We demonstrate the use of trapped ytterbium ions as quantum bits for quantum information processing. We implement fast, efficient state preparation and state detection of the first-order magnetic field-insensitive hyperfine levels of 171Yb+, with a measured coherence time of 2.5 seconds. The high efficiency and high fidelity of these operations is accomplished through the stabilization and frequency modulation of relevant laser sources.
We study the deterministic entanglement of a pair of neutral atoms trapped in an optical lattice by coupling to excited-state molecular hyperfine potentials. Information can be encoded in the ground-state hyperfine levels and processed by bringing atoms together pair-wise to perform quantum logical operations through induced electric dipole-dipole interactions. The possibility of executing both diagonal and exchange type entangling gates is demonstrated for two three-level atoms and a figure of merit is derived for the fidelity of entanglement. The fidelity for executing a CPHASE gate is calcu…
We introduce a technique to store and manipulate single x-ray photons which relies on dynamically controlled absorption via nuclear hyperfine magnetic splitting. This scheme is inherently suitable for storage, on-demand generation and dynamical manipulation of single x-ray photons, for instance, the manipulation of the temporal shape, temporal splitting, the interference between x-ray photons and the control of the polarization. Our approach opens up new paths in x-ray quantum information.
We demonstrate laser-driven two-qubit and single-qubit logic gates with fidelities 99.9(1)% and 99.9934(3)% respectively, significantly above the approximately 99% minimum threshold level required for fault-tolerant quantum computation, using qubits stored in hyperfine ground states of calcium-43 ions held in a room-temperature trap. We study the speed/fidelity trade-off for the two-qubit gate, for gate times between 3.8$μ$s and 520$μ$s, and develop a theoretical error model which is consistent with the data and which allows us to identify the principal technical sources of infidelity.
We demonstrate ultrafast coherent coupling between an atomic qubit stored in a single trapped cadmium ion and a photonic qubit represented by two resolved frequencies of a photon. Such ultrafast coupling is crucial for entangling networks of remotely-located trapped ions through photon interference, and is also a key component for realizing ultrafast quantum gates between Coulomb-coupled ions.
We prepare and detect the hyperfine state of a single 87Rb atom coupled to a fiber-based high finesse cavity on an atom chip. The atom is extracted from a Bose-Einstein condensate and trapped at the maximum of the cavity field, resulting in a reproducibly strong atom-cavity coupling. We use the cavity reflection and transmission signal to infer the atomic hyperfine state with a fidelity exceeding 99.92% in a read-out time of 100 microseconds. The atom is still trapped after detection.
Fast and efficient detection of the qubit state in trapped ion quantum information processing is critical for implementing quantum error correction and performing fundamental tests such as a loophole-free Bell test. In this work we present a simple qubit state detection protocol for a $^{171}$Yb$^+$ hyperfine atomic qubit trapped in a microfabricated surface trap, enabled by high collection efficiency of the scattered photons and low background photon count rate. We demonstrate average detection times of 10.5, 28.1 and 99.8\,$\upmu$s, corresponding to state detection fidelities of 99%, 99.85(1…
Advanced techniques for manipulation of internal states, standard in atomic physics, are demonstrated for a charged molecular species for the first time. We address individual hyperfine states of ro-vibrational levels of a diatomic ion by optical excitation of individual hyperfine transitions, and achieve controlled transfer of population into a selected hyperfine state. We use molecular hydrogen ions (HD^{+}) as a model system and employ a novel frequency-comb-based, continuous-wave 5 \mum laser spectrometer. The achieved spectral resolution is the highest obtained so far in the optical domai…
We perform spectroscopy on the hyperfine splitting of $^{85}$Rb atoms trapped in far-off-resonance optical traps. The existence of a spatially dependent shift in the energy levels is shown to induce an inherent dephasing effect, which causes a broadening of the spectroscopic line and hence an inhomogeneous loss of atomic coherence at a much faster rate than the homogeneous one caused by spontaneous photon scattering. We present here a number of approaches for reducing this inhomogeneous broadening, based on trap geometry, additional laser fields, and novel microwave pulse sequences. We then sh…
We propose and demonstrate a protocol for high-fidelity indirect readout of trapped ion hyperfine qubits, where the state of a $^9\text{Be}^+$ qubit ion is mapped to a $^{25}\text{Mg}^+$ readout ion using laser-driven Raman transitions. By partitioning the $^9\text{Be}^+$ ground state hyperfine manifold into two subspaces representing the two qubit states and choosing appropriate laser parameters, the protocol can be made robust to spontaneous photon scattering errors on the Raman transitions, enabling repetition for increased readout fidelity. We demonstrate combined readout and back-action e…
We propose an experimentally feasible scheme to achieve quantum computation based solely on geometric manipulations of a quantum system. The desired geometric operations are obtained by driving the quantum system to undergo appropriate adiabatic cyclic evolutions. Our implementation of the all-geometric quantum computation is based on laser manipulation of a set of trapped ions. An all-geometric approach, apart from its fundamental interest, promises a possible way for robust quantum computation.
