Gevorg Muradyan, Mariam Hovhannisyan
Intense, well-controlled regular light pulse trains start to play a crucial role in many fields of physics. We theoretically demonstrate a very simple and robust technique for generating such periodic ultrashort pulses from a continuous probe wave which propagates in a dispersive thermal gas media.
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Errors in quantum state identification with ultrashort pulses
本文从探测基本原理出发，证明超短脉冲等非平稳场的相干函数依赖场形状，导致超快源观测的聚束与超聚束不能指示场的量子态。
Quantum coherence between electronic states of a photoionized molecule and the resulting process of ultrafast electron-hole migration have been put forward as a possible quantum mechanism of charge-directed reactivity governing the photoionization-induced molecular decomposition. Attosecond experiments based on the indirect (fragment ion-based) characterization of the proposed electronic phenomena suggest that the photoionization-induced electronic coherence can survive for tens of femtoseconds, while some theoretical studies predict much faster decay of the coherence due to the quantum uncert…
We discuss the propagation of laser radiation through a medium of quantum prepared Λ-type atoms in order to enhance the insight into the physics of QS-PT generator suggested in Phys. Rev. A 80, 035801 (2009). We obtain analytical results which give a qualitatively corerct description of the outcoming series of ultrashort optical pulses and show that for the case of alkali vapor medium QS-PT generation may be implemented under ordinary experimental conditions.
The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond exclusively to electronic coherences, and thus such experiments can be used to form a test for electronic vs. vibrational oscillations in such systems. Here we demonstrate a method for practically implementing such a test, whereby pump-probe signals are taken at several different pulse durations and used to extrapolate to the ultrashort-pulse limit. We present…
Developing an analytical theory for atomic coherence driven by ultrashort laster pulses has proved to be challenging due to the breakdown of the rotating wave approximation (RWA). In this paper, we present an approximate, closed-form solution to the Schrodinger equation that describes a two-level atom under the excitation of a far-off-resonance, few-cycle pulse of arbitrary shape without invoking the RWA. As an example of its applicability, an analytical solution for Gaussian pulses is explicitly given. Comparisons with numerical solutions validate the accuracy our solution within the scope of…
Electronic interferometry with ultrashort plasmonic pulses
本文将超短单电子等离激元脉冲注入14微米Mach-Zehnder干涉仪，证明按需注入下量子相干性稳健，并首次揭示高频非绝热区域，为飞行量子比特的量子信息处理提供新路径。
The coherence properties of broadband down converted light are investigated theoretically and experimentally in both the classical and quantum mechanical frameworks. Although broadband down converted light is one-photon incoherent noise, it possesses unique two-photon coherence. Thus, for performing two-photon processes, down-converted light is equivalent to coherent ultrashort pulses in some aspects and to coherent CW laser radiation in others. This equivalence is theoretically established and experimentally demonstrated in the classical, high-power regime. Two applications that take advantag…
We analyze electronically excited nuclear wave functions and their coherence when subjecting a molecule to the action of natural, pulsed incoherent solar-like light, and to that of ultrashort coherent light assumed to have the same center frequencies and spectral bandwidths. Specifically, we compute the spatio-temporal dependence of the excited wave packets and their electronic coherence for these two types of light sources, on different electronic potential energy surfaces. The resultant excited state wave functions are shown to be qualitatively different, reflecting the light source from whi…
Electronic coherence is of utmost importance for the access and control of quantum-mechanical solid-state properties. Using a purely electronic observable, the photocurrent, we measure an electronic coherence time of 22 +/- 4 fs in graphene. The photocurrent is ideally suited to measure electronic coherence as it is a direct result of quantum path interference, controlled by the delay between two ultrashort two-color laser pulses. The maximum delay for which interference between the population amplitude injected by the first pulse interferes with that generated by the second pulse determines t…
Generation of ultrashort (~10ps) spontaneous emission pulses by quantum dots in a switched optical microcavity
本研究通过自由载流子脉冲注入开关 GaAs/AlAs 微柱腔，利用量子点集合体作为内部光源，实现了 6 至 300 皮秒的超短自发辐射脉冲，为超快成像和量子光子学提供了关键资源。
Controlling the wave function of free electrons is important to improve the spatial resolution of electron microscopes, the efficiency of electron interaction with sample modes of interest, and our ability to probe ultrafast materials dynamics at the nanoscale. In this context, attosecond electron compression has been recently demonstrated through interaction with the near fields created by scattering of ultrashort laser pulses at nanostructures followed by free electron propagation. Here, we show that control over electron pulse shaping, compression, and statistics can be improved by replacin…
Coherence-limited digital control of a superconducting qubit using a Josephson pulse generator at 3 K
利用约瑟夫森脉冲发生器在3K下实现超导量子比特的相干限制数字控制，提升了门保真度和退相干时间。
We present a general analysis for the interaction of a probe laser radiation with a coherently prepared molecular Raman medium. We describe a general formalism which includes dispersive effects, such as group velocity and group velocity dispersion (GVD). When dispersion is negligible, the analysis is especially simple and insightful. We show that molecular oscillations result in a modulated instantaneous susceptibility of the medium. The effect of the time-varying susceptibility on a probe laser pulse is two-fold: the output frequency becomes modulated because of the time-varying phase velocit…
Scaling of quantum computers to fault-tolerant levels relies critically on the integration of energy-efficient, stable, and reproducible qubit control and readout electronics. In comparison to traditional semiconductor control electronics (TSCE) located at room temperature, the signals generated by Josephson junction (JJ) based rf sources benefit from small device sizes, low power dissipation, intrinsic calibration, superior reproducibility, and insensitivity to ambient fluctuations. Previous experiments to co-locate qubits and JJ-based control electronics resulted in quasiparticle poisoning o…
Superconducting quantum computer is manufactured based on semiconductor process which makes qubits integration possible. At the same time, this kind of qubit exhibits high performance fidelity, de-coherence time, scalability and requires a programmable arbitrary waveform generator (AWG). This paper presents implementation of an AWG which composed of two gigabit samples per second (GSPS) sampling rate, 16 bit vertical resolution digital to analog converters (DACs). The AWG integrated with separate microwave devices onto a metal plate for the scale-up consideration. A special waveform sequence o…
The nature of excited states of open quantum systems produced by incoherent natural thermal light is analyzed based on a description of the generator of the dynamics. Natural thermal light is shown to generate long-lasting coherent dynamics because of (i) the super-Ohmic character of the radiation, and (ii) the absence of pure dephasing dynamics. In the presence of an environment, the long-lasting coherences induced by suddenly turned-on incoherent light dissipate and stationary coherences are established. As a particular application, dynamics in a subunit of the PC-645 light-harvesting comple…
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