We present a systematic approach based on Bloch vector's treatment and the Magnus quantum electrodynamical formalism to study qubit manipulation by a train of pulses. These investigations include one of the basic processes involved in quantum computation. The concrete calculations are performed for tunneling quantum dynamics, multiple resonance and off-resonance excitations of qubit driven by Gaussian pulses. In this way, the populations of qubit states due to multiple resonant interactions are investigated for various operational regimes including: single-pulse excitation, two-pulse excitation with phase shift between pulse envelopes being controlling parameter and for excitation with sequential pulses. In the last case, we demonstrate the formation of quasienergetic states and quasienergies of qubit driven by train of identical pulses. In this case the transition probability of qubit exhibits aperiodic oscillations, but also becomes periodically regular for definite values of the quasienergy.
We present an experimental demonstration as well as a theoretical model of an integrated circuit designed for the manipulation of a microwave field down to the single-photon level. The device is made of a superconducting resonator coupled to a transmission line via a second frequency-tunable resonator. The tunable resonator can be used as a tunable coupler between the fixed resonator and the transmission line. Moreover, the manipulation of the microwave field between the two resonators is possible. In particular, we demonstrate the swapping of the field from one resonator to the other by pulsi…
Silicon carbide (SiC) has become a key player in realization of scalable quantum technologies due to its ability to host optically addressable spin qubits and wafer-size samples. Here, we have demonstrated optically detected magnetic resonance (ODMR) with resonant excitation, and clearly identified the ground state energy levels of the NV centers in 4H-SiC. Coherent manipulation of NV centers in SiC has been achieved with Rabi and Ramsey oscillations. Finally, we show the successful generation and characterization of single nitrogen vacancy (NV) center in SiC employing ion implantation. Our re…
A scheme for controlling the entanglement of a two-qubit system by a local magnetic pulse is proposed. We show that the entanglement of the two-qubit system can be increased by sacrificing the coherence in ancillary degree of freedom, which is induced by a local manipulation.
We present rigorous and intuitive master equation models to study on-demand single photon sources from pulse-excited quantum dots coupled to cavities. We consider three methods of source excitation: resonant pi-pulse, off-resonant phonon-assisted inversion, and two-photon excitation of a biexciton-exciton cascade, and investigate the effect of the pulse excitation process on the quantum indistinguishability, efficiency, and purity of emitted photons. By explicitly modelling the time-dependent pulsed excitation process in a manner which captures non-Markovian effects associated with coupling to…
We propose a method to design pulses in a resonant three-level system to enhance the robustness of non-adiabatic geometric gate operations. By optimizing the shape of the pulse envelope, we show that the gate operations are more robust against frequency detuning than they are with Gaussian and square pulses. Our method provides a way to design pulses that can be employed in a system where robustness against frequency variations or inhomogeneous broadening is required,and may be extended to ensure robustness against other physical imperfections such as intensity fluctuations and random noises.
The resonant filtering method transforming frequency modulated radiation field into a train of short pulses is proposed to apply in optical domain. Effective frequency modulation can be achieved by electro-optic modulator or by resonant frequency modulation of the filter with a narrow absorption line. Due to frequency modulation narrow-spectrum CW radiation field is seen by the resonant filter as a comb of equidistant spectral components separated by the modulation frequency. Tuning narrow-bandwidth filter in resonance with $n$-th spectral component of the comb transforms the radiation field i…
We study the quantum dynamics of a two-level system driven by a pulse that starts near-resonant for small amplitudes, yielding nonadiabatic evolution, and induces an adiabatic evolution for larger amplitudes. This problem is analyzed in terms of lifting of degeneracy for rising amplitudes. It is solved exactly for the case of linear and exponential rising. Approximate solutions are given in the case of power law rising. This allows us to determine approximative formulas for the lineshape of resonant excitation by various forms of pulses such as truncated trig-pulses. We also analyze and explai…
Photon echo schemes are excellent candidates for high efficiency coherent optical memory. They are capable of high-bandwidth multi-pulse storage, pulse resequencing and have been shown theoretically to be compatible with quantum information applications. One particular photon echo scheme is the gradient echo memory (GEM). In this system, an atomic frequency gradient is induced in the direction of light propagation leading to a Fourier decomposition of the optical spectrum along the length of the storage medium. This Fourier encoding allows precision spectral manipulation of the stored light. I…
