Performances and stability of a 2.4 ton Gd organic liquid scintillator target for antineutrino detection
I. R. Barabanov, L. B. Bezrukov, C. Cattadori, N. A. Danilov, A. Di Vacri, Yu. S. Krilov, L. Ioannucci, E. A. Yanovich, M. Aglietta, A. Bonardi, G. Bruno, W. Fu… 展开作者
I. R. Barabanov, L. B. Bezrukov, C. Cattadori, N. A. Danilov, A. Di Vacri, Yu. S. Krilov, L. Ioannucci, E. A. Yanovich, M. Aglietta, A. Bonardi, G. Bruno, W. Fulgione, E. Kemp, A. S. Malguin, A. Porta, M. Selvi
In this work we report the performances and the chemical and physical properties of a (2 x 1.2) ton organic liquid scintillator target doped with Gd up to ~0.1%, and the results of a 2 year long stability survey. In particular we have monitored the amount of both Gd and primary fluor actually in solution, the optical and fluorescent properties of the Gd-doped liquid scintillator (GdLS) and its performances as a neutron detector, namely neutron capture efficiency and average capture time. The experimental survey is ongoing, the target being continuously monitored. After two years from the doping time the performances of the Gd-doped liquid scintillator do not show any hint of degradation and instability; this conclusion comes both from the laboratory measurements and from the "in-tank" measurements. This is the largest stable Gd-doped organic liquid scintillator target ever produced and continuously operated for a long period.
Over the course of several decades, organic liquid scintillators have formed the basis for successful neutrino detectors. Gadolinium-loaded liquid scintillators provide efficient background suppression for electron antineutrino detection at nuclear reactor plants. In the Double Chooz reactor antineutrino experiment, a newly developed beta-diketonate gadolinium-loaded scintillator is utilized for the first time. Its large scale production and characterization are described. A new, light yield matched metal-free companion scintillator is presented. Both organic liquids comprise the target and "G…
This study presents a new concept of segmented antineutrino detector based on hexagonal plastic scintillator bars for detecting antineutrinos from a nuclear reactor core. The choice of hexagonal scintillator bars is original and provides compactness. The proposed detector detects antineutrinos via inverse beta decay (IBD) with the prompt-delayed double coincidence. Owing to its segmented structure, the background, which satisfies the delayed coincidence condition can be eliminated by applying proper event selection cuts. In this manner, the main focus is to determine proper selection criteria …
We propose a new type segmented antineutrino detector made of plastic scintillators for the nuclear safeguard application. A small prototype was built and tested to measure background events. A satisfactory unmanned field operation of the detector system was demonstrated. Besides, a detailed Monte Carlo simulation code was developed to estimate the antineutrino detection efficiency of the detector.
We developed a segmented reactor-antineutrino detector made of plastic scintillators for application as a tool in nuclear safeguards inspection and performed mostly unmanned field operations at a commercial power plant reactor. At a position outside the reactor building, we measured the difference in reactor antineutrino flux above the ground when the reactor was active and inactive.
In this study, simulation-based design and optimization studies of a gadolinium loaded segmented plastic scintillator detector are presented for monitoring applications of nuclear reactors in Turkey using antineutrinos. For the first time in the literature, a multivariate analysis technique is introduced to suppress cosmic background for such a reactor antineutrino detector.
Several liters of an organic liquid scintillator (LS) loaded with Nd have been made. We report on performances of this scintillator in terms of optical properties, radiopurity and light yield for a Nd concentration of 6.5 g/l. A possible application to search for the 150Nd neutrinoless double beta decay with a 10-ton scale LS detector is discussed together with further improvements.
We regard the possibility of detecting the antineutrino flux producing by the $^{40}$K placing inside the Earth. Thermal flux of the Earth could be better understood with observing such a flux. Lower and upper limitations on the $^{40}$K antineutrino flux are presented.
