Sr lattice clock at 1x10^{-16} fractional uncertainty by remote optical evaluation with a Ca clock
A. D. Ludlow, T. Zelevinsky, G. K. Campbell, S. Blatt, M. M. Boyd, M. H. G. de Miranda, M. J. Martin, J. W. Thomsen, S. M. Foreman, Jun Ye, T. M. Fortier, J. E.… 展开作者
A. D. Ludlow, T. Zelevinsky, G. K. Campbell, S. Blatt, M. M. Boyd, M. H. G. de Miranda, M. J. Martin, J. W. Thomsen, S. M. Foreman, Jun Ye, T. M. Fortier, J. E. Stalnaker, S. A. Diddams, Y. Le Coq, Z. W. Barber, N. Poli, N. D. Lemke, K. M. Beck, C. W. Oates
Optical atomic clocks promise timekeeping at the highest precision and accuracy, owing to their high operating frequencies. Rigorous evaluations of these clocks require direct comparisons between them. We have realized a high-performance remote comparison of optical clocks over km-scale urban distances, a key step for development, dissemination, and application of these optical standards. Through this remote comparison and a proper design of lattice-confined neutral atoms for clock operation, we evaluate the uncertainty of a strontium (Sr) optical lattice clock at the 1x10-16 fractional level, surpassing the best current evaluations of cesium (Cs) primary standards. We also report on the observation of density-dependent effects in the spin-polarized fermionic sample and discuss the current limiting effect of blackbody radiation-induced frequency shifts.
A major outstanding problem for many quantum clock synchronization protocols is the hidden assumption of the availability of synchronized clocks within the protocol. In general, quantum operations between two parties do not have consistent phase definitions of quantum states, which introduce an unknown systematic phase error. We show that despite prior arguments to the contrary, it is possible to remove this unknown phase via entanglement purification. This closes the loophole for entanglement based quantum clock synchronization protocols, which are most compatible with current photon based lo…
The energy levels and electric dipole ($E1$) matrix elements of the ground state and low-lying excited states of Be atoms are calculated using the relativistic configuration interaction plus core polarization (RCICP) method. The static and dynamic $E1$, magnetic dipole ($M1$) and electric quadrupole ($E2$) polarizabilities as well as the hyperpolarizabilities of the $2s^2~^1S_0$ and $2s2p~^3P_0$ states are determined. Two magic wavelengths, 300.03 and 252.28 nm, of $2s^2~^1S_0 \rightarrow 2s2p~^3P_0$ clock transition are found. Then, the multipolar and nonlinear Stark shifts of the clock trans…
We analyze spin squeezing via Rydberg dressing in optical lattice clocks with random fractional filling. We compare the achievable clock stability in different lattice geometries, including unity-filled tweezer clock arrays and fractionally filled lattice clocks with varying dimensionality. We provide practical considerations and useful tools in the form of approximate analytical expressions and fitting functions to aid in the experimental implementation of Rydberg-dressed spin squeezing. We demonstrate that spin squeezing via Rydberg dressing in one-, two-, and three-dimensional optical latti…
With Hg atoms confined in an optical lattice trap in the Lamb-Dicke regime, we obtain a spectral line at 265.6 nm in which the full-width at half-maximum is <15Hz. Here we lock an ultrastable laser to this ultranarrow clock transition and achieve a fractional frequency stability of 5.4x10^(-15)/sqrt(tau) for tau<=400s. The highly stable laser light used for the atom probing is derived from a 1062.6 nm fiber laser locked to an ultrastable optical cavity that exhibits a mean drift rate of -6.0x10^(-17) s^(-1) (or -16.9 mHz.s^(-1) at 282 THz) over a five month period. A comparison between two suc…
In this paper, blackbody radiation (BBR) temperature rise seen by the $^{40}$Ca$^+$ ion confined in a miniature Paul trap and its uncertainty have been evaluated via finite-element method (FEM) modelling. The FEM model was validated by comparing with thermal camera measurements, which were calibrated by PT1000 resistance thermometer, at several points on a dummy trap. The input modelling parameters were analyzed carefully in detail, and their contributions to the uncertainty of environment temperature were evaluated on the validated FEM model. The result shows that the temperature rise seen by…
This article describes the recent progress of optical lattice clocks with neutral strontium ($^{87}$Sr), ytterbium ($^{171}$Yb) and mercury ($^{199}$Hg) atoms. In particular, we present frequency comparison between the clocks locally via an optical frequency comb and between two Sr clocks at remote sites using a phase-stabilized fibre link. We first review cryogenic Sr optical lattice clocks that reduce the room-temperature blackbody radiation shift by two orders of magnitude and serve as a reference in the following clock comparisons. Similar physical properties of Sr and Yb atoms, such as tr…
Over a two-year duration, we have compared the frequency of the 199Hg+ 5d106s 2S 1/2 (F=0)<-> 5d9 6s2 2D 5/2 (F=2) electric-quadrupole transition at 282 nm with the frequency of the ground-state hyperfine splitting in neutral 133Cs. These measurements show that any fractional time variation of the ratio nu(Cs)/nu(Hg) between the two frequencies is smaller than +/- 7 10^-15 / yr (1 sigma uncertainty). According to recent atomic structure calculations, this sets an upper limit to a possible fractional time variation of g(Cs) m_e / m_p alpha^6.0 at the same level.
