Viola Druzhinina, Marcel Mudrich, Florian Arnecke, Javier Madronero, Andreas Buchleitner
We show that the quantum reflection coefficient of ultracold heavy atoms scattering off a dielectric surface can be tuned in a wide range by suitable choice of surface and environment temperatures. This effect results from a temperature dependent long-range repulsive part of the van der Waals-Casimir-Polder-Lifshitz atom-surface interaction potential.
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Selective reflection Casimir-Polder spectroscopy in vapor cells: the influence of the thermal velocity distribution
本文针对选择性反射光谱此前采用的无限多普勒近似局限，扩展理论处理以纳入有限多普勒宽度影响，可分析超大Casimir-Polder相互作用区域、重新审视低激发态实验分析并助力确定量子摩擦特征。
We revisist the issue of entanglement of thermal equilibrium states in composite quantum systems. The possible scenarios are exemplified in bipartite qubit/qubit and qubit/qutrit systems.
We critically discuss the common belief that the thermal Casimir-Polder force can always be represented as a Matsubara sum, as it is true for the Casimir force. On the contrary, an exact treatment of the atom-field coupling reveals that for a ground-state atom, terms associated with virtual-photon absorption contribute to the force which are identified as a signature of non-equilibrium dynamics. Even the equilibrium force on a thermalized atom or molecule may be overestimated when using the ground-state polarizability instead of its thermal counterpart.
We provide an explicit analytical calculation that shows the asymptotic approach of the one dimensional Caldeira-Leggett model to thermal equilibrium in the high temperature and weak coupling limit. We investigate a free particle and a harmonic oscillator system, using both the Lindblad and the non-Lindblad type master equations for each case, and show that thermal equilibrium is reached exactly for the free particle and aproximately for the harmonic oscillator, irrespective of the initial preparation of the system. We also generalize our calculation to higher dimensions.
We characterize all Gaussian dynamical semigroups in continuous variables quantum systems of n-bosonic modes which have a thermal Gibbs state as a stationary solution. This is performed through an explicit relation between the diffusion and dissipation matrices, which characterize the semigroup dynamic, and the covariance matrix of the thermal equilibrium state. We also show that Alicki's quantum detailed-balance condition, based on a Gelfand-Naimark-Segal inner product, allows the determination of the temperature dependence of the diffusion and dissipation matrices, and the identification of …
To understand under which conditions thermodynamics emerges from the microscopic dynamics is the ultimate goal of statistical mechanics. Despite the fact that the theory is more than 100 years old, we are still discussing its foundations and its regime of applicability. A point of crucial importance is the definition of the notion of thermal equilibrium, which is given as the state that maximises the von Neumann entropy. Here we argue that it is necessary to propose a new way of describing thermal equilibrium, focused on observables rather than on the full state of the quantum system. We chara…
We study two two-level atomic quantum systems (qubits) placed close to a body held at a temperature different from that of the surrounding walls. While at thermal equilibrium the two-qubit dynamics is characterized by not entangled steady thermal states, we show that absence of thermal equilibrium may bring to the generation of entangled steady states. Remarkably, this entanglement emerges from the two-qubit dissipative dynamic itself, without any further external action on the two qubits, suggesting a new protocol to produce and protect entanglement which is intrinsically robust to environmen…
The problem of estimating the thermal corrections to Casimir and Casimir-Polder interactions in systems involving conducting plates has attracted considerable attention in the recent literature on dispersion forces. Alternative theoretical models, based on distinct low-frequency extrapolations of the plates reflection coefficient for transverse electric (TE) modes, provide widely different predictions for the magnitude of this correction. In this paper we examine the most widely used prescriptions for this reflection coefficient from the point of view of their consistency with the Bohr-van Lee…
Quantum Dynamics, Master Equation and Equilibrium for a Qubit Coupled to a Thermal Boson Field
本文解析推导了旋转波近似下量子比特与热玻色子环境耦合的精确主方程，分析了演化算子的长时间行为，并考察了系统达到热平衡的条件。
We study the energy shift and the Casimir-Polder force of an atom out of thermal equilibrium near the surface of a dielectric substrate. We first generalize, adopting the local source hypothesis, the formalism proposed by Dalibard, Dupont-Roc and Cohen-Tannoudji, which separates the contributions of thermal fluctuations and radiation reaction to the energy shift and allows a distinct treatment to atoms in the ground and excited states, to the case out of thermal equilibrium, and then use the generalized formalism to calculate the energy shift and the Casimir-Polder force of an isotropically po…
We study the two qubits Heisenberg XX chain with magnetic impurity in the presence of the external magnetic field and calculate the optimal fidelity of standard teleportation via the thermal equilibrium state. It is found that the combined influence of magnetic impurity and external magnetic field can increase the critical temperatures of entanglement and quantum teleportation without limit. The relation between two kinds of critical temperatures is revealed.
