We report on a series of 42 measurements of the transition frequency of the 429~THz (5s$^2$)~$^1$S$_0$--(5s5p)~$^3$P$_0$ line in $^{87}$Sr taken over three years from 2017 to 2019. They have been performed at the Physikalisch-Technische Bundesanstalt (PTB) between the laboratory strontium lattice clock and the primary caesium fountain clocks CSF1 and CSF2. The length of each individual measurement run has been extended by use of a hydrogen maser as flywheel to improve the statistical uncertainty given by the Cs clocks. We determine an averaged transition frequency of $429\:228\:004\:229\:873.00(0.07)$~Hz with $1.5\times10^{-16}$ fractional uncertainty, at the limit of the current realization of the unit hertz. Analysis of the data provides an improved limit on the coupling of the gravitational potential of the Sun to the proton--electron mass ratio $μ$, and confirms the limits on its temporal drift.
Improvements of the systematic uncertainty, frequency instability, and long-term reliability of the two caesium fountain primary frequency standards CSF1 and CSF2 at PTB (Physikalisch-Technische Bundesanstalt) are described. We have further investigated many of the systematic effects and made a number of modifications of the fountains. With an optically stabilized microwave oscillator, the quantum projection noise limited frequency instabilities are improved to $7.2 \times 10^{-14} (τ/1\,\mathrm{s})^{-1/2}$ for CSF1 and $2.5 \times 10^{-14} (τ/1\,\mathrm{s})^{-1/2}$ for CSF2 at high atom densi…
We report on the first frequency ratio measurement of an $^{115}$In+ single ion clock and a $^{87}$Sr optical lattice clock. A hydrogen maser serves as a reference oscillator to measure the ratio by independent optical combs. Over more than 90 000 seconds of measurement time, the frequency ratio $f_{\rm{In^+}}/f_{\rm{Sr}}$ is determined to be 2.952 748 749 874 863 4(21) with relative uncertainty of $7.0 \times 10^{-16}$. The measurement creates a new connection in the network of frequency ratios of optical clocks.
Optical lattice clocks are at the forefront of frequency metrology. Both the instability and systematic uncertainty of these clocks have been reported to be two orders of magnitude smaller than the best microwave clocks. For this reason, a redefinition of the SI second based on optical clocks seems possible in the near future. However, the operation of optical lattice clocks has not yet reached the reliability that microwave clocks have achieved so far. In this paper, we report on the operation of a strontium optical lattice clock that spans several weeks, with more than 80% uptime. We make us…
We demonstrate agreement between measurements and ab initio calculations of the frequency shifts caused by distributed cavity phase variations in the microwave cavity of a primary atomic fountain clock. Experimental verification of the finite element models of the cavities gives the first quantitative evaluation of this leading uncertainty and allows it to be reduced to delta nu / nu = 8.4\times10^-17. Applying these experimental techniques to clocks with improved microwave cavities will yield negligible distributed cavity phase uncertainties, less than \pm1\times10^-17.
We present an improvement of short term frequency stability of the integrating sphere cold atom clock after increasing the intensities of clock signals and optimizing the feedback loop of the clock. A short term frequency stability of $5.0\times10^{-13}τ^{-1/2}$ has been achieved and the limiting factors have been analyzed.