Aided by ultra-high resolution spectroscopy, the overall systematic uncertainty of the $^{1}S_{0}$-$^{3}P_{0}$ clock resonance for lattice-confined $^{87}$Sr has been characterized to $9\times10^{-16}$. This uncertainty is at a level similar to the Cs-fountain primary standard, while the potential stability for the lattice clocks exceeds that of Cs. The absolute frequency of the clock transition has been measured to be 429,228,004,229,874.0(1.1) Hz, where the $2.5\times10^{-15}$ fractional uncertainty represents the most accurate measurement of a neutral-atom-based optical transition frequency…
The optical lattice clock NICT-Sr1 regularly reports calibration measurements of the international timescale TAI. By comparing measurement results to the reports of eight Primary Frequency Standards, we find the absolute frequency of the $^{87}\mathrm{Sr}$ clock transition to be f(Sr)=$429\,228\,004\,229\,873.082(76)$, with a fractional uncertainty of less than 1.8x10$^{-16}$ approaching the systematic limits of the best realization of SI second. Our result is consistent with other recent measurements and further supported by the loop closure over the absolute frequencies of $^{87}\mathrm{Sr}$…
There has been tremendous progress in the performance of optical frequency standards since the first proposals to carry out precision spectroscopy on trapped, single ions in the 1970s. The estimated fractional frequency uncertainty of today's leading optical standards is currently in the $10^{-18}$ range, approximately two orders of magnitude better than that of the best caesium primary frequency standards. This exceptional accuracy and stability is resulting in a growing number of research groups developing optical clocks. While good review papers covering the topic already exist, more practi…
We present a mathematical framework adapted to the comparison of atomic clocks remotely connected by a complex network of optical or microwave links. This framework facilitates the computation of frequency ratios using a generic set of equations that are valid for a wide variety of clock architectures, making the comparison of a large number of clocks practical. This formalism suggests a generic data exchange protocol that can be used in clock comparison collaborations, for which data logging and decision taking are completely local procedures, independently implemented by the participants.
