Quantum dimer models and exotic orders

Quantum phases of ferromagnetically coupled dimers on Shastry-Sutherland lattice

The ground state (gs) of antiferromagnetically coupled dimers on the Shastry-Sutherland lattice (SSL) stabilizes many exotic phases and has been extensively studied. The gs properties of ferromagnetically coupled dimers on SSL are equally important but unexplored. In this model the exchange coupling along the $x$-axis ($J_x$) and $y$-axis ($J_y$) are ferromagnetic and the diagonal exchange coupling ($J$) is antiferromagnetic. In this work we explore the quantum phase diagram of ferromagnetically coupled dimer model numerically using density matrix renormalization group (DMRG) method. We note t…

Featureless quantum spin liquid, 1/3-magnetization plateau state and exotic thermodynamic properties of spin-1/2 frustrated Heisenberg antiferromagnet on an infinite Husimi lattice

By utilizing tensor-network-based methods, we investigate the zero- and finite-temperature properties of the spin-1/2 Heisenberg antiferromagnetic (HAF) model on an infinite Husimi lattice that contains 3/2 sites per triangle. The ground state of this model is found to possess vanishing local magnetization and is featureless; the spin-spin and dimer-dimer correlation functions are verified to decay exponentially; and its ground-state energy per site is determined to be $e_0=-0.4343(1)$, which is very close to that [$e_0=-0.4386(5)$] of the intriguing kagome HAF model. The magnetization curve s…

Quantum dimer model with extensive ground-state entropy on the kagome lattice

We introduce a quantum dimer model on the kagome lattice with kinetic terms allowing from 3 to 6 dimers to resonate around hexagons. Unlike models studied previously, the different resonance loops appears with different signs (given by the parity of the number of dimers involved). These signs naturally appear when performing the lowest-order overlap expansion (Rokhsar and Kivelson 1988) of the Heisenberg model. We demonstrate that the quantum dimer model has an extensive zero-temperature entropy and has very short-range dimer-dimer correlations. We discuss the possible relevance of this new ki…

Quantum dimer model on the kagome lattice: solvable dimer liquid and Ising gauge theory

We introduce quantum dimer models on lattices made of corner-sharing triangles. These lattices includes the kagome lattice and can be defined in arbitrary geometry. They realize fully disordered and gapped dimer-liquid phase with topological degeneracy and deconfined fractional excitations, as well as solid phases. Using geometrical properties of the lattice, several results are obtained exactly, including the full spectrum of a dimer-liquid. These models offer a very natural - and maybe the simplest possible - framework to illustrate general concepts such as fractionalization, topological ord…

Quantum Criticality in Dimerized Spin Ladders

We analyze a possibility of quantum criticality (gaplessness) in dimerized antiferromagnetic two- and three-leg spin-1/2 ladders. Contrary to earlier studies of these models, we examine different dimerization patterns in the ladder. We find that ladders with the columnar dimerization order have lower zero-temperature energies and they are always gapped. For the staggered dimerization order, we find the quantum critical lines, in agreement with earlier analyses. The bond mean-field theory we apply, demonstrates its quantitative accuracy and agrees with available numerical results. We conclude t…

Effective quantum dimer model for trimerized kagome antiferromagnet

An effective spin-orbit Hamiltonian is derived for a spin-1/2 trimerized kagome antiferromagnet in the second-order of perturbation theory in the ratio of two coupling constants. Low-energy singlet states of the obtained model are mapped to a quantum dimer model on a triangular lattice. The quantum dimer model is dominated by dimer resonances on a few shortest loops of the triangular lattice. Characteristic energy scale for the dimer model constitutes only a small fraction of the weaker exchange coupling constant.

Quantum phase transitions in disordered dimerized quantum spin models and the Harris criterion

We use quantum Monte Carlo simulations to study effects of disorder on the quantum phase transition occurring versus the ratio g=J/J' in square-lattice dimerized S=1/2 Heisenberg antiferromagnets with intra- and inter-dimer couplings J and J'. The dimers are either randomly distributed (as in the classical dimer model), or come in parallel pairs with horizontal or vertical orientation. In both cases the transition violates the Harris criterion, according to which the correlation-length exponent should satisfy nu >= 1. We do not detect any deviations from the three-dimensional O(3) universality…