We have investigated the analytical and numerical dynamics of entanglement for two qubits that interact with each other via Heisenberg XXX-type interaction and subject to local time-specific external kick and Gaussian pulse-type magnetic fields in x-y plane. The qubits have been assumed to be initially prepared in different pure separable and maximally entangled states and the effect of the strength and the direction of external fast pulses on concurrence has been investigated. The carefully designed kick or pulse sequences are found to enable one to obtain constant long-lasting entanglement w…
We study the dynamics of a two-level system driven by an off-resonant few-cycle pulse which has a phase jump $ϕ$ at $t=t_{0}$, in contrast to many cycle pulses, under non rotating-wave approximation (NRWA). We give a closed form analytical solution for the evolution of the probability amplitude $|C_{a} (t)|$ for the upper level. Using the appropriate pulse parameters like phase-jump $ϕ$, jump time $t_{0}$, pulse width $τ$, frequency $ν$ and Rabi frequency $Ω_{0}$ the population transfer, after the pulse is gone, can be optimized and for the pulse considered here, enhancement of $10^{6}-10^{8}$…
We have constructed a pulsed laser system for the manipulation of cold Rb atoms. The system combines optical telecommunications components and frequency doubling to generate light at 780 nm. Using a fast, fibre-coupled intensity modulator, output from a continuous laser diode is sliced into pulses with a length between 1.3 and 6.1 ns and a repetition frequency of 5 MHz. These pulses are amplified using an erbium-doped fibre amplifier, and frequency-doubled in a periodically poled lithium niobate crystal, yielding a peak power up to 12 W. Using the resulting light at 780 nm, we demonstrate Rabi…
We propose a new protocol to implement ultra-fast two-qubit phase gates with trapped ions using spin-dependent kicks induced by resonant transitions. By only optimizing the allocation of the arrival times in a pulse train sequence the gate is implemented in times faster than the trapping oscillation period $T<2π/ω$. Such gates allow us to increase the number of gate operations that can be completed within the coherence time of the ion-qubits favoring the development of scalable quantum computers.
We experimentally observe the action of multiple light pulses on the transverse motion of a continuous beam of fullerenes. The light potential is generated by non-resonant ultra-short laser pulses in perpendicular spatial overlap with the molecule beam. We observe a small but clear enhancement of the number of molecules in the center fraction of the molecular beam. Relatively low light intensity and short laser pulse duration prevent the molecule from fragmentation and ionization. Experimental results are confirmed by Monte Carlo trajectory simulations.
Machine Learning finds application in the quantum control and readout of qubits. In this work we apply Artificial Neural Networks to assist the manipulation and the readout of a prototypical molecular spin qubit - an Oxovanadium(IV) moiety - in two experiments designed to test the amplitude and the phase recognition, respectively. We first successfully use an artificial network to analyze the output of a Storage/Retrieval protocol with four input pulses to recognize the echo positions and, with further post selection on the results, to infer the initial input pulse sequence. We then apply an A…
We present a simple approach allowing to obtain analytical expressions for laser pulses that can drive a two-level system in an arbitrarily chosen way. The proposed scheme relates every desired population-evolution path to a single resonant laser pulse. It allows to drive the system from any initial superposition of the two states to a final state having the desired distribution of the populations. We exemplify the scheme with a concrete example, where the system is driven from a non-stationary superposition of states to one of its eigenstates. We argue that the proposed approach may have inte…
The three-electron configuration of gate-defined double quantum dots encodes a promising qubit for quantum information processing. I propose a two-qubit entangling gate using a pulse-gated manipulation procedure. The requirements for high-fidelity entangling operations are equivalent to the requirements for the pulse-gated single-qubit manipulations that have been successfully realized for Si QDs. This two-qubit gate completes the universal set of all-pulse-gated operations for the three-electron double-dot qubit and paves the way for a scalable setup to achieve quantum computation.
Existence of self-similar, superposed pulse-train solutions of the nonlinear, coupled Maxwell-Schrödinger equations, with the frequencies controlled by the oscillator strengths of the transitions, is established. Some of these excitations are specific to the resonant media, with energy levels in the configurations of $Λ$ and $N$ and arise because of the interference effects of cnoidal waves, as evidenced from some recently discovered identities involving the Jacobian elliptic functions. Interestingly, these excitations also admit a dual interpretation as single pulse-trains, with widely differ…
We have demonstrated that near complete coherence can be achieved in a four level double lambda-like systems using a train of ultra-short optical pulses. The effect of the Doppler broadening has been analyzed and a scheme has been proposed for establishing high and uniform coherence across different velocity groups in the atomic ensemble. We have also presented a novel scheme of excitation using chirped pulses and shown that in addition to generating coherence in the system it is possible to alter the translational states of the atoms.