For the past 15 years, tremendous progress within the fields of laser stabilization, optical frequency combs and atom cooling and trapping have allowed the realization of optical atomic clocks with unrivaled performances. These instruments can perform frequency comparisons with fractional uncertainties well below $10^{-17}$, finding applications in fundamental physics tests, relativistic geodesy, and time and frequency metrology. Even though most optical clocks are currently laboratory setups, several proposals for using these clocks for field measurements or within an optical clock network ha…
The pursuit of better atomic clocks has advanced many research areas, providing better quantum state control, new insights in quantum science, tighter limits on fundamental constant variation, and improved tests of relativity. The record for the best stability and accuracy is currently held by optical lattice clocks. This work takes an important step towards realizing the full potential of a many-particle clock with a state-of-the-art stable laser. Our 87Sr optical lattice clock now achieves fractional stability of 2.2e-16 at 1 s. With this improved stability, we perform a new accuracy evaluat…
We report a cascaded optical link of 1100 km for ultra-stable frequency distribution over an Internet fiber network. The link is composed of four spans for which the propagation noise is actively compensated. The robustness and the performance of the link are ensured by five fully automated optoelectronic stations, two of them at the link ends, and three deployed on the field and connecting the spans. This device coherently regenerates the optical signal with the heterodyne optical phase locking of a low-noise laser diode. Optical detection of the beat-note signals for the laser lock and the l…
Atomic clock frequency ratios with fractional uncertainty $\leq 3.2 \times 10^{-18}$
Atom Computing；JILA, National Institute of Standards and Technology and the University of Colorado（科罗拉多大学美国国家标准与技术研究院JILA实验室）；Department of Physics, University of Colorado（科罗拉多大学物理系）；Time and Frequency Division, National Institute of Standards and Technology（美国国家标准与技术研究院时间与频率部）；Statistical Engineering Division, National Institute of Standards and Technology（美国国家标准与技术研究院统计工程部）；Infleqtion
The rapid increase in accuracy and stability of optical atomic clocks compared to the caesium atomic clock as primary standard of time and frequency asks for a future re-definition of the second in the International System of Units (SI). The status of the optical clocks based on either single ions in radio-frequency traps or on neutral atoms stored in an optical lattice is described with special emphasis of the current work at the Physikalisch-Technische Bundesanstalt (PTB). Besides the development and operation of different optical clocks with estimated fractional uncertainties in the 10^-18 …
A Wannier-Stark optical lattice clock has demonstrated unprecedented measurement precision for optical atomic clocks. We present a systematic evaluation of the lattice light shift, a necessary next step for establishing this system as an accurate atomic clock. With precise control of the atomic motional states in the lattice, we report accurate measurements of the multipolar and the hyperpolar contributions and the operational lattice light shift with a fractional frequency uncertainty of 3.5$\times$10${}^{-19}$.
A black-body radiation (BBR) shifts of (nsnp ^3P_0) - (ns^2 ^1S_0) clock transition in divalent atoms Mg, Ca, Sr, and Yb are evaluated. A theory of multipolar BBR shifts is developed and its implications are discussed. At room temperatures, the resulting uncertainties in the BBR shifts are relatively large and substantially affect the projected 10^{-18} fractional accuracy of the optical-lattice-based clocks.
We present the first characterization of the spectral properties of superradiant light emitted from the ultra-narrow, 1 mHz linewidth optical clock transition in an ensemble of cold $^{87}$Sr atoms. Such a light source has been proposed as a next-generation active atomic frequency reference, with the potential to enable high-precision optical frequency references to be used outside laboratory environments. By comparing the frequency of our superradiant source to that of a state-of-the-art cavity-stabilized laser and optical lattice clock, we observe a fractional Allan deviation of $6.7(1)\time…
We report the observation of the higher order frequency shift due to the trapping field in a $^{87}$Sr optical lattice clock. We show that at the magic wavelength of the lattice, where the first order term cancels, the higher order shift will not constitute a limitation to the fractional accuracy of the clock at a level of $10^{-18}$. This result is achieved by operating the clock at very high trapping intensity up to $400 $kW/cm$^2$ and by a specific study of the effect of the two two-photon transitions near the magic wavelength.
We experimentally demonstrate agreement between two $^{176}$Lu$^+$ frequency references using correlation spectroscopy. From a comparison at different magnetic fields, we obtain a quadratic Zeeman coefficient of $-4.89264(88)\,\mathrm{Hz/mT^2}$, which gives a corresponding fractional frequency uncertainty contribution of just $2.5\times 10^{-20}$ for comparisons at typical operating fields of 0.1\,mT. A subsequent comparison with both systems at 0.1\,mT, demonstrates a fractional frequency difference of $(-2.0\pm(3.7)_\mathrm{stat}\pm(0.9)_\mathrm{sys})\times10^{-18}$, where `stat' and `sys' i…
We discuss the minimization of the Dick effect in an optical lattice clock. We show that optimizing the time sequence of operation of the clock can lead to a significant reduction of the clock stability degradation by the frequency noise of the interrogation laser. By using a non-destructive detection of the atoms, we are able to recycle most of the atoms between cycles and consequently to strongly reduce the time spent capturing the atoms in each cycle. With optimized parameters, we expect a fractional Allan deviation better than 2E-16$τ^{-1/2}$ for the lattice clock.
