We study the Kondo-Heisenberg model using a fermionic representation for the localized spins. The mean-field phase diagram exhibits a zero temperature quantum critical point separating a spin liquid phase where the f-conduction hybridization vanishes, and a Kondo phase where it does not. Two solutions can be stabilized in the Kondo phase, namely a uniform hybridization when the band masses of the conduction electrons and the f spinons have the same sign, and a modulated one when they have opposite sign. For the uniform case, we show that above a very small Fermi liquid temperature scale (~1 mK), the critical fluctuations associated with the vanishing hybridization have dynamical exponent z=3, giving rise to a specific heat coefficient that diverges logarithmically in temperature, as well as a conduction electron inverse lifetime that has a T log T behavior. Because the f spinons do not carry current, but act as an effective bath for the relaxation of the current carried by the conduction electrons, the latter result also gives rise to a T log T behavior in the resistivity. This behavior is consistent with observations in a number of heavy fermion metals.
The breakdown of the lattice Kondo effect in local-moment metals can lead to non-trivial forms of quantum criticality and a variety of non-Fermi-liquid phases. Given indications that Kondo-breakdown transitions involve criticality not only in the spin but also in the charge sector, we investigate the interplay of Kondo breakdown and strong valence fluctuations in generalized Anderson lattice models. We employ a parton mean-field theory to describe the transitions between deconfined fractionalized Fermi liquids and various confined phases. We find that rapid valence changes near Kondo breakdown…
Motivated by the observation of light surface states in SmB6, we examine the effects of surface Kondo breakdown in topological Kondo insulators. We present both numerical and analytic results which show that the decoupling of the localized moments at the surface disturbs the compensation between light and heavy electrons and dopes the Dirac cone. Dispersion of these uncompensated surface states are dominated by inter-site hopping, which leads to a much lighter quasiparticles. These surface states are also highly durable against the effects of surface magnetism and decreasing thickness of the s…
We propose that the thermoelectric power distinguishes two competing scenarios for quantum phase transitions in heavy fermions : the spin-density-wave (SDW) theory and breakdown of the Kondo effect. In the Kondo breakdown scenario, the Seebeck coefficient turns out to collapse from the temperature scale $E^{*}$, associated with quantum fluctuations of the Fermi surface reconfiguration. This feature differs radically from the physics of the SDW theory, where no reconstruction of the Fermi surface occurs, and can be considered as the hallmark of the Kondo breakdown theory. We test these ideas, u…
The breakdown of the Kondo effect may be the origin of the anomalous properties of the heavy-fermion compounds at low temperatures. We study the dynamics of one impurity embedded in an antiferromagnetic host at the quantum critical point and show that the impurity is not screened and develops a power law correlation function. This suggests that the breakdown of the Kondo effect can simply be a consequence of the system's proximity to the quantum critical point.
We consider a spin-1/2 Heisenberg chain coupled via a Kondo interaction to two-dimensional Dirac fermions. The Kondo interaction is irrelevant at the \textit{decoupled} fixed-point, leading to the existence of a Kondo-breakdown phase and a Kondo-breakdown critical point separating such a phase from a heavy Fermi liquid. We reach this conclusion on the basis of a renormalization group analysis, large-N calculations as well as extensive auxiliary-field quantum Monte Carlo simulations. We extract quantities such as the zero-bias tunneling conductance which will be relevant to future experiments i…
The unconventional critical behavior near magnetic quantum phase transitions in various heavy-fermion metals, apparently inconsistent with the standard spin-density-wave scenario, has triggered proposals on the breakdown of the Kondo effect at the critical point. Here we investigate, within one specific scenario, the fate of such a zero-temperature transition upon coupling of the electronic to lattice degrees of freedom. We study a Kondo-Heisenberg model with volume-dependent Kondo coupling -- this model displays both Kondo volume collapse and Kondo-breakdown transitions, as well as Lifshitz t…
We show that the scenario of multi-scale Kondo breakdown quantum critical point (QCP) gives rise to a divergent Grüneisen ratio with an anomalous exponent 0.7. In particular, we fit the experimental data of $YbRh_{2}(Si_{0.95}Ge_{0.05})_{2}$ for specific heat, thermal expansion, and Grüneisen ratio based on our simple analytic expressions. A reasonable agreement between the experiment and theory is found for the temperature range between 0.4 K and 10 K. We discuss how the Grüneisen ratio is a key measurement to discriminate between the Kondo breakdown and spin-density wave theories.