Statistical transmutation in doped quantum dimer models

We prove a "statistical transmutation" symmetry of doped quantum dimer models on the square, triangular and kagome lattices: the energy spectrum is invariant under a simultaneous change of statistics (i.e. bosonic into fermionic or vice-versa) of the holes and of the signs of all the dimer resonance loops. This exact transformation enables to define duality equivalence between doped quantum dimer Hamiltonians, and provides the analytic framework to analyze dynamical statistical transmutations. We investigate numerically the doping of the triangular quantum dimer model, with special focus on th…

Continuous interpolation between the fully frustrated Ising and quantum dimer models

We propose a new quantum model interpolating between the fully frustrated spin-1/2 Ising model in a transverse field and a dimer model. This model contains a resonating-valence-bond phase, including a line with an exactly solvable ground state of the Rokhsar-Kivelson type. We discuss the phase diagrams of this model on the square and triangular (in terms of the dimer representation) lattices.

Exact Solution and Correlations of a Quantum Dimer Model on the Checkerboard Lattice

We present analytic results for a special dimer model on the {\em non-bipartite} and {\em non-planar} checkerboard lattice that does not allow for parallel dimers surrounding diagonal links. We {\em exactly} calculate the number of closed packed dimer coverings on finite checkerboard lattices under periodic boundary conditions, and determine all dimer-dimer correlations. The latter are found to vanish beyond a certain distance. We find that this solvable model, despite being non-planar, is in close kinship with well-known paradigm-setting planar counterparts that allow exact mappings to $\math…

From exotic phases to microscopic Hamiltonians

We report recent analytical progress in the quest for spin models realising exotic phases. We focus on the question of `reverse-engineering' a local, SU(2) invariant S=1/2 Hamiltonian to exhibit phases predicted on the basis of effective models, such as large-N or quantum dimer models. This aim is to provide a point-of-principle demonstration of the possibility of constructing such microscopic lattice Hamiltonians, as well as to complement and guide numerical (and experimental) approaches to the same question. In particular, we demonstrate how to utilise peturbed Klein Hamiltonians to generate…

Quantum dimer models

These lecture notes aim to provide a self-contained, pedagogical introduction to the physics of local constraints, fractionalisation and topological liquids organised around the Rokhsar-Kivelson quantum dimer model. Topics and phenomena covered include emergent photons, SU(2) invariant spin liquids, valence-bond solids and Cantor deconfinement, along with an elementary introduction to the underlying theoretical models and methods.

Vison excitations in near-critical quantum dimer models

We study vison excitations in a quantum dimer model interpolating between the Rokhsar-Kivelson models on the square and triangular lattices. In the square-lattice case, the model is known to be critical and characterized by U(1) topological quantum numbers. Introducing diagonal dimers brings the model to a Z_2 resonating-valence-bond phase. We study variationally the emergence of vison excitations at low concentration of diagonal dimers, close to the critical point. We find that, in this regime, vison excitations are large in size and their structure resembles vortices in type-II superconducto…

Effective Quantum Dimer Model for the Kagome Heisenberg Antiferromagnet: Nearby Quantum Critical Point and Hidden Degeneracy

The low-energy singlet dynamics of the Quantum Heisenberg Antiferromagnet on the Kagome lattice is described by a quantitative Quantum Dimer Model. Using advanced numerical tools, the latter is shown to exhibit Valence Bond Crystal order with a large 36-site unit cell and hidden degeneracy between even and odd parities. Evidences are given that this groundstate lies in the vicinity of a $\mathbb{Z}_2$ dimer liquid region separated by a Quantum Critical Point. Implications regarding numerical analysis and experiments are discussed.

Magnetic field-induced transition in a quantum magnet described by the Quantum Dimer Model

The effect of a magnetic field on a gapped quantum magnet is described within the framework of the Quantum Dimer Model. A minimal model describing the proliferation of itinerant spinons above a critical field is proposed and investigated by Lanczos exact diagonalizations and quantum Monte Carlo simulations. For both square and triangular lattices, it is shown that spinons are fully polarized and Bose-condense. This offers a novel scenario of a Quantum Critical Point in the dimer-liquid phase (triangular lattice) characterized by the continuous appearance of a spinon superfluid density, contras…

Double Semion Phase in an Exactly Solvable Quantum Dimer Model on the Kagome Lattice