We experimentally investigate an optical clock based on $^{171}$Yb ($I=1/2$) atoms confined in an optical lattice. We have evaluated all known frequency shifts to the clock transition, including a density-dependent collision shift, with a fractional uncertainty of $3.4 \times 10^{-16}$, limited principally by uncertainty in the blackbody radiation Stark shift. We measured the absolute clock transition frequency relative to the NIST-F1 Cs fountain clock and find the frequency to be 518 295 836 590 865.2(0.7) Hz.
We consider the frequency shift in optical lattice clocks which arises from the coupling of the electronic motion to the atomic motion within the lattice. For the simplest of 3-D lattice geometries this coupling is shown to only affect clocks based on blue-detuned lattices. We have estimated the size of this shift for the prospective strontium lattice clock operating at the 390 nm blue-detuned magic wavelength. The resulting fractional frequency shift is found to be on the order of $10^{-18}$ and is largely overshadowed by the electric quadrupole shift. For lattice clocks based on more complex…
Recently invented and demonstrated, optical lattice clocks hold great promise for improving the precision of modern timekeeping. These clocks aim at the 10^-18 fractional accuracy, which translates into a clock that would neither lose or gain a fraction of a second over an estimated age of the Universe. In these clocks, millions of atoms are trapped and interrogated simultaneously, dramatically improving clock stability. Here we discuss the principles of operation of these clocks and, in particular, a novel concept of "magic" trapping of atoms in optical lattices. We also highlight recently pr…
We report on a frequency ratio measurement of a ${}^{199}$Hg-based optical lattice clock referencing a ${}^{87}$Sr-based clock. Evaluations of lattice light shift, including atomic-motion-dependent shift, enable us to achieve a total systematic uncertainty of $7.2 \times 10^{-17}$ for the Hg clock. The frequency ratio is measured to be $ν_{\rm Hg}/ν_{\rm Sr}=2.629\, 314\, 209\, 898\, 909\, 60(22)$ with a fractional uncertainty of $8.4 \times 10^{-17}$, which is smaller than the uncertainty of the realization of the SI second, i.e., the SI limit.
We demonstrate a high-performance coherent-population-trapping (CPT) Cs vapor cell atomic clock using the push-pull optical pumping technique (PPOP) in the pulsed regime, allowing the detection of high-contrast and narrow Ramsey-CPT fringes. The impact of several experimental parameters onto the clock resonance and short-term fractional frequency stability, including the laser power, the cell temperature and the Ramsey sequence parameters, has been investigated. We observe and explain the existence of a slight dependence on laser power of the central Ramsey-CPT fringe line-width in the pulsed …
We report a frequency measurement of the 1S0-3P0 transition of 87Sr atoms in an optical lattice clock. The frequency is determined to be 429 228 004 229 879 (5) Hz with a fractional uncertainty that is comparable to state-of-the-art optical clocks with neutral atoms in free fall. Two previous measurements of this transition were found to disagree by about 2x10^{-13}, i.e. almost four times the combined error bar, instilling doubt on the potential of optical lattice clocks to perform at a high accuracy level. In perfect agreement with one of these two values, our measurement essentially dissipa…
We present a new evaluation of an 87Sr optical lattice clock using spin polarized atoms. The frequency of the 1S0-3P0 clock transition is found to be 429 228 004 229 873.6 Hz with a fractional accuracy of 2.6 10^{-15}, a value that is comparable to the frequency difference between the various primary standards throughout the world. This measurement is in excellent agreement with a previous one of similar accuracy.