Collisions with background gas particles can shift the resonance frequencies of atoms in atomic clocks. The internal quantum states of atoms can also become entangled with their motional states due to the recoil imparted by a collision, which leads to a further shift of the clock frequency through the relativistic Doppler shift. It can be complicated to evaluate the Doppler and collisional frequency shifts for clock atoms in such entangled states, but estimates of these shifts are essential in order to improve the accuracy of optical atomic clocks. We present a formalism that describes collisi…
The medium-long term frequency stability of the integrating sphere cold atom clock was improved.During the clock operation, Rb atoms were cooled and manipulated using cooling light diffusely reflected by the inner surface of a microwave cavity in the clock. This light heated the cavity and caused a frequency drift from the resonant frequency of the cavity. Power fluctuations of the cooling light led to atomic density variations in the cavity's central area, which increased the clock frequency instability through a cavity pulling effect. We overcame these limitations with appropriate solutions.…
This article describes the recent progress of optical lattice clocks with neutral strontium ($^{87}$Sr), ytterbium ($^{171}$Yb) and mercury ($^{199}$Hg) atoms. In particular, we present frequency comparison between the clocks locally via an optical frequency comb and between two Sr clocks at remote sites using a phase-stabilized fibre link. We first review cryogenic Sr optical lattice clocks that reduce the room-temperature blackbody radiation shift by two orders of magnitude and serve as a reference in the following clock comparisons. Similar physical properties of Sr and Yb atoms, such as tr…
The temperature dependence of the Cs clock transition frequency in a vapor cell filled with Ne buffer gas has been measured. The experimental setup is based on the coherent population trapping (CPT) technique and a temporal Ramsey interrogation allowing a high resolution. A quadratic dependence of the frequency shift is shown. The temperature of the shift cancellation is evaluated. The actual Ne pressure in the cell is determined from the frequency shift of the 895nm optical transition. We can then determine the Cs-Ne collisional temperature coefficients of the clock frequency. These results c…
Collisions with background gas can perturb the transition frequency of trapped ions in an optical atomic clock. We develop a non-perturbative framework based on a quantum channel description of the scattering process, and use it to derive a master equation which leads to a simple analytic expression for the collisional frequency shift. As a demonstration of our method, we calculate the frequency shift of the Sr$^+$ optical atomic clock transition due to elastic collisions with helium.
We consider the frequency shift in optical lattice clocks which arises from the coupling of the electronic motion to the atomic motion within the lattice. For the simplest of 3-D lattice geometries this coupling is shown to only affect clocks based on blue-detuned lattices. We have estimated the size of this shift for the prospective strontium lattice clock operating at the 390 nm blue-detuned magic wavelength. The resulting fractional frequency shift is found to be on the order of $10^{-18}$ and is largely overshadowed by the electric quadrupole shift. For lattice clocks based on more complex…
We performed an absolute frequency measurement of the $^1S_{0}$-$^3P_{0}$ transition in $^{87}$Sr with a fractional uncertainty of $1.2 \times 10^{-15}$, which is less than one third that of our previous measurement. A caesium fountain atomic clock was used as a transfer oscillator to reduce the uncertainty of the link between a strontium optical lattice clock and the SI second. The absolute value of the transition frequency is 429 228 004 229 873.56(49) Hz.
We analyze both the s- and p-wave collision induced frequency shifts and propose a over-$π$ pulse scheme to cancel the shifts in optical lattice clocks interrogated by a Rabi pulse. The collisional frequency shifts are analytically solved as a function of the pulse area and the inhomogeneity of the Rabi frequencies. Experimentally measured collisional frequency shifts in an Yb optical lattice clock are in good agreement with the analytical calculations. Based on our analysis, the over-$π$ pulse combined with a small inhomogeneity below 0.1 allows a fractional uncertainty on a level of $10^{-18…
We report an s-wave collisional frequency shift of an atomic clock based on fermions. In contrast to bosons, the fermion clock shift is insensitive to the population difference of the clock states, set by the first pulse area in Ramsey spectroscopy, θ_1. The fermion shift instead depends strongly on the second pulse area θ_2. It allows the shift to be canceled, nominally at θ_2 = π/2, but correlations shift the null to slightly larger θ_2. The shift applies to optical lattice clocks and increases with the spatial inhomogeneity of the clock excitation field, naturally large at optical frequenci…
We perform spectroscopic observations of the 698-nm clock transition in $^{87}$Sr confined in an optical lattice using a laser linewidth transfer technique. A narrow-linewidth laser interrogating the clock transition is prepared by transferring the linewidth of a master laser (1064 nm) to that of a slave laser (698 nm) with a high-speed controllable fiber-based frequency comb. The Fourier-limited spectrum is observed for an 80-ms interrogating pulse. We determine that the absolute frequency of the 5s$^{2}$ $^{1}$S$_{0}$ - 5s5p $^{3}$P$_{0}$ clock transition in $^{87}$Sr is 429 228 004 229 872.…