Hyperfine atomic states are among the most promising candidates for qubit encoding in quantum information processing. In atomic systems, hyperfine transitions are typically driven through a two-photon Raman process by a laser field which is amplitude modulated at the hyperfine qubit frequency. Here, we introduce a new method for generating amplitude modulation by phase modulating a laser and reflecting it from a highly dispersive optical element known as a chirped Bragg grating (CBG). This approach is passively stable, offers high efficiency, and is compatible with high-power laser sources, en…
The beam splitter and phase shifter, which are the key elements in the experiments of light interference, are realized in the motion of trapped ions. Some applications, such as the creation of quantum motional states and the realization of Mach-Zehnder interferometer, are illustrated. Several detection methods of motional states used in the interferometer are also discussed.
A single laser-cooled and trapped 9Be+ ion is used to investigate methods of coherent quantum-state synthesis and quantum logic. We create and characterize nonclassical states of motion including "Schroedinger-cat" states. A fundamental quantum logic gate is realized which uses two states of the quantized ion motion and two ion internal states as qubits. We explore some of the applications for, and problems in realizing, quantum computation based on multiple trapped ions.
We use microwave induced adiabatic passages for selective spin flips within a string of optically trapped individual neutral Cs atoms. We position-dependently shift the atomic transition frequency with a magnetic field gradient. To flip the spin of a selected atom, we optically measure its position and sweep the microwave frequency across its respective resonance frequency. We analyze the addressing resolution and the experimental robustness of this scheme. Furthermore, we show that adiabatic spin flips can also be induced with a fixed microwave frequency by deterministically transporting the …
We demonstrate single-shot qubit readout with fidelity sufficient for fault-tolerant quantum computation, for two types of qubit stored in single trapped calcium ions. For an optical qubit stored in the (4S_1/2, 3D_5/2) levels of 40Ca+ we achieve 99.991(1)% average readout fidelity in one million trials, using time-resolved photon counting. An adaptive measurement technique allows 99.99% fidelity to be reached in 145us average detection time. For a hyperfine qubit stored in the long-lived 4S_1/2 (F=3, F=4) sub-levels of 43Ca+ we propose and implement a simple and robust optical pumping scheme …
Methods for, and limitations to, the generation of entangled states of trapped atomic ions are examined. As much as possible, state manipulations are described in terms of quantum logic operations since the conditional dynamics implicit in quantum logic is central to the creation of entanglement. Keeping with current interest, some experimental issues in the proposal for trapped-ion quantum computation by I. Cirac and P. Zoller (University of Innsbruck) are discussed. Several possible decoherence mechanisms are examined and what may be the more important of these are identified. Some potential…
We study the entanglement between the 2D vibrational motion and two ground state hyperfine levels of a trapped ion, Under particular conditions this entanglement depends on the parity of the total initial vibrational quanta. We study the robustness of this quantum coherence effect with respect to the presence of non-dissipative sources of decoherence, and of an imperfect initial state preparation.
We demonstrate tunable spin-spin couplings between trapped atomic ions, mediated by laser forces on multiple transverse collective modes of motion. A $σ_x σ_x$-type Ising interaction is realized between quantum bits stored in the ground hyperfine clock states of Yb ions. We demonstrate entangling gates and tailor the spin-spin couplings with two and three trapped ions. The use of closely-spaced transverse modes provides a new class of interactions relevant to quantum computing and simulation with large collections of ions in a single crystal.
