Terahertz (THz) waves have been significantly developed in the last fifteen years because of their great potential for applications in industrial and scientific communities1,2. The unique properties of THz waves as transparency for numerous materials and strong absorption for water-based materials are expected to broadly impact biosensing3 such as medical imaging4, chemical identifications5, and DNA recognition6. In particular, for accessing information within a scale comparable to the cell size where interactions between cell membrane and other organelle structures occur, micron size spatial resolution is required. Due to the large wavelength, however, the joint capability of THz near-field imaging with real-time acquisition, which is a highly desirable ability for observing real-time changes of in vivo sample, remains undone. Here, we report a real-time THz near-field microscope with a high dynamic range that can capture images of a 370 x 740 μm2 area at 35 frames per second. We achieve high spatial resolution on a large area by combining two novel techniques: THz pulse generation by tilted-pulse-front excitation7 and electro-optic (EO) balanced imaging detection using a thin crystal. To demonstrate the microscope capability, we reveal the field enhancement at the gap position of a dipole antenna after the irradiation of a THz pulse. Our results are the first demonstration of a direct quantification of a 2-dimensional subwavelength THz electric field taken in real-time.
We consider a periodically gated two-dimensional electron system, with a central gate finger biased independently creating a tunable plasmonic cavity in a planar plasmonic crystal. We demonstrate that the plasmons resonantly excited in the periodic plasmonic lattice by incident terahertz radiation can strongly pump the cavity plasmon modes leading to a deep sub-wavelength concentration of terahertz energy with giant electric field enhancement factor up to 10000.
Using a two-dipole model of an optical near-field of Scanning Near-field Optical Microscope tip, i. e. taking into account contributions of magnetic and electric dipoles, we propose and analyze a new type of 3D optical nanotrap found for certain relations between electric and magnetic dipoles. Electric field attains a minimum value in vacuum in the vicinity of the tip and hence such a trap is quite suitable for manipulations with cold atoms.
Terahertz (THz) wave shows great potential in non-destructive testing, bio detection and cancer imaging. Recent progresses on THz wave near-field probes/apertures enable mechanically raster scanning of an object's surface in the near-field region, while an efficient, non-scanning, non-invasive, deeply sub-diffraction-limited imaging still remains challenging. Here, we demonstrate a THz near-field microscopy using a reconfigurable spintronic THz emitter array (STEA) with computational ghost imaging. By illuminating an object with the reconfigurable STEA in near field and computing the correlati…
Excitation of antiferromagnetic spin waves in HoFeO$_{3}$ crystal combined with a split ring resonator (SRR) is studied using terahertz (THz) electromagnetic pulses. The magnetic field in the vicinity of the SRR induced by the incident THz electric field component excites and the Faraday rotation of the polarization of a near-infrared probe pulse directly measures oscillations that correspond to the antiferromagnetic spin resonance mode. The good agreement of the temperature-dependent magnetization dynamics with the calculation using the two-lattice Landau-Lifshitz-Gilbert equation confirms th…
Using an affordable ytterbium laser with sub-mJ of energy combined with a novel pulse compression technique, we demonstrate an extremely competitive state-of-the-art terahertz (THz) source with 53 mW of average power and 310 kV/cm at focus from the tilted-pulse front pumping scheme in lithium niobate at room temperature. Key points of this demonstration include the use of a pump pulse duration of 280 fs in combination with an echelon mirror. Our results present unmatched combined characteristics and are highly competitive with the existing THz sources pumped at the mJ range. This demonstration…
We present a metamaterial-based terahertz (THz) sensor for thickness measurements of subwavelength-thin materials and refractometry of liquids and liquid mixtures. The sensor operates in reflection geometry and exploits the frequency shift of a sharp Fano resonance minimum in the presence of dielectric materials. We obtained a minimum thickness resolution of 12.5 nm (1/16000 times the wavelength of the THz radiation) and a refractive index sensitivity of 0.43 THz per refractive index unit. We support the experimental results by an analytical model that describes the dependence of the resonance…