The absolute frequency of the 1S0-3P0 clock transition of 87Sr has been measured to be 429 228 004 229 873.65 (37) Hz using lattice-confined atoms, where the fractional uncertainty of 8.6x10-16 represents one of the most accurate measurements of an atomic transition frequency to date. After a detailed study of systematic effects, which reduced the total systematic uncertainty of the Sr lattice clock to 1.5x10-16, the clock frequency is measured against a hydrogen maser which is simultaneously calibrated to the US primary frequency standard, the NIST Cs fountain clock, NIST-F1. The comparison i…
We demonstrate a one-dimensional optical lattice clock with a spin-polarized fermionic isotope designed to realize a collision-shift-free atomic clock with neutral atom ensembles. To reduce systematic uncertainties, we developed both Zeeman shift and vector light-shift cancellation techniques. By introducing both an H-maser and a Global Positioning System (GPS) carrier phase link, the absolute frequency of the $^1S_0(F=9/2) - {}^3P_0(F=9/2)$ clock transition of the $^{87}$Sr optical lattice clock is determined as 429,228,004,229,875(4) Hz, where the uncertainty is mainly limited by that of the…
The knowledge of the frequency noise spectrum of a diode laser is of interest in several high resolution experiments. Specifically, in laser-pumped vapor cell clocks, it is well established that the laser frequency noise plays a role in affecting the clock performances. It is then important to characterize the frequency noise of a diode laser, especially since such measurements are rarely found in the literature and hardly ever provided by vendors. In this paper, we describe a technique based on a frequency-to-voltage converter that transforms the laser frequency fluctuations into voltage fluc…
The frequency ratio of the 1S0(F=1/2)-3P0(F=1/2) clock transition in 171Yb and the 1S0(F=9/2)-3P0(F=9/2) clock transition in 87Sr is measured by an optical-optical direct frequency link between two optical lattice clocks. We determined the ratio (ν_{Yb}/ν_{Sr}) to be 1.207 507 039 343 340 4(18) with a fractional uncertainty of 1.5x10^{-15}. The measurement uncertainty of the frequency ratio is smaller than that obtained from absolute frequency measurements using the International Atomic Time (TAI) link. The measured ratio agrees well with that derived from the absolute frequency measurement re…
We report on a frequency ratio measurement of a ${}^{199}$Hg-based optical lattice clock referencing a ${}^{87}$Sr-based clock. Evaluations of lattice light shift, including atomic-motion-dependent shift, enable us to achieve a total systematic uncertainty of $7.2 \times 10^{-17}$ for the Hg clock. The frequency ratio is measured to be $ν_{\rm Hg}/ν_{\rm Sr}=2.629\, 314\, 209\, 898\, 909\, 60(22)$ with a fractional uncertainty of $8.4 \times 10^{-17}$, which is smaller than the uncertainty of the realization of the SI second, i.e., the SI limit.
We report frequency measurement of the clock transition in an 115In+ ion sympathetically-cooled with Ca+ ions in a linear rf trap. The Ca+ ions are used as a probe of the external electromagnetic field and as the coolant for preparing the cold In+. The frequency is determined to be 1 267 402 452 901 049.9 (6.9) Hz by averaging 36 measurements using an optical frequency comb referenced to the frequency standards located in the same site.
We have measured the absolute frequency of the optical lattice clock based on $^{87}$Sr at PTB with an uncertainty of $3.9\times 10^{-16}$ using two caesium fountain clocks. This is close to the accuracy of today's best realizations of the SI second. The absolute frequency of the 5s$^2$ $^1$S$_0$-5s5p $^3$P$_0$ transition in $^{87}$Sr is 429,228,004,229,873.13(17) Hz. Our result is in excellent agreement with recent measurements performed in different laboratories worldwide. We improved the total systematic uncertainty of our Sr frequency standard by a factor of five and reach $3\times 10^{-17…
Time and frequency are the most accurately measurable quantities, providing foundations for science and modern technologies. The accuracy relies on the SI (Systéme International) second that refers to Cs microwave clocks with fractional uncertainties at $10^{-16}$. Recent revolutionary progress of optical clocks aims to achieve $1\times 10^{-18}$ uncertainty, which however has been hindered by long averaging-times or by systematic uncertainties. Here, we demonstrate optical lattice clocks with $^{87}$Sr atoms interrogated in a cryogenic environment to address the blackbody radiation-induced fr…
We have observed that the collisional frequency shift in primary caesium fountain clocks varies with the clock state population composition and, in particular, is zero for a given fraction of the |F = 4, mF = 0> atoms, depending on the initial cloud parameters. We present a theoretical model explaining our observations. The possibility of the collisional shift cancellation implies an improvement in the performance of caesium fountain standards and a simplification in their operation. Our results also have implications for test operation of fountains at multiple pi/2 pulse areas.