Quantum dimer models typically arise in various low energy theories like those of frustrated antiferromagnets. We introduce a quantum dimer model on the kagome lattice which stabilizes an alternative $\mathbb{Z}_2$ topological order, namely the so-called "double semion" order. For a particular set of parameters, the model is exactly solvable, allowing us to access the ground state as well as the excited states. We show that the double semion phase is stable over a wide range of parameters using numerical exact diagonalization. Furthermore, we propose a simple microscopic spin Hamiltonian for w…

Quantum Phase Transitions in Coupled Dimer Compounds

We study the critical properties in cubic systems of antiferromagnetically coupled spin dimers near magnetic-field induced quantum phase transitions. The quantum critical points in the zero-temperature phase diagrams are determined from quantum Monte Carlo simulations. Furthermore, scaling properties of the uniform magnetization and the staggered transverse magnetization across the quantum phase transition in magnetic fields are calculated. The critical exponents are derived from Ginzburg-Landau theory. We find excellent agreement between the quantum Monte Carlo simulations and the analytical …

"Nonmagnetic" Dimer Mott insulator induced by the coupling of spin with quantum electric dipoles

We present an effective dipolar-spin model based on the strong coupling analysis, which may explain the possible origin of the "spin liquid Mott insulator". The issue is related to the dimer Mott insulator reminiscent of the organic triangular lattice system, $κ$-ET$_2$Cu$_2$(CN)$_3$, whose gapless spin liquid state had been discussed in the context of geometrical frustration of exchange coupling, $J$, between spins on dimer orbitals. It turns out that another degrees of freedom within the insulator, {\it quantum electric-dipoles} on dimers, interacts with each other by the Coulomb interaction…

Quantum phase transition in a dimerized chain with hexamer distortion

We consider the dimerized spin-1/2 Heisenberg chain with spin hexameric distortion of the exchange pattern and study the zero-temperature phase diagram in the parameter space $(J_{1}, J_{2}, J_{3})$ by continuum-limit bosonization approach and the exact diagonalization method. The phase diagram is rich and has two gaped dimer phases. We obtain an estimate of the critical line separating the different gapped dimer phases by the bosonization approach. The existence of the transition line and the difference between dimer phases is checked numerically. The behavior of the energy gap and the dimer …

Quantum Statistics of Interacting Dimer Spin Systems

The compound TlCuCl3 represents a model system of dimerized quantum spins with strong interdimer interactions. We investigate the triplet dispersion as a function of temperature by inelastic neutron scattering experiments on single crystals. By comparison with a number of theoretical approaches we demonstrate that the description of Troyer, Tsunetsugu, and Wuertz [Phys. Rev. B 50, 13515 (1994)] provides an appropriate quantum statistical model for dimer spin systems at finite temperatures, where many-body correlations become particularly important.

Dynamics of the quantum dimer model on the triangular lattice: Soft modes and local resonating valence-bond correlations

We report on an exhaustive investigation of the dynamical dimer-dimer correlations in imaginary time for the quantum dimer model on the triangular lattice using the Green's function Monte Carlo method. We show in particular that soft modes develop upon reducing the dimer-dimer repulsion, indicating the presence of a second-order phase transition into an ordered phase with broken translational symmetry. We further investigate the nature of this ordered phase, for which a 12-site unit cell has been previously proposed, with the surprising result that significant Bragg peaks are only present at t…

具有Dzyaloshinsky-Moriya相互作用的量子自旋二聚体自旋动力学研究

Investigation of the spin dynamics of quantum spin dimers with Dzyaloshinsky-Moriya interaction

本研究通过绝热调控磁场，实现量子自旋螺旋二聚体从非磁性基态到经典螺旋态的转变，并利用可暂停的周期振荡操控量子态与磁构型，且可推广至偶数自旋链。

Deconfined quantum criticality and Neel order via dimer disorder

Recent results on the nature of the quantum critical point between Neel and valence bond solid(VBS) ordered phases of two dimensional quantum magnets are examined by an attack from the VBS side. This approach leads to an appealingly simple physical description, and further insight into the properties of the transition.