We show that a large number of ions stored in a Penning trap, and forming a 2D Coulomb crystal, provides an almost ideal system for scalable quantum computation and quantum simulation. In particular, the coupling of the internal states to the motion of the ions transverse to the crystal plane, allows one to implement two qubit quantum gates. We analyze in detail the decoherence induced by anharmonic couplings with in--plane hot vibrational modes, and show that very high gate fidelities can be achieved with current experimental set--ups.
We demonstrate quantum control of a large spin-angular momentum associated with the F=3 hyperfine ground state of 133Cs. A combination of time dependent magnetic fields and a static tensor light shift is used to implement near-optimal controls and map a fiducial state to a broad range of target states, with yields in the range 0.8-0.9. Squeezed states are produced also by an adiabatic scheme that is more robust against errors. Universal control facilitates the encoding and manipulation of qubits and qudits in atomic ground states, and may lead to improvement of some precision measurements.
We propose the implementation of a geometric-phase gate on magnetic-field-insensitive qubits with $\hatσ^z$-dependent forces for trapped ion quantum computing. The force is exerted by two laser beams in a Raman configuration. Qubit-state dependency is achieved by a small frequency detuning from the virtually-excited state. Ion species with excited states of long radiative lifetimes are used to reduce the chance of a spontaneous photon emission to less than 10$^{-8}$ per gate-run. This eliminates the main source of gate infidelity of previous implementations. With this scheme it seems possible …
The control of thermal decoherence via dynamical decoupling and via the quantum Zeno effect (Zeno control) is investigated for a model of trapped ion, where the dynamics of two low lying hyperfine states undergoes decoherence due to the thermal interaction with an excited state. Dynamical decoupling is a procedure that consists in periodically driving the excited state, while the Zeno control consists in frequently measuring it. When the control frequency is high enough, decoherence is shown to be suppressed. Otherwise, both controls may accelerate decoherence.
We report new techniques for driving high-fidelity stimulated Raman transitions in trapped ion qubits. An electro-optic modulator induces sidebands on an optical source, and interference between the sidebands allows coherent Rabi transitions to be efficiently driven between hyperfine ground states separated by 14.53 GHz in a single trapped 111Cd+ ion.
We present a method for achieving high fidelity state preparation and measurement (SPAM) using trapped ion hyperfine qubits with nuclear spins higher than $I = 1/2$. The ground states of these higher nuclear spin isotopes do not afford a simple frequency-selective state preparation scheme. We circumvent this limitation by stroboscopically driving strong and weak transitions, blending fast optical pumping using dipole transitions and narrow microwave or optical quadrupole transitions. We demonstrate this method with the $I=3/2$ isotope $^{137}\mbox{Ba}^+$ to achieve a SPAM infidelity of $\left(…
With a 9Be+ trapped-ion hyperfine-states qubit, we demonstrate an error probability per randomized single-qubit gate of 2.0(2) x 10^-5, below the threshold estimate of 10^-4 commonly considered sufficient for fault-tolerant quantum computing. The 9Be+ ion is trapped above a microfabricated surface-electrode ion trap and is manipulated with microwaves applied to a trap electrode. The achievement of low single-qubit-gate errors is an essential step toward the construction of a scalable quantum computer.
We propose an architecture and methodology for large-scale quantum simulations using hyperfine states of trapped-ions in an arbitrary-layout microtrap array with laserless interactions. An ion is trapped at each site, and the electrode structure provides for the application of single and pairwise evolution operators using only locally created microwave and radio-frequency fields. The avoidance of short-lived atomic levels during evolution effectively eliminates errors due to spontaneous scattering; this may allow scaling of quantum simulators based on trapped ions to much larger systems than c…
We demonstrate the reversible mapping of a coherent state of light with mean photon number n-bar ~= 1.1 to and from the hyperfine states of an atom trapped within the mode of a high finesse optical cavity. The coherence of the basic processes is verified by mapping the atomic state back onto a field state in a way that depends on the phase of the original coherent state. Our experiment represents an important step towards the realization of cavity QED-based quantum networks, wherein coherent transfer of quantum states enables the distribution of quantum information across the network.
Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a hyperfine interaction, using single-quantum and zero-quantum Ramsey fringes, by applying it to the system of a Nitrogen Vacancy (NV) center and a $^{13}$C nuclear spin in the 1$^{\mathrm{st}}$ shell. The zero-quantum Ramsey fringe, analogous to the quantum beat in a $Λ$-type level structure, particularly enhances the measurement precision for non-secular hyperfin…
Many systems used for quantum computing possess additional states beyond those defining the qubit. Leakage out of the qubit subspace must be considered when designing quantum error correction codes. Here we consider trapped ion qubits manipulated by Raman transitions. Zeeman qubits do not suffer from leakage errors but are sensitive to magnetic fields to first-order. Hyperfine qubits can be encoded in clock states that are insensitive to magnetic fields to first-order, but spontaneous scattering during the Raman transition can lead to leakage. Here we compare a Zeeman qubit ($^{174}$Yb$^+$) to…
Hyperfine-resolved laser excitation and detection of nuclear isomer in trapped $^{229}$Th$^{3+}$ ions
Institute of Theoretical Physics, Chinese Academy of Sciences（中国科学院理论物理研究所）；Center for Photonic Quantum Precision Measurement, Advanced Research Institute of Multidisciplinary Science, Beijing Institute of Technology（北京理工大学前沿交叉科学研究院光子量子精密测量中心）；Beijing Institute of Technology, State Key Laboratory of Environment Characteristics and Effects for Near-space（北京理工大学临近空间环境特性与效应省部共建国家重点实验室）；Johannes Gutenberg-University Mainz（美因茨约翰内斯·古腾堡大学）；Beijing Computational Science Research Center（北京计算科学研究中心）；School of Physical Sciences, University of Chinese Academy of Sciences（中国科学院大学物理科学学院）；School of Nuclear Science and Technology, University of Chinese Academy of Sciences（中国科学院大学核科学与技术学院）
We present a method that combines continuous and pulsed microwave radiation patterns to achieve robust interactions among hyperfine trapped ions placed in a magnetic field gradient. More specifically, our scheme displays continuous microwave drivings with modulated phases, phase flips, and $π$ pulses. This leads to high-fidelity entangling gates which are resilient against magnetic field fluctuations, changes on the microwave amplitudes, and crosstalk effects. Our protocol runs with arbitrary values of microwave power, which includes the technologically relevant case of low microwave intensiti…
We analyze the error in trapped-ion, hyperfine qubit, quantum gates due to spontaneous scattering of photons from the gate laser beams. We investigate single-qubit rotations that are based on stimulated Raman transitions and two-qubit entangling phase-gates that are based on spin-dependent optical dipole forces. This error is compared between different ion species currently being investigated as possible quantum information carriers. For both gate types we show that with realistic laser powers the scattering error can be reduced to below current estimates of the fault-tolerance error threshold…
Physical systems must fulfill a number of conditions to qualify as useful quantum bits (qubits) for quantum information processing, including ease of manipulation, long decoherence times, and high fidelity readout operations. Since these conditions are hard to satisfy with a single system, it may be necessary to combine different degrees of freedom. Here we discuss a possible system, based on electronic and nuclear spin degrees of freedom in trapped ions. The nuclear spin yields long decoherence times, while the electronic spin, in a magnetic field gradient, provides efficient manipulation, an…
Highly efficient, nearly deterministic, and isotope selective generation of Yb$^+$ ions by 1- and 2-color photoionization is demonstrated. State preparation and state selective detection of hyperfine states in \ybodd is investigated in order to optimize the purity of the prepared state and to time-optimize the detection process. Linear laser cooled Yb$^+$ ion crystals ions confined in a Paul trap are demonstrated. Advantageous features of different previous ion trap experiments are combined while at the same time the number of possible error sources is reduced by using a comparatively simple e…
In order to faithfully detect the state of an individual two-state quantum system (qubit) realized using, for example, a trapped ion or atom, state selective scattering of resonance fluorescence is well established. The simplest way to read out this measurement and assign a state is the threshold method. The detection error can be decreased by using more advanced detection methods like the time-resolved method or the $π$-pulse detection method. These methods were introduced to qubits with a single possible state change during the measurement process. However, there exist many qubits like the h…
