Quantum computers based on electron spins controlled by ultra-fast, off-resonant, single optical pulses
Susan M. Clark, Kai-Mei C. Fu, Thaddeus D. Ladd, Yoshihisa Yamamoto
备注：
4 pages, 4 figures, introduction is clarified, the section on two-qubit gates was expanded and much more detail about gate fidelities is given, figures were modified, one figure replaced with a figure showing gate fidelities for relevant parameters
We describe a fast quantum computer based on optically controlled electron spins in charged quantum dots that are coupled to microcavities. This scheme uses broad-band optical pulses to rotate electron spins and provide the clock signal to the system. Non-local two-qubit gates are performed by phase shifts induced by electron spins on laser pulses propagating along a shared waveguide. Numerical simulations of this scheme demonstrate high-fidelity single-qubit and two-qubit gates with operation times comparable to the inverse Zeeman frequency.
We propose a method to design pulses in a resonant three-level system to enhance the robustness of non-adiabatic geometric gate operations. By optimizing the shape of the pulse envelope, we show that the gate operations are more robust against frequency detuning than they are with Gaussian and square pulses. Our method provides a way to design pulses that can be employed in a system where robustness against frequency variations or inhomogeneous broadening is required,and may be extended to ensure robustness against other physical imperfections such as intensity fluctuations and random noises.
We study the quantum dynamics of a two-level system driven by a pulse that starts near-resonant for small amplitudes, yielding nonadiabatic evolution, and induces an adiabatic evolution for larger amplitudes. This problem is analyzed in terms of lifting of degeneracy for rising amplitudes. It is solved exactly for the case of linear and exponential rising. Approximate solutions are given in the case of power law rising. This allows us to determine approximative formulas for the lineshape of resonant excitation by various forms of pulses such as truncated trig-pulses. We also analyze and explai…
We propose a new protocol to implement ultra-fast two-qubit phase gates with trapped ions using spin-dependent kicks induced by resonant transitions. By only optimizing the allocation of the arrival times in a pulse train sequence the gate is implemented in times faster than the trapping oscillation period $T<2π/ω$. Such gates allow us to increase the number of gate operations that can be completed within the coherence time of the ion-qubits favoring the development of scalable quantum computers.
We present a simple approach allowing to obtain analytical expressions for laser pulses that can drive a two-level system in an arbitrarily chosen way. The proposed scheme relates every desired population-evolution path to a single resonant laser pulse. It allows to drive the system from any initial superposition of the two states to a final state having the desired distribution of the populations. We exemplify the scheme with a concrete example, where the system is driven from a non-stationary superposition of states to one of its eigenstates. We argue that the proposed approach may have inte…
Resonant spontaneous bremsstrahlung of an electron scattered by a nucleus in the field of two moderately strong pulsed laser waves is studied theoretically. The process is studied in detail within the interference kinematic region. This region is determined by scattering of particles in the same plane at predetermined angles, at that stimulated absorption and emission of photons of external pulsed waves by an electron occurs in correlated manner. The correspondence between the emission angle and the final-electron energy is established in the kinematic region where the resonant parametric inte…
Ultrachirped pulses for which the frequency chirp is of the order of the transition frequency of a two-level atom are examined. When the chirp is large enough, the resonance may be crossed twice, for positive and negative quadrature frequencies. In this scenario the analytic signal and quadrature decompositions of the field into amplitude and phase factors turn out to be quite different. The corresponding interaction pictures are strictly equivalent, but only as long as approximations are not applied. The domain of validity of the formal rotating wave approximation is dramatically enhanced usi…
We consider a quantum processor based on five qutrits represented by spins S=1, which is driven by radio fre-quency (RF) pulses selective in transitions between adjacent levels. Numerical simulation of the implementation of the quantum-adiabatic clustering algorithm was performed on the example of partitioning a set of six points into three groups. We find the amplitudes and durations of rectangular RF pulses, as well as the durations of free evolu-tion intervals in the control pulse sequence, which made it possible to engineer a time-dependent effective Hamilto-nian in the discrete-time appro…
