We report the experimental realisation of a versatile ring trap for ultracold atoms. The ring geometry is created by the time-averaged adiabatic potential resulting from the application of an oscillating magnetic bias field to a rf dressed quadrupole trap. Lifetimes for a Bose-Einstein condensate in the ring exceed 11s and the ring radius was continuously varied from 50$μ$m to 261$μ$m. An efficient method of loading the ring from a conventional TOP trap is presented together with a rotation scheme which introduces angular momentum into the system. The ring presents an opportunity to study the superfluid properties of a condensate in a multiply connected geometry and also has applications for matter-wave interferometry.
Reactive or elastic two-body collisions in an ultracold gas are affected by quantum statistics. In this paper, we study ensemble-averaged collision rates for a two-species fermionic gas. The two species may have different masses, densities and temperatures. We investigate how averaged collision rates are affected by the presence of Fermi spheres in the initial states; Pauli blocking of final states is not considered. It is shown that, independently on the details of the collision, Fermi-averaged collision rates deviate from Boltzmann-averaged ones, particularly for a gas with strong imbalance …
We demonstrate a novel class of trapping potentials, time-averaged adiabatic potentials (TAAP) which allows the generation of a large variety of traps and waveguides for ultracold atoms. Multiple traps can be coupled through controllable tunneling barriers or merged altogether. We present analytical expressions for pancake-, cigar-, and ring- shaped traps. The ring-geometry is of particular interest for guided matter-wave interferometry as it provides a perfectly smooth waveguide of controllable diameter, and thus a tunable sensitivity of the interferometer.
We report the first experimental realization of ultracold atoms confined in a time-averaged, adiabatic potential (TAAP). This novel trapping technique involves using a slowly oscillating ($\sim$ kHz) bias field to time-average the instantaneous potential given by dressing a bare magnetic potential with a high frequency ($\sim$ MHz) magnetic field. The resultant potentials provide a convenient route to a variety of trapping geometries with tunable parameters. We demonstrate the TAAP trap in a standard time-averaged orbiting potential trap with additional Helmholtz coils for the introduction of …
We present the first experimental demonstration of a multiple-radiofrequency dressed potential for the configurable magnetic confinement of ultracold atoms. We load cold $^{87}$Rb atoms into a double well potential with an adjustable barrier height, formed by three radiofrequencies applied to atoms in a static quadrupole magnetic field. Our multiple-radiofrequency approach gives precise control over the double well characteristics, including the depth of individual wells and the height of the barrier, and enables reliable transfer of atoms between the available trapping geometries. We have cha…
We propose a scheme to dynamically synthesize a space-periodic effective magnetic field for neutral atoms by time-periodic magnetic field pulses. When atomic spin adiabatically follows the direction of the effective magnetic field, an adiabatic scalar potential together with a geometric vector potential emerges for the atomic center-of-mass motion, due to the Berry phase effect. While atoms hop between honeycomb lattice sites formed by the minima of the adiabatic potential, complex Peierls phase factors in the hopping coefficients are induced by the vector potential, which facilitate a topolog…
We study the growth dynamics of ordered structures of strongly interacting polar molecules in optical lattices. Using dipole blockade of microwave excitations, we map the system onto an interacting spin-1/2 model possessing ground states with crystalline order, and describe a way to prepare these states by non-adiabatically driving the transitions between molecular rotational levels. The proposed technique bypasses the need to cross a phase transition and allows for the creation of ordered domains of considerably larger size compared to approaches relying on adiabatic preparation.