We present a characterization of a small (9-liter) and mobile 0.1% 6Li-doped pulse-shape-sensitive plastic scintillator antineutrino detector called SANDD (Segmented AntiNeutrino Directional Detector), constructed for the purpose of near-field reactor monitoring with sensitivity to antineutrino direction. SANDD comprises three different types of module. A detailed Monte Carlo simulation code was developed to match and validate the performance of each of the three modules. The combined model was then used to produce a prediction of the performance of the entire detector. Analysis cuts were esta…
We introduce a novel approach to investigate CP violation in the neutrino sector, based on the simultaneous detection of $ν_e$ and $\barν_e$ stemming from the oscillation of $ν_μ$ and $\barν_μ$ produced in the decay at rest of $π$s and $μ$s at a beam dump. This approach relies on a novel liquid scintillator detector technology expected to yield unprecedented identification of $ν_e$ and $\barν_e$ charged-current interactions, which we investigate by means of Montecarlo simulations. Here we report preliminary results concerning both the detection technique and its physics reach.
The DANSS project is aimed at creating a relatively compact neutrino spectrometer which does not contain any flammable or other dangerous liquids and may therefore be located very close to the core of an industrial power reactor. As a result, it is expected that high neutrino flux would provide about 15,000 IBD interactions per day in the detector with a sensitive volume of 1 m$^3$. High segmentation of the plastic scintillator will allow to suppress a background down to a 1% level. Numerous tests performed with a simplified pilot prototype DANSSino under a 3 GW$_{th}$ reactor of the Kalinin N…
A meter-long, 23-liter EJ-309 liquid scintillator detector has been constructed to study the light collection and pulse-shape discrimination performance of elongated scintillator cells for the PROSPECT reactor antineutrino experiment. The magnitude and uniformity of light collection and neutron/gamma discrimination power in the energy range of antineutrino inverse beta decay products have been studied using gamma and spontaneous fission calibration sources deployed along the cell long axis. We also study neutron-gamma discrimination and light collection abilities for differing PMT and reflecto…
The fluorescence decay-time constants have been measured for several scintillator mixtures based on phenyl-o-xylylethane (PXE) and linear alkylbenzene (LAB) solvents. The resulting values are of relevance for the physics performance of the proposed large-volume liquid scintillator detector LENA (Low Energy Neutrino Astronomy). In particular, the impact of the measured values to the search for proton decay via p -> K+ antineutrino is evaluated in this work.
In this work, the simulation of optical photons is carried out in an antineutrino detector module consisting of a plastic scintillator connected to light guides and photomultipliers on both ends, which is considered to be used for remote reactor monitoring in the field of nuclear safety. Using Monte Carlo (MC) based GEANT4 simulation, numerous parameters influencing the light collection and thereby the energy resolution of the antineutrino detector module are studied: e.g., degrees of scintillator surface roughness, reflector type, and its ap- plying method onto scintillator and light guide su…
The Daya Bay Antineutrino Detector gas system is designed to protect the liquid scintillator targets of the antineutrino detectors against degradation and contamination from exposure to ambient laboratory air. The gas system is also used to monitor the leak tightness of the antineutrino detector assembly. The cover gas system constantly flushes the gas volumes above the liquid scintillator with dry nitrogen to minimize oxidation of the scintillator over the five year lifetime of the experiment. This constant flush also prevents the infiltration of radon or other contaminants into these detecti…
The electron antineutrino spectrum in the Stereo reactor experiment (ILL Grenoble) is measured via the inverse beta decay signals in an organic liquid scintillator. The six target cells of the Stereo detector are filled with about 1800 litres of Gd-loaded liquid scintillator optimised for the requirements of the experiment. These target cells are surrounded by similar cells containing liquid scintillator without the Gd-loading. The development and characteristics of these scintillators are reported. In particular, the transparency, light production and pulse shape discrimination capabilities o…
A detector material or configuration that can provide an unambiguous indication of neutron capture can substantially reduce random coincidence backgrounds in antineutrino detection and capture-gated neutron spectrometry applications. Here we investigate the performance of such a material, a composite of plastic scintillator and $^6$Li$_6^{nat}$Gd$(^{10}$BO$_{3})_{3}$:Ce (LGB) crystal shards of ~1 mm dimension and comprising 1% of the detector by mass. While it is found that the optical propagation properties of this material as currently fabricated are only marginally acceptable for antineutri…
Purification of the 278 tons of liquid scintillator and 889 tons of buffer shielding for the Borexino solar neutrino detector was performed with a system that combined distillation, water extraction, gas stripping and filtration. The purification of the scintillator achieved unprecedented low backgrounds for the large scale liquid scintillation detector. This paper describes the principles of operation, design, construction and commissioning of the purification system, and reviews the requirements and methods to achieve system cleanliness and leak-tightness.
