Despite its fundamental role in the dynamics of compressible fluids, bulk viscosity has received little experimental attention and there remains a paucity of measured data. Acoustic spectroscopy provides a robust and accurate approach to measuring this parameter. Working from the Navier-Stokes model of a compressible fluid one can show that the bulk viscosity makes a significant and measurable contribution to the frequency-squared acoustic attenuation. Here we employ this methodology to determine the bulk viscosity of Millipore water over a temperature range of 7 to 50 degrees Celsius. The measured attenuation spectra are consistent with the theoretical predictions, while the bulk viscosity of water is found to be approximately three times larger than its shear counterpart, reinforcing its significance in acoustic propagation. Moreover, our results demonstrate that this technique can be readily and generally applied to fluids to accurately determine their temperature dependent bulk viscosities.
Acoustic streaming can be generated around sharp structures, even when the acoustic wavelength is much larger than the vessel size. This sharp-edge streaming can be relatively intense, \textcolor{blue}{owing to the strongly focused inertial effect experienced by the acoustic flow near the tip.} We conducted experiments with Particle Image Velocimetry to quantify this streaming flow through the influence of liquid viscosity $ν$, from 1 mm$^2$/s to 30 mm$^2$/s, and acoustic frequency $f$ from 500 Hz to 3500 Hz. Both quantities supposedly influence the thickness of the viscous boundary layer $δ= …
Acoustic wave attenuation due to vibrational and rotational molecular relaxation, under simplifying assumptions of near-thermodynamic equilibrium and absence of molecular dissociations, can be accounted for by specifying a bulk viscosity coefficient $μ_B$. In this paper, we propose a simple frequency-dependent bulk viscosity model which, under such assumptions, accurately captures wave attenuation rates from infrasonic to ultrasonic frequencies in Navier--Stokes and lattice Boltzmann simulations. The proposed model can be extended to any gas mixture for which molecular relaxation timescales an…
This article investigates how the acoustic propulsion of cone-shaped colloidal particles that are exposed to a traveling ultrasound wave depends on the viscosity of the fluid surrounding the particles. Using acoustofluidic computer simulations, we found that the propulsion of such nano- and microcones decreases strongly and even changes sign for increasing shear viscosity. In contrast, we found only a weak dependence of the propulsion on the bulk viscosity. The obtained results are in line with the findings of previous theoretical and experimental studies.
We explore the behaviour of barotropic and irrotational fluids with a small viscosity under the effect of first-order acoustic perturbations. We discuss, following the extant literature, the difficulties in gleaning an acoustic geometry in the presence of viscosity. In order to obviate various technical encumbrances, when viscosity is present, for an extraction of a possible acoustic geometry, we adopted a method of double perturbations, whereby dynamical quantities such as the velocity field and potential undergo a perturbation both in viscosity and in an external acoustic stimulus. The resul…
In this paper we study the motion of a surface gravity wave with viscosity. In particular we prove two well-posedness results. On the one hand, we establish the local solvability in Sobolev spaces for arbitrary dissipation. On the other hand, we establish the global well-posedness in Wiener spaces for a sufficiently large viscosity. These results are the first rigorous proofs of well-posedness for the Dias, Dyachenko \& Zakharov system ({\em Physics Letters A} 2008) modelling gravity waves with viscosity when surface tension is not taken into account.