First-order quantum phase transition in the orthogonal-dimer spin chain

We investigate the low-energy properties of the orthogonal-dimer spin chain characterized by a frustrated dimer-plaquette structure. When the competing antiferromagnetic couplings are varied, the first-order quantum phase transition occurs between the dimer and the plaquette phases, which is accompanied by nontrivial features due to frustration: besides the discontinuity in the lowest excitation gap at the transition point, a sharp level-crossing occurs for the spectrum in the plaquette phase. We further reveal that the plateau in the magnetization curve at 1/4 of the full moment dramatically …

Field dependent thermodynamics and Quantum Critical Phenomena in the dimerized spin system Cu2(C5H12N2)2Cl4

Experimental data for the uniform susceptibility, magnetization and specific heat for the material Cu2(C5H12N2)2Cl4 (abbreviated CuHpCl) as a function of temperature and external field are compared with those of three different dimerized spin models: alternating spin-chains, spin-ladders and the bilayer Heisenberg model. It is shown that because this material consists of weakly coupled spin-dimers, much of the data is insensitive to how the dimers are coupled together and what the effective dimensionality of the system is. When such a system is tuned to the quantum critical point by applicatio…

Phase diagram of an extended quantum dimer model on the hexagonal lattice

We introduce a quantum dimer model on the hexagonal lattice that, in addition to the standard three-dimer kinetic and potential terms, includes a competing potential part counting dimer-free hexagons. The zero-temperature phase diagram is studied by means of quantum Monte Carlo simulations, supplemented by variational arguments. It reveals some new crystalline phases and a cascade of transitions with rapidly changing flux (tilt in the height language). We analyze perturbatively the vicinity of the Rokhsar-Kivelson point, showing that this model has the microscopic ingredients needed for the "d…

DMRG investigation of constrained models: from quantum dimer and quantum loop ladders to hard-boson and Fibonacci anyon chains

Motivated by the presence of Ising transitions that take place entirely in the singlet sector of frustrated spin-1/2 ladders and spin-1 chains, we study two types of effective dimer models on ladders, a quantum dimer model and a quantum loop model. Building on the constraints imposed on the dimers, we develop a Density Matrix Renormalization Group algorithm that takes full advantage of the relatively small Hilbert space that only grows as Fibonacci number. We further show that both models can be mapped rigorously onto a hard-boson model first studied by Fendley, Sengupta and Sachdev [Phys. Rev…

Topological Quantum Many-Body Scars in Quantum Dimer Models on the Kagome Lattice

We present a class of quantum dimer models on the kagome lattice with full translational invariance that feature a quantum many-body scar state of analytically known entanglement properties within their spectra. Using exact diagonalization on lattices of up to 60 sites, we show that non-scar states conform to the eigenstate thermalization hypothesis. Specifically, we show that energies are distributed according to the Gaussian ensemble expected of their respective symmetry sector, illustrate the existence of the scar from bipartite entanglement properties, and demonstrate revival phenomena in …

Sequence of first-order quantum phase transitions in a frustrated spin half dimer-plaquette chain

We study the frustrated dimer-plaquette quantum spin chain for ferromagnetic dimer bonds. This quantum system undergoes a series of first-order ground-state phase transitions driven by frustration or by a magnetic field. We find that the different nature of the ground-state phases has a strong influence on the magnetization curve as well as the low-temperature thermodynamics. In particular, the magnetization curve exhibits plateaus and jumps, the number of which depends on the strength of frustration. The temperature dependence of the susceptibility may either show activated spin-gap behaviour…

Multicolored quantum dimer models, resonating valence-bond states, color visons, and the triangular-lattice t_2g spin-orbital system

The spin-orbital model for triply degenerate t_2g electrons on a triangular lattice has been shown to be dominated by dimers: the phase diagram contains both strongly resonating, compound spin-orbital dimer states and quasi-static, spin-singlet valence-bond (VB) states. To elucidate the nature of the true ground state in these different regimes, the model is mapped to a number of quantum dimer models (QDMs), each of which has three dimer colors. The generic multicolored QDM, illustrated for the two- and three-color cases, possesses a topological color structure, "color vison" excitations, and …

Exact solution of a two-species quantum dimer model for pseudogap metals

We present an exact ground state solution of a quantum dimer model introduced in Ref.[1], which features ordinary bosonic spin-singlet dimers as well as fermionic dimers that can be viewed as bound states of spinons and holons in a hole-doped resonating valence bond liquid. Interestingly, this model captures several essential properties of the metallic pseudogap phase in high-$T_c$ cuprate superconductors. We identify a line in parameter space where the exact ground state wave functions can be constructed at an arbitrary density of fermionic dimers. At this exactly solvable line the ground sta…

An RVB phase in the triangular lattice quantum dimer model

We study the quantum dimer model on the triangular lattice, which is expected to describe the singlet dynamics of frustrated Heisenberg models in phases where valence bond configurations dominate their physics. We find, in contrast to the square lattice, that there is a truly short ranged resonating valence bond (RVB) phase with no gapless collective excitations and with deconfined, gapped, spinons for a {\it finite} range of parameters. We also establish the presence of three crystalline phases in this system.