Population leakage outside the qubit subspace presents a particularly harmful source of error that cannot be handled by standard error correction methods. Using a trapped $^{171}$Yb$+$ ion, we demonstrate an optical pumping scheme to suppress leakage errors in atomic hyperfine qubits. The selection rules and narrow linewidth of a quadrupole transition are used to selectively pump population out of leakage states and back into the qubit subspace. Each pumping cycle reduces the leakage population by a factor of $\sim3$, allowing for an exponential suppression in the number of cycles. We use inte…
We implement all single-qubit operations with fidelities significantly above the minimum threshold required for fault-tolerant quantum computing, using a trapped-ion qubit stored in hyperfine "atomic clock" states of $^{43}$Ca$^+$. We measure a combined qubit state preparation and single-shot readout fidelity of 99.93%, a memory coherence time of $T^*_2=50$ seconds, and an average single-qubit gate fidelity of 99.9999%. These results are achieved in a room-temperature microfabricated surface trap, without the use of magnetic field shielding or dynamic decoupling techniques to overcome technica…
$^{133}\text{Ba}^+$ has been identified as an attractive ion for quantum information processing due to the unique combination of its spin-1/2 nucleus and visible wavelength electronic transitions. Using a microgram source of radioactive material, we trap and laser-cool the synthetic $A$ = 133 radioisotope of barium II in a radio-frequency ion trap. Using the same, single trapped atom, we measure the isotope shifts and hyperfine structure of the $6^2 \text{P}_{1/2}$ $\leftrightarrow$ $6^2 \text{S}_{1/2}$ and $6^2 \text{P}_{1/2}$ $\leftrightarrow$ $5^2 \text{D}_{3/2}$ electronic transitions that…
A promising scheme for building scalable quantum simulators and computers is the synthesis of a scalable system using interconnected subsystems. A prerequisite for this approach is the ability to faithfully transfer quantum information between subsystems. With trapped atomic ions, this can be realized by transporting ions with quantum information encoded into their internal states. Here, we measure with high precision the fidelity of quantum information encoded into hyperfine states of a 171Yb+ ion during ion transport in a microstructured Paul trap. Ramsey spectroscopy of the ion's internal s…
We demonstrate a coherence time of 2.1(1)~s for electron spin superposition states of a single trapped $^{40}$Ca$^+$ ion. The coherence time, measured with a spin-echo experiment, corresponds to residual rms magnetic field fluctuations $\leq$~2.7$\times$10$^{-12}$~T. The suppression of decoherence induced by fluctuating magnetic fields is achieved by combining a two-layer $μ$-metal shield, which reduces external magnetic noise by 20 to 30~dB for frequencies of 50~Hz to 100~kHz, with Sm$_2$Co$_{17}$ permanent magnets for generating a quantizing magnetic field of 0.37~mT. Our results extend the …
We propose a pulsed dynamical decoupling protocol as the generator of tunable, fast, and robust quantum phase gates between two microwave-driven trapped ion hyperfine qubits. The protocol consists of sequences of $π$-pulses acting on ions that are oriented along an externally applied magnetic field gradient. In contrast to existing approaches, in our design the two vibrational modes of the ion chain cooperate under the influence of the external microwave driving to achieve significantly increased gate speeds. Our scheme is robust against the dominant noise sources, which are errors on the magn…
Validity conditions for the adiabatic approximation are useful tools to understand and predict the quantum dynamics. Remarkably, the resonance phenomenon in oscillating quantum systems has challenged the adiabatic theorem. In this scenario, inconsistencies in the application of quantitative adiabatic conditions have led to a sequence of new approaches for adiabaticity. Here, by adopting a different strategy, we introduce a validation mechanism for the adiabatic approximation by driving the quantum system to a non-inertial reference frame. More specifically, we begin by considering several rele…
The recently demonstrated trapping and laser cooling of $^{133}$Ba$^+$ has opened the door to the use of this nearly ideal atom for quantum information processing. However, before high fidelity qubit operations can be performed, a number of unknown state energies are needed. Here, we report measurements of the $^2$P$_{3/2}$ and $^2$D$_{5/2}$ hyperfine splittings, as well as the $^2$P$_{3/2}$$\leftrightarrow$ $^2$S$_{1/2}$and $^2$P$_{3/2}$ $\leftrightarrow$ $^2$D$_{5/2}$ transition frequencies. Using these transitions, we demonstrate high fidelity $^{133}$Ba$^+$ hyperfine qubit manipulation wit…
Simultaneous measurement of multiple qubits stored in hyperfine levels of trapped 111Cd+ ions is realized with an intensified charge-coupled device (CCD) imager. A general theory of fluorescence detection for hyperfine qubits is presented and applied to experimental data. The use of an imager for photon detection allows for multiple qubit state measurement with detection fidelities of greater than 98%. Improvements in readout speed and fidelity are discussed in the context of scalable quantum computation architectures.