Spatial adiabatic passage processes for ultracold atoms trapped in tunnel-coupled cylindrically symmetric concentric potentials are investigated. Specifically, we discuss the matter-wave analogue of the rapid adiabatic passage (RAP) technique for a high fidelity and robust loading of a single atom into a harmonic ring potential from a harmonic trap, and for its transport between two concentric rings. We also consider a system of three concentric rings and investigate the transport of a single atom between the innermost and the outermost rings making use of the matter-wave analogue of the stimu…
We report two novel techniques for cooling and rotating Bose-Einstein condensates in a dilute rubidium vapour that highlight the control and versatility afforded over cold atom systems by time-averaged adiabatic potentials (TAAPs). The intrinsic loss channel of the TAAP has been successfully employed to evaporatively cool a sample of trapped atoms to quantum degeneracy. The speed and efficiency of this process compares well with that of conventional forced rf-evaporation. In an independent experiment, we imparted angular momentum to a cloud of atoms forming a Bose-Einstein condensate by introd…
We present a joint experimental and theoretical analysis to assess the adiabatic experimental preparation of ultracold bosons in optical lattices aimed at simulating the three-dimensional Bose-Hubbard model. Thermometry of lattice gases is realized from the superfluid to the Mott regime by combining the measurement of three-dimensional momentum-space densities with ab-initio quantum Monte Carlo (QMC) calculations of the same quantity. The measured temperatures across the superfluid-to-Mott transition are in agreement with isentropic lines reconstructed via QMC for the experimental parameters o…
We propose a scheme to realize lattice potentials of sub-wavelength spacing for ultracold atoms. It is based on spin-dependent optical lattices with a time-periodic modulation. We show that the atomic motion is well described by the combined action of an effective, time-independent, lattice of small spacing, together with a micro-motion associated with the time-modulation. A numerical simulation shows that an atomic gas can be adiabatically loaded into the effective lattice ground state, for timescales comparable to the ones required for adiabatic loading of standard optical lattices. We gener…
Quantum many-body phases offer unique properties and emergent phenomena, making them an active area of research. A promising approach for their experimental realization in model systems is to adiabatically follow the ground state of a quantum Hamiltonian from a product state of isolated particles to one that is strongly-correlated. Such protocols are relevant also more broadly in coherent quantum annealing and adiabatic quantum computing. Here we explore one such protocol in a system of ultracold atoms in an optical lattice. A fully magnetized state is connected to a correlated zero-magnetizat…
The ability to generate and tune quantized persistent supercurrents is crucial for building superconducting or atomtronic devices with novel functionalities. In ultracold atoms, previous methods for generating quantized supercurrents are generally based on dynamical processes to prepare atoms in metastable excited states. Here we show that arbitrary quantized circulation states can be adiabatically prepared and tuned as the ground state of a ring-shaped Bose-Einstein condensate by utilizing spin-orbital-angular-momentum (SOAM) coupling and an external potential. There exists superfluid hystere…
Interesting spin Hamiltonians can be realized with ultracold atoms in a two-component Mott insulator (2CMI). It was recently demonstrated that the application of a magnetic field gradient to the 2CMI enables new techniques of thermometry and adiabatic cooling. Here we present a theoretical description which provides quantitative analysis of these two new techniques. We show that adiabatic reduction of the field gradient is capable of cooling below the Curie or Néel temperature of certain spin ordered phases.
We introduce a model to study the collisions of two ultracold diatomic molecules in one dimension interacting via pairwise potentials. We present results for this system, and argue that it offers lessons for real molecular collisions in three dimensions. We analyze the distribution of the adiabatic potentials in the hyperspherical coordinate representation as well as the distribution of the four-body bound states in the adiabatic approximation (i.e. no coupling between adiabatic channels). It is found that while the adiabatic potential distribution transitions from chaotic to non-chaotic as th…
We characterize the disorder induced localization in momentum space for ultracold atoms in one-dimensional incommensurate lattices, according to the dual Aubry-André model. For low disorder the system is localized in momentum space, and the momentum distribution exhibits time-periodic oscillations of the relative intensity of its components. The behavior of these oscillations is explained by means of a simple three-mode approximation. We predict their frequency and visibility by using typical parameters of feasible experiments. Above the transition the system diffuses in momentum space, and th…
We report the observation of quantum dynamical oscillations of ultracold atomic gases in the F and D bands of a single-well optical lattice. We are able to control the Bragg reflections at the Brillouin zone edge up to the third order. As a result, we can switch the quantum dynamics from oscillations across both the F and D bands to oscillations only within the F-band. Our capability to observe these remarkable oscillations comes from the innovative non-adiabatic technique which allows us to load ultracold atoms efficiently to the G-band of an optical lattice.