An Al$^+$ clock with $1.6\times10^{-18}$ systematic uncertainty and its frequency ratios
Physikalisch-Technische Bundesanstalt（德国联邦物理技术研究院）；Institut für Quantenoptik, Leibniz Universität Hannover（汉诺威莱布尼茨大学量子光学研究所）；Laboratoire Kastler Brossel, Sorbonne Université, CNRS, ENS-PSL Research University, Collège de France（索邦大学、法国国家科学研究中心、巴黎文理研究大学、法兰西公学院卡斯特尔-布罗塞尔实验室）
We investigate systematic errors associated with a common modulation technique used for phase sensitive detection of a coherent population trapping (CPT) resonance. In particular, we show that modification of the CPT resonance lineshape due to the presence of off-resonant fields leads to frequency shifts which may limit the stability of CPT-based atomic clocks. We also demonstrate that an alternative demodulation technique greatly reduces these effects.
We have quantified collisional losses, decoherence and the collision shift in a one-dimensional optical lattice clock with bosonic 88Sr. The lattice clock is referenced to the highly forbidden transition 1S0 - 3P0 at 698 nm, which becomes weakly allowed due to state mixing in a homogeneous magnetic field. We were able to quantify three decoherence coefficients, which are due to dephasing collisions, inelastic collisions between atoms in the upper and lower clock state, and atoms in the upper clock state only. Based on the measured coefficients, we determine the operation parameters at which a …
We report on the first absolute transition frequency measurement at the 10^{-15} level with a single, laser-cooled 40Ca+ ion in a linear Paul trap. For this measurement, a frequency comb is referenced to the transportable Cs atomic fountain clock of LNE-SYRTE and is used to measure the S1/2-D5/2 electric-quadrupole transition frequency. After the correction of systematic shifts, the clock transition frequency f_Ca+ = 411 042 129 776 393.2 (1.0) Hz is obtained, which corresponds to a fractional uncertainty within a factor of three of the Cs standard. Future improvements are expected to lead to …
A caesium fountain clock is operated utilizing a microwave oscillator that derives its frequency stability from a stable laser by means of a fiber-laser femtosecond frequency comb. This oscillator is based on the technology developed for optical clocks and replaces the quartz based microwave oscillator commonly used in fountain clocks. As a result, a significant decrease of the frequency instability of the fountain clock is obtained, reaching 0.74E-14 at 100 s averaging time. We could demonstrate that for a significant range of detected atom numbers the instability is limited by quantum projec…
We report direct measurements of the frequency ratio of the 642 THz ${}^2S_{1/2} (F=0)$--${}^2F_{7/2} (F=3)$ electric octupole transition in ${}^{171}\mathrm{Yb}^+$ and the 429 THz ${}^1S_0$--${}^3P_0$ transition in ${}^{87}\mathrm{Sr}$. A series of 107 measurements has been performed at the Physikalisch-Technische Bundesanstalt between December 2012 and October 2019. Long-term variations of the ratio are larger than expected from the individual measurement uncertainties of few $10^{-17}$. The cause of these variations remains unknown. Even taking these into account, we find a fractional uncer…
Optical atomic clocks have already overcome the eighteenth decimal digit of instability and uncertainty demonstrating incredible control over external perturbations of the clock transition frequency. At the same time there is an increasing demand for atomic and ionic transitions with minimal sensitivity to external fields, with practical operational wavelengths and robust readout protocols. One of the goals is to simplify clock's operation maintaining its relative uncertainty at low 10-18 level. It is especially important for transportable and envisioned space-based optical clocks. We proved e…
For the past 15 years, tremendous progress within the fields of laser stabilization, optical frequency combs and atom cooling and trapping have allowed the realization of optical atomic clocks with unrivaled performances. These instruments can perform frequency comparisons with fractional uncertainties well below $10^{-17}$, finding applications in fundamental physics tests, relativistic geodesy, and time and frequency metrology. Even though most optical clocks are currently laboratory setups, several proposals for using these clocks for field measurements or within an optical clock network ha…