When an acoustic wave travels in a lossy medium such as a liquid, it progressively transfers its pseudo-momentum to the fluid, which results in a steady acoustic streaming. Remarkably, the phenomenon involves a balance between sound attenuation and shear, such that viscosity vanishes in the final expression of the velocity field. For this reason, the effect of viscosity has long been ignored in acoustic streaming experiments. Here, we show experimentally that the viscosity plays a major role in cavities such as the streaming induced by surface acoustic waves in sessile droplets. We develop a n…
A microscopic model able to describe simultaneously the dynamic viscosity and the self-diffusion coefficient of fluids is presented. This model is shown to emerge from the introduction of fractional calculus in a usual model of condensed matter physics based on an elastic energy functional. The main feature of the model is that all measurable quantities are predicted to depend in a non-trivial way on external parameters (e.g. the experimental set-up geometry, in particular the sample size). On the basis of an unprecedented comparative analysis of a collection of published experimental data, th…
Surface acoustic waves (SAW) can concentrate micro-particles in droplets within seconds. Yet, the mechanism is not clear and existing explanations fail by several orders of magnitude. In this paper, we analyze the effect of fluid viscosity and particle size on SAW-driven collective particle dynamics in droplets. In most of our experiments, the particles do not aggregate but instead remain away from the droplet center, thereby forming "black holes". We show that the black holes are due to steric hindrance wherein the poloidal streamlines that should drive particles to the center of the droplet …
Acoustic Signatures of Pinch-Off Cavities During Water-Entry
College of Shipbuilding Engineering, Harbin Engineering University（哈尔滨工程大学船舶工程学院）；Nanhai Institute of Harbin Engineering University（哈尔滨工程大学南海研究院）；Southampton Ocean Engineering Joint Institute, Harbin Engineering University（哈尔滨工程大学南安普顿海洋工程联合学院）；National Key Lab of Ship Structural Safety, Harbin Engineering University（哈尔滨工程大学船舶结构安全国家重点实验室）
In this letter, we derive the Korteweg-de Vries (KdV) equation corresponding to the surface dynamics of a shallow depth ($h$) two-dimensional fluid with odd viscosity ($ν_o$) subject to gravity ($g$) in the long wavelength weakly nonlinear limit. In the long wavelength limit, the odd viscosity term plays the role of surface tension albeit with opposite signs for the right and left movers. We show that there exists two regimes with a sharp transition point within the applicability of the KdV dynamics, which we refer to as weak $(|ν_o|< \sqrt{gh^3}/6)$ and strong $(|ν_o|> \sqrt{gh^3}/6)$ parity-…
We employ a millimeter-scale piezoelectric acoustic actuator, which generates MHz-frequency surface acoustic waves (SAWs) in a solid substrate, to actively coat a drop of water by a macroscopic film of silicon oil as a paradigm for a small scale and low power coating system. We build upon previous studies on SAW induced dynamic wetting of a solid substrate, also known as the acoustowetting phenomena, to actively drive a model low surface-energy liquid -- silicon oil -- coat a model liquid object -- a sessile drop of water. The oil film spreads along the path of the propagating SAW and comes in…
Acoustic signals generated by filamentation of ultrashort TW laser pulses in water are characterized experimentally. Measurements reveal a strong influence of input pulse duration on the shape and intensity of the acoustic wave. Numerical simulations of the laser pulse nonlinear propagation and the subsequent water hydrodynamics and acoustic wave generation show that the strong acoustic emission is related to the mechanism of superfilamention in water. The elongated shape of the plasma volume where energy is deposited drives the far-field profile of the acoustic signal, which takes the form of…
The aim of this paper is to present a modeling for the rheological behavior of simple liquids as a function of the amplitude of the imposed shear stress or strain. The elastic mode theory (Ref. 6) is first generalized to take into account the fact that during a flow experiment, mechanical energy is injected in a system initially at thermodynamic equilibrium. This generalized theory can be seen as a particular aspect of the general problem of perturbation by the measurement, associated with that of the coupling between fluctuation and dissipation. This generalization leads to a "finitary" chara…
We use both theory and experiment to study the response of {\it partially wetting} films of water and surfactant solutions to a propagating MHz vibration in the solid substrate in the form of a Rayleigh surface acoustic wave (SAW). The SAW invokes a drift of mass in the liquid film, which is associated with the Schlichting boundary layer flow (also known as the Schlichting streaming). We study thin films that are governed by a balance between the drift and capillary stress alone. We demonstrate weak capillary contributions, such as for silicon oil films, support dynamic wetting and lead to the…