The design of a self-complementary metallic checkerboard pattern achieves broadband, dispersion-less, and maximized absorption, concentrating in the deep subwavelength resistive connections between squares, without any theoretical limitation on the energy absorbing area. Here, we experimentally and numerically investigate the electromagnetic response in the limit of extremely small connections. We show that finite conductivity and randomness in a near-self-complementary checkerboard pattern plays a crucial role in producing a frequency-independent energy loss in the terahertz frequency region.…
In this paper, a new structure is proposed which is expected to realize dual-band electromagnetically induced transparency (EIT)-like effect in terahertz spectrum. It can be regarded as a metamaterial of grating-like elements composed of dual-band U-shaped resonators. The near-field coupling between bright modes can produce EIT-like effect. After optimizing the parameters, our numerical simulated results are in good agreement with the theoretical analysis. The EIT-like effect can significantly reduce the group speed near the transparent window, may gain more significant potential applications …
We experimentally study the effect of near field coupling on the transmission of light in terahertz metasurfaces, possessing slightly distinctive SRR resonances. Our results show that the interplay between the strengths of electric and magnetic dipoles, modulates the amplitude of resulting electromagnetically induced transmission, probed under different types of asymmetries in the coupled system. We employ a two-particle model to theoretically study the influence of the near field coupling between bright and quasi-dark modes on the transmission properties of the coupled system and we find an e…
Spatiotemporal Terahertz Emission Nanoscopy of Spintronic Photocurrents
RPTU Kaiserslautern-Landau（凯泽斯劳滕-兰道莱布尼茨理工学院）；Fraunhofer Institute for Industrial Mathematics ITWM（弗劳恩霍夫工业数学研究所）；Freie Universität Berlin（柏林自由大学）；Hangzhou International Innovation Institute, Beihang University（北京航空航天大学杭州国际创新学院）；School of Electronic and Information Engineering, Beihang University（北京航空航天大学电子与信息工程学院）；School of Engineering, Brown University（布朗大学工程学院）；University of Lille, CNRS, Centrale Lille, Université Polytechnique Hauts-de-France（里尔大学、法国国家科学研究中心、中央里尔理工学院、上法兰西高等工业大学联合实验室）；Zhangjiang Laboratory（张江实验室）
Terahertz fields can be dramatically enhanced as they propagate through nanometer-sized slits. The enhancement is mediated by significant accumulation of the induced surface charges on the surrounding metal. This enhancement is shown here to be dynamically modulated and the nanoslits are gradually shunted using a copropagating optical beam. The terahertz fields are found to skirt the nanoscale photo-excited region underneath the slits, scattering to the far field and rigorously mapping the near field.
In recent years several methods to overcome diffraction limit in the far field microscopy have been demonstrated. Still the problem of superresolution is reliably solved only for fluorescent microscopy, giving a resolution of up to 20-30nm. Obtaining the optical resolution lower than 100nm without fluorescent dyes requires using rather slow and complicated technique of scanning near filed optical microscope (SNOM). We propose and demonstrate a method of optical near field acquisition by far-field microscope through observation of nanoparticles Brownian motion in immersion liquid. The resolutio…
We designed and implemented a gradient index metasurface for the in-plane focusing of confined terahertz surface waves. We measured the spatial propagation of the surface waves by two-dimensional mapping of the complex electric field using a terahertz near-field spectroscope. The surface waves were focused to a diameter of 500 \micro m after a focal length of approx. 2 mm. In the focus, we measured a field amplitude enhancement of a factor of 3.
We demonstrate a terahertz (THz) frequency comb that is flexible in terms of its frequency range and the number and spacing of comb lines. We use a combination of near-infrared laser diodes, phase modulation and opto-electronic frequency conversion. The THz comb lines are characterized to be < 10 MHz by resolving the pressure dependent collisional broadening of an ammonia molecule rotational mode.
We theoretically and numerically demonstrate an actively tunable slow light in a hybrid metal-graphene metamaterial in the terahertz (THz) regime. In the unit cell, the near field coupling between the metallic elements including the bright cut wire resonator and the dark double split-ring resonator gives rises to a pronounced transmission peak. By positioning a monolayer graphene under the dark mode resonator, an active modulation of the near field coupling is achieved via shifting the Fermi level of graphene. The physical origin can be attributed to the variation in the damping rate of the da…
High energy terahertz pulses are produced by optical rectification (OR) in organic crystals DAST and DSTMS by a Ti:sapphire amplifier system centered at 0.8 microns. The simple scheme provides broadband spectra between 1 and 5 THz, when pumped by collimated 60 fs near-infrared pump pulse and it is scalable in energy. Fluence-dependent conversion efficiency and damage threshold are reported as well as optimized OR at visible wavelength.