Ising transition in dimerized XY quantum spin chain

In the present paper, we proposed a simple spin-1/2 model which provides a exactly solvable example to study the Ising criticality with central charge c=1/2. By mapping it onto the real Majorana fermions, the Ising critical behavior is explored explicitly, although its bosonized form is not the double frequency sine-Gordon model.

A Generalized Quantum Dimer Model Applied to the Frustrated Heisenberg Model on the Square Lattice: Emergence of a Mixed Columnar-Plaquette Phase

Aiming to describe frustrated quantum magnets with non-magnetic singlet ground states, we have extended the Rokhsar-Kivelson (RK) loop-expansion to derive a generalized Quantum Dimer Model containing only connected terms up to arbitrary order. For the square lattice frustrated Heisenberg antiferromagnet (J1-J2-J3 model), an expansion up to 8th order shows that the leading correction to the original RK model comes from dimer moves on length-6 loops. This model free of the original sign problem is treated by advanced numerical techniques. The results suggest that a rotationally anisotropic plaqu…

Electronic quasiparticles in the quantum dimer model: density matrix renormalization group results

We study a recently proposed quantum dimer model for the pseudogap metal state of the cuprates. The model contains bosonic dimers, representing a spin-singlet valence bond between a pair of electrons, and fermionic dimers, representing a quasiparticle with spin-$1/2$ and charge $+e$. By density matrix renormalization group calculations on a long but finite cylinder, we obtain the ground-state density distribution of the fermionic dimers for a number of different total densities. From the Friedel oscillations at open boundaries, we deduce that the Fermi surface consists of small hole pockets ne…

Engineering SU(2) invariant spin models to mimic quantum dimer physics on the square lattice

We consider the spin-1/2 hamiltonians proposed by Cano and Fendley [J. Cano and P. Fendley, Phys. Rev. Lett. 105, 067205 (2010)] which were built to promote the well-known Rokshar-Kivelson (RK) point of quantum dimer models to spin-1/2 wavefunctions. We first show that these models, besides the exact degeneracy of RK point, support gapless spinless excitations as well as a spin gap in the thermodynamic limit, signatures of an unusual spin liquid. We then extend the original construction to create a continuous family of SU(2) invariant spin models that reproduces the phase diagram of the quantu…

The plaquette phase of the square lattice quantum dimer model

The plaquette phase of the square lattice quantum dimer model is studied using a continuous-time reptation quantum Monte Carlo method for lattices of sizes up to 48x48 sites. We determine the location of the phase transition between the columnar and plaquette phases to occur at V_c/J=0.60 +- 0.05 which is significantly larger than inferred from previous exact diagonalization studies on smaller lattices. Offdiagonal correlation functions are obtained. They exhibit long-range order in the plaquette phase but not at the Rokhsar-Kivelson point. We also observe significant finite-size corrections t…

Quantum oscillations and criticality in a fermionic and bosonic dimer model for the cuprates

We study quantum oscillations for a system of fermionic and bosonic dimers and compare the results to those experimentally observed in the cuprate superconductors in their underdoped regime. Based on gauge invariance, we argue that the charge carriers obey the Onsager quantization condition and quantum oscillations take on a Lifshitz-Kosevich form. We obtain the effective mass and find good qualitative agreement with experiments if we tune the model to the point where the observed mass divergence at optimum doping is associated to a van Hove singularity at which four free-dimer Fermi pockets t…

具有可调单离子各向异性的spin-1 Kitaev链中的自发二聚化、自旋向列序与解禁闭量子临界点

Spontaneous dimerization, spin-nematic order, and deconfined quantum critical point in a spin-1 Kitaev chain with tunable single-ion anisotropy

本文利用密度矩阵重整化群方法研究具有可调单离子各向异性的spin-1 Kitaev链，揭示了自旋向列相、二聚化相与反铁磁相间的相变，并发现“Landau禁止”的连续相变，为解禁闭量子临界点提供了新平台。