In this work we model and realize stimulated Raman adiabatic passage (STIRAP) in the diatomic $\mathrm{^{23}Na^{40}K}$ molecule from weakly bound Feshbach molecules to the rovibronic ground state via the $\left|v_d=5,J=Ω=1\right\rangle$ excited state in the $d^3Π$ electronic potential. We demonstrate how to set up a quantitative model for polar molecule production by taking into account the rich internal structure of the molecules and the coupling laser phase noise. We find excellent agreement between the model predictions and the experiment, demonstrating the applicability of the model in the…
We report the long-time nonlinear dynamical evolution of ultracold atomic gases in the P-band of an optical lattice. A Bose-Einstein condensate (BEC) is fast and efficiently loaded into the Pband at zero quasi-momentum with a non-adiabatic shortcut method. For the first one and half milliseconds, these momentum states undergo oscillations due to coherent superposition of different bands, which are followed by oscillations up to 60ms of a much longer period. Our analysis shows the dephasing from the nonlinear interaction is very conducive to the long-period oscillations induced by the variable …
We develop the theory for the Adiabatic Raman Photoassociation (ARPA) of ultracold atoms to form ultracold molecules in the presence of scattering resonances. Based on a computational method in which we replace the continuum with a discrete set of "effective modes", we show that the existence of resonances greatly aids in the formation of deeply bound molecular states. We illustrate our general theory by computationally studying the formation of $^{85}$Rb$_2$ molecules from pairs of colliding ultracold $^{85}$Rb atoms. The single-event transfer yield is shown to have a near-unity value for wid…
Investigating Friedel oscillations in ultracold gases would complement the studies performed on solid state samples with scanning-tunneling microscopes. In atomic quantum gases interactions and external potentials can be tuned freely and the inherently slower dynamics allow to access non-equilibrium dynamics following a potential or interaction quench. Here, we examine how Friedel oscillations can be observed in current ultracold gas experiments under realistic conditions. To this aim we numerically calculate the amplitude of the Friedel oscillations which a potential barrier provokes in a 1D …
The ground-state properties of a few spin-1/2 fermions with different masses and interacting via short-range contact forces are studied within an exact diagonalization approach. It is shown that, depending on the shape of the external confinement, different scenarios of the spatial separation between components manifested by specific shapes of the density profiles can be obtained in the strong interaction limit. We find that the ground-state of the system undergoes a specific transition between orderings when the confinement is changed adiabatically from a uniform box to a harmonic oscillator …
Alkaline-earth(-like) ultracold atoms, trapped in optical lattices and in the presence of an external gauge field, can stabilise Mott insulating phases characterised by density and magnetic order. We show that this property can be used to realise a topological fractional pump. Our analysis is based on a many-body adiabatic expansion and on time-dependent matrix-product-states numerical simulations. We characterise the pumping protocol by including both finite-size and non-adiabatic corrections. For a specific form of atom-atom interaction, we present an exactly-solvable model of a fractional p…
Variational and diffusion quantum Monte Carlo (VMC and DMC) calculations of the properties of the zero-temperature fermionic gas at unitarity are reported. The ratio of the energy of the interacting to the non-interacting gas for a system of 128 particles is calculated to be 0.4517(3) in VMC and 0.4339(1) in the more accurate DMC method. The spherically-averaged pair-correlation functions, momentum densities, and one-body density matrices are very similar in VMC and DMC, but the two-body density matrices and condensate fractions show some differences. Our best estimate of the condensate fracti…
Time-averaged trapping potentials have played an important role in the development of the field of ultracold atoms. Despite their widespread application, there is not yet a complete understanding of when a system can be considered time-averaged. Here we use Floquet theory to analyse the lowest energy state of time-periodic trapping potentials, and characterise the transition from a localised state in a slowly moving trap to a delocalised state in a rapidly oscillating time-averaged potential. We investigate how the driving parameters affect the density and phase of the Floquet ground state, an…