We study the Casimir-Lifshitz force and the radiative heat transfer in a system consisting of three bodies held at three independent temperatures and immersed in a thermal environment, the whole system being in a stationary configuration out of thermal equilibrium. The theory we develop is valid for arbitrary bodies, i.e. for any set of temperatures, dielectric and geometrical properties, and describes each body by means of its scattering operators. For the three-body system we provide a closed-form unified expression of the radiative heat transfer and of the Casimir-Lifshitz force (both in an…
We propose a superconducting circuit that shows a super-radiant phase transition (SRPT) in the thermal equilibrium. The existence of the SRPT is confirmed analytically in the limit of an infinite number of artificial atoms. We also perform numerical diagonalization of the Hamiltonian with a finite number of atoms and observe an asymptotic behavior approaching the infinite limit as the number of atoms increases. The SRPT can also be interpreted intuitively in a classical analysis.
We analyse the evolution of a quantum oscillator in a finite temperature environment using the quantum state diffusion (QSD) picture. Following a treatment similar to that of reference [7] we identify stationary solutions of the corresponding Itô equation. We prove their global stability and compute typical time scales characterizing the localization process. The recovery of the density matrix in approximately diagonal form enables us to verify the approach to thermal equilibrium in the long time limit and we comment on the connection between QSD and the decoherent histories approach.
We investigate the creation of entanglement between two quantum emitters interacting with a realistic common stationary electromagnetic field out of thermal equilibrium. In the case of two qubits we show that the absence of equilibrium allows the generation of steady entangled states, which is inaccessible at thermal equilibrium and is realized without any further external action on the two qubits. We first give a simple physical interpretation of the phenomenon in a specific case and then we report a detailed investigation on the dependence of the entanglement dynamics on the various physical…
We investigate spatial entanglement in a system of spinless non-interacting bosons in a one dimensional harmonic trap described by the grand canonical ensemble. We find the lower bound for the amount of spatial entanglement contained in the average state of two bosons in the trap and show that it exists for arbitrary high temperatures.
We investigate a two-level system in resonant contact with a larger environment. The environment typically is in a canonical state with a given temperature initially. Depending on the precise spectral structure of the environment and the type of coupling between both systems, the smaller part may relax to a canonical state with the same temperature as the environment (i.e. thermal relaxation) or to some other quasi equilibrium state (non thermal relaxation). The type of the (quasi) equilibrium state can be related to the distribution of certain properties of the energy eigenvectors of the tota…
Geometric phase of a two-level atom near a dielectric nanosphere out of thermal equilibrium
本文研究了二能级原子在非热平衡介电纳米球环境中的几何相位，发现GP修正取决于光子态局部密度和非平衡有效参数，且倏逝波激发可显著增强GP，为量子计算资源研究奠定基础。
We consider the problem of keeping an arbitrary state $ρ_s$ out of thermal equilibrium. We find that counter-acting thermalisation using only a resource system which is in a stationary state at the initial time and a system-resource interaction that preserves the global energy is possible if and only if the target state $ρ_s$ is block-diagonal in the eigenbasis of the system's Hamiltonian $H_s.$ As a consequence, we compute the extra work the operator must provide by tuning the resource-system interaction to overcome this constraint. This quantity, which is interpreted as the work needed to pr…
The effects of initial conditions and system parameters on entanglement dynamics and asymptotic entanglement for a two-qubit anisotropic XY Heisenberg system in the presence of an inhomogeneous magnetic field and spin-orbit interaction are investigated. We suppose that each qubit interacts with a separate thermal reservoir which is held in its own temperature. The effects of the parameters of the system and environment like spin-orbit interaction and temperature difference of reservoirs are also discussed.