A method for energy and radius reconstruction with simulated charge information in a ton-scale liquid scintillator detector like Taishan Antineutrino Observatory
Institute of High Energy Physics, Chinese Academy of Sciences（中国科学院高能物理研究所）；Kaiping Neutrino Research Center（开平中微子研究中心）；Department of Applied Sciences, School of Engineering and Technology, CGC University（CGC大学工程技术学院应用科学系）；TIANFU Cosmic Ray Research Center（天府宇宙线研究中心）
The Daya Bay Reactor Neutrino Experiment has measured the neutrino mixing angle θ_{13} to world-leading precision. The experiment uses eight antineutrino detectors filled with 20-tons of gadolinium-doped liquid scintillator to detect antineutrinos emitted from the Daya Bay nuclear power plant through the inverse beta decay reaction. The precision measurement of sin^{2}2θ_{13} relies on the relative antineutrino interaction rates between detectors at near (400 m) and far (roughly 1.8 km) distances from the nuclear reactors. The measured interaction rate in each detector is directly proportional…
New experimental research programs in the field of neutrino physics are calling for new detectors with large masses, high energy resolution and good background rejection capabilities. This paper presents a novel hybrid organic/inorganic scintillator, which is able to improve on all three aspects simultaneously. This scintillator consists of microscopic grains of inorganic crystals suspended in an organic scintillating carrier medium. Due to multiple scattering off the crystals, this scintillator appears opaque over longer distances and is intended for use in specialized detectors. Thanks to th…
A liquid scintillator (LS) is developed for the Taishan Antineutrino Observatory (TAO), a ton-level neutrino detector to measure the reactor antineutrino spectrum with sub-percent energy resolution by adopting Silicon Photomultipliers (SiPMs) as photosensor. To reduce the dark noise of SiPMs to an acceptable level, the LS has to work at -50 degree or lower. A customized apparatus based on a charge-coupled device (CCD) is developed to study the transparency of the liquid samples in a cryostat. We find that the water content in LS results in transparency degradation at low temperature, which can…
We report on the production and characterization of liquid scintillators for the detection of electron antineutrinos by the Daya Bay Reactor Neutrino Experiment. One hundred eighty-five tons of gadolinium-loaded (0.1% by mass) liquid scintillator (Gd-LS) and two hundred tons of unloaded liquid scintillator (LS) were successfully produced from a linear-alkylbenzene (LAB) solvent in six months. The scintillator properties, the production and purification systems, and the quality assurance and control (QA/QC) procedures are described.
Measurement of Light Yield Response of Gd-compatible Water-based Liquid Scintillator with the Brookhaven 1-ton testbed
Chung-Ang University（中央大学）；University of California at Berkeley（加州大学伯克利分校）；Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室）；Brookhaven National Laboratory（布鲁克海文国家实验室）；The Pennsylvania State University（宾夕法尼亚州立大学）；Bronx Community College（布朗克斯社区学院）；University of Alabama（阿拉巴马大学）；Stony Brook University（石溪大学）
Organic liquid scintillators are used in many neutrino physics experiments of the past and present. In particular for low energy neutrinos when realtime and energy information are required, liquid scintillators have several advantages compared to other technologies. In many cases the organic liquid needs to be loaded with metal to enhance the neutrino signal over background events. Several metal loaded scintillators of the past suffered from chemical and optical instabilities, limiting the performance of these neutrino detectors. Different ways of metal loading are described in the article wit…
A large-volume liquid scintillator can be used as a tracking detector to measure high-energy neutrino events, like atmospheric neutrinos and neutrino beams. The lepton flavor recognition is almost absolute above 1 GeV. The energy resolution is 2--5 %, the main uncertainties coming from nuclear physics and poorly recognized hadrons. At GeV scale antineutrinos may be statistically distinguishable from neutrinos by neutron and proton signals.