Off-resonant error for a driven quantum system refers to interactions due to the input drives having non-zero spectral overlap with unwanted system transitions. For the cross-resonance gate, this includes leakage as well as off-diagonal computational interactions that lead to bit-flip error on the control qubit. In this work, we quantify off-resonant error, with more focus on the less studied off-diagonal control interactions, for a direct CNOT gate implementation. Our results are based on numerical simulation of the dynamics, while we demonstrate the connection to time-dependent Schrieffer-Wo…
Ultrachirped pulses for which the frequency chirp is of the order of the transition frequency of a two-level atom are examined. When the chirp is large enough, the resonance may be crossed twice, for positive and negative quadrature frequencies. In this scenario the analytic signal and quadrature decompositions of the field into amplitude and phase factors turn out to be quite different. The corresponding interaction pictures are strictly equivalent, but only as long as approximations are not applied. The domain of validity of the formal rotating wave approximation is dramatically enhanced usi…
Electro-optic time lenses are promising experimental components for photonic spectral-temporal processing of quantum information. We report a stable method to realize an electro-optic time lens, which relies on the amplification of an electronic response of a fast photodiode. The method does not require a repetitive clock and may be applied to aperiodic optical signals. We experimentally demonstrate the approach using single-photon pulses and directly verify its aperiodicity. The approach will enable construction of complex electro-optic temporal optical systems.
We investigate the evolution of extreme ultraviolet (XUV) spectral lineshapes in an optically-thick helium gas under near-infrared (IR) perturbation. In our experimental and theoretical work, we systematically vary the IR intensity, time-delay, gas density and IR polarization parameters to study lineshape modifications induced by collective interactions, in a regime beyond the single atom response of a thin, dilute gas. In both experiment and theory, we find that specific features in the frequency-domain absorption profile, and their evolution with propagation distance, can be attributed to th…
We report measurements of the time-dependent phases of the leak and retrieved pulses obtained in EIT storage experiments with metastable helium vapor at room temperature. In particular, we investigate the influence of the optical detuning at two-photon resonance, and provide numerical simulations of the full dynamical Maxwell-Bloch equations, which allow us to account for the experimental results.
We examine coherent memory manipulation in a $Λ$-type medium, using the second order solution presented by Groves, Clader and Eberly [J. Phys. B: At. Mol. Opt. Phys. 46, 224005 (2013)] as a guide. The analytical solution obtained using the Darboux transformation and a nonlinear superposition principle describes complicated soliton-pulse dynamics which, by an appropriate choice of parameters, can be simplified to a well-defined sequence of pulses interacting with the medium. In this report, this solution is reviewed and put to test by means of a series of numerical simulations, encompassing all…
An efficient technique to produce a periodic sequence of ultrashort pulses of recoilless gamma-radiation via its transmission through the optically thick vibrating resonant absorber was demonstrated recently [Nature, 508, 80 (2014)]. In this work we extend the theoretical analysis to the case of a set of multiple absorbers. We consider an analytical model describing the control of spectral content of a frequency modulated gamma-radiation by selective correction of amplitudes and initial phases of some spectral components, using, respectively, the resonant absorption or dispersion of nuclei. On…
Solutions to the Maxwell-Bloch equations for a $Λ$ system are computed using the single-soliton Darboux transformation and the nonlinear superposition principle. These allow complete control of information deposited by a signal pulse (with the help of an auxiliary control pulse) in the coherence of the medium's ground states by injecting sub-sequential pulses. Additionally, we study the encoding of two signal pulses and their manipulation by a control pulse and show that multipulse storage and control are possible as long as the imprints made by encoding the signal pulses are sufficiently sepa…
We consider a quantum processor based on five qutrits represented by spins S=1, which is driven by radio fre-quency (RF) pulses selective in transitions between adjacent levels. Numerical simulation of the implementation of the quantum-adiabatic clustering algorithm was performed on the example of partitioning a set of six points into three groups. We find the amplitudes and durations of rectangular RF pulses, as well as the durations of free evolu-tion intervals in the control pulse sequence, which made it possible to engineer a time-dependent effective Hamilto-nian in the discrete-time appro…
We describe a fast quantum computer based on optically controlled electron spins in charged quantum dots that are coupled to microcavities. This scheme uses broad-band optical pulses to rotate electron spins and provide the clock signal to the system. Non-local two-qubit gates are performed by phase shifts induced by electron spins on laser pulses propagating along a shared waveguide. Numerical simulations of this scheme demonstrate high-fidelity single-qubit and two-qubit gates with operation times comparable to the inverse Zeeman frequency.
