We performed an experimental test of the Kochen-Specker theorem based on an inequality derived from the Peres-Mermin proof, using spin-path (momentum) entanglement in a single neutron system. Following the strategy proposed by Cabello et al. [Phys. Rev. Lett. 100, 130404 (2008)], a Bell-like state was generated and three expectation values were determined. The observed violation 2.291 +/- 0.008 > 1 clearly shows that quantum mechanical predictions cannot be reproduced by noncontextual hidden variables theories.
Previous experimental tests of quantum contextuality based on the Bell-Kochen-Specker (BKS) theorem have demonstrated that not all observables among a given set can be assigned noncontextual eigenvalue predictions, but have never identified which specific observables must fail such assignment. We now remedy this shortcoming by showing that BKS contextuality can be confined to particular observables by pre- and postselection, resulting in anomalous weak values that we measure using modern neutron interferometry. We construct a confined contextuality witness from weak values, which we measure ex…
We show that an experimental demonstration of quantum contextuality using 2 degrees of freedom of single neutrons based on a violation of an inequality derived from the Peres-Mermin proof of the Kochen-Specker theorem would be more conclusive than those obtained from previous experiments involving pairs of ions [M. A. Rowe et al., Nature (London) 409, 791 (2001)] and single neutron [Y. Hasegawa et al., Nature (London) 425, 45 (2003)] based on violations of Clauser-Horne-Shimony-Holt-like inequalities.
We report a single-neutron optical experiment to demonstrate the violation of a Bell-like inequality. Entanglement is achieved not between particles, but between the degrees of freedom, in this case, for a single-particle. The spin-{\small 1/2} property of neutrons are utilized. The total wave function of the neutron is described in a tensor product Hilbert space. A Bell-like inequality is derived not by a non-locality but by a contextuality. Joint measurements of the spinor and the path properties lead to the violation of a Bell-like inequality. Manipulation of the wavefunction in one Hilbert…
Entanglement between degrees of freedom, namely between the spin, path and (total) energy degrees of freedom, for single neutrons is exploited. We implemented a triply entangled Greenberger-Horne-Zeilinger(GHZ)-like state and coherently manipulated relative phases of two-level quantum subsystems. An inequality derived by Mermin was applied to analyze the generated GHZ-like state: we determined the four expectation values and finally obtained M=2.558 +/- 0.004 which is clearly above the threshold of 2. This demonstrates the violation of a Mermin-like inequality for triply entangled GHZ-like sta…
We develop an operator-based description of two types of multimode-entangled single-neutron quantum optical devices: Wollaston prisms and radio-frequency spin flippers in inclined magnetic field gradients. This treatment is similar to the approach used in quantum optics, and is convenient for the analysis of quantum contextuality measurements in certain types of neutron interferometers. We describe operationally the way multimode-entangled single-neutron states evolve in these devices, and provide expressions for the associated operators describing the dynamics, in the limit in which the neutr…
A neutron interferometric test of interaction-free detection of the presence of an absorbing object in one arm of a neutron interferometer has been performed. Despite deviations from the ideal performance characteristics of a Mach-Zehnder interferometer it could be shown that information is obtained without interaction.
We analyse a recently reported neutron interference experiment to measure a geometric phase and attempt to bring out the inadequacy of the ``phase modulo 2π" approach to the geometric phase. A modified neutron interferometer experiment to observe 2nπphase changes of topological origin resulting from closed circuits around singularities in the parameter space of the experiment is proposed.
The energy eigenstates of a spin$-\frac{1}{2}$ particle in a magnetic field confined to a plane, define a planar spin. If the particle moves adiabatically around a loop in this plane, it picks up a topological Berry phase that can only be an integer multiple of $π$. We propose a neutron interferometry test of the Berry phase for a circulating planar spin induced by a magnetic field caused by a very long current-carrying straight wire perpendicular to the plane. This Berry phase causes destructive interference in the direction of the incoming beam of thermal neutrons moving through a triple-Lau…
We analyze the coherence properties of polarized neutrons, after they have interacted with a magnetic field or a phase shifter undergoing different kinds of statistical fluctuations. We endeavor to probe the degree of disorder of the distribution of the phase shifts by means of the loss of quantum mechanical coherence of the neutron. We find that the notion of entropy of the shifts and that of decoherence of the neutron do not necessarily agree. In some cases the neutron wave function is more coherent, even though it has interacted with a more disordered medium.
