S. J. Kuhn, S. McKay, J. Shen, N. Geerits, R. M. Dalgliesh, E. Dees, A. A. M. Irfan, F. Li, S. Lu, V. Vangelista, D. V. Baxter, G. Ortiz, S. R. Parnell, W. M. Snow, R. Pynn
The development of direct probes of entanglement is integral to the rapidly expanding field of complex quantum materials. Here we test the robustness of entangled neutrons as a quantum probe by measuring the Clauser-Horne-Shimony-Holt contextuality witness while varying the beam properties. Specifically, we prove that the entanglement of the spin and path subsystems of individual neutrons prepared in two different experiments using two different apparatuses persists even after varying the entanglement length, coherence length, and neutron energy difference of the paths. The two independent apparatuses acting as entangler-disentangler pairs are static-field magnetic Wollaston prisms and resonance-field radio frequency flippers. Our results show that the spatial and energy properties of the neutron beam may be significantly altered without reducing the contextuality witness value below the Tsirelson bound, meaning that maximum entanglement is preserved. We also show that two paths may be considered distinguishable even when separated by less than the neutron coherence length. This work is the key step in the realization of the new modular, robust technique of entangled neutron scattering.
We consider two ensembles of qubit dissipating into two overlapping environments, that is with a certain number of qubit in common that dissipate into both environments. We then study the dynamics of bipartite entanglement between the two ensembles by excluding the common qubit. To get analytical solutions for an arbitrary number of qubit we consider initial states with a single excitation and show that the largest amount of entanglement can be created when excitations are initially located among side (non common) qubit. Moreover, the stationary entanglement exhibits a monotonic (resp. non-mon…
Entanglement generated from polar molecules of two-dimensional rotation is investigated in a static electric field. The electric field modulates the rotational properties of molecules, leading to distinctive entanglement. The concurrence is used to estimate the degree of entanglement. When the electric field is applied parallel or perpendicular to the intermolecular direction, the concurrences reveal two overlapping features. Such a pronounced signature corresponds to the coexistence of all Bell-like states. The characteristics of Bell-like states and overlapping concurrences are kept independ…
We demonstrate how quantum entanglement can be directly witnessed in the quasi-1D Heisenberg antiferromagnet KCuF$_3$. We apply three entanglement witnesses --- one-tangle, two-tangle, and quantum Fisher information --- to its inelastic neutron spectrum, and compare with spectra simulated by finite-temperature density matrix renormalization group (DMRG) and classical Monte Carlo methods. We find that each witness provides direct access to entanglement. Of these, quantum Fisher information is the most robust experimentally, and indicates the presence of at least bipartite entanglement up to at …
We compute the proton-neutron entanglement entropy in the interacting nuclear shell model for a variety of nuclides and interactions. Some results make intuitive sense, for example that the shell structure, as governed by single-particle and monopole energies, strongly affects the energetically available space and thus the entanglement entropy. We also find a surprising result: that the entanglement entropy at low excitation energy tends to decrease for nuclides when $N \neq Z$. While we provide evidence this arises from the physical nuclear force by contrasting with random two-body interactio…
We present experimental evidence of the generation of distinct types of genuine multipartite entanglement between three degrees of freedom, two internal and one external degree of freedom, within single-neutron quantum systems. This is achieved via the development of new spin manipulation apparatuses for neutron interferometry and the genuine multipartite entanglement is detected via appropriately designed and optimized non-linear witnesses. Via the applied criteria we reveal even finer properties of the type of the genuine multipartite entanglement that is produced in the experiment. In a sub…
It is now experimentally possible to entangle thousands of qubits, and efficiently measure each qubit in parallel in a distinct basis. To fully characterize an unknown entangled state of $n$ qubits, one requires an exponential number of measurements in $n$, which is experimentally unfeasible even for modest system sizes. By leveraging (i) that single-qubit measurements can be made in parallel, and (ii) the theory of perfect hash families, we show that all $k$-qubit reduced density matrices of an $n$ qubit state can be determined with at most $e^{\mathcal{O}(k)} \log^2(n)$ rounds of parallel me…
Violation of a Bell-like inequality for a spin-energy entangled neutron state has been confirmed in a polarimetric experiment. The proposed inequality, in Clauser-Horne-Shimony-Holt (CHSH) formalism, relies on correlations between the spin and energy degree of freedom in a single-neutron system. The entangled states are generated utilizing a suitable combination of two radio-frequency fields in a neutron polarimeter setup. The correlation function S is determined to be 2.333+/-0.005, which violates the Bell-like CHSH inequality by more than 66 standard deviations.
