tie geometry, experimental results are reproduced …
We report a broadband terahertz time-domain spectroscopy (THz-TDS) which enables twenty vibrational modes of adenosine nucleoside to be resolved in a wide frequency range of 1-20 THz. The observed spectroscopic features of adenosine are in good agreement with the published spectra obtained using Fourier Transform Infrared Spectroscopy (FTIR) and Raman spectroscopy. This much-extended bandwidth leads to enhanced material characterization capability as it provides spectroscopic information on both intra-molecular and inter-molecular vibrations. In addition, we also report a low-cost Frequency Mo…
Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multi-heterodyne spectroscopy using two terahertz quantum cascade laser combs. With just 100 $μ$s of integration time, we achieve peak signal-to-noise ratios exceeding 60 dB and a spectral coverage greater than 250 GHz centered at 2.8 THz. Even with room-temperature detectors we are able to achieve peak signal-to-noise ratios of 50 dB, and as a proof-of-principle we use these…
In this paper, we employ the novel design of the metamaterial half-wave plate by using the multiple layers of the metamaterials with some specific rotation angles. The rotation angles are given by composite pulse control which is the well-known quantum control technique. A big advantage of this method can analytically calculate the rotation angles and can be easily extended to the multiple layers. The more layers of the metamaterials can present more bandwidth of half-wave plate. In this paper, we present 1, 3, 5, 7 configurations of layers of a metamaterial half-wave plate and we demonstrate …
Terahertz (THz) Time domain spectroscopy (THz-TDS) is a broadband spectroscopic technique spreading its uses in multiple fields: in science from material science to biology, in industry where it measures the thickness of a paint layer during the painting operation. Using such practical commercial apparatus with broad spectrum for gas spectroscopy could be a major asset for air quality monitoring and tracking of atmospheric composition. However, gas spectroscopy needs high resolution and the usual approach in THz-TDS, where the recorded time trace is Fourier transform, suffers from resolution l…
In this study, terahertz (THz) absorption and transmission of monolayer MoS$_{2}$ was calculated under different carrier concentrations. Results showed that the THz absorption of monolayer MoS$_{2}$ is very small even under high carrier concentrations and large incident angle. Equivalent loss of the THz absorption is the total sum of reflection and absorption that is one to three grades lower than that of graphene. The monolayer MoS$_{2}$ transmission is much larger than that of the traditional GaAs and InAs two-dimensional electron gas. The field-effect tubular structure formed by the monolay…
Light-matter interactions are key in providing fundamental information about materials. Even in the linear-response regime, the spectroscopic response of a material encodes in it many properties of the ground state as well as of its excitations. This knowledge has been critical in our understanding of novel quantum materials, and the further improvement and extensions of linear spectroscopy will continue to be key in the exploration of novel states of matter. We report the development of broadband circular polarization spectroscopy in the terahertz range of the electromagnetic spectrum. We tak…
Nonlinear couplings between photons and electrons in new materials give rise to a wealth of interesting nonlinear phenomena. This includes frequency mixing, optical rectification or nonlinear current generation, which are of particular interest for generating radiation in spectral regions that are difficult to access, such as the terahertz gap. Owing to its specific linear dispersion and high electron mobility at room temperature, graphene is particularly attractive for realizing strong nonlinear effects. However, since graphene is a centrosymmetric material, second-order nonlinearities a prio…
Platforms for all-optical computing possess photonic circuits made of silicon-based channels, metal wires or optical fibers, etc. However, such solid waveguides suffer from the lack of reversibility and reconfigurability if facing the next generation of light-guiding-light (LGL) computing scheme, which envisions circuitry-free and rapidly reconfigurable systems powered by dynamic interactions between light beams. Here, we proposed the ubiquitous air as a restorable LGL signal manipulation medium with transient air-plasma waveguide circuits. Briefly, by focusing femtosecond laser beams in the f…
Transmission through photoexcited semiconductors is used to temporally and spectrally shape a Terahertz pulse. By adjusting the optical pump-THz probe delay, we experimentally introduce a polar asymmetry in the pulse profile as high as 92%. To shape the spectrum, we apply the same technique after strongly chirping the Terahertz pulse. This led to significant reshaping of the spectrum with a 52% upshift of spectrum median. Pulse shaping techniques introduced here are of particular importance for temporal and spectral shape-sensitive THz nonlinear experiments.
The invisibility cloak has been a long-standing dream for many researchers over the decades. The introduction of transformational optics has revitalized this field by providing a general method to design material distributions to hide the subject from detection. By transforming space and light propagation, a three-dimensional (3D) object is perceived as having a reduced number of dimensions, in the form of points, lines, and thin sheets, making it "undetectable" judging from the scattered field. Although a variety of cloaking devices have been reported at microwave and optical frequencies, the…
Plasmonic metamaterials and metasurfaces offer new opportunities in developing high performance terahertz emitters and detectors beyond the limitations of conventional nonlinear materials. However, simple meta-atoms for second-order nonlinear applications encounter fundamental trade-offs in the necessary symmetry breaking and local-field enhancement due to radiation damping that is inherent to the operating resonant mode and cannot be controlled separately. Here we present a novel concept that eliminates this restriction obstructing the improvement of terahertz generation efficiency in nonline…
The design of a self-complementary metallic checkerboard pattern achieves broadband, dispersion-less, and maximized absorption, concentrating in the deep subwavelength resistive connections between squares, without any theoretical limitation on the energy absorbing area. Here, we experimentally and numerically investigate the electromagnetic response in the limit of extremely small connections. We show that finite conductivity and randomness in a near-self-complementary checkerboard pattern plays a crucial role in producing a frequency-independent energy loss in the terahertz frequency region.…