We study both the electrical and thermal transport near the heavy-fermion quantum critical point (QCP), identified with the breakdown of the Kondo effect as an orbital selective Mott transition. We show that the contribution to the electrical conductivity comes mainly from conduction electrons while the thermal conductivity is given by both conduction electrons and localized fermions (spinons), scattered with dynamical exponent $z = 3$. This scattering mechanism gives rise to a quasi-linear temperature dependence of the electrical and thermal resistivity. The characteristic feature of the Kond…
The Kondo breakdown scenario has been claimed to allow the $T$-linear resistivity in the vicinity of the Kondo breakdown quantum critical point, two cornerstones of which are the dynamical exponent $z = 3$ quantum criticality for hybridization fluctuations in three dimensions and irrelevance of vertex corrections for transport due to the presence of localized electrons. We revisit the issue of vertex corrections in electrical transport coefficients. Assuming that two kinds of bosonic degrees of freedom, hybridization excitations and gauge fluctuations, are in equilibrium, we derive coupled qua…
We study the finite-frequency inter-band transition peak in the optical conductivity of a heavy fermion system close to a Kondo breakdown quantum critical point, where the lattice Kondo temperature vanishes. As the system approaches the phase transition from the heavy Fermi liquid side, we find a new cross-over regime where the peak position is related to, but is not directly proportional to, the lattice Kondo scale. In particular, the position of the peak moves to lower energies, but remains finite at the critical point. On the other hand, the peak value changes non-monotonically and eventual…
We show within the slave boson technique, that the Anderson lattice model exhibits a Kondo breakdown quantum critical point (KB-QCP) where the hybridization goes to zero at zero temper- ature. At this fixed point, the f-electrons experience as well a selective Mott transition separating a local-moment phase from a Kondo-screened phase. The presence of a multi-scale QCP in the An- derson lattice in the absence of magnetism is discussed in the context of heavy fermion compounds. This study is the first evidence for a selective Mott transition in the Anderson lattice.
Motivated by recent Hall-effect experiment in YbRh$_2$Si$_2$, we study ground state properties of a Kondo lattice model in a two-dimensional square lattice using variational Monte Carlo method. We show that there are two types of phase transition, antiferromagnetic transition and topological one (Fermi surface reconstruction). In a wide region of parameters, these two transitions occur simultaneously without the breakdown of Kondo screening, accompanied by a discontinuous change of the Hall coefficient. This result is consistent with the experiment and gives a novel theoretical picture for the…
We consider Dirac electrons on the honeycomb lattice Kondo coupled to spin-1/2 degrees of freedom on the kagome lattice. The interactions between the spins are chosen along the lines of the Balents-Fisher-Girvin model that is known to host a $\mathbb{Z}_2$ spin liquid and a ferromagnetic phase. The model is amenable to sign free auxiliary field quantum Monte Carlo simulations. While in the ferromagnetic phase the Dirac electrons acquire a gap, they remain massless in the $\mathbb{Z}_2$ spin liquid phase due to the breakdown of Kondo screening. Since our model has an odd number of spins per uni…
One of the challenges in strongly correlated electron systems, is to understand the anomalous electronic behavior that develops at an antiferromagnetic quantum critical point (QCP), a phenomenon that has been extensively studied in heavy fermion materials. Current theories have focused on the critical spin fluctuations and associated break-down of the Kondo effect. Here we argue that the abrupt change in Fermi surface volume that accompanies heavy fermion criticality leads to critical charge fluctuations. Using a model one dimensional Kondo lattice in which each moment is connected to a separa…
We show that the inclusion of nonlocal correlation effects in a variational wave function for the ground state of a topological Anderson lattice Hamiltonian is capable of describing both topologically trivial insulating phases and nontrivial ones characterized by an indirect gap, as well as its closure at the transition into a metallic phase. The method, though applied to an oversimplified model, thus captures the metallic and insulating states that are indeed observed in a variety of Kondo semiconductors, while accounting for topologically nontrivial band structures.