We have observed the stationary interference oscillations of a triple-entangled neutron state in an interferometric experiment. Time-dependent interaction with two radio-frequency (rf) fields enables coherent manipulation of an energy degree of freedom in a single neutron. The system is characterized by a multiply entangled state governed by a Jaynes-Cummings Hamiltonian. The experimental results confirm coherence of the manipulation as well as the validity of the description.
The Kochen-Specker theorem theoretically shows evidence of the incompatibility of noncontextual hidden variable theories with quantum mechanics. Quantum contextuality is a more general concept than quantum non-locality which is quite well tested in experiments by using Bell inequalities. Within neutron interferometry we performed an experimental test of the Kochen-Specker theorem with an inequality, which identifies quantum contextuality, by using spin-path entanglement in a single neutron system. Here entanglement is achieved not between different particles, but between degrees of freedom, i.…
We study two different decoherence modes for entangled qubits by considering a Liouville - von Neumann master equation. Mode A is determined by projection operators onto the eigenstates of the Hamiltonian and mode B by projectors onto rotated states. We present solutions for general and for Bell diagonal states and calculate for the later the mixedness and the amount of entanglement given by the concurrence. We propose a realization of the decoherence modes within neutron interferometry by applying fluctuating magnetic fields. An experimental test of the Kraus operator decomposition describing…
Bragg diffraction is comparable to a hard-wall reflection if the Bragg condition is exactly fulfilled. However, in a neutron interferometer in the gravitational field (COW experiment) this is not the case and the momentum transfers should not be described by hard wall reflection, as it has been done in the commented article. Instead, and quite similar to the atom case, each mirror or beam splitter creates a constant momentum transfer given by the reciprocal lattice vector of the Bragg crystal. To lowest order there are no differences between the atom and the neutron case.
Einstein's theory of general relativity and quantum theory form the two major pillars of modern physics. However, certain inertial properties of a particle's intrinsic spin are inconspicuous while the inertial properties of mass are well known. Here, by performing a neutron interferometric experiment, we observe phase shifts arising as a consequence of the spin's coupling with the angular velocity of a rotating magnetic field. The resulting phase shifts linearly depend on the frequency of the rotation of the magnetic field. Our results agree well with the predictions derived from the Pauli - S…
The question of whether quantum phenomena can be explained by classical models with hidden variables is the subject of a long lasting debate. In 1964, Bell showed that certain types of classical models cannot explain the quantum mechanical predictions for specific states of distant particles. Along this line, some types of hidden variable models have been experimentally ruled out. An intuitive feature for classical models is non-contextuality: the property that any measurement has a value which is independent of other compatible measurements being carried out at the same time. However, the res…
In neutron interferometric experiments using polarized neutrons coherent spin-rotation control is required. In this letter we present a new method for Larmor spin-rotation around an axis parallel to the outer guide field using topology optimized 3D printed magnets. The use of 3D printed magnets instead of magnetic coils avoids unwanted inductances and offers the advantage of no heat dissipation, which prevents potential loss in interferometric contrast due to temperature gradients in the interferometer. We use topology optimization to arrive at a design of the magnet geometry that is optimized…
We present a detailed analysis of the time series of time-stamped neutron counts obtained by single-neutron interferometry. The neutron counting statistics display the usual Poissonian behavior, but the variance of the neutron counts does not. Instead, the variance is found to exhibit a dependence on the phase-shifter setting which can be explained by a probabilistic model that accounts for fluctuations of the phase shift. The time series of the detection events exhibit long-time correlations with amplitudes that also depend on the phase-shifter setting. These correlations appear as damped osc…
We present a split-beam neutron interferometric experiment to test the non-cyclic geometric phase tied to the spatial evolution of the system: the subjacent two-dimensional Hilbert space is spanned by the two possible paths in the interferometer and the evolution of the state is controlled by phase shifters and absorbers. A related experiment was reported previously by some of the authors [Hasegawa et al., PRA 53, 2486 (1996)] to verify the cyclic spatial geometric phase. The interpretation of this experiment, namely to ascribe a geometric phase to this particular state evolution, has met seve…
A discrete-event approach, which has already been shown to give a cause-and-effect explanation of many quantum optics experiments, is applied to single-neutron interferometry experiments. The simulation algorithm yields a logically consistent description in terms of individual neutrons and does not require the knowledge of the solution of a wave equation. It is shown that the simulation method reproduces the results of several single-neutron interferometry experiments, including experiments which, in quantum theoretical language, involve entanglement. Our results demonstrate that classical (no…
In 1975, two experimental groups have independently observed the 4$π$-symmetry of neutrons' spin, when passing through a static magnetic field, using a three-blade interferometer made from a single perfect Si-crystal (analogous to the Mach-Zehnder interferometer of light optics). In this article, we provide a complete analysis of the experiment, both from a theoretical and conceptual point of view. Firstly, we solve the Schrödinger equation in the weak potential approximation, to obtain the amplitude of the refracted and forward refracted beams, produced by the passage of neutrons through one …
We analyze the dynamics of neutron beams in interferometry experiments using quantum dynamical semigroups. We show that these experiments could provide stringent limits on the non-standard, dissipative terms appearing in the extended evolution equations.