Transition metal (TM) defects in silicon carbide (SiC) are a promising platform in quantum technology, especially because some TM defects emit in the telecom band. We develop a theory for the interaction of an active electron in the $D$-shell of a TM defect in SiC with the TM nuclear spin and derive the effective hyperfine tensor within the Kramers doublets formed by the spin-orbit coupling. Based on our theory we discuss the possibility to exchange the nuclear and electron states with potential applications for nuclear spin manipulation and long-lived nunclear-spin based quantum memories.
We experimentally realize an enhanced Raman control scheme for neutral atoms that features an intrinsic suppression of the two-photon carrier transition, but retains the sidebands which couple to the external degrees of freedom of the trapped atoms. This is achieved by trapping the atom at the node of a blue detuned standing wave dipole trap, that acts as one field for the two-photon Raman coupling. The improved ratio between cooling and heating processes in this configuration enables a five times lower fundamental temperature limit for resolved sideband cooling. We apply this method to perfor…
We propose to use a large cloud of cold trapped ions as a medium for quantum optics and quantum information experiments. Contrary to most recent realizations of qubit manipulation based on a small number of trapped and cooled ions, we study the case of traps containing a macroscopic number of ions. We consider in particular the implementation of a quantum memory for quantum information stored in continuous variables and study the impact of the relevant physical parameters on the expected performances of the system.
We investigate the electric manipulation of a single electron spin in a single gate-defined quantum dot. We observe that so-far neglected differences between the hyperfine and spin-orbit mediated electric dipole spin resonance conditions have important consequences at high magnetic fields. In experiments using adiabatic rapid passage to invert the electron spin, we observe an unusually wide and asymmetric response as a function of magnetic field. Simulations support the interpretation of the lineshape in terms of four different resonance conditions. These findings may lead to isotope-selective…
We propose a new design for a quantum information processor where qubits are encoded into Hyperfine states of ions held in a linear array of individually tailored microtraps and sitting in a spatially varying magnetic field. The magnetic field gradient introduces spatially dependent qubit transition frequencies and a type of spin-spin interaction between qubits. Single and multi-qubit manipulation is achieved via resonant microwave pulses as in liquid-NMR quantum computation while the qubit readout and reset is achieved through trapped-ion fluorescence shelving techniques. By adjusting the mic…
We experimentally investigate the resonance fluorescence spectrum of single 171Yb and 172Yb ions which are laser cooled to the Lamb-Dicke regime in a radiofrequency trap. While the fluorescence scattering of 172Yb is continuous, the 171Yb fluorescence is interrupted by quantum jumps because a nonvanishing rate of spontaneous transitions leads to electron shelving in the metastable hyperfine sublevel 2D3/2(F=2). The average duration of the resulting dark periods can be varied by changing the intensity of a repumping laser field. Optical heterodyne detection is employed to analyze the fluorescen…
We demonstrate the initialisation, read-out and high-speed manipulation of a qubit stored in a single 87 Rb atom trapped in a submicron-size optical tweezer. Single qubit rotations are performed on a sub-100 ns time scale using two-photon Raman transitions. Using the ``spin-echo'' technique, we measure an irreversible dephasing time of 34 ms. The read-out of the single atom qubit is at the quantum projection noise limit when averaging up to 1000 individual events.
We consider the quantum processor based on a chain of trapped ions to propose an architecture wherein the motional degrees of freedom of trapped ions (position and momentum) could be exploited as the computational Hilbert space. We adopt a continuous-variables approach to develop a toolbox of quantum operations to manipulate one or two vibrational modes at a time. Together with the intrinsic non-linearity of the qubit degree of freedom, employed to mediate the interaction between modes, arbitrary manipulation and readout of the ionic wave function could be achieved.