The next generation of very-short-baseline reactor experiments will require compact detectors operating at surface level and close to a nuclear reactor. This paper presents a new detector concept based on a composite solid scintillator technology. The detector target uses cubes of polyvinyltoluene interleaved with $^6$LiF:ZnS(Ag) phosphor screens to detect the products of the inverse beta decay reaction. A multi-tonne detector system built from these individual cells can provide precise localisation of scintillation signals, making efficient use of the detector volume. Monte Carlo simulations …
Environmental radioactivity is a dominant background for rare decay search experiments, and it is difficult to completely remove such an impurity from detector vessels. We propose a scintillation balloon as the active vessel of a liquid scintillator in order to identify this undesirable radioactivity. According to our feasibility studies, the scintillation balloon enables the bismuth--polonium sequential decay to be tagged with a 99.7\% efficiency, assuming a KamLAND (Kamioka Liquid scintillator AntiNeutrino Detector)-type liquid scintillator detector. This tagging of sequential decay using al…
JUNO is a 20 kt Liquid Scintillator Antineutrino Detector currently under construction in the south of China. This report reviews JUNO's physics programme related to all neutrino sources but reactor antineutrinos, namely neutrinos from supernova burst, solar neutrinos and geoneutrinos.
Three-dimensional finely grained plastic scintillator detectors bring many advantages in particle detectors, allowing a massive active target which enables a high-precision tracking of interaction products, excellent calorimetry and a sub-nanosecond time resolution. Whilst such detectors can be scaled up to several-tonnes, as required by future neutrino experiments, a relatively long production time, where each single plastic-scintillator element is independently manufactured and machined, together with potential challenges in the assembly, complicates their realisation. In this manuscript we …
In order to carry out research in the field of possible existence of a sterile neutrino the laboratory based on SM-3 reactor (Dimitrovgrad, Russia) was created to search for oscillations of reactor antineutrino. The prototype of a multi-section neutrino detector with liquid scintillator volume of 350 l was installed in the middle of 2015. It is a moveable inside the passive shielding detector, which can be set at distance range from 6 to 11 meters from the reactor core. Measurements of antineutrino flux at such short distances from the reactor core are carried out with moveable detector for th…
The Jiangmen Underground Neutrino Observatory (JUNO) uses 20k tons of liquid scintillator (LS)to detect neutrinos. The content of radioactive substances in the liquid scintillator will affect theexperimental results. JUNO will use counter current water extraction to reduce the radioactive metalions inside the LS. In this article, The factors that affect the final water extraction like the partitioncoefficient and the factors that affect it, the optimal mass transfer droplet size, the flow rate ratio,theoretical stage and different working mode (LS as continuous phase or dispersed phase) have b…
Electron antineutrinos are detected in organic liquid scintillator based neutrino experiments by means of the inverse beta decay, producing both a positron and a neutron. The positron may form a bound state together with an electron, called positronium (Ps). The longer-lived spin state of Ps, orthopositronium (o-Ps) has a lifetime of about $3\,\mathrm{ns}$ in organic liquid scintillators (LS). Its formation changes the time distribution of photon emission, which affects positron reconstruction algorithms and allows the application of pulse shape discrimination (PSD) to distinguish electron fro…
The NUCLEUS experiment aims at measuring the coherent elastic scattering of nuclear reactor antineutrinos off nuclei using cryogenic calorimeters. Operating at an overburden of 3m.w.e., muon-induced backgrounds are expected to be dominant. It is therefore essential to develop an efficient muon veto, with a detection efficiency of more than 99%. This will be realized in NUCLEUS through a compact cube assembly of plastic scintillator panels. In order to prevent a large unshielded area where the cryostat intersects the shielding arrangement without unnecessarily increasing the induced detector de…
