Systematic measurements of mass-ratio distributions for fission following collisions of $^{48}$Ti projectiles with even-even target nuclei from $^{144}$Sm to $^{208}$Pb have been made at sub-barrier energies. They show the presence of quasifission, and depend strongly on target nucleus deformation and the fissility of the composite nucleus. A new framework to analyse systematic mass-ratio measurements allows direct comparison with the trends expected from shell structure, independent of assumptions or fits. This indicates that quasi-fission mass distributions show trends consistent with low energy mass-asymmetric fission of the same actinide elements.
Mass distributions of fission fragments arising from the slow quasi-fission process have been derived by comparing the measured distributions with the theoretical distributions based on compound nuclear fission model for several reactions. The mass-distributions corresponding to quasi-fission events for all the systems show the following common features: (1) they are double peaked with fixed peak-centroids and nearly same width at different incident energies, (2) the yield of quasi-fission events decreases with the increasing projectile energy, and (3) peak corresponding to lighter fragment is…
Fission of atomic nuclei often produces mass asymmetric fragments. However, the origin of this asymmetry was believed to be different in actinides and in the sub-lead region [A. Andreyev {\it et al.}, Phys. Rev. Lett. {\bf 105}, 252502 (2010)]. It has recently been argued that quantum shell effects stabilising pear shapes of the fission fragments could explain the observed asymmetries in fission of actinides[G. Scamps and C. Simenel, Nature {\bf 564}, 382 (2018)]. This interpretation is tested in the sub-lead region using microscopic mean-field calculations of fission based on the Hartree-Fock…
Quantum shell effects are known to affect the formation of fragments in nuclear fission. Shell effects also affect quasi-fission reactions occurring in heavy-ion collisions. Systematic time-dependent Hartree-Fock simulations of 50Ca+176Yb collisions show that the mass equilibration between the fragments in quasi-fission is stopped when they reach similar properties to those in the asymmetric fission mode of the 226Th compound nucleus. Similar shell effects are then expected to determine the final repartition of nucleons between the nascent fragments in both mechanisms. Future experimental stud…
Dissipative dynamics of nuclear fission is a well confirmed phenomenon described either by a Kramers-modified statistical model or by a dynamical model employing the Langevin equation. Though dynamical models as well as statistical models incorporating fission delay are found to explain the measured fission observables in many studies, it nonetheless shows conflicting results for shell closed nuclei in the mass region 200. Analysis of recent data for neutron shell closed nuclei in excitation energy range 40$-$80 MeV failed to arrive at a satisfactory description of the data and attributed the …
A regular pattern, revealing the leading role of the light-fragment nuclear charge, is found to emerge from a consistent analysis of the experimental information collected recently on low-energy asymmetric fission of neutron-deficient nuclei around lead. The observation is corroborated by a theoretical investigation within a microscopic framework, suggesting the importance of proton configurations driven by quadrupole-octupole correlations. This is in contrast to the earlier theoretical interpretations in terms of dominant neutron shells. The survey of a wider area of the nuclear chart by a se…
Nuclear fission is still one of the most complex physical processes we can observe in nature due to the interplay of macroscopic and microscopic nuclear properties that decide the result. An example of this coupling is the presence of nuclear dissipation as an important ingredient that contributes to drive the dynamics and has a clear impact on the time of the process. However, different theoretical interpretations, and scarce experimental data make it poorly understood. In this letter, we present the first experimental determination of the dissipation energy in fission as a function of the fr…
Presence of closed proton and/or neutron shells causes deviation from macroscopic properties of nuclei which are understood in terms of the liquid drop model. It is important to investigate experimentally the stabilizing effects of shell closure, if any, against fission. This work aims to investigate probable effects of proton shell ($Z = 82$) closure in the compound nucleus, in enhancing survival probability of the evaporation residues formed in heavy ion-induced fusion-fission reactions. Evaporation residue cross sections have been measured for the reactions $^{19}$F+$^{180}$Hf, $^{19}$F+$^{…
Despite the recent experimental and theoretical progress in the investigation of the nuclear fission process, a complete description still represents a challenge in nuclear physics because it is a very complex dynamical process, whose description involves the coupling between intrinsic and collective degrees of freedom, as well as different quantum-mechanical phenomena. To improve on the existing data on nuclear fission, we produce fission reactions of heavy nuclei in inverse kinematics by using quasi-free (p,2p) scattering, which induce fission through particle-hole excitations that can range…
Fission of $^{180}$Hg produces mass asymmetric fragments which are expected to be influenced by deformed shell-effects at N=56 in the heavy fragment and Z=34 in the light fragment [G. Scamps and C. Simenel, arXiv:1904.01275 (2019)]. To investigate both shell-effects and to determine which one has the main influence on the asymmetry in the region of the $^{180}$Hg, we produce a systematic of Constraint-Hartree-Fock calculations in nuclei with similar N/Z ratio than the $^{178}$Pt. It is found that N=56 determines the asymmetry of systems in this region of the nuclear chart.