We have considered theoretically the feasibility of the broadband quantum memory based on the resonant tripod-type atomic configuration. In this case, the writing of a signal field is carried out simultaneously into two channels, and characterized by an excitation of two spin waves of the atomic ensemble. With simultaneous read out from both channels quantum properties of the original signal are mapped on the retrieval pulse no worse than in the case of memory based on Lambda-type atomic configuration. At the same time new possibilities are opened up for manipulation of quantum states associat…
We demonstrate that the current laser technology used for field-free molecular alignment via a cascade of Raman rotational transitions allows for observing long-discussed non-linear quantum phenomena in the dynamics of the periodically kicked rotor. This includes the scaling of the absorbed energy near the conditions of quantum resonance and Anderson-like localisation in the angular momentum. Based on these findings, we suggest a novel approach to tunable selective rotational excitation and alignment in a molecular mixture, using trains of short laser pulses. We demonstrate the efficiency of t…
We demonstrate generation of a pulsed stream of electrically triggered single photons in resonance fluorescence, by applying high frequency electrical pulses to a single quantum dot in a p-i-n diode under resonant laser excitation. Single photon emission was verifed, with the probability of multiple photon emission reduced to 2.8%. We show that despite the presence of charge noise in the emission spectrum of the dot, resonant excitation acts as a filter to generate narrow bandwidth photons.
We report successful manipulation of non-classical atomic spin states. We generate squeezed spin states by a spin quantum nondemolition measurement, and apply an off-resonant circularly-polarized light pulse to the atoms. By changing the pulse duration, we have clearly observed a rotation of anisotropic quantum noise distribution in good contrast with the case of manipulation of a coherent spin state where the quantum noise distribution is always isotropic. This is an important step for quantum state tomography, quantum swapping, and precision spectroscopic measurement.
We present an analytical treatment of coherent excitation of a Two-Level Atom driven by a far-off resonant classical field. A class of pulse envelope is obtained for which this problem is exactly solvable. The solutions are given in terms of Heun function which is a generalization of the Hypergeometric function. The degeneracy of Heun to Hypergeometric equation can give all the exactly solvable pulse shapes of Gauss Hypergeometric form, from the generalized pulse shape obtained here. We discuss the application of the results obtained to the generation of XUV.
For neutral atom qubits, the residual thermal motion of the cold atoms constitutes a major challenge that limits the accessible two-qubit gate fidelity. Recently, an interesting type of two-qubit controlled-PHASE quantum gate protocol has been introduced for neutral atom qubit platform, which relies upon off-resonant modulated driving and Rydberg blockade effect. Building upon this progress, we have further developed an upgrade in the form of dual-pulse off-resonant modulated driving. Besides the inherent advantages of avoiding shelving population in Rydberg levels, not necessarily requiring i…
We discuss procedures for error-tolerant spin control in environments that permit transient, large-angle reorientation of magnetic bias field. Short sequences of pulsed, non-resonant magnetic field pulses in a laboratory-frame meridional plane are derived. These are shown to have band-pass excitation properties comparable to established amplitude-modulated, resonant pulses used in high, static-field magnetic resonance. Using these meridional pulses, we demonstrate robust $z$ inversion in proton ($^{1}$H) nuclear magnetic resonance near earth's field.
A dynamic quantum control of three-color lights in an optically dense medium is presented. We discuss how effectively to stop traveling three-color light pulses in the medium by using three control laser fields at near resonant transitions satisfying electromagnetically induced transparency. This opens a door to the quantum coherent control of multiple traveling light pulses for quantum memory and quantum switching, which are essential components in multi-party quantum optical communications.
We present a quantum manipulation of a traveling light pulse using double atomic coherence for two-color stationary light and quantum frequency conversion. The quantum frequency conversion rate of the traveling light achieved by the two-color stationary light phenomenon is near unity. We theoretically discuss the two-color stationary light for the frequency conversion process in terms of pulse area, energy transfer and propagation directions. The resulting process may apply the coherent interactions of a weak field to nonlinear quantum optics such as quantum nondemolition measurement.