The Daya Bay reactor antineutrino experiment has recently measured the neutrino mixing parameter sin22θ13 by observing electron antineutrino disappearance over kilometer-scale baselines using six antineutrino detectors at near and far distances from reactor cores at the Daya Bay nuclear power complex. Liquid scintillator contained in transparent target vessels is used to detect electron antineutrinos via the inverse beta-decay reaction. The Daya Bay experiment will operate for about five years yielding a precision measurement of sin22θ13. We report on long-term studies of poly(methyl methacryl…
In this study, the conceptual design and physics simulations of a near-field Water-based Liquid Scintillator (WbLS) detector placed 100 meters from the Akkuyu Nuclear Power Plant (ANPP), currently under construction and aiming at being Turkey's first nuclear power plant, is presented. The ANPP is an excellent opportunity for neutrino studies and the development of an R&D program for neutrino detectors in Turkey. The Reactor Neutrino Experiments of Turkey (RNET) program includes a compact and portable detector with a 2.5-ton volume of WbLS and a ~30% photo-coverage, and the program is planned t…
The cosmic rays data collected using a large area plastic scintillator array ISMRAN (Indian Scintillator Matrix for Reactor AntiNeutrino) are presented. The data collected serve as a useful benchmark of cosmogenic background in a non-reactor environment for the future measurements of electron-antineutrinos to be performed using the ISMRAN setup. The zenith angle distribution of the atmospheric muons has been measured and compared with Monte Carlo expectations. The detector setup was further used to measure the lifetime distribution of stopped muons and extract their rates inside the detector m…
Core-collapse supernovae produce an intense burst of electron antineutrinos in the few-tens-of-MeV range. Several Large Liquid Scintillator-based Detectors (LLSD) are currently operated worldwide, being very effective for low energy antineutrino detection through the Inverse Beta Decay (IBD) process. In this article, we develop a procedure for the prompt extraction of the supernova location by revisiting the details of IBD kinematics over the broad energy range of supernova neutrinos. Combining all current scintillator-based detector, we show that one can locate a canonical supernova at 10 kpc…
This study investigates the deployment of a medium-scale neutrino detector near Turkey's first nuclear power plant, the Akkuyu Nuclear Power Plant. The aim of this detector is to become a modular testbed for new technologies in the fields of new detection media and innovative photosensors. Such technologies include Water-based Liquid Scintillator (WbLS), Large Area Picosecond Photo-Detectors (LAPPDs), dichroic Winston cones, and large area silicon photomultiplier modules. The detector could be used for instantaneous monitoring of the Akkuyu Nuclear Power Plant via its antineutrino flux. In add…
The JSNS$^{2}$ (J-PARC Sterile Neutrino Search at J-PARC Spallation Neutron Source) experiment will search for neutrino oscillations over a 24 m short baseline at J-PARC. The JSNS$^{2}$ inner detector will be filled with 17 tons of gadolinium-loaded liquid scintillator (LS) with an additional 31 tons of unloaded LS in the intermediate $γ$-catcher and outer veto volumes. JSNS$^{2}$ has chosen Linear Alkyl Benzene (LAB) as an organic solvent because of its chemical properties. The unloaded LS was produced at a refurbished facility, originally used for scintillator production by the RENO experime…
We propose the first truly directional antineutrino detector for antineutrinos above the hydrogen inverse beta decay (IBD) threshold, with potential applications including monitoring for nuclear nonproliferation, spatially mapping geo-neutrinos, characterizing the diffuse supernova neutrino background, and searching for new physics in the neutrino sector. The detector consists of adjacent and separated target and capture scintillator planes. IBD events take place in the target layers, which are thin enough to allow the neutrons to escape without scattering elastically. The neutrons are detecte…
Future generations of liquid scintillator neutrino experiments will require stably loading tons of candidate isotopes into kiloton-scale detectors, representing a significant chemical challenge. Nanoparticles containing the candidate isotopes provide a promising method for this loading. Additionally, the unique optical properties of nanoparticles can enhance detection and background discrimination. Perovskite nanocrystals are particularly attractive due to the reliability of their crystal structure and their easily-scalable synthesis. We present here the first study of lead-based perovskite na…