We have considered theoretically the feasibility of the broadband quantum memory based on the resonant tripod-type atomic configuration. In this case, the writing of a signal field is carried out simultaneously into two channels, and characterized by an excitation of two spin waves of the atomic ensemble. With simultaneous read out from both channels quantum properties of the original signal are mapped on the retrieval pulse no worse than in the case of memory based on Lambda-type atomic configuration. At the same time new possibilities are opened up for manipulation of quantum states associat…
The resonant filtering method transforming frequency modulated radiation field into a train of short pulses is proposed to apply in optical domain. Effective frequency modulation can be achieved by electro-optic modulator or by resonant frequency modulation of the filter with a narrow absorption line. Due to frequency modulation narrow-spectrum CW radiation field is seen by the resonant filter as a comb of equidistant spectral components separated by the modulation frequency. Tuning narrow-bandwidth filter in resonance with $n$-th spectral component of the comb transforms the radiation field i…
We study the dynamics of a two-level system driven by an off-resonant few-cycle pulse which has a phase jump $ϕ$ at $t=t_{0}$, in contrast to many cycle pulses, under non rotating-wave approximation (NRWA). We give a closed form analytical solution for the evolution of the probability amplitude $|C_{a} (t)|$ for the upper level. Using the appropriate pulse parameters like phase-jump $ϕ$, jump time $t_{0}$, pulse width $τ$, frequency $ν$ and Rabi frequency $Ω_{0}$ the population transfer, after the pulse is gone, can be optimized and for the pulse considered here, enhancement of $10^{6}-10^{8}$…
The actual theoretical research investigates the resonant high-energy spontaneous bremsstrahlung of ultrarelativistic electrons with considerable energies in the field of a nucleus and a quasimonochromatic laser wave. Under the resonant conditions within the laser field the intermediate virtual electron transforms into the real particle. As a result, the accomplished analysis defines that the polar emission angle characterizes the frequency of a spontaneous photon. The study derives the expressions for the resonant differential cross-sections of the represented processes that realize simultane…
We present an analytical treatment of coherent excitation of a Two-Level Atom driven by a far-off resonant classical field. A class of pulse envelope is obtained for which this problem is exactly solvable. The solutions are given in terms of Heun function which is a generalization of the Hypergeometric function. The degeneracy of Heun to Hypergeometric equation can give all the exactly solvable pulse shapes of Gauss Hypergeometric form, from the generalized pulse shape obtained here. We discuss the application of the results obtained to the generation of XUV.
The ability to enhance resonant signals and eliminate the non-resonant background is analyzed for Coherent Anti-Stokes Raman Scattering (CARS). The analysis is done at a specific frequency as well as for broadband excitation using femtosecond pulse-shaping techniques. An appropriate objective functional is employed to balance resonant signal enhancement against non-resonant background suppression. Optimal enhancement of the signal and minimization of the background can be achieved by shaping the probe pulse alone while keeping the pump and Stokes pulses in transform-limited-form (TLF). In some…
We experimentally investigate the atom optics kicked particle at quantum resonance using finite duration kicks. Even though the underlying process is quantum interference it can be well described by an $ε$-pseudoclassical model. The $ε$-pseudoclassical model agrees well with our experiments for a wide range of parameters. We investigate the parameters yielding maximal momentum transfer to the atoms and find that this occurs in the regime where neither the short pulse approximation nor the Bragg condition is valid. Nonetheless, the momentum transferred to the atoms can be predicted using a simp…
Existence of self-similar, superposed pulse-train solutions of the nonlinear, coupled Maxwell-Schrödinger equations, with the frequencies controlled by the oscillator strengths of the transitions, is established. Some of these excitations are specific to the resonant media, with energy levels in the configurations of $Λ$ and $N$ and arise because of the interference effects of cnoidal waves, as evidenced from some recently discovered identities involving the Jacobian elliptic functions. Interestingly, these excitations also admit a dual interpretation as single pulse-trains, with widely differ…
A simple method for the production of ultrashort light pulses (USPs) with suppressed photon fluctuations is considered. The method is based on self-phase modulation (SPM) of an USP in a nonlinear medium (optical fibre) and subsequent transmission of pulse through a dispersive optical element.
