Spectroscopic features revealing the coherent interaction of a degenerate two-level atomic system with two optical fields are examined. A model for the numerical calculation of the response of a degenerate two-level system to the action of an arbitrarily intense resonant pump field and a weak probe in the presence of a magnetic field is presented. The model is valid for arbitrary values of the total angular momentum of the lower and upper levels and for any choice of the polarizations of the optical waves. Closed and open degenerate two-level systems are considered. Predictions for probe absorption and dispersion, field generation by four-wave-mixing, population modulation and Zeeman optical pumping are derived. On all these observables, sub-natural-width coherence resonances are predicted and their spectroscopic features are discussed. Experimental spectra for probe absorption and excited state population modulation in the D2 line of Rb vapor are presented in good agreement with the calculations
Polarization squeezing is shown to occur in non-degenerate parametric amplification of coherent light and the degree of squeezing at interaction time $T$ can be as large as $1-e^{-2T}$. This gives $86.4\%$ polarization squeezing for $T=1$ and $98.2\%$ for $T=2$. One simple case when this occurs is on taking initially plane polarized light having equal amplitudes in the two modes that finally has equal intensities of two circular polarizations. This suggest the experimental settings of parameters to achieve this extent of polarization squeezing in coherent light.
A particularly simple setup is introduced to study the influence of time-delayed coherent feedback on the optical squeezing properties of the degenerate parametric amplifier (DPA). The possibility for significantly enhanced squeezing is demonstrated both on resonance and in sidebands, at a reduced pump power compared to the case without feedback. We study a broad range of operating parameters and their influence on the characteristic squeezing of the system. A classical analysis of the system dynamics reveals the connection between the feedback-modified landscape of stability and enhanced sque…
Quantum coherent feedback control is a measurement-free control method fully preserving quantum coherence. In this paper we show how time-delayed quantum coherent feedback can be used to control the degree of squeezing in the output field of a cavity containing a degenerate parametric oscillator. We focus on the specific situation of Pyragas-type feedback control where time-delayed signals are fed back directly into the quantum system. Our results show how time-delayed feedback can enhance or decrease the degree of squeezing as a function of time delay and feedback strength.
We present the quantum theory of coherent Ising machines based on networks of degenerate optical parametric oscillators (DOPOs). In a simple model consisting of two coupled DOPOs, both positive-$P$ representation and truncated Wigner representation predict quantum correlation and inseparability between the two DOPOs in spite of the open-dissipative nature of the system. Here, we apply the truncated Wigner representation method to coherent Ising machines with thermal, vacuum, and squeezed reservoir fields. We find that the probability of finding the ground state of a one-dimensional Ising model…
We study polarization squeezing of a light beam initially in the coherent state using the nonlinear interaction hamiltonian $ H=k\big(\hat a_{x}^{\dagger2}+{\hat a_{x}}^2\big)$. For the degree of polarization squeezing, we use a definition written in the final form by the authors and also used in earlier papers. We find that the polarization squeezing can be very high and the degree of polarization squeezing can be less than unity by a very small amount. We achieve the polarization squeezing even for very low beam intensity under some conditions involving phase angles in the polarization modes…
Non-equilibrium photon correlations of coherently excited single quantum systems can reveal their internal quantum dynamics and provide spectroscopic access. Here we propose and discuss the fundamentals of a coherent photon coincidence spectroscopy based on the application of laser pulses with variable delay and the detection of an time-averaged two-photon coincidence rate. For demonstration, two simple but important cases, i.e., an exciton - biexciton in a quantum dot and two coupled quantum emitters, are investigated based on quantum dynamics simulations demonstrating that this nonlinear spe…
Recently, the coherent Ising machine (CIM) as a degenerate optical parametric oscillator (DOPO) network has been researched to solve Ising combinatorial optimization problems. We formulate a theoretical model for the CIM with discrete-time measurement feedback processes, and perform numerical simulations for the simplest network, composed of two degenerate optical parametric oscillator pulses with the anti-ferromagnetic mutual coupling. We evaluate the extent to which quantum coherence exists during the optimization process.