We illustrate how geometric gauge forces and topological phase effects emerge in quantum systems without employing assumptions that rely on adiabaticity. We show how geometric magnetism may be harnessed to engineer novel quantum devices including a velocity sieve, a component in mass spectrometers, for neutral atoms or neutrons. We outline a possible experimental setup that demonstrates topological interferometry for neutral spin 1/2 systems.
We consider tests of short-distance modifications of gravity based on neutron interferometry in the scenario of large extra dimensions. Avoiding the non-computability problem in the calculation of the internal gravitational potential of extended sources, typical of models with zero-width brane, we determine the neutron optical potential associated with the higher-dimension gravitational interaction between the incident neutron and a material medium in the context of thick brane theories. Proceeding this way, we identify the physical quantity of the extra dimension model that the neutron interf…
Perfect single-crystal neutron interferometers are adversely sensitive to environmental disturbances, particularly mechanical vibrations. The sensitivity to vibrations results from the slow velocity of thermal neutrons and the long measurement time that are encountered in a typical experiment. Consequently, to achieve a good interference solutions for reducing vibration other than those normally used in optical experiments must be explored. Here we introduce a geometry for a neutron interferometer that is less sensitive to low-frequency vibrations. This design may be compared with both dynamic…
If scattering amplitudes are ordinary complex numbers (not quaternions) there is a universal algebraic relationship between the six coherent cross sections of any three scatterers (taken singly and pairwise). A violation of this relationship would indicate either that scattering amplitudes are quaternions, or that the superposition principle fails. Some possible experimental tests involve neutron interferometry, K_S-meson regeneration, and low energy proton-proton scattering.
We present phase shift measurements for neutron matter waves in vacuum and in low pressure Helium using a method originally developed for neutron scattering length measurements in neutron interferometry. We search for phase shifts associated with a coupling to scalar fields. We set stringent limits for a scalar chameleon field, a prominent quintessence dark energy candidate. We find that the coupling constant $β$ is less than 1.9 $\times10^7$~for $n=1$ at 95\% confidence level, where $n$ is an input parameter of the self--interaction of the chameleon field $φ$ inversely proportional to $φ^n$.
In recent years there has been an enormous progress in matter wave interferometry. The Colella- Overhauser-Werner (COW) type of neutron interferometer and the Kasevich-Chu (K-C) atom interferometer, are the prototype of such devices and the issue of whether they are sensitive to relativistic effects has recently aroused much controversy. We examine the question of to what extent the gravitational red shift, and the related twin paradox effect can be seen in both of these atom and neutron interferometers. We point out an asymmetry between the two types of devices. Because of this, the non-vanis…
A zero-area four-blade perfect crystal neutron interferometer (NI) possess a decoherence-free subspace (DFS) for low-frequency mechanical vibrations and thus is easier to site. %has the potential to broaden the application of crystal-based neutron interferometry to a higher number of neutron sources. However, unlike the standard three-blade Mach-Zehnder NI the ideal contrast of this four-blade NI geometry is less than one. By applying a recently introduced quantum information model for dynamical diffraction we show that the contrast for the four-blade DFS NI can be increased by offsetting the …
We discuss a discrete-event simulation approach, which has been shown to give a unified cause-and-effect description of many quantum optics and single-neutron interferometry experiments. The event-based simulation algorithm does not require the knowledge of the solution of a wave equation of the whole system, yet reproduces the corresponding statistical distributions by generating detection events one-by-one. It is showm that single-particle interference and entanglement, two important quantum phenomena, emerge via information exchange between individual particles and devices such as beam spli…
Ongoing fascination with quantum mechanics keeps driving the development of the wide field of quantum-optics, including its neutron-optics branch. Application of neutron-optical methods and, especially, neutron interferometry and polarimetry has a long-standing tradition for experimental investigations of fundamental quantum phenomena. We give an overview of related experimental efforts made in recent years.