The propagation of a step pulse through a thick resonant absorber with homogeneously broadened absorption line is considered. It is shown that a specific subradiant state is naturally developed in the absorber due to the formation of the spatial domains of the atomic coherence with opposite phases. It is proposed to divide the absorber into slices in accord with these domains and place the phase shifters in front of the first slice and between the other slices. If the phase shifters are switched on simultaneously at a particular moment of time, elapsed from the beginning of the step pulse, a s…
We present rigorous and intuitive master equation models to study on-demand single photon sources from pulse-excited quantum dots coupled to cavities. We consider three methods of source excitation: resonant pi-pulse, off-resonant phonon-assisted inversion, and two-photon excitation of a biexciton-exciton cascade, and investigate the effect of the pulse excitation process on the quantum indistinguishability, efficiency, and purity of emitted photons. By explicitly modelling the time-dependent pulsed excitation process in a manner which captures non-Markovian effects associated with coupling to…
Quantum computing exploits the quantum-mechanical nature of matter to exist in multiple possible states simultaneously. This new approach promises to revolutionize the present form of computing. As an approach to quantum computing, we discuss ultrafast laser pulse shaping, in particular, the acousto-optic modulator based Fourier-Transform pulse-shaper, which has the ability to modulate tunable high power ultrafast laser pulses. We show that optical pulse shaping is an attractive route to quantum computing since shaped pulses can be transmitted over optical hardware and the same infrastructure …
We present a systematic approach based on Bloch vector's treatment and the Magnus quantum electrodynamical formalism to study qubit manipulation by a train of pulses. These investigations include one of the basic processes involved in quantum computation. The concrete calculations are performed for tunneling quantum dynamics, multiple resonance and off-resonance excitations of qubit driven by Gaussian pulses. In this way, the populations of qubit states due to multiple resonant interactions are investigated for various operational regimes including: single-pulse excitation, two-pulse excitatio…
We investigate the evolution of extreme ultraviolet (XUV) spectral lineshapes in an optically-thick helium gas under near-infrared (IR) perturbation. In our experimental and theoretical work, we systematically vary the IR intensity, time-delay, gas density and IR polarization parameters to study lineshape modifications induced by collective interactions, in a regime beyond the single atom response of a thin, dilute gas. In both experiment and theory, we find that specific features in the frequency-domain absorption profile, and their evolution with propagation distance, can be attributed to th…
We report measurements of the time-dependent phases of the leak and retrieved pulses obtained in EIT storage experiments with metastable helium vapor at room temperature. In particular, we investigate the influence of the optical detuning at two-photon resonance, and provide numerical simulations of the full dynamical Maxwell-Bloch equations, which allow us to account for the experimental results.
An efficient technique to produce a periodic sequence of ultrashort pulses of recoilless gamma-radiation via its transmission through the optically thick vibrating resonant absorber was demonstrated recently [Nature, 508, 80 (2014)]. In this work we extend the theoretical analysis to the case of a set of multiple absorbers. We consider an analytical model describing the control of spectral content of a frequency modulated gamma-radiation by selective correction of amplitudes and initial phases of some spectral components, using, respectively, the resonant absorption or dispersion of nuclei. On…
We discuss procedures for error-tolerant spin control in environments that permit transient, large-angle reorientation of magnetic bias field. Short sequences of pulsed, non-resonant magnetic field pulses in a laboratory-frame meridional plane are derived. These are shown to have band-pass excitation properties comparable to established amplitude-modulated, resonant pulses used in high, static-field magnetic resonance. Using these meridional pulses, we demonstrate robust $z$ inversion in proton ($^{1}$H) nuclear magnetic resonance near earth's field.
We solve a finite range two-channel model for three resonant identical bosons. The model provides a minimal description of the various magnetic Feshbach resonances in single species ultra-cold bosonic systems, including off-resonant scattering. We obtain important insights into the interpretation of seminal experiments: the three-body recombination rate measured in Sodium and the Efimov resonances observed in Caesium. This approach quantifies non universal effects appearing for a finite magnetic field detuning.
We report on time-resolved pulsed four-wave mixing (FWM) signals in a thermal Rubidium vapor involving a Rydberg state. We observe FWM signals with dephasing times up to 7 ns, strongly dependent on the excitation bandwidth to the Rydberg state. The excitation to the Rydberg state is driven by a pulsed two-photon transition on ns time scales. Combined with a third cw de-excitation laser, a strongly directional and collective emission is generated according to a combination of the phase matching effect and averaging over Doppler classes. In contrast to a previous report [1] using off-resonant FW…
For neutral atom qubits, the residual thermal motion of the cold atoms constitutes a major challenge that limits the accessible two-qubit gate fidelity. Recently, an interesting type of two-qubit controlled-PHASE quantum gate protocol has been introduced for neutral atom qubit platform, which relies upon off-resonant modulated driving and Rydberg blockade effect. Building upon this progress, we have further developed an upgrade in the form of dual-pulse off-resonant modulated driving. Besides the inherent advantages of avoiding shelving population in Rydberg levels, not necessarily requiring i…
Off-resonant error for a driven quantum system refers to interactions due to the input drives having non-zero spectral overlap with unwanted system transitions. For the cross-resonance gate, this includes leakage as well as off-diagonal computational interactions that lead to bit-flip error on the control qubit. In this work, we quantify off-resonant error, with more focus on the less studied off-diagonal control interactions, for a direct CNOT gate implementation. Our results are based on numerical simulation of the dynamics, while we demonstrate the connection to time-dependent Schrieffer-Wo…
It is shown that the magnetic state decoherence produced by collisions in a thermal vapor can be suppressed by the application of a train of ultrafast optical pulses.