Motivated by recent experimental advances in ultracold atomic gases placed in cavities, we study the influence of the atom-cavity coupling on the Fermi gases trapped in optical lattices. By adiabatic elimination of the cavity photon field, the atom-cavity coupling gives rise to effective long-range interactions. It results in a variety of two-body scattering processes, during which the atomic pairs can acquire an additional center-of-mass momentum. This reveals the possibility of Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superfluids in which the atomic pairing momentum is nonzero. By inspecting …
We theoretically consider non-interacting fermions confined to optical lattices and apply a lattice amplitude modulation that we choose to be either homogeneous or of superlattice geometry. We study the atom excitation rate to higher Bloch bands which can be measured by adiabatic band mapping. We find that the atom excitation rate shows a clear signature of the temperature dependent Fermi distribution in the lowest band of the equilibrium lattice as excitations are quasimomentum-resolved. Based on typical experimental parameters and incorporating a trapping potential, we find that thermometry …
All light has structure, but only recently it has become possible to construct highly controllable and precise potentials so that most laboratories can harness light for their specific applications. In this chapter, we review the emerging techniques for high-resolution and configurable optical trapping of ultracold atoms. We focus on optical deflectors and spatial light modulators in the Fourier and direct imaging configurations. These optical techniques have enabled significant progress in studies of superfluid dynamics, single-atom trapping, and underlie the emerging field of atomtronics. Th…
We propose a scheme of "$R$-type" photoassociative adiabatic passage (PAP) to create polar molecular condensates from two different species of ultracold atoms. Due to the presence of a quasi-coherent population trapping state in the scheme, it is possible to associate atoms into molecules with a \textit{low-power} photoassociation (PA) laser. One remarkable advantage of our scheme is that a tunable atom-molecule coupling strength can be achieved by using a time-dependent PA field, which exhibits larger flexibility than using a tunable magnetic field. In addition, our results show that the PA i…
We present a new technique for producing two- and three-dimensional Rashba-type spin-orbit couplings for ultracold atoms without involving light. The method relies on a sequence of pulsed inhomogeneous magnetic fields imprinting suitable phase gradients on the atoms. For sufficiently short pulse durations, the time-averaged Hamiltonian well approximates the Rashba Hamiltonian. Higher order corrections to the energy spectrum are calculated exactly for spin-1/2 and perturbatively for higher spins. The pulse sequence does not modify the form of rotationally symmetric atom-atom interactions. Final…
We present experimental evidence of the successful closed-loop optimization of the dynamics of cold atoms in an optical lattice. We optimize the loading of an ultracold atomic gas minimizing the excitations in an array of one-dimensional tubes (3D-1D crossover) and we perform an optimal crossing of the quantum phase-transition from a Superfluid to a Mott-Insulator in a three-dimensional lattice. In both cases we enhance the experiment performances with respect to those obtained via adiabatic dynamics, effectively speeding up the process by more than a factor three while improving the quality o…
In order to study ultracold charge-transfer processes in hybrid atom-ion traps, we have mapped out the potential energy curves and molecular parameters for several low lying states of the Rb, Yb$^+$ system. We employ both a multi-reference configuration interaction (MRCI) and a full configuration interaction (FCI) approach. Turning points, crossing points, potential minima and spectroscopic molecular constants are obtained for the lowest five molecular states. Long-range parameters, including the dispersion coefficients are estimated from our {\it ab initio} data. The separated-atom ionization…
