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arXiv 0909.1956cond-mat.mes-hall
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分子磁体的共振隧穿和近藤隧穿

Resonant and Kondo tunneling through molecular magnets

Florian Elste, Carsten Timm

摘要:

通过分子磁体的运输研究在政权的强耦合的铅。我们考虑一个共振隧穿模型,其中量子点或分子中的电子自旋通过交换相互作用耦合到另外的局部各向异性自旋。两个相反的制度占主导地位的共振隧穿和近藤运输,分别被认为是。在共振隧穿制度,杂质自旋的定态计算任意强的分子铅耦合使用主方程的方法,它对待交换相互作用微扰。我们发现,即使杂化能量超过热能,微分电导中的特征精细结构仍然存在。运输近藤政权内的图解方法进行了研究。我们表明,磁各向异性引起分裂的近藤峰在低偏置电压。

英文摘要:

Transport through molecular magnets is studied in the regime of strong coupling to the leads. We consider a resonant-tunneling model where the electron spin in a quantum dot or molecule is coupled to an additional local, anisotropic spin via exchange interaction. The two opposite regimes dominated by resonant tunneling and by Kondo transport, respectively, are considered. In the resonant-tunneling regime, the stationary state of the impurity spin is calculated for arbitrarily strong molecule-lead coupling using a master-equation approach, which treats the exchange interaction perturbatively. We find that the characteristic fine structure in the differential conductance persists even if the hybridization energy exceeds thermal energies. Transport in the Kondo regime is studied within a diagrammatic approach. We show that magnetic anisotropy gives rise to a splitting of the Kondo peak at low bias voltages.

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