Terahertz (THz) imaging has the ability to see through otherwise opaque materials. However, due to the long wavelengths of THz radiation (λ=300μm at 1THz), far-field THz imaging techniques are heavily outperformed by optical imaging in regards to the obtained resolution. In this work we demonstrate near-field THz imaging with a single-pixel detector. We project a time-varying optical mask onto a silicon wafer which is used to spatially modulate a pulse of THz radiation. The far-field transmission corresponding to each mask is recorded by a single element detector and this data is used to recon…
We are reporting on terahertz generation from organic crystal BNA using a 1.15 to 1.55 um near infrared pump. We observed a very large emission spectrum extending up to 7 THz, compared to 2.5 THz from Ti:Sa pump in previous reports. The maximum optical-to-THz conversion efficiency in our experiment was 0.8% at 1 kHz repetition rate and without saturation leading to a peak electric field of 1 GV/m. Our results show pronounced phase matching privilege for intense terahertz generation using a pump in the 1.15 to 1.25 um range where high energy near infrared pump sources operate.
In this work we report two designs of subwavelength fibers packaged for practical terahertz wave guiding. We describe fabrication, modeling and characterization of microstructured polymer fibers featuring a subwavelength-size core suspended in the middle of a large porous outer cladding. This design allows convenient handling of the subwavelength fibers without distorting their modal profile. Additionally, the air-tight porous cladding serves as a natural enclosure for the fiber core, thus avoiding the need for a bulky external enclosure for humidity-purged atmosphere. Fibers of 5 mm and 3 mm …
We propose a novel scheme to generate single-cycle terahertz (THz) pulses via reflection of an optical femtosecond pulse train from a thin layer of nonlinear resonant medium. Our method is based on a coherent control of low-frequency oscillations and free induction decay in the medium. The specific single-cycle shape of generated THz pulses requires a plane wavefront and detection in the near field. Our theoretical results pave the way to a new, simple and high-efficiency way to generate single-cycle waveshape-tunable terahertz pulses.
We studied the effects on the terahertz transmission of gammadion metamatials by adjusting the size and periodicity of the metamaterial, while keeping the periodicity and size fixed, respectively. The terahertz transmission responses of these metamaterials were analyzed using terahertz time domain spectroscopy as well as finite difference time domain electromagnetic simulations. We have found that increasing size or periodicity results in a red shift of the resonant frequency, and that increasing size or decreasing periodicity results in the formation of a second resonant frequency. We associa…
In ultrabroadband terahertz electro-optic sampling, spectral filtering of the gate pulse can strongly reduce the quantum noise while the signal level is only weakly affected. The concept is tested for phase-matched electro-optic detection of field transients centered at 45 THz with 12-fs near-infrared gate pulses in AgGaS2. Our new approach increases the experimental signal-to-noise ratio by a factor of 3 compared to standard electro-optic sampling. Under certain conditions an improvement factor larger than 5 is predicted by our theoretical analysis.
Carrier conversion from terahertz wave to dual-wavelength near-infrared light injection-locking to optical comb using asynchronous nonpolarimetric electro-optic downconversion with electro-optic polymer modulator
The active control of matter by strong electromagnetic fields is of growing importance, with applications all across the optical spectrum from the extreme-ultraviolet to the far-infrared. In recent years, phase-stable terahertz (THz) fields have shown tremendous potential in the observation and manipulation of elementary excitations in complex systems. The combination of concepts from attosecond science with advanced THz technology facilitates novel spectroscopic schemes, such as THz streaking. In general, driving charges at lower frequency enhances interaction energies and can promote drastic…
We theoretically study the generation of terahertz (THz) radiation by two-color filamentation of ultrashort laser pulses with different wavelengths. We consider wavelengths in the range from 0.6 to 10.6 $μ$m, thus covering the whole range of existing and future powerful laser sources in the near, mid and far-infrared. We show how different parameters of two-color filaments and generated THz pulses depend on the laser wavelength. We demonstrate that there is an optimal laser wavelength for two-color filamentation that provides the highest THz conversion efficiency and results in generation of e…
Near-field optical microscopes with two independent tips for simultaneous excitation and detection can be essential tools for studying localized optical phenomena on the subwavelength scale. Here, we report on the implementation of a fully automated and robust dual-tip scanning near-field optical microscope (SNOM), in which the excitation tip is stationary, while the detection tip automatically scans the surrounding area. To monitor and control the distance between the two probes, mechanical interactions due to shear forces are used. We experimentally investigate suitable scan parameters and f…
The tilted-pulse-front setup utilizing a diffraction grating is one of the most successful methods to generate single- to few-cycle terahertz pulses. However, the generated terahertz pulses have a large spatial inhomogeneity, due to the noncollinear phase matching condition and the asymmetry of the prism-shaped nonlinear crystal geometry, especially when pushing for high optical-to-terahertz conversion efficiency. A 3D+1 (x,y,z,t) numerical model is necessary in order to fully investigate the terahertz generation problem in the tilted-pulse-front scheme. We compare in detail the differences be…
We have developed theory for the interaction of THz radiation with a sub-wavelength metallic grating. The structure of electric fields of the electromagnetic wave under the metallic grating has been studied in the near-field zone. Spatial distributions of the electric field components and the electric energy density have been obtained for the transmitted wave through the grating. An effect of strong local enhancement of the electric field has been detected. Spatial dependences of the polarization of the transmitted wave has been analyzed for the near-field zone.