Recent progress in manipulating atomic and condensed matter systems has instigated a surge of interest in non-equilibrium physics, including many-body dynamics of trapped ultracold atoms and ions, near-field radiative heat transfer, and quantum friction. Under most circumstances the complexity of such non-equilibrium systems requires a number of approximations to make theoretical descriptions tractable. In particular, it is often assumed that spatially separated components of a system thermalize with their immediate surroundings, although the global state of the system is out of equilibrium. T…
The thermal Casimir-Lifshitz force among two bodies held at different temperatures displays striking features that are absent in systems in thermal equilibrium. The manifestation of this force has been observed so far only in Bose-Einstein condensates close to a heated substrate, but never between two macroscopic bodies. Observation of the thermal Casimir-Lifhitz force out of thermal equilibrium with conventional Casimir setups is very difficult, because for experimentally accessible separations the thermal force is small compared to the zero-temperature quantum Casimir force, unless prohibiti…
Thermalization is the dynamical process by which a many-body system evolves toward a thermal equilibrium state that maximizes its entropy. In certain cases, however, the establishment of thermal equilibrium is significantly slowed down and a phenomenon of pre-thermalization can emerge. It describes the initial relaxation toward a quasi-steady state after a perturbation. While having similar properties to their thermal counterparts, pre-thermal states exhibit a partial memory of initial conditions. Here, we observe the dynamical formation of a pre-thermal state in a non-equilibrium, two-dimensi…
We develop an exact method for computing Casimir forces and the power of radiative heat transfer between two arbitrary nanostructured surfaces out of thermal equilibrium. The method is based on a generalization of the scattering approach recently used in investigations on the Casimir effect. Analogously to the equilibrium case, we find that also out of thermal equilibrium the shape and composition of the surfaces enter only through their scattering matrices. The expressions derived provide exact results in terms of the scattering matrices of the intervening surfaces.
We study the thermalization of an elementary quantum system modeled by a two-level atom interacting with stationary electromagnetic fields out of thermal equilibrium near a dielectric slab. The slab is held at a temperature different from that of the region where the atom is located. We find that when the slab is a nonabsorbing and nondispersive dielectric of a finite thickness $ d$, no out of thermal equilibrium effects appear as far as the thermalization of the atom is concerned, and a finite thick dielectric slab with a tiny imaginary part in the relative permittivity $\operatorname{Im} ε$ …
A framework for the investigation of disordered quantum systems in thermal equilibrium is proposed. The approach is based on a dynamical model--which consists of a combination of a double-bracket gradient flow and a uniform Brownian fluctuation--that `equilibrates' the Hamiltonian into a canonical distribution. The resulting equilibrium state is used to calculate quenched and annealed averages of quantum observables.
Based on the view that thermal equilibrium should be characterized through macroscopic observations, we develop a general theory about typicality of thermal equilibrium and the approach to thermal equilibrium in macroscopic quantum systems. We first formulate the notion that a pure state in an isolated quantum system represents thermal equilibrium. Then by assuming, or proving in certain classes of nontrivial models (including that of two bodies in thermal contact), large-deviation type bounds (which we call thermodynamic bounds) for the microcanonical ensemble, we prove that to represent ther…
The circumstances under which a system reaches thermal equilibrium, and how to derive this from basic dynamical laws, has been a major question from the very beginning of thermodynamics and statistical mechanics. Despite considerable progress, it remains an open problem. Motivated by this issue, we address the more general question of equilibration. We prove, with virtually full generality, that reaching equilibrium is a universal property of quantum systems: Almost any subsystem in interaction with a large enough bath will reach an equilibrium state and remain close to it for almost all times…
Thermal states are the bedrock of statistical physics. Nevertheless, when and how they actually arise in closed quantum systems is not fully understood. We consider this question for systems with local Hamiltonians on finite quantum lattices. In a first step, we show that states with exponentially decaying correlations equilibrate after a quantum quench. Then we show that the equilibrium state is locally equivalent to a thermal state, provided that the free energy of the equilibrium state is sufficiently small and the thermal state has exponentially decaying correlations. As an application, we…
Different non-equilibrium situations have recently been considered when studying the thermal Casimir--Polder interaction with a body. We show that the Keldysh Green function method provides a very general common framework for such studies where non-equilibrium of either the atom or the body with the environment can be accounted for. We apply the results to the case of ground state polar molecules out of equilibrium with their environment, observing several striking effects. We consider thermal Casimir--Polder potentials in planar configurations, and new results for a molecule in a cylindrical …