Entanglement between degrees of freedom, namely between the spin, path and (total) energy degrees of freedom, for single neutrons is exploited. We implemented a triply entangled Greenberger-Horne-Zeilinger(GHZ)-like state and coherently manipulated relative phases of two-level quantum subsystems. An inequality derived by Mermin was applied to analyze the generated GHZ-like state: we determined the four expectation values and finally obtained M=2.558 +/- 0.004 which is clearly above the threshold of 2. This demonstrates the violation of a Mermin-like inequality for triply entangled GHZ-like sta…
We discuss a discrete-event simulation approach, which has been shown to give a unified cause-and-effect description of many quantum optics and single-neutron interferometry experiments. The event-based simulation algorithm does not require the knowledge of the solution of a wave equation of the whole system, yet reproduces the corresponding statistical distributions by generating detection events one-by-one. It is showm that single-particle interference and entanglement, two important quantum phenomena, emerge via information exchange between individual particles and devices such as beam spli…
This letter details a simple scheme to entangle two neutrons by successive scattering from a macroscopic sample. In zero magnetic field the entanglement falls as the sample size increases. However, by applying a field and tuning the momentum of the neutrons, one can achieve a substantial degree of entanglement irrespective of the size of the sample.
For both cases with and without interactions, bipartite entanglement of two-fermions from a Fermi gas in a trap is investigated. We show how the entanglement depends on the locations of the two fermions and the total number of particles. Fermions at the verge of trap have longer entanglement distance (beyond it, the entanglement disappears) than those in the center. We derive a lower limitation to the average overlapping for two entangled fermions in the BCS ground state, it is shown to be $\sqrt{Q/2M}$, a function of Cooper pair number $Q$ and total number of occupied energy levels $M$.
The development of qualitatively new measurement capabilities is often a prerequisite for critical scientific and technological advances. The dramatic progress made by modern probe techniques to uncover the microscopic structure of matter is fundamentally rooted in our control of two defining traits of quantum mechanics: discreteness of physical properties and interference phenomena. Magnetic Resonance Imaging, for instance, exploits the fact that protons have spin and can absorb photons at frequencies that depend on the medium to image the anatomy and physiology of living systems. Scattering …
Centre for Quantum Technologies（量子技术中心）；Nanyang Technological University（南洋理工大学）；School of Electrical and Electronic Engineering, Nanyang Technological University（南洋理工大学电气与电子工程学院）；Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University（南洋理工大学物理与数学科学学院物理与应用物理系）；Weifang University（潍坊学院）；Singapore University of Technology and Design（新加坡科技设计大学）；Universität Siegen（锡根大学）
We demonstrate that inelastic neutron scattering technique can be used to indirectly detect and measure the macroscopic quantum correlations quantified by both entanglement and discord in a quantum magnetic material, VODPO4 . 1D2O. The amount of quantum correlations is obtained 2 by analyzing the neutron scattering data of magnetic excitations in isolated V4+ spin dimers. Our quantitative analysis shows that the critical temperature of this material can reach as high as Tc = 82.5 K, where quantum entanglement drops to zero. Significantly, quantum discord can even survive at Tc = 300 K and may …
Photon-nucleon entanglement in Compton scattering at low and high energies
Physics Department, Brookhaven National Laboratory（布鲁克海文国家实验室物理系）；RIKEN BNL Research Center, Brookhaven National Laboratory（理化学研究所布鲁克海文研究中心）；Université Paris-Saclay - CEA - IRFU（巴黎萨克雷大学-法国原子能和替代能源委员会-核物理研究所）；Center for Frontiers in Nuclear Science, Stony Brook University（纽约州立大学石溪分校核科学前沿中心）
The characterization of quantum information quantifiers has attracted a considerable attention of the scientific community, since they are a useful tool to verify the presence of quantum correlations in a quantum system. In this context, in the present work we show a theoretical study of some quantifiers, such as entanglement witness, entanglement of formation, Bell's inequality violation and geometric quantum discord as a function of the diffractive properties of neutron scattering. We provide one path toward identifying the presence of quantum correlations and quantum nonlocality in a molecu…
A discrete-event approach, which has already been shown to give a cause-and-effect explanation of many quantum optics experiments, is applied to single-neutron interferometry experiments. The simulation algorithm yields a logically consistent description in terms of individual neutrons and does not require the knowledge of the solution of a wave equation. It is shown that the simulation method reproduces the results of several single-neutron interferometry experiments, including experiments which, in quantum theoretical language, involve entanglement. Our results demonstrate that classical (no…