We start from Feynman`s idea to use negative probabilities to describe the two slit experiment and other quantum interfernce experiments. Formally by using negative probability distributions we can explain the results of the two slit experiment on the basis of the pure corpuscular picture of quantum mechnanics. However, negative probabilities are absurd objects in the framework of the standard Kolmogorov theory of probability. We present a large class of non-Kolmogorovean probability models where negative probabilities are well defined on the frequency basis. These are models with probabilitie…
The development of direct probes of entanglement is integral to the rapidly expanding field of complex quantum materials. Here we test the robustness of entangled neutrons as a quantum probe by measuring the Clauser-Horne-Shimony-Holt contextuality witness while varying the beam properties. Specifically, we prove that the entanglement of the spin and path subsystems of individual neutrons prepared in two different experiments using two different apparatuses persists even after varying the entanglement length, coherence length, and neutron energy difference of the paths. The two independent app…
Complex molecules are intriguing objects at the interface between quantum and classical phenomena. Compared to the electrons, neutrons, or atoms studied in earlier matter-wave experiments, they feature a much more complicated internal structure, but can still behave as quantum objects in their center-of-mass motion. Molecules may involve a large number of vibrational modes and highly excited rotational states, they can emit thermal photons, electrons, or even atoms, and they exhibit large cross sections for collisional interactions with residual background gases. This makes them ideal candidat…
We review an event-based simulation approach which reproduces the statistical distributions of wave theory not by requiring the knowledge of the solution of the wave equation of the whole system but by generating detection events one-by-one according to an unknown distribution. We illustrate its applicability to various single photon and single neutron interferometry experiments and to two Bell test experiments, a single-photon Einstein-Podolsky-Rosen experiment employing post-selection for photon pair identification and a single-neutron Bell test interferometry experiment with nearly $100\%$ …
High contrast matter-wave interferometry is essential in various fundamental quantum mechanical experiments as well as for technical applications. Thereby, contrast and sensitivity are typically reduced by decoherence and dephasing effects. While decoherence accounts for a general loss of quantum information in a system due to entanglement with the environment, dephasing is due to collective time-dependent external phase shifts, which can be related to temperature drifts, mechanical vibrations or electromagnetic oscillations. In contrast to decoherence, dephasing can in principle be reversed. …
For precise measurements with polarized neutrons high efficient spin-manipulation is required. We developed several neutron optical elements suitable for a new sophisticated setup, i.e., DC spin-turners and Larmor-accelerators which diminish thermal disturbances and depolarisation considerably. The gain in performance is exploited demonstrating violation of a Bell-like inequality for a spin-path entangled single-neutron state. The obtained value of S=2.365(13), which is much higher than previous measurements by neutron interferometry, is 28 $σ$ above the limit of S=2 predicted by contextual hi…
We propose an experimental approach to {\it macro}scopically test the Kochen-Specker theorem (KST) with superconducting qubits. This theorem, which has been experimentally tested with single photons or neutrons, concerns the conflict between the contextuality of quantum mechnaics (QM) and the noncontextuality of hidden-variable theories (HVTs). We first show that two Josephson charge qubits can be controllably coupled by using a two-level data bus produced by a Josephson phase qubit. Next, by introducing an approach to perform the expected joint quantum measurements of two separated Josephson …
Pendellösung length-scale neutron and X-ray interferometry
Institute for Quantum Computing, University of Waterloo（滑铁卢大学量子计算研究所）；Department of Physics and Astronomy, University of Waterloo（滑铁卢大学物理与天文学系）；Department of Chemistry, University of Waterloo（滑铁卢大学化学系）；Centre for Cold Matter, Blackett Laboratory, Imperial College London（伦敦帝国理工学院布莱克特实验室冷物质中心）；Diamond Light Source Ltd.（钻石光源有限公司）；Neutron Scattering Division, Oak Ridge National Laboratory（橡树岭国家实验室中子散射部）；National Institute of Standards and Technology（美国国家标准与技术研究院）；Physics Department, University of Toronto（多伦多大学物理系）；STFC-Rutherford Appleton Laboratory, ISIS Facility（STC-鲁瑟福阿普尔顿实验室ISIS设施）；Department of Physics, University at Buffalo, State University of New York（纽约州立大学布法罗分校物理系）
Optics and interferometry with matter waves is the art of coherently manipulating the translational motion of particles like neutrons, atoms and molecules. Coherent atom optics is an extension of techniques that were developed for manipulating \emph{internal} quantum states. Applying these ideas to translational motion required the development of techniques to localize atoms and transfer population coherently between distant localities. In this view position and momentum are (continuouse) quantum mechanical degree of freedom analogous to discrete internal quantum states. In our contribution we…
The analysis of phase shifts in executed and proposed interferometry experiments on photons and neutrons neglected forces exerted at the boundaries of spatial constrictions. When those forces are included it is seen that the observed phenomena are not in fact geometric in nature. A new proposal to be published by Allman et al. avoids that pitfall.