Terahertz spectral range (frequencies of 0.1-1 THz) has recently emerged as the next frontier for non-destructive imaging, industrial sensing and ultra-fast wireless communications. Here, we review several classes of materials such as simple metals, semiconductors, high-k dielectrics, polar materials, zero gap materials, as well as structured materials that can support strongly localised electromagnetic modes at material interfaces in the Terahertz spectral range. We present the basic theory of surface waves, detail the requirement of strong modal confinement and low loss for the surface waves…
We describe a method to map the standing-wave pattern inside a Fabry-Perot optical cavity with sub-wavelength resolution by perturbing it with a commercially available scanning near-field optical microscope (SNOM) tip. The method is applied to a fiber Fabry-Perot microcavity. We demonstrate its use to determine the relative position of the antinodes at two different wavelengths. In addition, we use the SNOM tip as a point-like source allowing precise positioning of a microscope objective with respect to the cavity mode.
We present a superconducting metamaterial saturable absorber at terahertz frequencies. The absorber consists of an array of split ring resonators (SRRs) etched from a 100nm YBaCu3O7 (YBCO) film. A polyimide spacer layer and gold ground plane are deposited above the SRRs, creating a reflecting perfect absorber. Increasing either the temperature or incident electric field (E) decreases the superconducting condensate density and corresponding kinetic inductance of the SRRs. This alters the impedance matching in the metamaterial, reducing the peak absorption. At low electric fields, the absorption…
Imaging applications in the terahertz (THz) frequency range are severely restricted by diffraction. Near-field scanning probe microscopy is commonly employed to enable mapping of the THz electromagnetic fields with sub-wavelength spatial resolution, allowing intriguing scientific phenomena to be explored such as charge carrier dynamics in nanostructures and THz plasmon-polaritons in novel 2D materials and devices. High-resolution THz imaging, so far, has been relying predominantly on THz detection techniques that require either an ultrafast laser or a cryogenically-cooled THz detector. Here, w…
A proof of concept for high speed near-field imaging with sub-wavelength resolution using SLM is presented. An 8 channel THz detector array antenna with an electrode gap of 100 um and length of 5 mm is fabricated using the commercially available GaAs semiconductor substrate. Each array antenna can be excited simultaneously by spatially reconfiguring the optical probe beam and the THz electric field can be recorded using 8 channel lock-in amplifiers. By scanning the probe beam along the length of the array antenna, a 2D image can be obtained with amplitude, phase and frequency information.
A new principle of subwavelength imaging based on frequency scanning is considered. It is shown that it is possible to reconstruct the spatial profile of an external field exciting an array (or coupled arrays) of subwavelength-sized resonant particles with a frequency scan over the whole band of resonating array modes. During the scan it is enough to measure and store the values of the near field at one or at most two points. After the scan the distribution of the near field can be reconstructed with simple post-processing. The proposed near-field microscope has no moving parts.
High-order harmonic generation by femtosecond laser pulse in the presence of a moderately strong terahertz (THz) field is studied under the strong field approximation, showing a simple proportionality of near-cutoff even-order harmonic (NCEH) amplitude to the THz electric field. The formation of the THz induced-NCEHs is analytically shown for both continuous wave and Gaussian pulse. The perturbation analysis with regard to the frequency ratio of the THz field to the femtosecond pulse shows the THz-induced NCEHs originates from its first-order correction, and the available parametric conditions…
Near-field imaging with terahertz (THz) waves is emerging as a powerful technique for fundamental research in photonics and across physical and life sciences. Spatial resolution beyond the diffraction limit can be achieved by collecting THz waves from an object through a small aperture placed in the near-field. However, light transmission through a sub-wavelength size aperture is fundamentally limited by the wave nature of light. Here, we conceive a novel architecture that exploits inherently strong evanescent THz field arising within the aperture to mitigate the problem of vanishing transmiss…
In this paper the design for an absorbing metamaterial with near unity absorbance in terahertz region is presented. The absorber's unit cell structure consists of two metamaterial resonators that couple to electric and magnetic fields separately. The structure allows us to maximize absorption by varying dielectric material and thickness and, hence the effective electrical permittivity and magnetic permeability.