We investigate the spectral properties of a finite laser-driven lattice of ultracold Rydberg atoms exploiting the dipole blockade effect in the frozen Rydberg gas regime. Uniform one-dimensional lattices as well as lattices with variable spacings are considered. In the case of a weak laser coupling, we find a multitude of many-body Rydberg states with well-defined excitation properties which are adiabatically accessible starting from the ground state. A comprehensive analysis of the degeneracies of the spectrum as well as of the single and pair excitations numbers of the eigenstates is perform…
We investigate the existence of the $macroscopic$ $quantum$ $phase$ in trapped ultracold quantum degenerate gases, such as Bose-Einstein condensate, in an asymmetrical two-dimensional magnetic lattice. We show the key to adiabatically control the tunneling in the new two-dimensional magnetic lattice by means of external magnetic bias fields. The macroscopic quantum phase signature is identified as a Rabi-like oscillation when solving the system of coupled time-dependent differential equations, described here by the Boson Josephson Junctions (BJJs). In solving the system of the BJJs we used an …
A protocol is proposed for the rapid coherent loading of a Bose-Einstein condensate into the ground state of an optical lattice, without residual excitation associated with the breakdown of adiabaticity. The driving potential required to assist the rapid loading is derived using the fast forward technique, and generates the ground state in any desired short time. We propose an experimentally feasible loading scheme using a bichromatic lattice potential, which approximates the fast-forward driving potential with high fidelity.
Quantum simulations with ultracold atoms typically create atomic wavefunctions with structures at optical length scales, where direct imaging suffers from the diffraction limit. In analogy to advances in optical microscopy for biological applications, we use a non-linear atomic response to surpass the diffraction limit. Exploiting quantum interference, we demonstrate imaging with super-resolution of $λ/100$ and excellent temporal resolution of 500 ns. We characterize our microscope's performance by measuring the ensemble averaged wavefunction of atoms within the unit cells of an optical lattic…
We report on the creation of bosonic NaCs molecules in their absolute rovibrational ground state via stimulated Raman adiabatic passage. We create ultracold gases with up to 22,000 dipolar NaCs molecules at a temperature of 300(50) nK and a peak density of $1.0(4) \times 10^{12}$ cm$^{-3}$. We demonstrate comprehensive quantum state control by preparing the molecules in a specific electronic, vibrational, rotational, and hyperfine state. Employing the tunability and strength of the permanent electric dipole moment of NaCs, we induce dipole moments of up to 2.6 D. Dipolar systems of NaCs molecu…
We report on the creation of ultracold 84Sr2 molecules in the electronic ground state. The molecules are formed from atom pairs on sites of an optical lattice using stimulated Raman adiabatic passage (STIRAP). We achieve a transfer efficiency of 30% and obtain 4x10^4 molecules with full control over the external and internal quantum state. STIRAP is performed near the narrow 1S0-3P1 intercombination transition, using a vibrational level of the 0u potential as intermediate state. In preparation of our molecule association scheme, we have determined the binding energies of the last vibrational l…
We design and explore a shortcut to adiabaticity (STA) for changing the interaction strength between two ultracold, harmonically trapped bosons. Starting from initially uncorrelated, non-interacting particles, we assume a time-dependent tuning of the inter-particle interaction through a Feshbach resonance, such that the two particles are strongly interacting at the end of the driving. The efficiency of the STA is then quantified by examining the thermodynamic properties of the system, such as the irreversible work, which is related to the out-of-equilibrium excitations in the system. We also q…
We report on two-photon photoassociation (PA) spectroscopy of ultracold heteronuclear LiRb molecules. This is used to determine the binding energies of the loosely bound levels of the electronic ground singlet and the lowest triplet states of LiRb. We observe strong two-photon PA lines with power broadened line widths greater than 20 GHz at relatively low laser intensity of 30 W/cm$^{2}$. The implication of this observation on direct atom to molecule conversion using stimulated Raman adiabatic passage (STIRAP) is discussed and the prospect for electronic ground state molecule production is the…