A direct and complete measurement of isotopic fission-fragment yields of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced with an average excitation energy of 8.3 MeV in one-neutron transfer reactions between a $^{238}$U beam and a $^{9}$Be target at Coulomb barrier energies. The fission fragments were detected and isotopically identified using the VAMOS++ spectrometer at the GANIL facility. This measurement allows to directly evaluate the fission models at excitation energies of fast neutrons, relevant for next-generation nuclear reactors. The pres…
Fission Hindrance in hot 216Th: Evaporation Residue Measurements
用ATLAS碎片质量分析仪测量了能量为165、174、185、196、205、215、225、236、246和257 MeV的32 S +184 W的聚变蒸发残余物截面。与统计模型计算的数据进行了比较，发现需要一个随激发能增加的核耗散强度来再现激发函数。与以前发表的数据的比较表明，耗散强度强烈依赖于壳结构的核系统。
Level structure of light neutron-rich La isotopes beyond the N=82 shell closure
GANIL, CEA/DRF-CNRS/IN2P3（法国国家大加速器研究中心）；Shandong University（山东大学）；Weihai Research Institute of Industrial Technology of Shandong University（山东大学威海工业技术研究院）；Vanderbilt University（范德堡大学）；Variable Energy Cyclotron Centre（变能回旋加速器中心）；Homi Bhabha National Institute（霍米·巴巴国立研究所）；Sun Yat-sen University（中山大学）；Institute for Basic Science（基础科学研究院）；Université Paris-Saclay（巴黎萨克雷大学）；Institute of Nuclear Physics PAN（波兰科学院核物理研究所）；Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）；Université de Strasbourg（斯特拉斯堡大学）；Tata Institute of Fundamental Research（塔塔基础研究所）；Tsinghua University（清华大学）
Background: Quasifission and fusion-fission are primary mechanisms to prevent the production of superheavy elements. The recent experimental measurements reveal that the fusion-evaporation cross section in the $3n$ reaction channel of $^{48}$Ca+$^{239}$Pu is 50 times lower than using $^{244}$Pu as target nucleus. However, the precise mechanisms of this remarkable isotopic dependence are not well understood. Purpose: To understand the experimental observation of the rapid decrease of stability of superheavy nuclei as the neutron number decreases, the theoretical studies of quasifission and fusi…
Beta-delayed neutron emission and $β$-delayed fission ($β$df) probabilities were calculated for heavy, neutron-rich nuclei using the Los Alamos coupled Quasi-Particle Random Phase Approximation plus Hauser-Feshbach (QRPA+HF) approach. In this model, the compound nucleus is initially populated by $β$-decay and is followed through subsequent statistical decays taking into account competition between neutrons, $γ$-rays and fission. The primary output of these calculations includes branching ratios along with neutron and $γ$-ray spectra. We find a relatively large region of heavy nuclides where th…
To disentangle the role of shell effects and dynamics, fission fragment mass distributions of $^{191}$Au, a nucleus in the newly identified island of mass asymmetric fission in the sub-lead region, have been measured down to excitation energy of $\approx$20 MeV above the fission barrier via two different entrance channels, viz. $^{16}$O+$^{175}$Lu and $^{37}$Cl+$^{154}$Sm reactions. Apart from having signature of the shell effects in both the cases, clear experimental evidence of quasifission has been observed in the mass distributions of the Cl induced reaction, that has also been substantiat…
Isotopic fission yields of ${}^{240}$Pu as a function of the excitation energy
GANIL, CNRS/IN2P3, CEA/DRF（GANIL，法国国家科学研究中心/欧洲核子研究组织，法国原子能和替代能源委员会）；IGFAE - Universidade de Santiago de Compostela（圣地亚哥-德孔波斯特拉大学 IGFAE 研究所）；IJC Lab, Université Paris-Saclay, CNRS/IN2P3（巴黎萨克雷大学 IJC 实验室，法国国家科学研究中心/欧洲核子研究组织）；IFIC, Centro Mixto Universidad de Valencia-CSIC（瓦伦西亚大学-西班牙国家科学研究理事会混合中心 IFIC）；CINTECX, Universidade de Vigo（维戈大学 CINTECX 研究中心）；CEA Saclay, DRF/IRFU/SPhN（法国原子能和替代能源委员会萨克雷园区，研究与技术发展部/核物理研究所）
Potential energy surfaces and fission barriers of superheavy nuclei are analyzed in the macroscopic-microscopic model. The Lublin-Strasbourg Drop (LSD) is used to obtain the macroscopic part of the energy, whereas the shell and pairing energy corrections are evaluated using the Yukawa-folded potential. A standard flooding technique has been used to determine the barrier heights. It was shown the Fourier shape parametrization containing only three deformation parameters reproduces well the nuclear shapes of nuclei on their way to fission. In addition, the non-axial degree of freedom is taken in…
A study of medium-mass heavy-ion reactions leading to two fragments in the exit channel from barrier to 18A MeV is proposed. A special focus is made on fission and quasi-fission for events with two fragments ($Z\geq10$) in the exit channel selected. Reactions induced by $^{129}Xe$ projectiles on $^{nat}Sn$ and on $^{197}Au$ at energies ranging from $8A$ MeV to $18A$ MeV were analyzed. Using the fragment ($Z\geq10$) multiplicity equal to 2, fission and quasi-fission events were studied for the lowest beam energies using the fission fragment charge distributions, the total kinetic energy distrib…
Constraining the equation of state of nuclear matter from competition of fusion and quasi-fission in the reactions leading to production of the superheavy elements