Fiber-based remote comparison of $^{87}$Sr lattice clocks in 24 km distant laboratories is demonstrated. The instability of the comparison reaches $5\times10^{-16}$ over an averaging time of 1000 s, which is two orders of magnitude shorter than that of conventional satellite links and is limited by the instabilities of the optical clocks. By correcting the systematic shifts that are predominated by the differential gravitational redshift, the residual fractional difference is found to be $(1.0\pm7.3)\times10^{-16}$, confirming the coincidence between the two clocks. The accurate and speedy com…
We report the first accuracy evaluation of an optical lattice clock based on the 1S0 - 3P0 transition of an alkaline earth boson, namely 88Sr atoms. This transition has been enabled using a static coupling magnetic field. The clock frequency is determined to be 429 228 066 418 009(32) Hz. The isotopic shift between 87Sr and 88Sr is 62 188 135 Hz with fractional uncertainty 5.10^{-7}. We discuss the conditions necessary to reach a clock accuracy of 10^{-17} or less using this scheme.
The absolute frequency of the 1S0-3P0 clock transition of 87Sr has been measured to be 429 228 004 229 873.65 (37) Hz using lattice-confined atoms, where the fractional uncertainty of 8.6x10-16 represents one of the most accurate measurements of an atomic transition frequency to date. After a detailed study of systematic effects, which reduced the total systematic uncertainty of the Sr lattice clock to 1.5x10-16, the clock frequency is measured against a hydrogen maser which is simultaneously calibrated to the US primary frequency standard, the NIST Cs fountain clock, NIST-F1. The comparison i…
We present a measurement of the absolute frequency of the 5s$^2$ $^1$S$_0$ to 5s5p $^3$P$_0$ transition in $^{87}$Sr, which is a secondary representation of the SI second. We describe the optical lattice clock apparatus used for the measurement, and we focus in detail on how its systematic frequency shifts are evaluated with a total fractional uncertainty of $1 \times 10^{-17}$. Traceability to the International System of Units is provided via comparison to International Atomic Time (TAI). Gathering data over 5- and 15-day periods, with the lattice clock operating on average 74$\%$ of the time…
We performed an absolute frequency measurement of the $^1S_{0}$-$^3P_{0}$ transition in $^{87}$Sr with a fractional uncertainty of $1.2 \times 10^{-15}$, which is less than one third that of our previous measurement. A caesium fountain atomic clock was used as a transfer oscillator to reduce the uncertainty of the link between a strontium optical lattice clock and the SI second. The absolute value of the transition frequency is 429 228 004 229 873.56(49) Hz.
We analyze both the s- and p-wave collision induced frequency shifts and propose a over-$π$ pulse scheme to cancel the shifts in optical lattice clocks interrogated by a Rabi pulse. The collisional frequency shifts are analytically solved as a function of the pulse area and the inhomogeneity of the Rabi frequencies. Experimentally measured collisional frequency shifts in an Yb optical lattice clock are in good agreement with the analytical calculations. Based on our analysis, the over-$π$ pulse combined with a small inhomogeneity below 0.1 allows a fractional uncertainty on a level of $10^{-18…
We study ultranarrow $5s_{1/2}$ - $4f_{5/2}$ transitions in Nd$^{13+}$ and Sm$^{15+}$ and demonstrate that they lie in the optical region. The transitions are insensitive to external perturbations. At the same time they are sensitive to the variation of the fine structure constant $α$. The fractional accuracy of the frequency of the transitions can be smaller than $10^{-19}$, which may provide a basis for atomic clocks of superb accuracy. Sensitivity to the variation of $α$ approaches $10^{-20}$ per year.
