In computing the spectra of quantum mechanical systems one encounters the Fourier transforms of time correlation functions, as given by the quantum regression theorem for systems described by master equations. Quantum state diffusion (QSD) gives a useful method of solving these problems by unraveling the master equation into stochastic trajectories; but there is no generally accepted definition of a time correlation function for a single QSD trajectory. In this paper we show how QSD can be used to calculate these spectra directly; by formally solving the equations which arise, we arrive at a natural definition for a two-time correlation function in QSD, which depends explicitly on both the stochastic noise of the particular trajectory and the time of measurement, and which agrees in the mean with the ensemble average definition of correlation functions.
We investigate time-dependent stochastic disorder in the one-dimensional Jaynes-Cummings-Hubbard model and show that it gives rise to diffusive behaviour. We find that disorder correlation frequency is effective in controlling the level of diffusivity. In the defectless system the mean squared displacement (MSD), which is a measure of the diffusivity, increases with increasing disorder frequency. Contrastingly, when static defects are present the MSD increases with disorder frequency only at lower frequencies; at higher frequencies, increasing disorder frequency actually reduces the MSD.
Quantum chaos is linked to Brownian diffusion of the underlying quantum energy level-spacing sequences. The level-spacings viewed as functions of their order execute random walks which imply uncorrelated random increments of the level-spacings while the integrability to chaos transition becomes a change from Poisson to Gauss statistics for the level-spacing increments. This universal nature of quantum chaotic spectral correlations is numerically demonstrated for eigenvalues from random tight binding lattices and for zeros of the Riemann zeta function.
We experimentally verify the analytical expressions that exist for the diffusion rate in the quantum delta kicked rotor system for small numbers of kicks. We show development of diffusion resonances from two to five kicks, and of multiple resonances for high kick strengths. Furthermore, we show that, in contrast to classical predictions, the results are purely periodic in the kick period, and reproduce the predicted quantum- and diffusion resonances.
We present a model of an N-qubit channel where consecutive qubits experience correlated random rotations. Our model is an extension to the standard decoherence-free subsystems approach (DFS) which assumes that all the qubits experience the same disturbance. The variation of rotations acting on consecutive qubits is modeled as diffusion on the SU(2) group. The model may be applied to spins traveling in a varying magnetic field, or to photons passing through a fiber whose birefringence fluctuates over the time separation between photons. We derive an explicit formula describing the action of the…
Spectral diffusion is the phenomenon of random jumps in the emission wavelength of narrow lines. This phenomenon is a major hurdle for applications of solid state quantum emitters like quantum dots, molecules or diamond defect centers in an integrated quantum optical technology. Here, we provide further insight into the underlying processes of spectral diffusion of the zero phonon line of single nitrogen vacancy centers in nanodiamonds by using a novel method based on photon correlation interferometry. The method works although the spectral diffusion rate is several orders of magnitude higher …
Quantum diffusion, as developed in the 1990s, could explain how a system, subject to measurement, goes into an eigenstate of the measured observable. Here it is shown that quantum diffusion theory can be interpreted as a result within linear relativistic quantum mechanics. Thus, in contrast to what is widely believed, quantum measurement can be analyzed within the theory of quantum mechanics itself.