We study the deconfined quantum critical point of the Kondo-Heisenberg lattice in three dimensions using a fermionic representation for the localized spins. The mean-field phase diagram exhibits a zero temperature quantum critical point separating a spin liquid phase where the hybridization vanishes and a Kondo phase where it does not. Two solutions can be stabilized in the Kondo phase, namely a uniform hybridization when the band masses of the conduction electrons and the spinons have the same sign, and a modulated one when they have opposite sign. For the uniform case, we show that above a v…
We report that nonmagnetic heavy-fermion (HF) iron oxypnictide CeFePO with two-dimensional XY-type anisotropy shows a metamagnetic behavior at the metamagnetic field H_M \simeq 4 T perpendicular to the c-axis and that a critical behavior is observed around H_M. Although the magnetic character is entirely different from that in other Ce-based HF metamagnets, H_M in these metamagnets is linearly proportional to the inverse of the effective mass, or to the temperature where the susceptibility shows a peak. This finding suggests that H_M is a magnetic field breaking the local Kondo singlet, and th…
The phase diagram of the Bose-Fermi Kondo model contains an SU(2)-invariant Kondo-screened phase separated by a continuous quantum phase transition from a Kondo-destroyed local moment phase. We analyze the effect of the Berry phase term of the spin path integral on the quantum critical properties of this quantum impurity model. For a range of the power-law exponent characterizing the spectral density of the dissipative bosonic bath, neglecting the influence of the Berry phase term makes the fixed point Gaussian. For the same range of the spectral density exponent, incorporating the Berry phase…
We study the Kondo alloy model on a square lattice using dynamical mean-field theory (DMFT) for Kondo substitution and disorder effects, together with static mean-field approximations. We computed and analyzed photoemission properties as a function of electronic filling $n_c$, Kondo impurity concentration $x$, and strength of Kondo temperature $T_K$. We provide a complete description of the Angle Resolved Photoemission Spectroscopy (ARPES) signals expected in the paramagnetic Kondo phases. By analyzing the Fermi surface, we observe the Lifshitz-like transition predicted previously for strong $…
We study the low energy states of the Kondo alloy model (KAM) as function of the magnetic impurity concentration per site, x, and the conduction electron average site occupation, nc. In previous works, two different Fermi liquid regimes had been identified at strong Kondo coupling JK, that may be separated by a transition at x=nc. Here, we analyze the KAM for finite JK on a Bethe lattice structure. First, using the mean-field coherent potential approximation (DMFT-CPA) which is exact at lattice coordination Z=infty, we show that the real part of the local potential scattering may be located ou…
The interaction between strong correlation and Berry curvature is an open territory of in the field of quantum materials. Here we report large anomalous Hall conductivity in a Kondo lattice ferromagnet USbTe which is dominated by intrinsic Berry curvature at low temperatures. However, the Berry curvature induced anomalous Hall effect does not follow the scaling relation derived from Fermi liquid theory. The onset of the Berry curvature contribution coincides with the Kondo coherent temperature. Combined with ARPES measurement and DMFT calculations, this strongly indicates that Berry curvature …
We develop the quantum Boltzman equation approach for the Kondo breakdown quantum critical point, involved with two bands for conduction electrons and localized fermions. Particularly, the role of vertex corrections in transport is addressed, crucial for non-Fermi liquid transport of temperature linear dependence. Only one band of spinons may be considered for scattering with gauge fluctuations, and their associated vertex corrections are introduced in the usual way, where divergence of self-energy corrections is cancelled by that of vertex corrections, giving rise to the physically meaningful…
Kondo scaling of $4f$-electron states and the Kondo singlet breakdown in heavy fermions
Helmholtz-Zentrum Berlin für Materialien und Energie（柏林亥姆霍兹材料与能源中心）；Heidelberg University（海德堡大学）；Synchrotron SOLEIL（SOLEIL同步辐射中心）；Université de Rennes, CNRS, Institut des Sciences Chimiques de Rennes-UMR6226（雷恩大学，法国国家科学研究中心，雷恩化学科学研究所）；Université de Lorraine, CNRS, Institut Jean Lamour（洛林大学，法国国家科学研究中心，让·拉穆尔研究所）；National Synchrotron Radiation Research Center（国家同步辐射研究中心）