We report on the isotope shift between ${}^{88}$Sr and ${}^{87}$Sr on the ${}^1S_0 - {}^3P_0$ clock transitions. The interleaved operation of an optical lattice clock with two isotopes allows the canceling out of common perturbations, such as the quadratic Zeeman shift, the clock-light shift, and the blackbody radiation shift. The isotope shift is determined to be 62 188 134.004(10) Hz, where the major uncertainty is introduced by the collisional shift that is distinct for each isotope. Our result allows us to determine the frequency of $^{88}$Sr-$^{87}$Sr optical lattice clocks with a fractio…
We develop a method of spectroscopy that uses a weak static magnetic field to enable direct optical excitation of forbidden electric-dipole transitions that are otherwise prohibitively weak. The power of this scheme is demonstrated using the important application of optical atomic clocks based on neutral atoms confined to an optical lattice. The simple experimental implementation of this method -- a single clock laser combined with a DC magnetic field-- relaxes stringent requirements in current lattice-based clocks (e.g., magnetic field shielding and light polarization), and could therefore ex…
Ultra-precise optical clocks in space will allow new studies in fundamental physics and astronomy. Within an European Space Agency (ESA) program, the Space Optical Clocks (SOC) project aims to install and to operate an optical lattice clock on the International Space Station (ISS) towards the end of this decade. It would be a natural follow-on to the ACES mission, improving its performance by at least one order of magnitude. The payload is planned to include an optical lattice clock, as well as a frequency comb, a microwave link, and an optical link for comparisons of the ISS clock with ground…
We present an analysis of the different types of noise from the detection and interrogation laser in our strontium lattice clock. We develop a noise model showing that in our setup quantum projection noise--limited detection is possible if more than 130~atoms are interrogated. Adding information about the noise spectrum of our clock laser with sub-$10^{-16}$ fractional frequency instability allows to infer the clock stability for different modes of operation. Excellent agreement with experimental observations for the instability of the difference between two interleaved stabilizations is found…
The advent of novel measurement instrumentation can lead to paradigm shifts in scientific research. Optical atomic clocks, due to their unprecedented stability and uncertainty, are already being used to test physical theories and herald a revision of the International System of units (SI). However, to unlock their potential for cross-disciplinary applications such as relativistic geodesy, a major challenge remains. This is their transformation from highly specialized instruments restricted to national metrology laboratories into flexible devices deployable in different locations. Here we repor…
Optical atomic clocks using highly-charged ions hold an intriguing promise of metrology at the 19th significant figure. Here we study transitions within the $4f^{12}$ ground-state electronic configuration of highly charged ions. We consider isotopes lacking hyperfine structure and show that the detrimental effects of coupling of electronic quadrupole moments to gradients of trapping electric field can be effectively reduced by using specially chosen virtual clock transitions. The estimated systematic fractional clock accuracy is shown to be below $10^{-19}$.
We have demonstrated a direct frequency comparison between two $^{87}{\rm Sr}$ lattice clocks operated in intercontinentally separated laboratories in real time. Two-way satellite time and frequency transfer technique based on the carrier phase was employed for a direct comparison with a baseline of 9 000 km between Japan and Germany. A clock comparison was achieved for 83 640 s resulting in a fractional difference of $(1.1\pm1.6) \times 10^{-15}$, where the statistical part is the biggest contribution to the uncertainty. This measurement directly confirms the agreement of the two optical cloc…
We report improved frequency ratio measurement with $^{87}$Sr and $^{171}$Yb optical lattice clocks at the National Metrology Institute of Japan (NMIJ). The $^{87}$Sr optical lattice clock is enhanced with several major modifications and is re-evaluated with a reduced uncertainty of $1.1\times10^{-16}$. We employed a $^{171}$Yb optical lattice clock with an uncertainty of $4\times10^{-16}$ that was developed for contributing to International Atomic Time (TAI). The measurement result is $ν_{\mathrm{Yb}}/ν_{\mathrm{Sr}}$ = 1.207 507 039 343 338 58(49)$_{\mathrm{sys}}$(6)$_{\mathrm{stat}}$ with a…
We demonstrate state-of-the-art technique of an active clock to provide a continuous superradiant lasing signal using an ensemble of trapped Cs atoms in the optical lattice. A magic wavelength of the proposed |7S1/2; F = 4, MF = 0> - |6P3/2; F = 3, MF = 0> clock transition in Cs atom is identified at 1181 nm for constructing the optical lattice. Pertinent optical lines are also found for pumping and repumping atoms from their ground states. A fractional uncertainty about 10-15 level to the clock frequency has been predicted by carrying out rigorous calculations of several atomic properties. Th…