We report improved frequency ratio measurement with $^{87}$Sr and $^{171}$Yb optical lattice clocks at the National Metrology Institute of Japan (NMIJ). The $^{87}$Sr optical lattice clock is enhanced with several major modifications and is re-evaluated with a reduced uncertainty of $1.1\times10^{-16}$. We employed a $^{171}$Yb optical lattice clock with an uncertainty of $4\times10^{-16}$ that was developed for contributing to International Atomic Time (TAI). The measurement result is $ν_{\mathrm{Yb}}/ν_{\mathrm{Sr}}$ = 1.207 507 039 343 338 58(49)$_{\mathrm{sys}}$(6)$_{\mathrm{stat}}$ with a…
We search for ultralight scalar dark matter candidates that induce oscillations of the fine structure constant, the electron and quark masses, and the quantum chromodynamics energy scale with frequency comparison data between an $^{171}$Yb optical lattice clock and a $^{133}$Cs fountain microwave clock that span 298 days with an uptime of 15.4 $\%$. New limits on the couplings of the scalar dark matter to electrons and gluons in the mass range from $10^{-22}$ eV/$c^{2}$ to $10^{-20}$ eV/$c^{2}$ are set, assuming that each of these couplings is the dominant source of the modulation in the frequ…
We present a comprehensive study of the frequency shifts associated with the lattice potential for a Sr lattice clock. By comparing two such clocks with a frequency stability reaching $5\times 10^{-17}$ after a one hour integration time, and varying the lattice depth up to $U_0=900 \, E_r$ with $E_r$ being the recoil energy, we evaluate lattice related shifts with an unprecedented accuracy. We put the first experimental upper bound on the recently predicted frequency shift due to the magnetic dipole (M1) and electric quadrupole (E2) interactions. This upper bound is significantly smaller than …
We present a theoretical analysis of the Stark effect in the hyperfine structure of the cesium ground-state. We have used third order perturbation theory, including diagonal and off-diagonal hyperfine interactions, and have identified terms which were not considered in earlier treatments. A numerical evaluation using perturbing levels up to n=18 yields new values for the tensor polarizability $α_2(6S_{1/2})$ and for the Stark shift of the clock transition frequency in cesium. The polarizabilities are in good agreement with experimental values, thereby removing a 40-year-old discrepancy. The cl…
We report the direct excitation of the highly forbidden (6s^2) 1S0 - (6s6p) 3P0 optical transition in two odd isotopes of ytterbium. As the excitation laser frequency is scanned, absorption is detected by monitoring the depletion from an atomic cloud at ~70 uK in a magneto-optical trap. The measured frequency in 171Yb (F=1/2) is 518,295,836,593.2 +/- 4.4 kHz. The measured frequency in 173Yb (F=5/2) is 518,294,576,850.0 +/- 4.4 kHz. Measurements are made with a femtosecond-laser frequency comb calibrated by the NIST cesium fountain clock and represent nearly a million-fold reduction in uncertai…
Transition frequencies of atoms and ions are among the most accurately accessible quantities in nature, playing important roles in pushing the frontiers of science by testing fundamental laws of physics, in addition to a wide range of applications such as satellite navigation systems. Atomic clocks based on optical transitions approach uncertainties of $10^{-18}$, where full frequency descriptions are far beyond the reach of the SI second. Frequency ratios of such super clocks, on the other hand, are not subject to this limitation. They can therefore verify consistency and overall accuracy for…
We experimentally investigate an optical clock based on $^{171}$Yb ($I=1/2$) atoms confined in an optical lattice. We have evaluated all known frequency shifts to the clock transition, including a density-dependent collision shift, with a fractional uncertainty of $3.4 \times 10^{-16}$, limited principally by uncertainty in the blackbody radiation Stark shift. We measured the absolute clock transition frequency relative to the NIST-F1 Cs fountain clock and find the frequency to be 518 295 836 590 865.2(0.7) Hz.