Competition between the Kondo effect and Ruderman-Kittel-Kasuya-Yosida interaction in the two-impurity Kondo problem can be phenomenologically described by the Rasul-Schlottmann spin model. We revisit this model from the quantum entanglement perspective by calculating both the inter-impurity entanglement and the local Kondo entanglement, the latter being the entanglement between a local magnetic impurity and its spatially nearby conduction electron. A groundstate phase diagram is derived and a discontinuous breakdown of the local Kondo entanglement is found at the singular point, associated co…
Quantum Monte Carlo studies of U(1) lattice gauge models of Kondo breakdown
Institut für Theoretische Physik und Astrophysik and Würzburg-Dresden Cluster of Excellence ct.qmat, Universität Würzburg（维尔茨堡大学理论与天体物理研究所及维尔茨堡-德累斯顿ct.qmat卓越集群）
We show that for the half-filled Kondo lattice model on the honeycomb lattice a Kondo breakdown occurs at small Kondo couplings $J_k$ within the magnetically ordered phase. Our conclusions are based on auxiliary field quantum Monte Carlo simulations of the so-called composite fermion spectral function. Within a U(1) gauge theory formulation of the Kondo model, it becomes apparent that a Higgs mechanism dictates the weight of the resonance in the spectral function. For the honeycomb lattice we observe that for small $J_k$ the quasiparticle pole gives way to incoherent spectral weight but it rem…
The topology and spin-orbital polarization of two-dimensional (2D) surface electronic states have been extensively studied in this decade. One major interest in them is their close relationship with the parities of the bulk (3D) electronic states. In this context, the surface is often regarded as a simple truncation of the bulk crystal. Here we show breakdown of the bulk-related in-plane rotation symmetry in the topological surface states (TSSs) of the Kondo insulator SmB$_6$. Angle-resolved photoelectron spectroscopy (ARPES) performed on the vicinal SmB$_6$(001)-$p$(2$\times$2) surface showed…
Emergence of a symmetry-broken Chern insulator near a moiré Kondo breakdown
Shanghai Jiao Tong University（上海交通大学）；Cornell University（康奈尔大学）；Kavli Institute at Cornell for Nanoscale Science（康奈尔纳米科学卡弗里研究所）；Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；Tsung-Dao Lee Institute, Shanghai Jiao Tong University（上海交通大学李政道研究所）；National Institute for Materials Science（国立材料研究所）；Hefei National Laboratory（合肥国家实验室）；Max Planck Institute for the Structure and Dynamics of Matter（马克斯·普朗克物质结构动力学研究所）
Flat-Band Driven Kondo Breakdown and Reentrant Effects in Heavy-Fermion Moiré Superlattices
Institute of Software Technology, German Aerospace Center（德国航空航天中心软件技术研究所）；Theoretical Division, Los Alamos National Laboratory（洛斯阿拉莫斯国家实验室理论部）；Center for Integrated Nanotechnologies, Los Alamos National Laboratory（洛斯阿拉莫斯国家实验室集成纳米技术中心）；Department of Physics, Condensed Matter Theory, TU Dortmund University（多特蒙德工业大学凝聚态理论物理系）
A review of the low temperature properties of Kondo lattice systems is presented within the mean-field approximation, focusing on the different characteristic energy scales. The Kondo temperature, T_K, and the Fermi liquid coherence energy, T_0, are analyzed as functions of the electronic filling, the shape of the non-interacting density of states, and the concentration of magnetic moments. These two scales can vanish, corresponding to a breakdown of the Kondo effect when an external magnetic field is applied. The Kondo breakdown can also be reached by adding a superexchange term to the Kondo …
Strange metal behavior arises in heavy fermion metals close to antiferromagnetic transitions. An increasing amount of experiments indicates a link of such behavior to a Kondo breakdown quantum critical point. To shed light on this intriguing problem, we study the 2D Kondo-Heisenberg model using a dynamical large-N multichannel Schwinger boson approach. We identify and characterize the quantum phase transition from an antiferromagnetically ordered ground state to a Kondo-dominated paramagnetic state, and attribute a jump in certain phase shift to Kondo breakdown. In addition, we calculate trans…
We have simulated a half-filled $1D$ $p$-wave periodic Anderson model with numerically exact projector quantum Monte Carlo technique, and the system is indeed located in the Haldane-like state as detected in previous works on the $p$-wave Kondo lattice model, though the soluble non-interacting limit corresponds to the conventional $Z_{2}$ topological insulator. The site-resolved magnetization in an open boundary system and strange correlator for the periodic boundary have been used to identify the mentioned topological states. Interestingly, the edge magnetization in the Haldane-like state is …