A theory of thermal and nonthermal radiation in a vacuum background of arbitrary temperature generated by relativistic polarizable particle with spin is proposed. When the particle rotates, radiation is produced by vacuum fluctuations even in the case of zero temperature of the system. In the ultrarelativistic case, the spectral-angular intensity of radiation is concentrated along the velocity of the particle. At finite temperatures of particle and vacuum, the particle temperature (in its rest frame) rather quickly acquires an equilibrium magnitude depending on the velocities of rotation and u…
Stalled response near thermal equilibrium in periodically driven systems
本文研究孤立多体量子系统在中等强度周期性扰动下的响应，发现当系统接近热平衡时驱动效应被强烈抑制，呈现停滞响应现象，并通过数值、解析和定性论证予以证实。
We consider an isolated, macroscopic quantum system. Let H be a micro-canonical "energy shell," i.e., a subspace of the system's Hilbert space spanned by the (finitely) many energy eigenstates with energies between E and E + delta E. The thermal equilibrium macro-state at energy E corresponds to a subspace H_{eq} of H such that dim H_{eq}/dim H is close to 1. We say that a system with state vector psi in H is in thermal equilibrium if psi is "close" to H_{eq}. We show that for "typical" Hamiltonians with given eigenvalues, all initial state vectors psi_0 evolve in such a way that psi_t is in t…
We explore the perspective of considering the squeezed thermal reservoir as an equilibrium reservoir in a generalized Gibbs ensemble with two non-commuting conserved quantities. We outline the main properties of such a reservoir in terms of the exchange of energy, both heat and work, and entropy, giving some key examples to clarify its physical interpretation. This new paradigm allows for a correct and insightful interpretation of all thermodynamical features of the squeezed thermal reservoir, as well as other similar non-thermal reservoirs, including the characterization of reversibility and …
It is shown, that Bose-Einstein condensation can occur not only in spatially extended equilibrium systems, but also in the systems far from thermal equilibrium, which show order-disorder phase transition. The investigation is performed by solving the Complex Ginzburg-Landau equation, a universal model for nonequilibrium order-disorder phase transitions.
We perform photon-assisted-tunneling (PAT) experiments on a GaAs double quantum dot device under high microwave excitation power. Photon-assisted absorption of up to 14 photons is observed, when electron temperature (>1K) are far above the lattice temperature. Signatures of Landau-Zener-Stückelberg (LZS) interference are found even in this non-equilibrium PAT spectrum. In addition, the charge state relaxation time T_1~8ns measured in this out of thermal equilibrium double quantum dot is in agreement with other previous reports.
Casimir-Lifshitz force between graphene-based structures out of thermal equilibrium
本文研究石墨烯平行结构在非平衡温度条件下的Casimir-Lifshitz力，发现通过调节石墨烯化学势可实现力的原位调控，包括力从吸引变为排斥及非单调变化等异常行为。
We generalize the method of third quantization to a unified exact treatment of Redfield and Lindblad master equations for open quadratic systems of n fermions in terms of diagonalization of 4n x 4n matrix. Non-equilibrium thermal driving in terms of the Redfield equation is analyzed in detail. We explain how to compute all physically relevant quantities, such as non-equilibrium expectation values of local observables, various entropies or information measures, or time evolution and properties of relaxation. We also discuss how to exactly treat explicitly time dependent problems. The general fo…
We study the internal dynamics of an elementary quantum system placed close to a body held at a temperature different from that of the surrounding radiation. We derive general expressions for lifetime and density matrix valid for bodies of arbitrary geometry and dielectric permittivity. Out of equilibrium, the thermalization process and steady states become both qualitatively and quantitatively significantly different from the case of radiation at thermal equilibrium. For the case of a three-level atom close to a slab of finite thickness, we predict the occurrence of population inversion and a…
We demonstrate that the Casimir-Polder force for a molecule near the surface of a real dielectric substrate out of thermal equilibrium displays distinctive behaviors as compared to that at thermal equilibrium. In particular, when the molecule-substrate separation is much less than the molecular transition wave-length, the CP force in the high temperature limit can be dramatically manipulated by varying the relative magnitude of the temperatures of the substrate and the environment so that the attractive-to-repulsive transition can occur beyond certain a threshold temperature of either the subs…
We consider the notion of thermal equilibrium for an individual closed macroscopic quantum system in a pure state, i.e., described by a wave function. The macroscopic properties in thermal equilibrium of such a system, determined by its wave function, must be the same as those obtained from thermodynamics, e.g., spatial uniformity of temperature and chemical potential. When this is true we say that the system is in macroscopic thermal equilibrium (MATE). Such a system may however not be in microscopic thermal equilibrium (MITE). The latter requires that the reduced density matrices of small su…
We consider the thermal equilibrium distribution at inverse temperature $β$, or canonical ensemble, of the wave function $Ψ$ of a quantum system. Since $L^2$ spaces contain more nondifferentiable than differentiable functions, and since the thermal equilibrium distribution is very spread-out, one might expect that $Ψ$ has probability zero to be differentiable. However, we show that for relevant Hamiltonians the contrary is the case: with probability one, $Ψ$ is infinitely often differentiable and even analytic. We also show that with probability one, $Ψ$ lies in the domain of the Hamiltonian.