We use paramagnetic Faraday rotation to study spin noise spectrum from unpolarized Rb vapor in a tightly focused probe beam in the presence of N$_2$ buffer gas. We derive an analytical form for the diffusion component of the spin noise time-correlation function in a Gaussian probe beam. We also obtain analytical forms for the frequency spectrum of the spin noise in the limit of a tightly focused or a collimated Gaussian beam in the presence of diffusion. In particular, we find that in a tightly focused probe beam the spectral lineshape can be independent of the buffer gas pressure. Experimenta…
Capturing non-Markovian dynamics of open quantum systems is generally a challenging problem, especially for strongly-interacting many-body systems. In this work, we combine recently developed non-Markovian quantum state diffusion techniques with tensor network methods to address this challenge. As a first example, we explore a Hubbard-Holstein model with dissipative phonon modes, where this new approach allows us to quantitatively assess how correlations spread in the presence of non-Markovian dissipation in a 1D many-body system. We find regimes where correlation growth can be enhanced by the…
Diffusion noise is a major source of spectral line broadening in liquid state nano-scale nuclear magnetic resonance with shallow nitrogen-vacancy centres, whose main consequence is a limited spectral resolution. This limitation arises by virtue of the widely accepted assumption that nuclear spin signal correlations decay exponentially in nano-NMR. However, a more accurate analysis of diffusion shows that correlations survive for a longer time due to a power-law scaling, yielding the possibility for improved resolution and altering our understanding of diffusion at the nano-scale. Nevertheless,…
The paper contains the proof that the diffusion ensemble of point wise particles with the intensity depending on the grain of spatial resolution serves as the satisfactory approximation of one quantum particle dynamics.
We demonstrate the relevance of complex Gaussian stochastic processes to the stochastic state vector description of non-Markovian open quantum systems. These processes express the general Feynman-Vernon path integral propagator for open quantum systems as the classical ensemble average over stochastic pure state propagators in a natural way. They are the coloured generalization of complex Wiener processes in quantum state diffusion stochastic Schrodinger equations.
A new approach to thermo-quantum diffusion is proposed and a nonlinear quantum Smoluchowski equation is derived, which describes classical diffusion in the field of the Bohm quantum potential. A nonlinear thermo-quantum expression for the diffusion front is obtained, being a quantum generalization of the classical Einstein law. The quantum diffusion at zero temperature is also described and a new dependence of the position dispersion on time is derived. A stochastic Bohm-Langevin equation is also proposed.
The recently reported relativistic formulation of the well-known non-relativistic quantum state diffusion is seriously mistaken. It predicts, for instance, inconsistent measurement outcomes for the same system when seen by two different inertial observers.
Riemannian metric on real 2n-dimensional space associated with the equation governing complex diffusion of pure states of an open quantum system is introduced and studied. Examples of a qubit under the influence of dephasing and thermal environments are used to show that the curvature of the diffusion metric is a good indicator of the properties of the environment dominated evolution and its stability.
We study the quantum Arnol'd diffusion for a particle moving in a quasi-1D waveguide bounded by a periodically rippled surface, in the presence of the time-periodic electric field. It was found that in a deep semiclassical region the diffusion-like motion occurs for a particle in the region corresponding to a stochastic layer surrounding the coupling resonance. The rate of the quantum diffusion turns out to be less than the corresponding classical one, thus indicating the influence of quantum coherent effects. Another result is that even in the case when such a diffusion is possible, it termin…
A diffusion process is usually assumed for the phase of the order parameter of a Bose system of finite size. The theoretical basis is limited to the so called Bogoliubov approximation. We show that a suitable generalization of the Hartree-Fock-Bogoliubov approach recovers phase diffusion.
The dynamics of a kicked quantum system undergoing repeated measurements of momentum is investigated. A diffusive behavior is obtained even when the dynamics of the classical counterpart is not chaotic. The diffusion coefficient is explicitly computed for a large class of Hamiltonians and compared to the classical case.
The quantum diffusion of a particle in an initially localized state on a cyclic lattice with N sites is studied. Diffusion and reconstruction time are calculated. Strong differences are found for even or odd number of sites and the limit N->infinit is studied. The predictions of the model could be tested with micro - and nanotechnology devices.