Hidden dimer order in the quantum compass model

We introduce an exact spin transformation that maps frustrated Z_{i,j}Z_{i,j+1} and X_{i,j}X_{i+1,j} spin interactions along the rows and columns of the quantum compass model (QCM) on an LxL square lattice to (L-1)x(L-1) quantum spin models with 2(L-1) classical spins. Using the symmetry properties we unravel the hidden dimer order in the QCM, with equal two-dimer correlations <X_{i,i}X_{i+1,i}X_{k,l}X_{k+1,l}> and <X_{i,i}X_{i+1,i}X_{l,k}X_{l+1,k}> in the ground state, which is independent of the actual interactions. This order coexists with Ising-type spin correlations which decay with dista…

Zero-Temperature Properties of the Quantum Dimer Model on the Triangular Lattice

Using exact diagonalizations and Green's function Monte Carlo simulations, we have studied the zero-temperature properties of the quantum dimer model on the triangular lattice on clusters with up to 588 sites. A detailed comparison of the properties in different topological sectors as a function of the cluster size and for different cluster shapes has allowed us to identify different phases, to show explicitly the presence of topological degeneracy in a phase close to the Rokhsar-Kivelson point, and to understand finite-size effects inside this phase. The nature of the various phases has been …

Doping quantum dimer models on the square lattice

A family of models is proposed to describe the motion of holes in a fluctuating quantum dimer background on the square lattice. Following Castelnovo et al. [Ann. Phys. (NY) 318, 316 (2005)], a generalized Rokhsar-Kivelson Hamiltonian at **finite doping** which can be mapped on a **doped** interacting classical dimer model is constructed. A simple physical extension of this model is also considered. Using numerical computations and simple considerations based on the above exact mapping, we determine the phase diagram of the model showing a number of quantum phases typical of a doped Mott insula…

Double-semion topological order from exactly solvable quantum dimer models

We construct a generalized quantum dimer model on two-dimensional nonbipartite lattices including the triangular lattice, the star lattice and the kagome lattice. At the Rokhsar-Kivelson (RK) point, we obtain its exact ground states that are shown to be a fully gapped quantum spin liquid with the double-semion topological order. The ground-state wave function of such a model at the RK point is a superposition of dimer configurations with a nonlocal sign structure determined by counting the number of loops in the transition graph. We explicitly demonstrate the double-semion topological order in…

Ferromagnetic Quantum Critical Point in FeGa3 Tuned by Mixed-Valence Fe Dimers

The magnetic, transport, and thermal properties of single crystals of the series Fe(Ga1-xGex)3 are reported. Pure FeGa3 is a nonmagnetic semiconductor, that when doped with small concentrations of Ge (extrinsic electrons), passes through an insulator-to-metal transition and displays non-Fermi liquid (NFL) behavior. Moreover, we observer clear signatures of a ferromagnetic quantum critical point (FM-QCP) in this system at x = 0.052. The mechanism of the local moment formation is consistent with a one-electron reduction of Fe dimer singlets, a unique structural feature in FeGa3, where the densit…

非厄米特量子双模模型与瑞利德数组中量子自旋液体的制备

Preparation of a Quantum Spin Liquid in Non-Hermitian Quantum Dimer Models and Rydberg Arrays

通过非厄米特性在瑞利德原子数组中实现非厄米特量子双模模型的自旋液体态制备。

Quantum Dimer Model on the triangular lattice: Semiclassical and variational approaches to vison dispersion and condensation

After reviewing the concept of vison excitations in Z_2 dimer liquids, we study the liquid-crystal transition of the Quantum Dimer Model on the triangular lattice by means of a semiclassical spin-wave approximation to the dispersion of visons in the context of a "soft-dimer" version of the model. This approach captures some important qualitative features of the transition: continuous nature of the transition, linear dispersion at the critical point, and \sqrt{12}x\sqrt{12} symmetry-breaking pattern. In a second part, we present a variational calculation of the vison dispersion relation at the …

Magnetic field-induced phase transitions in a weakly coupled s = 1/2 quantum spin dimer system Ba$_{3}$Cr$_{2}$O$_{8}$

By using bulk magnetization, electron spin resonance (ESR), heat capacity, and neutron scattering techniques, we characterize the thermodynamic and quantum phase diagrams of Ba$_3$Cr$_2$O$_8$. Our ESR measurements indicate that the low field paramagnetic ground state is a mixed state of the singlet and the S$_z$ = 0 triplet for $H \perp c$. This suggests the presence of an intra-dimer Dzyaloshinsky-Moriya (DM) interaction with a DM vector perpendicular to the c-axis.