Neutral atom array serves as an ideal platform to study the quantum logic gates, where intense efforts have been devoted to improve the two-qubit gate fidelity. We report our recent findings in constructing a different type of two-qubit controlled-PHASE quantum gate protocol with neutral atoms enabled by Rydberg blockade, which aims at both robustness and high-fidelity. It relies upon modulated driving pulse with specially tailored smooth waveform to gain appropriate phase accumulations for quantum gates. The major features include finishing gate operation within a single pulse, not necessaril…
Intense, well-controlled regular light pulse trains start to play a crucial role in many fields of physics. We theoretically demonstrate a very simple and robust technique for generating such periodic ultrashort pulses from a continuous probe wave which propagates in a dispersive thermal gas media.
We study the photoionization and autoionization of Helium atom subject to ultrashort laser pulses by using a Feshbach formalism in the time domain. We solve the time-dependent Schrödinger equation in terms of a configuration interaction (CI) spectral method, in which the total wavefunction is expanded with configurations defined within bound-like ($\mathcal{Q}$) and scattering-like ($\mathcal{P}$) halfspaces. The method allowsone to provide accurate descriptions of both the atomic structure (energy positions and widths) and the photodynamics. We illustrate our approach by i) calculating the ti…
Experimental and numerical investigation of single-beam and pump-probe interaction with a resonantly absorbing dense extended medium under strong and weak field-matter coupling is presented. Significant probe beam amplification and conical emission were observed. Under relatively weak pumping and high medium density, when the condition of strong coupling between field and resonant matter is fulfilled, the probe amplification spectrum has a form of spectral doublet. Stronger pumping leads to the appearance of a single peak of the probe beam amplification at the transition frequency. The greater…
A new approach to single-qubit operations using exchange interactions of single electrons in gate-defined quantum dots has recently been demonstrated: the resonant exchange qubit. We show that two-qubit operations, specifically the CPHASE gate, can be performed between resonant exchange qubits very straightforwardly, using a single exchange pulse. This is in marked contrast to the best known protocols for exchange qubits where such a gate requires many pulses so that leakage processes arising from the exchange interaction can be overcome. For resonant exchange qubits a simple two-qubit gate is…
We model the formation of stable heteronuclear molecules via pulsed Raman photoassociation of a two-component Bose-Einstein condensate near a strong Feshbach resonance, for both counterintuitive and intuitive pulse sequencing. Compared to lasers alone, weak Raman photoassociation is enhanced by as much as a factor of ten (five) for a counterintuitive (intuitive) pulse sequence, whereas strong Raman photoassociation is barely enhanced at all--regardless of pulse sequence. Stronger intra-atom, molecule, or atom-molecule collisions lead to an expected decrease in conversion efficiency, but strong…
We demonstrate generation of a pulsed stream of electrically triggered single photons in resonance fluorescence, by applying high frequency electrical pulses to a single quantum dot in a p-i-n diode under resonant laser excitation. Single photon emission was verifed, with the probability of multiple photon emission reduced to 2.8%. We show that despite the presence of charge noise in the emission spectrum of the dot, resonant excitation acts as a filter to generate narrow bandwidth photons.
Fiber guided optical signal propagating in a Erbium doped nonlinear resonant medium is known to produce cleaner solitonic pulse, described by the self induced transparency (SIT) coupled to nonlinear Schroedinger equation. We discover two new possibilities hidden in its integrable structure, for amplification and control of the optical pulse. Using the variable soliton width permitted by the integrability of this model, the broadening pulse can be regulated by adjusting the initial population inversion of the opant atoms. The effect can be enhanced by another innovative application of its const…