A physics package for a compact cold atomic clock is hereby presented. The uniqueness of this package is its small dimensions that enable, for the first time, implementation of a primary cold atomic clock in a standard package of 3U height (=133mm). These dimensions are made possible by using an in-vacuum Microwave (MW) Loop Gap Resonator (LGR) whose length and diameter can be reduced from those of a typical resonator. Following our presentation of the design, we analyze the homogeneity of the MW field amplitude and phase. We find that the expected clock instability due to non-uniformity of th…
We propose a new class of atomic microwave clocks based on the hyperfine transitions in the ground state of aluminum or gallium atoms trapped in optical lattices. For these elements magic wavelengths exist at which both levels of the hyperfine doublet are shifted at the same rate by the lattice laser field, cancelling its effect on the clock transition. Our analysis of various systematic effects shows that, while offering an improved control over systematic errors, the accuracy of the proposed microwave clock is competitive to that of the state-of-the-art primary frequency standard.
We have performed ab initio calculations of the frequency shift induced by a static electric field on the cesium clock hyperfine transition. The calculations are used to find the frequency shifts due to blackbody radiation. Our result ($δν/E^2=-2.26(2)\times 10^{-10}$Hz/(V/m)$^2$) is in good agreement with early measurements and ab initio calculations performed in other groups. We present arguments against recent claims that the actual value of the effect might be smaller. The difference ($\sim$ 10%) between ab initio and semiempirical calculations is due to the contribution of the continuum s…
We present a new interrogation scheme for the next generation of quantum clocks to suppress frequency-shifts induced by laser probing fields themselves based on Generalized Hyper-Ramsey resonances. Sequences of composite laser pulses with specific selection of phases, frequency detunings and durations are combined to generate a very efficient and robust frequency locking signal with almost a perfect elimination of the light-shift from off resonant states and to decouple the unperturbed frequency measurement from the laser's intensity. The frequency lock point generated from synthesized error s…
In the last ten years extraordinary results in time and frequency metrology have been demonstrated. Frequency-stabilization techniques for continuous-wave lasers and femto-second optical frequency combs have enabled a rapid development of frequency standards based on optical transitions in ultra-cold neutral atoms and trapped ions. As a result, today's best performing atomic clocks tick at an optical rate and allow scientists to perform high-resolution measurements with a precision approaching a few parts in $10^{18}$. This paper reviews the history and the state of the art in optical-clock re…
We describe an optical frequency stabilization scheme of a microwave oscillator that is used for the interrogation of primary caesium fountain clocks. Because of its superior phase noise properties, this scheme, which is based on an ultrastable laser and a femtosecond laser frequency comb, overcomes the frequency instability limitations of fountain clocks given by the previously utilized quartz-oscillator-based frequency synthesis. The presented scheme combines the transfer of the short-term frequency instability of an optical cavity and the long-term frequency instability of a hydrogen maser …
We have carried out concurrent optical frequency measurements of the $(6s^{2})\,^{1}S_{0} -(6s6p)\,^{3}P_{1}$ ($F=\frac{3}{2}$) and $(6s^{2})\,^{1}S_{0} -(6s6p)\,^{3}P_{0}$ transitions in $^{171}$Yb, and in so doing have determined the frequency separation between the $^{3}P_{0}$ ($F=\frac{1}{2}$) and $^{3}P_{1}$ ($F=\frac{3}{2}$) levels with an uncertainty in the ppb range. The knowledge of this frequency interval will aid experiments relying on the $^{1}S_{0}-\,^{3}P_{0}$ line in $^{171}$Yb and $^{173}$Yb without access to highly accurate frequency standards.