The use of electron beams is ubiquitous; electron microscopy, scanning tunneling microscopy, electron lithography, and electron diffractometry all use well-collimated and focused beams. On the other hand, quantum degenerate electron beams do currently not exist. The realization of such beams may impact all electron beam technologies and are interesting to pursue. Past attempts to reach degeneracy were hampered by the low degeneracy of continuously emitting electron sources. With the recent advent of ultra-short electron pulses, high degeneracy is expected. Coulomb repulsion and low quantum coh…
In this paper we construct coherent states for the two-dimensional Morse potential. We find the dependence of the spectrum on the physical parameters and use this to understand the emergence of accidental degeneracies. It is observed that, under certain conditions pertaining to the irrationality of the parameters, accidental degeneracies do not appear and as such energy levels are at most two-fold degenerate. After defining a non-degenerate spectrum and set of states for the 2D Morse potential, we construct generalised coherent states and discuss the spatial distribution of their probability d…
A chirped-pulse quantum control scheme applicable to Coherent Anti-Stokes Raman Scattering spectroscopy, named as C-CARS, is presented aimed at maximizing the vibrational coherence in molecules. It implies chirping of three incoming pulses in the four-wave mixing process of CARS, the pump, the Stokes and the probe, to fulfil the conditions of adiabatic passage. The scheme is derived in the framework of rotating wave approximation and adiabatic elimination of excited state manifold simplifying the four-level model system into a ``super-effective'' two level system. The robustness, spectral sele…
We present a microscopic theory for nonlinear optical spectroscopy of N molecules in an optical cavity. A quantum Langevin analytical expression is derived for the time- and frequency-resolved signals accounting for arbitrary numbers of vibrational excitations. We identify clear signatures of the polariton-polaron interaction from multidimensional projections of the signal, e.g., pathways and timescales. Cooperative dynamics of cavity polaritons against intramolecular vibrations is revealed, along with a cross talk between long-range coherence and vibronic coupling that may lead to localizatio…
Employing the master equation for a three-level laser driven by coherent light and coupled to a squeezed vacuum reservoir, we obtain stochastic differential equations associated with the normal ordering. Using the solutions of the stochastic differential equations, we calculate the quadrature variance, the squeezing spectrum, the mean photon number, and the variance of the photon number. It turns out that the degree of squeezing increases with the linear gain coefficient or the squeeze parameter. It is also found that the driving coherent light decreases the mean photon number.
Environment-assisted squeezing in a coherently driven non-Hermitian degenerate parametric oscillator
Adama Science and Technology University（阿达马科学与技术大学）；Khalifa University of Science and Technology（哈利法科学技术大学）；Durban University of Technology（德班理工大学）；Arba Minch University（阿尔巴明奇大学）
Multi-dimensional spectroscopy represents a particularly insightful tool for investigating the interplay of nuclear and electronic dynamics, which plays an important role in a number of photophysical processes and photochemical reactions. Here we present a coherent state representation of the vibronic dynamics and of the resulting response functions for the widely used linearly displaced oscillator model. Analytical expressions are initially derived for the case of third-order response functions in an N-level system, with ground state initialization of the oscillator (zero-temperature limit). …
First-order phase transition in atom-molecule quantum degenerate mixtures with coherent three-body recombination
Missouri University of Science and Technology（密苏里科技大学）；Ben-Gurion University of the Negev（内盖夫本古里安大学）；Harvard & Smithsonian（哈佛大学与史密森尼学会）；University of Chicago（芝加哥大学）
We develop an ultrafast frequency-resolved Raman spectroscopy with entangled photons for polyatomic molecules in condensed phases, to probe the electronic and vibrational coherences. Using quantum correlation between the photons, the signal shows the capability of both temporal and spectral resolutions that are not accessible by either classical pulses or the fields without entanglement. We develop a microscopic theory for this Raman spectroscopy, revealing the electronic coherence dynamics which often shows a rapid decay within $\sim$50fs. The heterodyne-detected Raman signal is further devel…