In this paper, we consider the quantum correlations, coherence and entanglement, in neutrino oscillation. We find that the $l_{1}$-norm as a coherence measure is equal to sum of the three possible concurrences for measuring the entanglement among different flavor modes which were calculated in the paper by (M. Blasone et al., Europhys. Lett., {\bf 112}, 20007). Our result shows that the origin of the flavor entanglement in neutrino oscillation is the same as that of quantum coherence. Furthermore, in the wave packet framework, the variation of $l_{1}$-norm is investigated by varying the wave p…
Clustered quantum materials provide a new platform for the experimental study of many-body entanglement. Here we address a simple model of a single-molecule nano-magnet featuring N interacting spins in a transverse field. The field can induce an entanglement transition (ET). We calculate the magnetisation, low-energy gap and neutron-scattering cross-section and find that the ET has distinct signatures, detectable at temperatures as high as 5% of the interaction strength. The signatures are stronger for smaller clusters.
We report on criteria to detect entanglement between the light modes of two crossed optical cavities by analyzing the transverse deflection patterns of an atomic beam. The photon exchange between the modes and the atoms occurs around the overlapping nodes of associated standing waves, which generates the two-dimensional (2D) version of the Optical Stern-Gerlach (OSG) effect. In this optical cross-cavity setup, we show that the discrete signatures of the fields states, left in the momentum distribution of the deflected atoms, may reveal entanglement for a certain class of two-mode states. For a…
We report a single-neutron optical experiment to demonstrate the violation of a Bell-like inequality. Entanglement is achieved not between particles, but between the degrees of freedom, in this case, for a single-particle. The spin-{\small 1/2} property of neutrons are utilized. The total wave function of the neutron is described in a tensor product Hilbert space. A Bell-like inequality is derived not by a non-locality but by a contextuality. Joint measurements of the spinor and the path properties lead to the violation of a Bell-like inequality. Manipulation of the wavefunction in one Hilbert…
We demonstrate the ability to extract a spin-entangled state of two neutral atoms via postselection based on a measurement of their spatial configuration. Typically, entangled states of neutral atoms are engineered via atom-atom interactions. In contrast, in our work we use Hong-Ou-Mandel interference to postselect a spin-singlet state after overlapping two atoms in distinct spin states on an effective beam splitter. We verify the presence of entanglement and determine a bound on the postselected fidelity of a spin-singlet state of $\left(0.62 \pm 0.03\right)$. The experiment has direct analog…
The Kochen-Specker theorem theoretically shows evidence of the incompatibility of noncontextual hidden variable theories with quantum mechanics. Quantum contextuality is a more general concept than quantum non-locality which is quite well tested in experiments by using Bell inequalities. Within neutron interferometry we performed an experimental test of the Kochen-Specker theorem with an inequality, which identifies quantum contextuality, by using spin-path entanglement in a single neutron system. Here entanglement is achieved not between different particles, but between degrees of freedom, i.…
This thesis examines some of the more fundamental requirements of a successful quantum computation, namely the ability to transmit quantum information with maximum efficiency, and the creation of entanglement. I focus specifically on neutron entanglement, showing that the spins of two or more distinct neutrons can be measurably entangled by forward-scattering from an isotropic medium. The interpretation of `time' in scattering experiments is also discussed. I present a simple treatment based on the Heisenberg S-matrix, from which it emerges that in certain situations the quantum-mechanical tim…
We discuss a discrete-event, particle-based simulation approach which reproduces the statistical distributions of Maxwell's theory and quantum theory by generating detection events one-by-one. This event-based approach gives a unified cause-and-effect description of quantum optics experiments such as single-photon Mach-Zehnder interferometer, Wheeler's delayed choice, quantum eraser, double-slit, Einstein-Podolsky-Rosen-Bohm and Hanbury Brown-Twiss experiments, and various neutron interferometry experiments at a level of detail which is not covered by conventional quantum theoretical descripti…