It is shown that discrete-event simulation accurately reproduces the experimental data of a single-neutron interferometry experiment [T. Denkmayr {\sl et al.}, Nat. Commun. 5, 4492 (2014)] and provides a logically consistent, paradox-free, cause-and-effect explanation of the quantum Cheshire cat effect without invoking the notion that the neutron and its magnetic moment separate. Describing the experimental neutron data using weak-measurement theory is shown to be useless for unravelling the quantum Cheshire cat effect.
A novel method was recently proposed and experimentally realized for characterizing a quantum state by directly measuring its complex probability amplitudes in a particular basis using so-called weak values. Recently Vallone and Dequal showed theoretically that weak measurements are not a necessary condition to determine the weak value [Phys. Rev. Lett. 116, 040502 (2016)]. Here we report a measurement scheme used in a matter-wave interferometric experiment in which the neutron path system's quantum state was characterized via direct measurements using both strong and weak interactions. Experi…
The joint realm of quantum mechanics and the general-relativistic description of gravitation is becoming increasingly accessible to terrestrial experiments and observations. In this essay we study the emerging indications of the violation of equivalence principle (VEP). While the solar neutrino anomaly may find its natural explanation in a VEP, the statistically significant discrepancy observed in the gravitationally induced phases of neutron interferometry seems to be the first indication of a VEP. However, such a view would seem immediately challenged by the atomic interferometry results. Th…
In a July 2014 Nature Communications paper, Denkmayr et al. claim to have instantiated the so-called quantum Cheshire Cat experiment using neutron interferometry. Crucial to this claim are the weak values which must imply the quantum Cheshire Cat interpretation, i.e., "the neutron and its spin are spatially separated" in their experiment. While they measured the correct weak values for the quantum Cheshire Cat interpretation, the corresponding implications do not obtain because, as we show, those weak values were measured with both a quadratic and a linear magnetic field Bz interaction. We sho…
A recent neutron interferometry experiment claims to demonstrate a paradoxical phenomena dubbed the "quantum Cheshire Cat" \cite{Denkmayr2014}. We have reproduced and extended these results with an equivalent optical interferometer. The results suggest that the photon travels through one arm of the interferometer, while its polarization travels through the other. However, we show that these experimental results belong to the domain where quantum and classical wave theories coincide; there is nothing uniquely quantum about the illusion of this cheshire cat.
Among the known particles, the neutron takes a special position, as it provides experimental access to all four fundamental forces and a wide range of hypothetical interactions. Despite being unstable, free neutrons live long enough to be used as test particles in interferometric, spectroscopic, and scattering experiments probing low-energy scales. As was already recognized in the 1970s, fundamental concepts of quantum mechanics can be tested in neutron interferometry using silicon perfect-single-crystals. Besides allowing for tests of uncertainty relations, Bell inequalities and alike, neutro…
The development of qualitatively new measurement capabilities is often a prerequisite for critical scientific and technological advances. The dramatic progress made by modern probe techniques to uncover the microscopic structure of matter is fundamentally rooted in our control of two defining traits of quantum mechanics: discreteness of physical properties and interference phenomena. Magnetic Resonance Imaging, for instance, exploits the fact that protons have spin and can absorb photons at frequencies that depend on the medium to image the anatomy and physiology of living systems. Scattering …
This paper discusses a possible resolution of the nonobjectivity-nonlocality dilemma in quantum mechanics in 'the light of experimental tests of the Bell inequality for two entangled photons and a Bell-like inequality for a single neutron. My conclusion is that these experiments show that quantum mechanics is nonobjective: that is, the values of physical observables cannot be assigned to a system before measurement. Bell's assumption of nonlocality has to be rejected as having no direct experimental confirmation, at least thus far. I also consider the relationships between nonobjectivity and c…