Recent quantum oscillation experiments on SmB$_6$ pose a paradox, for while the angular dependence of the oscillation frequencies suggest a 3D bulk Fermi surface, SmB$_6$ remains robustly insulating to very high magnetic fields. Moreover, a sudden low temperature upturn in the amplitude of the oscillations raises the possibility of quantum criticality. Here we discuss recently proposed mechanisms for this effect, contrasting bulk and surface scenarios. We argue that topological surface states permit us to reconcile the various data with bulk transport and spectroscopy measurements, interpretin…
SmB6 is a proposed topological Kondo insulator where the presence of topological nontriviality can be tuned by variations in the Sm valence. Experimentally, Sm valence can be changed by tuning stoichiometry of SmB6. We show that Raman scattering can detect vacancies lower than 1% of Sm sites in SmB6 crystal by probing the intensity of defect-induced scattering of the acoustic phonon branch at 10~meV. In the electronic Raman spectra of SmB6 at temperatures below 130~K, we observe features developing in A$_{1g}$ and E$_g$ symmetries at 100 and 41~meV which we assign to excitations between hybrid…
We present an X-ray photoemission study of the heavy-fermion system CeCu$_{6-x}$Au$_x$ across the magnetic quantum phase transition of this compound at temperatures above the single-ion Kondo temperature $T_K$. In dependence of the Au concentration $x$ we observe a sudden change of the $f$-occupation number $n_f$ and the core-hole potential $U_{df}$ at the critical concentration $x_c=0.1$. We interpret these findings in the framework of the single-impurity Anderson model. Our results are in excellent agreement with findings from earlier UPS measurements %\cite{klein08qpt} and provide further i…
Kondo breakdown induced by non-Hermitian complex hybridization
Research Institute for Innovation and Co-Creation, Osaka Metropolitan University（大阪公立大学创新与共创研究所）；Department of Physics, Osaka Metropolitan University（大阪公立大学物理系）；Nambu Yoichiro Institute of Theoretical and Experimental Physics (NITEP), Osaka Metropolitan University（大阪公立大学南部阳一郎理论实验物理研究所）；Department of Physics, Institute of Science Tokyo（东京科学大学物理系）；Department of Physics, University of Tokyo（东京大学物理系）；Fundamental Quantum Science Program, TRIP Headquarters, RIKEN（理化学研究所TRIP总部基础量子科学项目）；Department of Physics, Ritsumeikan University（立命馆大学物理系）；Department of Materials Engineering Science, University of Osaka（大阪大学材料工程科学系）
Motivated by recent experiments, we study a quasi-one dimensional model of a Kondo lattice with Ferromagnetic coupling between the spins. Using bosonization and dynamical large-N techniques we establish the presence of a Fermi liquid and a magnetic phase separated by a local quantum critical point, governed by the Kondo breakdown picture. Thermodynamic properties are studied and a gapless charged mode at the quantum critical point is highlighted.
Kondo effect is a prominent quantum phenomenon describing the many-body screening of a local magnetic impurity. Here, we reveal a new type of non-magnetic Kondo behavior generated by gauge fluctuations in strongly-correlated baths. We show that a non-magnetic bond defect not only introduces the potential scattering but also locally enhances the gauge fluctuations. The local gauge fluctuations further mediate a pseudospin exchange interaction that produces an asymmetric Kondo fixed point in low-energy. The gauge-fluctuation-induced Kondo phenomena do not exhibit the characteristic resistivity b…
In a recent paper of Nandkishore and Senthil [arxiv:1201.5998 (2012)], a concept of orthogonal metal has been introduced to reinterpret the disordered state of slave-spin representation in the Hubbard model as an exotic gapped metallic state. We extend this concept to study the corresponding quantum phase transition in the extended Anderson lattice model. It is found that the disordered state of slave spins in this model is an orbital-selective orthogonal metal, a generalization of the concept of the orthogonal metal in the Hubbard model. Near the quantum critical point the essential behaviors…
We have studied the antiferromagnetic quantum phase transition of a 2D Kondo-Heisenberg square lattice using the non-linear sigma model. A renormalization group analysis of the competing Kondo -- RKKY interaction was carried out to 1-loop order in the $ε$ expansion, and a new quantum critical point is found, dominated by Kondo fluctuations. In addition, the spin-wave velocity scales logarithmically near the new QCP, i.e breakdown of hydrodynamic behavior. The results allow us to propose a new phase diagram near the AFM fixed point of this 2D Kondo lattice model.