The surface-atom Casimir-Polder-Lifshitz force out of thermal equilibrium is investigated in the framework of macroscopic electrodynamics. Particular attention is devoted to its large distance limit that shows a new, stronger behaviour with respect to the equilibrium case. The frequency shift produced by the surface-atom force on the the center-of-mass oscillations of a harmonically trapped Bose-Einstein condensate and on the Bloch oscillations of an ultra-cold fermionic gas in an optical lattice are discussed for configurations out of thermal equilibrium.
A large class of isolated quantum system in a pure state can equilibrate and serve as a heat bath. We show that once the equilibrium is reached, any of its subsystems that is much smaller than the isolated system is thermalized such that the subsystem is governed by the Gibbs distribution. Within this theoretical framework, the celebrated superposition principle of quantum mechanics leads to a prediction of a thermalized subsystem with multiple temperatures when the isolated system is in a superposition state of energy eigenstates of multiple distinct energy scales. This multiple-temperature s…
We investigate the force acting between two parallel plates held at different temperatures. The force reproduces, as limiting cases, the well known Casimir-Lifshitz surface-surface force at thermal equilibrium and the surface-atom force out of thermal equilibrium recently derived by M. Antezza \emph{et al.}, Phys. Rev. Lett. {\bf 95}, 113202 (2005). The asymptotic behavior of the force at large distances is explicitly discussed. In particular when one of the two bodies is a rarefied gas the force is not additive, being proportional to the square root of the density. Nontrivial cross-over regio…
Minimum-Time Transitions between Thermal Equilibrium States of the Quantum Parametric Oscillator
本文利用几何最优控制方法，解决了量子参量振子热平衡态间最短时间过渡问题，发现了一种新的最优解形式。
The Casimir-Polder-Lifshitz force felt by an atom near the surface of a substrate is calculated out of thermal equilibrium in terms of the dielectric function of the material and of the atomic polarizability. The new force decays like $1/z^3$ at large distances (i.e. slower than at equilibrium), exhibits a sizable temperature dependence and is attractive or repulsive depending on whether the temperature of the substrate is higher or smaller than the one of the environment. Our predictions can be relevant for experiments with ultracold atomic gases. Both dielectric and metal substrates are cons…
The eigenstate thermalization hypothesis (ETH) and the theory of linear response (LRT) are celebrated cornerstones of our understanding of the physics of many-body quantum systems out of equilibrium. While the ETH provides a generic mechanism of thermalization for states arbitrarily far from equilibrium, LRT extends the successful concepts of statistical mechanics to situations close to equilibrium. In our work, we connect these cornerstones to shed light on the route to equilibrium for a class of properly prepared states. We unveil that, if the off-diagonal part of the ETH applies, then the r…
We develop fluctuational electrodynamics for media with nonlinear optical response in and out of thermal equilibrium. Starting from the stochastic nonlinear Helmholtz equation and using the fluctuation dissipation theorem, we obtain perturbatively a deterministic nonlinear Helmholtz equation for the average field, the physical linear response, as well as the fluctuations and Rytov currents. We show that the effects of nonlinear optics, in or out of thermal equilibrium, can be taken into account with an effective, system-aware dielectric function. We discuss the heat radiation of a planar, nonl…
A simple procedure for obtaining superpositions of macroscopically distinct states is proposed and analyzed. We find that a thermal equilibrium state can be converted into such a state when a single global measurement of a macroscopic observable, such as the total magnetization, is made. This method is valid for systems with macroscopic degrees of freedom and finite (including zero) temperature. The superposition state is obtained with a high (low) probability when the measurement is made with a high (low) resolution. We find that this method is feasible in an experiment.
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