We report on a theoretical analysis of the phase-shift in compact atomic clocks working either with cold or thermal atoms. It is well known that in a microwave cavity with electromagnetic losses, a traveling wave adds to the standing wave of a given resonant mode. We calculate the spatial varying phase related to this travelling wave for two geometries of interest in clock applications, the cylindrical cavity and the spherical cavity. Due to their motion, the atoms probe different regions of the cavity and then experience different phases of the interrogating microwave field. We show that this…
We report on the design of a segmented linear Paul trap for optical clock applications using trapped ion Coulomb crystals. For an optical clock with an improved short-term stability and a fractional frequency uncertainty of 10^-18, we propose 115In+ ions sympathetically cooled by 172Yb+. We discuss the systematic frequency shifts of such a frequency standard. In particular, we elaborate on high precision calculations of the electric radiofrequency field of the ion trap using the finite element method. These calculations are used to find a scalable design with minimized excess micromotion of th…
The mid-term fractional frequency stability of miniaturized atomic clocks can be limited by light-shift effects. In this Letter, we demonstrate the implementation of a symmetric Auto-Balanced Ramsey (SABR) interrogation sequence in a microcell-based atomic clock based on coherent population trapping (CPT). Using this advanced protocol, the sensitivity of the clock frequency to laser power, microwave power and laser frequency variations is reduced, at least by one order of magnitude, in comparison with continuous-wave (CW) or Ramsey interrogation schemes. Light-shift mitigation obtained with th…
The current SI second based on the atomic hyperfine transition in the ground state of 133Cs is expected to be replaced by a new definition based on optical frequency standards, whose estimated uncertainty has now been established two orders of magnitude lower than the accuracy of the best Cs primary standards. However, such a redefinition of the second is hindered by the fact that many atomic species are potential contenders to become the new primary frequency standard. In this paper, we propose to resolve this issue by defining a composite frequency unit based on the weighted geometric mean o…
We present a measurement of the absolute frequency of the 5s$^2$ $^1$S$_0$ to 5s5p $^3$P$_0$ transition in $^{87}$Sr, which is a secondary representation of the SI second. We describe the optical lattice clock apparatus used for the measurement, and we focus in detail on how its systematic frequency shifts are evaluated with a total fractional uncertainty of $1 \times 10^{-17}$. Traceability to the International System of Units is provided via comparison to International Atomic Time (TAI). Gathering data over 5- and 15-day periods, with the lattice clock operating on average 74$\%$ of the time…
We report on the observation of a dc Stark frequency shift at the $10^{-13}$ level by comparing two strontium optical lattice clocks. This frequency shift arises from the presence of electric charges trapped on dielectric surfaces placed under vacuum close to the atomic sample. We show that these charges can be eliminated by shining UV light on the dielectric surfaces, and characterize the residual dc Stark frequency shift on the clock transition at the $10^{-18}$ level by applying an external electric field. This study shows that the dc Stark shift can play an important role in the accuracy b…
As optical clocks are improved to reach the frequency uncertainty below the 10$^{-17}$ level, the frequency shift due to the blackbody radiation (BBR) has been one of the major systematic effects hindering further improvement. To evaluate the BBR shift of an Yb optical lattice clock at KRISS, we installed an in-vacuum BBR shield and made radiation thermometry using a black-coated-sphere thermal probe. After we quantitatively measured the conduction loss of the thermal probe and the effects of all the external radiation sources, we determined the temperature at the atom trap site with an uncert…
We measured the absolute frequency of the $^1S_0$ - $^3P_0$ transition of $^{171}$Yb atoms confined in a one-dimensional optical lattice relative to the SI second. The determined frequency was 518 295 836 590 863.38(57) Hz. The uncertainty was reduced by a factor of 14 compared with our previously reported value in 2013 due to the significant improvements in decreasing the systematic uncertainties. This result is expected to contribute to the determination of a new recommended value for the secondary representations of the second.
We demonstrated transferring the stability of one highly stable clock laser operating at 729 nm to another less stable laser operating at 698 nm. The two different wavelengths were bridged using an optical frequency comb. The improved stability of the clock laser at 698 nm enabled us to evaluate the systematic frequency shifts of the Sr optical lattice clock with shorter averaging time. We determined the absolute frequency of the clock transition 1S0 - 3P0 in 87Sr to be 429 228 004 229 873.9 (1.4) Hz referenced to the SI second on the geoid via International Atomic Time (TAI).