Robust stimulated Raman exact passages are requisite for controlling nonlinear quantum systems, with the wide applications ranging from ultracold molecules, non-linear optics to superchemistry. Inspired by shortcuts to adiabaticity, we propose the fast-forward scaling of stimulated Raman adiabatic processes with the nonlinearity involved, describing the transfer from an atomic Bose-Einstein condensate to a molecular one by controllable external fields. The fidelity and robustness of atom-molecule conversion are shown to surpass those of conventional adiabatic passages, assisted by fast-forward…
A method is proposed to drive an ultrafast non-adiabatic dynamics of an ultracold gas trapped in a box potential. The resulting state is free from spurious excitations associated with the breakdown of adiabaticity, and preserves the quantum correlations of the initial state up to a scaling factor. The process relies on the existence of an adiabatic invariant and the inversion of the dynamical self-similar scaling law dictated by it. Its physical implementation generally requires the use of an auxiliary expulsive potential analogous to those used in soliton control. The method is extended to a …
The microscopic onset of irreversibility is finally becoming an experimental subject. Recent experiments on microscopic open and even isolated systems have measured statistical properties associated with entropy production, and hysteresis-like phenomena have been seen in cold atom systems with dissipation (i.e. effectively open systems coupled to macroscopic reservoirs). Here we show how experiments on isolated systems of ultracold atoms can show dramatic irreversibility like cooking an egg. In our proposed experiments, a slow forward-and-back parameter sweep will sometimes fail to return the …
We report on the observation of an elementary exchange process in an optically trapped ultracold sample of atoms and Feshbach molecules. We can magnetically control the energetic nature of the process and tune it from endoergic to exoergic, enabling the observation of a pronounced threshold behavior. In contrast to relaxation to more deeply bound molecular states, the exchange process does not lead to trap loss. We find excellent agreement between our experimental observations and calculations based on the solutions of three-body Schrödinger equation in the adiabatic hyperspherical representat…
We examine the spectral structure and many-body dynamics of two and three repulsively interacting bosons trapped in a one-dimensional double-well, for variable barrier height, inter-particle interaction strength, and initial conditions. By exact diagonalization of the many-particle Hamiltonian, we specifically explore the dynamical behaviour of the particles launched either at the single particle ground state or saddle point energy, in a time-independent potential. We complement these results by a characterisation of the cross-over from diabatic to quasi-adiabatic evolution under finite-time s…
We theoretically investigate the prospects for photoassociation (PA) of Rb$_3$, in particular at close range. We provide an overview of accessible states and possible transitions. The major focus is placed on the calculation of equilibrium structures, the survey of spin-orbit effects and the investigation of transition dipole moments. Furthermore we discuss Franck-Condon overlaps and special aspects of trimers including the (pseudo) Jahn-Teller effect and the resulting topology of adiabatic potential-energy surfaces. With this we identify concrete and suitable PA transitions to potentially pro…
We associate Sr atom pairs on sites of a Mott insulator optically and coherently into weakly-bound ground-state molecules, achieving an efficiency above 80\%. This efficiency is 2.5 times higher than in our previous work [S. Stellmer, B. Pasquiou, R. Grimm, and F. Schreck, Phys. Rev. Lett. 109, 115302 (2012)] and obtained through two improvements. First, the lifetime of the molecules is increased beyond one minute by using an optical lattice wavelength that is further detuned from molecular transitions. Second, we compensate undesired dynamic light shifts that occur during the stimulated Raman…
We report on the creation of an ultracold dipolar gas of fermionic $^{23}$Na$^{40}$K molecules in their absolute rovibrational and hyperfine ground state. Starting from weakly bound Feshbach molecules, we demonstrate hyperfine resolved two-photon transfer into the singlet ${\rm X}^1Σ^+ |v{=}0,J{=}0\rangle$ ground state, coherently bridging a binding energy difference of 0.65 eV via stimulated rapid adiabatic passage. The spin-polarized, nearly quantum degenerate molecular gas displays a lifetime longer than 2.5 s, highlighting NaK's stability against two-body chemical reactions. A homogeneous …