We present an effective field theory for the Kondo lattice, which can exhibit, in a certain range of parameters, a non Fermi liquid paramagnetic phase at the brink of a zero temperature Anti Ferromagnetic (AF) transition. The model is derived in a natural way from the bosonic Kondo-Heisenberg model, in which the Kondo resonances are treated as true (but damped) Grassmann fields. One loop Renormalization Group (RG) treatment of this model gives a phase diagram for the Kondo lattice as a function of $ J_K $ where, for $ J_K< J_c$ the system shows AF order, for $J_K> J_1$ one has the heavy electr…
We present results of high-resolution, low-temperature measurements of the Hall coefficient, thermopower, and specific heat on stoichiometric YbRh2Si2. They support earlier conclusions of an electronic (Kondo-breakdown) quantum critical point concurring with a field induced antiferromagnetic one. We also discuss the detachment of the two instabilities under chemical pressure. Volume compression/expansion (via substituting Rh by Co/Ir) results in a stabilization/weakening of magnetic order. Moderate Ir substitution leads to a non-Fermi-liquid phase, in which the magnetic moments are neither ord…
We propose a new phenomenological framework for three classes of Kondo lattice materials that incorporates the interplay between the fluctuations associated with the antiferromagnetic quantum critical point and those produced by the hybridization quantum critical point that marks the end of local moment behavior. We show that these fluctuations give rise to two distinct regions of quantum critical scaling: hybridization fluctuations are responsible for the logarithmic scaling in the density of states of the heavy electron Kondo liquid that emerges below the coherence temperature T*; while the …
We investigate f-electron charge susceptibility in a two-impurity Anderson model on the basis of Wilson's numerical renormalization group method. The f-electron charge susceptibility diverges logarithmically at the critical point of this model when conduction-electron bands exhibit particle-hole symmetry. Although the critical point disappears without the particle-hole symmetry, the f-electron charge fluctuation is much more enhanced near the crossover regime between the Kondo-Yosida singlet and intersite spin-singlet states than that in the single-impurity case. This result shows that charge …
Unconventional quantum criticality in heavy-fermion systems has been extensively analyzed in terms of a critical destruction of the Kondo effect. Motivated by a recent demonstration of quantum criticality in a mixed-valent heavy-fermion system, β-YbAlB4, we study a particle-hole-asymmetric Anderson impurity model with a pseudogapped density of states. We demonstrate Kondo destruction at a mixed-valent quantum critical point, where a collapsing Kondo energy scale is accompanied by a singular charge-fluctuation spectrum. Both spin and charge responses scale with energy over temperature (ω/T) and…
We study a localized spin coupled to an Anderson impurity to model the situation found in higher transition metal or rare earth compounds like e.g.\ LaMnO$_3$ or Gd monopnictides. We find that, even for large quantum numbers of the localized spin, quantum fluctuations play an essential role for the case of ferromagnetic coupling between the spin and the impurity levels. For antiferromagnetic coupling, a description in terms of a classical spin is appropriate.
Experiments in heavy-fermion metals and related theoretical work suggest that critical local-moment fluctuations can play an important role near a zero-temperature phase transition. We study such fluctuations at the quantum critical point of a Kondo impurity model in which the density of band states vanishes as |E|^r at the Fermi energy (E = 0). The local spin response is described by a set of critical exponents that vary continuously with r. For 0 < r < 1, the dynamical susceptibility exhibits omega/T scaling with a fractional exponent, implying that the critical point is interacting.
Quantum criticality in Yb(Rh0.97Co0.03)2Si2 is investigated by means of resistivity and magnetoresistance. The partial substitution of Co leads to a stabilization of the magnetism as expected according to the application of chemical pressure for Yb systems. However, the signature of the Kondo-breakdown remains at the same position in the temperature-magnetic field phase diagram compared to stoichiometric YbRh2Si2. As a consequence, the Kondo-breakdown is situated within the antiferromagnetic phase. These results fit well within the global phase diagram under chemical pressure [1].
We use hard x-ray photoemission spectroscopy (HAXPES) to investigate the electronic structure of YbAl2, for which the Yb valence has not been consistently reported to date. The bulk sensitivity and the analytical simplicity provided by the Yb 3d core-level HAXPES allow a reliable determination of the mean valence of Yb ions. For YbAl2, it is evaluated to be +2.20, which remains nearly unchanged below 300 K. The Kondo resonance peak with an extremely high Kondo temperature (above 2000 K) is clearly identified in the valence-band spectra. The results indicate that a coherent Kondo state can be r…
In a Kondo lattice, the spin exchange coupling between a local spin and the conduction electrons acquires nonlocal contributions due to conduction electron scattering from surrounding local spins and the subsequent RKKY interaction. It leads to a hitherto unrecognized interference of Kondo screening and the RKKY interaction beyond the Doniach scenario. We develop a renormalization group theory for the RKKY-modified Kondo vertex. The Kondo temperature, $T_K(y)$, is suppressed in a universal way, controlled by the antiferromagnetic RKKY coupling parameter $y$. Complete spin screening ceases to e…