We report on the design of a segmented linear Paul trap for optical clock applications using trapped ion Coulomb crystals. For an optical clock with an improved short-term stability and a fractional frequency uncertainty of 10^-18, we propose 115In+ ions sympathetically cooled by 172Yb+. We discuss the systematic frequency shifts of such a frequency standard. In particular, we elaborate on high precision calculations of the electric radiofrequency field of the ion trap using the finite element method. These calculations are used to find a scalable design with minimized excess micromotion of th…
Electrometry is performed using Rydberg states to evaluate the quadratic Stark shift of the $5s^2$ $^1\textrm{S}_0-5s5p$ $^3\textrm{P}_0$ clock transition in strontium. By measuring the Stark shift of the highly excited $5s75d\;^1\textrm{D}_2$ state using electromagnetically induced transparency, we characterize the electric field with sufficient precision to provide tight constraints on the systematic shift to the clock transition. Using the theoretically derived, and experimentally verified, polarizability for this Rydberg state we can measure the residual field with an uncertainty well belo…
We show that optical spectroscopy of Rydberg states can provide accurate {\em in situ} thermometry at room-temperature. Transitions from a metastable state to Rydberg states with principal quantum numbers of 25 to 30 have 200 times larger fractional frequency sensitivities to blackbody radiation than the Strontium clock transition. We demonstrate that magic wavelength lattices exist for both Strontium and Ytterbium transitions between the metastable and Rydberg states. Frequency measurements of Rydberg transitions with $10^{-16}$ accuracy provide $10 \, \mathrm{mK}$ resolution and yield a blac…
We propose here a few selective highly charged ions (HCIs), namely Ni$^{12+}$ and Cu$^{13+}$, Pd$^{12+}$ and Ag$^{13+}$, that not only promise to be very high accurate optical clocks below $10^{-19}$ uncertainties, but also offer quality factors larger than $10^{15}$ and yet possess simple atomic structures for the experimental set-up. Moreover, these ions have strong optical magnetic-dipole (M1) transitions than the previously proposed HCI clocks. They can be used for the cooling and detection techniques. To demonstrate the projected fractional uncertainties below $10^{-19}$ level, we have es…
Time and frequency are the most accurately measurable quantities, providing foundations for science and modern technologies. The accuracy relies on the SI (Systéme International) second that refers to Cs microwave clocks with fractional uncertainties at $10^{-16}$. Recent revolutionary progress of optical clocks aims to achieve $1\times 10^{-18}$ uncertainty, which however has been hindered by long averaging-times or by systematic uncertainties. Here, we demonstrate optical lattice clocks with $^{87}$Sr atoms interrogated in a cryogenic environment to address the blackbody radiation-induced fr…
Atomic clocks have recently reached a fractional timing precision of $<10^{-18}$. We point out that an array of atomic clocks, distributed along the Earth's orbit around the Sun, will have the sensitivity needed to detect the time dilation effect of mHz gravitational waves (GWs), such as those emitted by supermassive black hole binaries at cosmological distances. Simultaneous measurement of clock-rates at different phases of a passing GW provides an attractive alternative to the interferometric detection of temporal variations in distance between test masses separated by less than a GW wavelen…
We report on a series of 42 measurements of the transition frequency of the 429~THz (5s$^2$)~$^1$S$_0$--(5s5p)~$^3$P$_0$ line in $^{87}$Sr taken over three years from 2017 to 2019. They have been performed at the Physikalisch-Technische Bundesanstalt (PTB) between the laboratory strontium lattice clock and the primary caesium fountain clocks CSF1 and CSF2. The length of each individual measurement run has been extended by use of a hydrogen maser as flywheel to improve the statistical uncertainty given by the Cs clocks. We determine an averaged transition frequency of $429\:228\:004\:229\:873.0…
As optical clocks are improved to reach the frequency uncertainty below the 10$^{-17}$ level, the frequency shift due to the blackbody radiation (BBR) has been one of the major systematic effects hindering further improvement. To evaluate the BBR shift of an Yb optical lattice clock at KRISS, we installed an in-vacuum BBR shield and made radiation thermometry using a black-coated-sphere thermal probe. After we quantitatively measured the conduction loss of the thermal probe and the effects of all the external radiation sources, we determined the temperature at the atom trap site with an uncert…
We report on transferring 1E-16-level fractional frequency stability of a "master laser" operated at 1.5 μm to a "slave laser" operated at 698 nm, using a femtosecond fiber comb as transfer oscillator. With the 698 nm laser, the 1S_0 - 3P_0 clock transition of 87Sr was resolved to a Fourier-limited line width of 1.5 Hz (before: 10 Hz). Potential noise sources contributed by the frequency comb are discussed in detail.