Statistics of holes and nature of superfluid phases in Quantum dimer models

Quantum Dimer Models (QDM) arise as low energy effective models for frustrated magnets. Some of these models have proven successful in generating a scenario for exotic spin liquid phases with deconfined spinons. Doping, i.e. the introduction of mobile holes, has been considered within the QDM framework and partially studied. A fundamental issue is the possible existence of a superconducting phase in such systems and its properties. For this purpose, the question of the statistics of the mobile holes (or "holons") shall be addressed first. Such issues are studied in details in this paper for ge…

Impurity-doped Kagome Antiferromagnet: A Quantum Dimer Model Approach

The doping of quantum Heisenberg antiferromagnets on the kagome lattice by non-magnetic impurities is investigated within the framework of a generalized quantum dimer model (QDM) describing a) the valence bond crystal (VBC), b) the dimer liquid and c) the critical region on equal footing. Following the approach by Ralko et al. [Phys. Rev. Lett. 101, 117204 (2008)] for the square and triangular lattices, we introduce the (minimal) extension of the QDM on the Kagome lattice to account for spontaneous creation of mobile S=1/2 spinons at finite magnetic field. Modulations of the dimer density (at …

Phase separation and flux quantization in the doped quantum dimer model on the square and triangular lattices

The doped two-dimensional quantum dimer model is investigated by numerical techniques on the square and triangular lattices, with significantly different results. On the square lattice, at small enough doping, there is always a phase separation between an insulating valence-bond solid and a uniform superfluid phase, whereas on the triangular lattice, doping leads directly to a uniform superfluid in a large portion of the RVB phase. Under an applied Aharonov-Bohm flux, the superfluid exhibits quantization in terms of half-flux quanta, consistent with Q=2e elementary charge quanta in transport p…

Quantum Melting of Magnetic Order in an Organic Dimer-Mott Insulating System

Quantum entanglement effects between the electronic spin and charge degrees of freedom are examined in an organic molecular solid, termed a dimer-Mott insulating system, in which molecular dimers are arranged in a crystal as fundamental units. A low energy effective model includes an antisymmetric exchange interaction, as one of the dominant magnetic interactions. This interaction favors a 90 degree spin configuration, and competes with the Heisenberg-type exchange interaction. Stabilities of the magnetic ordered phases are examined by using the spin-wave theory, as well as the Schwinger-boson…

Spontaneous dimer order, excitation spectrum, and quantum phase transitions in the J1-J2 Heisenberg model

We overview some recent work and present new results on the ground state properties and the spectrum of excitations of the two-dimensional frustrated Heisenberg antiferromagnet. Spontaneous dimer order is present in the quantum disordered phase of this model. We study the stability and analyze the structure of the spectrum, including the two-particle singlet excitation branch throughout the disordered phase, as well as in the vicinity of the Neel critical point. The variation of the dimer order parameter is also given, and it is argued that near the critical point it reflects the presence of t…

Interaction between static holes in a quantum dimer model on the kagome lattice

A quantum dimer model (QDM) on the kagome lattice with an extensive ground-state entropy was recently introduced [Phys. Rev. B 67, 214413 (2003)]. The ground-state energy of this QDM in presence of one and two static holes is investigated by means of exact diagonalizations on lattices containing up to 144 kagome sites. The interaction energy between the holes (at distances up to 7 lattice spacings) is evaluated and the results show no indication of confinement at large hole separations.

Search for quantum electronic dipoles in the dimerized κ-(BEDT-TTF)2Cu[N(CN)2]Cl salt

The Mott insulator κ-(BEDT-TTF)2Cu[N(CN)2]Cl consists of molecular dimers arranged on an anisotropic triangular lattice and develops a canted antiferromagnetic ground state. It has recently been suggested that this system features purely electronic ferroelectricity which requires an electric dipole moment. Optical spectroscopy clearly rules out charge imbalance in this system, which excludes the existence of quantum electric dipoles on the dimers and subsequently a dipolar spin coupling. We suggest that the prominent in-plane dielectric response in κ-(BEDT-TTF)2Cu[N(CN)2]Cl is due to short-ran…