Terahertz subwavelength imaging aims at developing THz microscopes able to resolve deeply subwavelength features. To improve the spatial resolution beyond the diffraction limit, a current trend is to use various subwavelength probes to convert the near-field to the far-field. These techniques, while offering significant gains in spatial resolution, inherently lack the ability to rapidly obtain THz images due to the necessity of slow pixel-by-pixel raster scan and often suffer from low light throughput. In parallel, in the visible spectral range, several super-resolution imaging techniques were…
Terahertz (THz) near-field imaging is a flourishing discipline [1], with applications from fundamental studies of beam propagation [2,3] to the characterisation of metameterials [4,5] and waveguides [6,7]. Beating the diffraction limit typically involves rastering structures or detectors with length scale shorter than the radiation wavelength; in the THz domain this has been achieved using a number of techniques including scattering tips [8,9] and apertures [10]. Alternatively, mapping THz fields onto an optical wavelength and imaging the visible light removes the requirement for scanning a lo…
Strong-field mid-infrared pump--terahertz (THz) probe spectroscopy has been proven as a powerful tool for light control of different orders in strongly correlated materials. We report the construction of an ultrafast broadband infrared pump--THz probe system in reflection geometry. A two-output optical parametric amplifier is used for generating mid-infrared pulses with GaSe as the nonlinear crystal. The setup is capable of pumping bulk materials at wavelengths ranging from 1.2 $μ$m to 15 $μ$m and beyond, and detecting the subtle, transient photoinduced changes in the reflected electric field …
Bound states in the continuum (BICs) represent a new paradigm in photonics due to the full suppression of radiation losses. However, this suppression has also hampered their direct observation. By using a double terahertz (THz) near-field technique that allows the local excitation and detection of the THz amplitude, we are able to map for the first time the electromagnetic field of BICs over extended areas, unveiling the field-symmetry protection that suppresses far-field radiation. This investigation, done for metasurfaces of dimer rod resonators, reveals the in-plane extension and formation …
The generation of THz radiation from ionizing two-color femtosecond pulses propagating in metallic hollow waveguides filled with Ar is numerically studied. We observe a strong reshaping of the low-frequency part of the spectrum. Namely, after several millimeters of propagation the spectrum is extended from hundreds of GHz up to ~150 THz. For longer propagation distances, nearly single-cycle near-infrared pulses with wavelengths around 4.5 um are obtained by appropriate spectral filtering, with an efficiency of up to 0.25%.
Terahertz radiation by optical rectification has been observed at room temperature in a hydrogen-bonded organic molecular ferroelectric crystal, 2-phenyl malondialdehyde (PhMDA). The radiated electromagnetic wave consisted of a single-cycle terahertz pulse with a temporal width of $\sim$ 0.5 ps. The terahertz radiation amplitude divided by the sample thickness in PhMDA was nearly equivalent to that in a typical terahertz wave emitter ZnTe. This is attributable to a long coherence length in the range of 130 $\sim$ 800 $μ$m for the terahertz radiation from PhMDA. We also discussed the possibilit…
Giant enhancement of terahertz high-harmonic generation by cavity engineering of a three-dimensional Dirac semimetal
TU Dortmund University（多特蒙德工业大学）；CNR-Istituto Nanoscienze（国家研究委员会纳米科学研究所）；Scuola Normale Superiore（比萨高等师范学院）；University of Basel（巴塞尔大学）；Fudan University（复旦大学）；Shanghai Research Center for Quantum Sciences（上海量子科学研究中心）；Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）
Superconducting quantum circuits are one of the leading quantum computing platforms. To advance superconducting quantum computing to a point of practical importance, it is critical to identify and address material imperfections that lead to decoherence. Here, we use terahertz Scanning Near-field Optical Microscopy (SNOM) to probe the local dielectric properties and carrier concentrations of wet-etched aluminum resonators on silicon, one of the most characteristic components of the superconducting quantum processors. Using a recently developed vector calibration technique, we extract the THz pe…