Optical signals obtained by the material response to classical laser fields are given by nonlinear response functions which can be expressed by sums over various quantum pathways of matter. We show that some pathways can be selected by using nonclassical fields, through the entanglement of photon and material pathways, which results in a different-power law dependence on the incoming field intensity. Spectrally overlapping stimulated Raman scattering (SRS) and two-photon-absorption (TPA) pathways in a pump probe experiment are separated by controlling the degree of entanglement of pairs of inc…
Entanglement between quantum dots transmitted via Majorana wire: Insights from the fermionic negativity, concurrence and quantum mutual information
Rzeszów University of Technology（热舒夫理工大学）；University of Opole（奥波莱大学）；A. Mickiewicz University（亚当·密茨凯维奇大学）；M. Curie-Skłodowska University（玛丽亚·居里-斯克沃多夫斯卡大学）
We develop an operator-based description of two types of multimode-entangled single-neutron quantum optical devices: Wollaston prisms and radio-frequency spin flippers in inclined magnetic field gradients. This treatment is similar to the approach used in quantum optics, and is convenient for the analysis of quantum contextuality measurements in certain types of neutron interferometers. We describe operationally the way multimode-entangled single-neutron states evolve in these devices, and provide expressions for the associated operators describing the dynamics, in the limit in which the neutr…
We demonstrate that the magnetic susceptibility of strongly alternating antiferromagnetic spin-1/2 chains is an entanglement witness. Specifically, magnetic susceptibility of copper nitrate (CN) measured in 1963 (Berger et al., Phys. Rev. 132, 1057 (1963)) cannot be described without presence of entanglement. A detailed analysis of the spin correlations in CN as obtained from neutron scattering experiments (Xu et al., Phys. Rev. Lett. 84, 4465 (2000)) provides microscopic support for this interpretation. We present a quantitative analysis resulting in the critical temperature of 5K in both, co…
Quantum entanglement is a key resource, which grants quantum systems the ability to accomplish tasks that are classically impossible. Here, we apply Feynman's sum-over-histories formalism to interacting bipartite quantum systems and introduce entanglement measures for bipartite quantum histories. Based on the Schmidt decomposition of the matrix comprised of the Feynman propagator complex coefficients, we prove that bipartite quantum histories are entangled if and only if the Schmidt rank of this matrix is larger than 1. The proposed approach highlights the utility of using a separable basis fo…
Ultraviolet structure of entanglement harvesting from energy density and other quadratic couplings
University of Waterloo（滑铁卢大学）；Institute for Quantum Computing, University of Waterloo（滑铁卢大学量子计算研究所）；Perimeter Institute for Theoretical Physics（理论物理前沿研究所）
A discrete-event simulation approach which provides a cause-and-effect description of many experiments with photons and neutrons exhibiting interference and entanglement is applied to a recent single-neutron experiment that tests (generalizations of) Heisenberg's uncertainty relation. The event-based simulation algorithm reproduces the results of the quantum theoretical description of the experiment but does not require the knowledge of the solution of a wave equation nor does it rely on concepts of quantum theory. In particular, the data satisfies uncertainty relations derived in the context …
We investigate quantum coherences in the presence of noise by entangling the spin and path degrees of freedom of the output neutron beam from a noisy three-blade perfect crystal neutron interferometer. We find that in the presence of dephasing noise on the path degree of freedom the entanglement of the output state reduces to zero, however the quantum discord remains non-zero for all noise values. Hence even in the presence of strong phase noise non-classical correlations persist between the spin and path of the neutron beam. This indicates that measurements performed on the spin of the neutro…
The lack of methods to experimentally detect and quantify entanglement in quantum matter impedes our ability to identify materials hosting highly entangled phases, such as quantum spin liquids. We thus investigate the feasibility of using inelastic neutron scattering (INS) to implement a model-independent measurement protocol for entanglement based on three entanglement witnesses: one-tangle, two-tangle, and quantum Fisher information (QFI). We perform high-resolution INS measurements on Cs$_2$CoCl$_4$, a close realization of the $S=1/2$ transverse-field XXZ spin chain, where we can control en…
We performed an experimental test of the Kochen-Specker theorem based on an inequality derived from the Peres-Mermin proof, using spin-path (momentum) entanglement in a single neutron system. Following the strategy proposed by Cabello et al. [Phys. Rev. Lett. 100, 130404 (2008)], a Bell-like state was generated and three expectation values were determined. The observed violation 2.291 +/- 0.008 > 1 clearly shows that quantum mechanical predictions cannot be reproduced by noncontextual hidden variables theories.