The engineering problems involving clay under non-isothermal conditions (e.g., geothermal energy harvest, landfill cover system, and nuclear waste disposal) are multiscale and multiphysics by nature. The nanoscale hydrodynamics of clay at elevated temperature is essential in developing a physics-based multiscale model for clay under non-isothermal conditions. The nonequilibrium molecular dynamics (NEMD) is a useful tool to study the nanoscale hydrodyndamics of clay. This article presents an NEMD modeling of hydrodynamics of clay nanopores at elevated temperatures. Water flow confined in pyroph…
Initially, the acoustic field forced the droplets into an oblate spheroid shape, though the counteracting force of the cooling stream caused them to circularize. Droplet geometry was thus the net result of streaming forces and surface tension at the acoustic boundary layer/air-liquid interface. Nucleation was determined to be neither homogeneous nor heterogeneous but secondary, and thus dependent on the cooling rate and not on the degree of supercooling. It was likely initiated by aerosolized ice particles from the air or from droplets that had already nucleated and broken up. The latter secon…
Using classical as well as ab-initio molecular dynamics simulations, we calculate the frequency-dependent shear viscosity of pure water and water-glycerol mixtures. In agreement with recent experiments, we find deviations from Newtonian-fluid behavior in the THz regime. Based on an extension of the Maxwell model, we introduce a viscoelastic model to describe the observed viscosity spectrum of pure water. We find four relaxation modes in the spectrum which we attribute to i) hydrogen-bond network topology changes, ii) hydrogen-bond stretch vibrations of water pairs, iii) collective vibrations o…
Macro-textured superhydrophobic surfaces can reduce droplet-substrate contact times of impacting water droplets, however, surface designs with similar performance for significantly more viscous liquids are missing, despite their importance in nature and technology such as for chemical shielding, food staining repellency, and supercooled (viscous) water droplet removal in anti-icing applications. Here, we introduce a deterministic, controllable and up-scalable method to fabricate superhydrophobic surfaces with a 3D-printed architecture, combining arrays of alternating surface protrusions and in…
We study a three-wave truncation of a recently proposed damped/forced high-order nonlinear Schrödinger equation for deep-water gravity waves under the effect of wind and viscosity. The evolution of the norm (wave-action) and spectral mean of the full model are well captured by the reduced dynamics. Three regimes are found for the wind-viscosity balance: we classify them according to the attractor in the phase-plane of the truncated system and to the shift of the spectral mean. A downshift can coexist with both net forcing and damping, i.e., attraction to period-1 or period-2 solutions. Upshift…
Separation of bacterial spores from flowing water in macro-scale cavities by ultrasonic standing waves
利用超声波驻波从稳定的水流中分离出微米级的细菌孢子（蜡状芽孢杆菌）。横截面为0.0254 m x 0.0254 m的超声波谐振器设计有用于水流的流动入口和出口，以确保流入和流出流管的谐振器部分的层流条件。一个直径为0.01905米的PZT-4，标称2 MHz的换能器用于在谐振器中产生超声驻波。声谐振器从换能器面到相对的反射器壁为0.0356 m，其中声场在与水流方向正交的方向上。在固定频率激励下，孢子集中在声辐射力的稳定位置处，并被捕获在谐振器区域中。研究了换能器电压和频率对谐振腔中孢子捕获效率的影响。成功分离B。以40-250 ml/min的典型体积流率从水中分离蜡状芽孢，在40 ml/min的单程中获得了15%的效率。
By varying the oil volume fraction, the microscopic droplet size and the macroscopic rheology of emulsions are investigated in a Taylor-Couette (TC) turbulent shear flow. Although here oil and water in the emulsions have almost the same physical properties (density and viscosity), unexpectedly, we find that oil-in-water (O/W) and water-in-oil (W/O) emulsions have very distinct hydrodynamic behaviors, i.e., the system is clearly asymmetric. By looking at the micro-scales, the average droplet diameter hardly changes with the oil volume fraction neither for O/W nor for W/O. However, for W/O it is…
Nanofluidics is an emerging field offering innovative solutions for energy harvesting and desalination. The efficiency of these applications depends strongly on liquid-solid slip, arising from a favorable ratio between viscosity and interfacial friction. Using molecular dynamics simulations, we show that wall slip increases strongly when water is cooled below its melting point. For water on graphene, the slip length is multiplied by up to a factor of five and reaches $230$nm at the lowest simulated temperature, $T \sim 225$K; experiments in nanopores can reach much lower temperatures and could…
This paper describes a simple and inexpensive method of measuring viscosity of a Newtonian fluid using the ball drop technique and an inexpensive point and shoot ~1000 frame per second camera. We successfully measured the viscosity of glycerol and glycerol-water mixture with high precision. We used three different size copper balls of diameters 0.8 mm, 1.59 mm, and 2.38 mm to check the accuracy of the measured viscosity in different concentrations of glycerol-water mixer solutions ranging from 50% to 100% (pure glycerol). Our measurements are in excellent agreement with the measurements conduc…