The reactor neutrino and gallium anomalies can be tested with a 3-4 PBq (75-100 kCi scale) 144Ce-144Pr antineutrino beta-source deployed at the center or next to a large low-background liquid scintillator detector. The antineutrino generator will be produced by the Russian reprocessing plant PA Mayak as early as 2014, transported to Japan, and deployed in the Kamioka Liquid Scintillator Anti-Neutrino Detector (KamLAND) as early as 2015. KamLAND's 13 m diameter target volume provides a suitable environment to measure the energy and position dependence of the detected neutrino flux. A characteri…
Antineutrinos from a nuclear reactor comprise an unshieldable signal which carries information about the core. A gadolinium-doped, water-based Cherenkov detector could detect reactor antineutrinos for mid- to far-field remote reactor monitoring for non-proliferation applications. Two novel and independent reconstruction and analysis pathways have been developed and applied to a number of representative reactor signals to evaluate the sensitivity of a kiloton-scale, gadolinium-doped Cherenkov detector as a remote monitor. The sensitivity of four detector configurations to nine reactor signal co…
This article describes the setup and performance of the near and far detectors in the Double Chooz experiment. The electron antineutrinos of the Chooz nuclear power plant were measured in two identically designed detectors with different average baselines of about 400 m and 1050 m from the two reactor cores. Over many years of data taking the neutrino signals were extracted from interactions in the detectors with the goal of measuring a fundamental parameter in the context of neutrino oscillation, the mixing angle θ13. The central part of the Double Chooz detectors was a main detector comprisi…
The Jiangmen Underground Neutrino Observatory (JUNO) is designed to study neutrino mass hierarchy and measure three of the neutrino oscillation parameters with high precision using reactor antineutrinos. It is also able to study many other physical phenomena, including supernova neutrinos, solar neutrinos, geo-neutrinos, atmosphere neutrinos, and so forth. The central detector of JUNO contains 20,000~tons of liquid scintillator (LS) and about 18,000 20-inch photomultiplier tubes (PMTs), which is the largest liquid scintillator one under construction in the world up today. The energy resolution…
The Daya Bay experiment measures sin^2 2θ_13 using functionally identical antineutrino detectors located at distances of 300 to 2000 meters from the Daya Bay nuclear power complex. Each detector consists of three nested fluid volumes surrounded by photomultiplier tubes. These volumes are coupled to overflow tanks on top of the detector to allow for thermal expansion of the liquid. Antineutrinos are detected through the inverse beta decay reaction on the proton-rich scintillator target. A precise and continuous measurement of the detector's central target mass is achieved by monitoring the the …
A new experiment, which is called as NEOS (NEutrino Oscillation at Short baseline), is proposed on the site of Hanbit reactors at Yonggwang, South Korea, to investigate a reactor antineutrino anomaly. A homogeneous NEOS detector having a 1000-L target volume has been constructed and deployed at the tendon gallery ~25 m away from the reactor core. A linear alkylbenzene (LAB) is used as a main base solvent of the NEOS detector. Furthermore, a di-isopropylnaphthalene (DIN) is added to improve the light output and pulse shape discrimination (PSD) ability. The ratio of LAB to DIN is 90:10. PPO (3 g…
Pulse shape discrimination (PSD) is one of the most distinctive features of liquid scintillators. Since the introduction of the scintillation techniques in the field of particle detection, many studies have been carried out to characterize intrinsic properties of the most common liquid scintillator mixtures in this respect. Several application methods and algorithms able to achieve optimum discrimination performances have been developed. However, the vast majority of these studies have been performed on samples of small dimensions. The Counting Test Facility, prototype of the solar neutrino ex…
An upgrade of the long baseline neutrino experiment T2K near detector ND280 is currently being developed with the goal to reduce systematic uncertainties in the prediction of number of events at the far detector Super-Kamiokande. The upgrade program includes the design and construction of a new highly granular fully active scintillator detector with 3D WLS fiber readout as a neutrino target. The detector of about $200\times 180\times 60~cm^3$ in size and a mass of $\sim$2.2~tons will be assembled from about $2\times10^6$ plastic scintillator cubes of $1\times1\times1~cm^3$. Each cube is read o…