We devise a phase-coherent three-pulse protocol to probe the polariton dynamics in a trapped-ion quantum simulation. In contrast to conventional nonlinear signals, the presented scheme does not change the number of excitations in the system, allowing for the investigation of the dynamics within an $N$-excitation manifold. In the particular case of a filling factor one ($N$ excitations in an $N$-ion chain), the proposed interaction induces coherent transitions between a delocalized phonon superfluid and a localized atomic insulator phase. Numerical simulations of a two-ion chain demonstrate tha…
Cryogenic operation in conjunction with new test-mass materials promises to reduce the sensitivity limitations from thermal noise in gravitational-wave detectors. The currently most advanced materials under discussion are crystalline silicon as a substrate with amorphous silicon-based coatings. They require, however, operational wavelengths around 2 $\mathrmμ$m to avoid laser absorption. Here, we present a light source at 2128 nm based on a degenerate optical parametric oscillator (DOPO) to convert light from a 1064 nm non-planar ring-oscillator (NPRO). We achieve an external conversion effici…
Multi-electron semiconductor quantum dots have found wide application in qubits, where they enable readout and enhance polarizability. However, coherent control in such dots has typically been restricted to only the lowest two levels, and such control in the strongly interacting regime has not been realized. Here we report quantum control of eight different resonances in a silicon-based quantum dot. We use qubit readout to perform spectroscopy, revealing a dense set of energy levels with characteristic spacing far smaller than the single-particle energy. By comparing with full configuration in…
Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission measurement of frequency-entangled broadband photon pairs generated via parametric down-conversion with a monochromatic laser. It is observed that state-to-state dynamics in the system under study are temporally resolved by adjusting the path difference between the entangled twin beams when the entanglement time is sufficiently short. The non-classical photon corr…
Analysis of the frequency shift in coherent population trapping resonance's dynamic continuous-wave spectroscopy at the phase-jump modulation and its comparison with the conventional approach
P. N. Lebedev Physical Institute of the Russian Academy of Sciences（俄罗斯科学院列别杰夫物理研究所）
Recent work applying multidimentional coherent electronic spectroscopy at dilute samples in the gas phase is reviewed. The development of refined phase-cycling approaches with improved sensitivity has opened-up new opportunities to probe even dilute gas-phase samples. In this context, first results of 2-dimensional spectroscopy performed at doped helium droplets reveal the femtosecond dynamics upon electronic excitation of cold, weakly-bound molecules, and even the induced dynamics from the interaction with the helium environment. Such experiments, offering well-defined conditions at low tempe…
Attosecond four-wave mixing spectroscopy using an XUV pulse and two noncollinear near-infrared pulses is employed to measure Rydberg wavepacket dynamics resulting from extreme ultraviolet excitation of a 3s electron in atomic argon into a series of autoionizing 3s-1np Rydberg states around 29 eV. The emitted signals from individual Rydberg states exhibit oscillatory structure and persist well beyond the expected lifetimes of the emitting Rydberg states. These results reflect substantial contributions of longer-lived Rydberg states to the four wave mixing emission signals of each individually d…
The Fano lineshape arises from the interference of two excitation pathways to reach a continuum. Its generality has resulted in a tremendous success in explaining the lineshapes of many one-dimensional spectroscopies - absorption, emission, scattering, conductance, photofragmentation - applied to very varied systems - atoms, molecules, semiconductors and metals. Unravelling a spectroscopy into a second dimension reveals the relationship between states in addition to decongesting the spectra. Femtosecond-resolved two-dimensional electronic spectroscopy (2DES) is a four-wave mixing technique tha…