We show that quantum diffusion near the quantum critical point can provide a highly very efficient mechanism of open-system quantum annealing. It is based on the diffusion-mediated recombination of excitations. For an Ising spin chain coupled to a bosonic bath, excitation diffusion in a transverse field sharply slows down as the system moves away from the quantum critical region. This leads to spatial correlations and effective freezing of the excitation density. We find that obtaining an approximate solution via the diffusion-mediated quantum annealing can be faster than via closed-system qua…
By modelling quantum systems as emerging from a (classical) sub-quantum thermodynamics, the quantum mechanical "decay of the wave packet" is shown to simply result from sub-quantum diffusion with a specific diffusion coefficient varying in time due to a particle's changing thermal environment. It is thereby proven that free quantum motion strictly equals ballistic diffusion. The exact quantum mechanical trajectory distributions and the velocity field of the Gaussian wave packet are thus derived solely from classical physics. Moreover, also quantum motion in a linear (e.g., gravitational) poten…
Quantum diffusion is studied via dissipative Madelung hydrodynamics. Initially the wave packet spreads ballistically, than passes for an instant through normal diffusion and later tends asymptotically to a sub-diffusive law. It is shown that the apparent quantum diffusion coefficient is not a universal physical parameter since it depends on the initial wave packet preparation. The overdamped quantum diffusion of an electron in the field of a periodic potential is also investigated; in this case the wave packet spreads logarithmically in time. Thermo-quantum diffusion of heavier particles as hy…
We present a simple approach to the fixed phase method in Quantum Monte Carlo. This applies to electrons in molecules and electron gas and is straightforwardly extended to the Schrödinger equation with magnetic field.
Extensive coherent control over quantum chaotic diffusion using the kicked rotor model is demonstrated and its origin in deviations from random matrix theory is identified. Further, the extent of control in the presence of external decoherence is established. The results are relevant to both areas of quantum chaos and coherent control.
We study the spreading of a quantum-mechanical wavepacket in a one-dimensional tight-binding model with a noisy potential, and analyze the emergence of classical diffusion from the quantum dynamics due to decoherence. We consider a finite correlation time of the noisy environment, and treat the system by utilizing the separation of fast (dephasing) and slow (diffusion) processes. We show that classical diffusive behavior emerges at long times, and we calculate analytically the dependence of the classical diffusion coefficient on the noise magnitude and correlation time. This method provides a …
A quantum Markovian activated atom-surface diffusion model with interacting adsorbates is proposed for the intermediate scattering function, which is shown to be complex-valued and factorizable into a classical-like and a quantum-mechanical factor. Applications to the diffusion of Na atoms on flat (weakly corrugated) and corrugated-Cu(001) surfaces at different coverages and surface temperatures are analyzed. Quantum effects are relevant to diffusion at low surface temperatures and coverages even for relatively heavy particles, such as Na atoms, where transport by tunneling is absent.
Non-Markovian quantum state diffusion (NMQSD) provides a powerful approach to the dynamics of an open quantum system in bosonic environments. Here we develop an NMQSD method to study the open quantum system in fermionic environments. This problem involves anticommutative noise functions (i.e., Grassmann variables) that are intrinsically different from the noise functions of bosonic baths. We obtain the NMQSD equation for quantum states of the system and the non-Markovian master equation. Moreover, we apply this NMQSD method to single and double quantum-dot systems.
We study the fingerprint of the Arnol'd diffusion in a quantum system of two coupled nonlinear oscillators with a two-frequency external force. In the classical description, this peculiar diffusion is due to the onset of a weak chaos in a narrow stochastic layer near the separatrix of the coupling resonance. We have found that global dependence of the quantum diffusion coefficient on model parameters mimics, to some extent, the classical data. However, the quantum diffusion happens to be slower that the classical one. Another result is the dynamical localization that leads to a saturation of t…
We study an analog of the classical Arnol'd diffusion in a quantum system of two coupled non-linear oscillators one of which is governed by an external periodic force with two frequencies. In the classical model this very weak diffusion happens in a narrow stochastic layer along the coupling resonance, and leads to an increase of total energy of the system. We show that the quantum dynamics of wave packets mimics, up to some extent, global properties of the classical Arnol'd diffusion. This specific diffusion represents a new type of quantum dynamics, and may be observed, for example, in 2D se…