We investigate the role of the collective antisymmetric state in entanglement creation by spontaneous emission in a system of two non-overlapping two-level atoms. We calculate and illustrate graphically populations of the collective atomic states and the Wootters entanglement measure (concurrence) for two sets of initial atomic conditions. Our calculations include the dipole-dipole interaction and a spatial separation between the atoms that the antisymmetric state of the system is included throughout even for small interatomic separations. It is shown that spontaneous emission can lead to a tr…
We study two different decoherence modes for entangled qubits by considering a Liouville - von Neumann master equation. Mode A is determined by projection operators onto the eigenstates of the Hamiltonian and mode B by projectors onto rotated states. We present solutions for general and for Bell diagonal states and calculate for the later the mixedness and the amount of entanglement given by the concurrence. We propose a realization of the decoherence modes within neutron interferometry by applying fluctuating magnetic fields. An experimental test of the Kraus operator decomposition describing…
The problem of the complete transfer of quantum states and entanglement in a four qubits system composed of two single-mode cavities and two two-level atoms is investigated. The transfer of single and double excitation states is discussed for two different coupling configurations between the qubits. In the first, the coupling is mediated by the atoms that simultaneously couple to the cavity modes. In the second configuration, each atom resides inside one of the cavities and the coupling between the cavities is mediated by the overlapping field modes. A proper choice of basis states allows to i…
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Quantum entanglement is a quantum mechanical phenomenon where the quantum state of a many-body system with many degrees of freedom cannot be described independently of the state of each body with a given degree of freedom, no matter how far apart in space each body is. Entanglement is not only considered a resource in quantum information but also believed to affect complex condensed matter systems. Detecting and quantifying multi-particle entanglement in a many-body system is thus of fundamental significance for both quantum information science and condensed matter physics. Here, we detect and…
Dissipation engineering is a powerful framework for quantum state preparation and autonomous error correction in few-qubit systems. In this work, we examine the scalability of this approach and give three criteria which any dissipative state stabilization protocol should satisfy to be truly scalable as the number of qubits grows. Besides the requirement that it can be constructed in a resource-efficient manner from simple-to-engineer building blocks, a scalable protocol must also exhibit favorable scaling of the stabilization time with the increase in system size. We present a family of protoc…
We utilize single-crystal neutron diffraction to study the $C2/m$ structure of potassium hydrogen carbonate (KHCO$_3$) and macroscopic quantum entanglement above the phase transition at $T_c = 318$ K. Whereas split atom sites could be due to disorder, the diffraction pattern at 340 K evidences macroscopic proton states identical to those previously observed below $T_c$ by F. Fillaux et al., (2006 \textit{J. Phys.: Condens. Matter} \textbf{18} 3229). We propose a theoretical framework for decoherence-free proton states and the calculated differential cross-section accords with observations. The…
We propose a hardware architecture and protocol for connecting many local quantum processors contained within an optical cavity. The scheme is compatible with trapped ions or Rydberg arrays, and realizes teleported gates between any two qubits by distributing entanglement via single-photon transfers through a cavity. Heralding enables high-fidelity entanglement even for a cavity of moderate quality. For processors composed of trapped ions in a linear chain, a single cavity with realistic parameters successfully transfers photons every few $μ$s, enabling the any-to-any entanglement of 20 ion ch…
The so-called quantum measurement problems are solved from a new perspective. One of the main observations is that the basic entities of our world are {\it particles}, elementary or composite. It follows that each elementary process, hence each measurement process at its core, is a spacetime, pointlike, event. Another key idea is that, when a microsystem $ψ$ gets into contact with the experimental device, factorization of $ψ$ rapidly fails and entangled mixed states appear. The wave functions for the microsystem-apparatus coupled system for different measurement outcomes then lack overlapping …
Although various physical systems have been explored to produce entangled states involving electromagnetic, strong, and weak interactions, the gravity has not yet been touched in practical entanglement generation. Here, we propose an experimentally feasible scheme for generating spin entangled neutron pairs via the Earth's gravitational field, whose productivity can be one pair in every few seconds with the current technology. The scheme is realized by passing two neutrons through a specific rectangular cavity, where the gravity adjusts the neutrons into entangled state. This provides a simple…