The ability to enhance resonant signals and eliminate the non-resonant background is analyzed for Coherent Anti-Stokes Raman Scattering (CARS). The analysis is done at a specific frequency as well as for broadband excitation using femtosecond pulse-shaping techniques. An appropriate objective functional is employed to balance resonant signal enhancement against non-resonant background suppression. Optimal enhancement of the signal and minimization of the background can be achieved by shaping the probe pulse alone while keeping the pump and Stokes pulses in transform-limited-form (TLF). In some…
In this work, we demonstrate the use of frequency-tunable superconducting NbTiN coplanar waveguide microresonators for multi-frequency pulsed electron spin resonance (ESR) experiments. By applying a bias current to the center pin, the resonance frequency ($\sim$7.6 GHz) can be continuously tuned by as much as 95 MHz in 270 ns without a change in the quality factor of 3000 at 2K. We demonstrate the ESR performance of our resonators by measuring donor spin ensembles in silicon and show that adiabatic pulses can be used to overcome magnetic field inhomogeneities and microwave power limitations du…
We experimentally investigate the atom optics kicked particle at quantum resonance using finite duration kicks. Even though the underlying process is quantum interference it can be well described by an $ε$-pseudoclassical model. The $ε$-pseudoclassical model agrees well with our experiments for a wide range of parameters. We investigate the parameters yielding maximal momentum transfer to the atoms and find that this occurs in the regime where neither the short pulse approximation nor the Bragg condition is valid. Nonetheless, the momentum transferred to the atoms can be predicted using a simp…
A quasi-classical model (QCM) of molecular dynamics in intense femtosecond laser fields has been developed, and applied to a study of the effect of an ultrashort `control' pulse on the vibrational motion of a deuterium molecular ion in its ground electronic state. A nonadiabatic treatment accounts for the initial ionization-induced vibrational population caused by an ultrashort `pump' pulse. In the QCM, the nuclei move classically on the molecular potential as it is distorted by the laser-induced Stark shift and transition dipole. The nuclei then adjust to the modified potential, non-destructi…
A spatially-selective and internal-state-selective triggering pulse is an important component to realize the unitary dynamical state-locking process which may be used to realize the reversible and unitary halting protocol and construct the unstructured quantum search process based on the tensor-product Hilbert-space symmetric structure and the unitary quantum dynamics. In this paper it is shown how a spatially-selective and internal-state-selective triggering pulse is constructed generally in the quantum system of a single atom. Rigorous theoretical calculation and error estimation, which are …
The ability to coherently spectrally manipulate quantum information has the potential to improve qubit rates across quantum channels and find applications in optical quantum computing. In this paper we present experiments that use a multi-element solenoid combined with the three-level gradient echo memory scheme to perform precision spectral manipulation of optical pulses. These operations include bandwidth and frequency manipulation, spectral filtering of separate frequency components, as well as time-delayed interference between pulses with both the same, and different, frequencies. These op…
We report on time-resolved pulsed four-wave mixing (FWM) signals in a thermal Rubidium vapor involving a Rydberg state. We observe FWM signals with dephasing times up to 7 ns, strongly dependent on the excitation bandwidth to the Rydberg state. The excitation to the Rydberg state is driven by a pulsed two-photon transition on ns time scales. Combined with a third cw de-excitation laser, a strongly directional and collective emission is generated according to a combination of the phase matching effect and averaging over Doppler classes. In contrast to a previous report [1] using off-resonant FW…
Dynamic control of a weak quantum probe light pulse for the generation and quantum manipulations of a stationary multi-color (MC-) light field in a resonant coherent atomic medium using electromagnetically induced transparency is proposed. The manipulations have been analyzed based on the analytical solution of the adiabatic limit in the evolution of MC-light fields resulting from interaction of the slow probe light with the new fields generated in the nondegenerate multi-wave mixing scheme. We have found a critical stopping condition for the MC-light fields where the group velocity of light s…
We model the formation of stable heteronuclear molecules via pulsed Raman photoassociation of a two-component Bose-Einstein condensate near a strong Feshbach resonance, for both counterintuitive and intuitive pulse sequencing. Compared to lasers alone, weak Raman photoassociation is enhanced by as much as a factor of ten (five) for a counterintuitive (intuitive) pulse sequence, whereas strong Raman photoassociation is barely enhanced at all--regardless of pulse sequence. Stronger intra-atom, molecule, or atom-molecule collisions lead to an expected decrease in conversion efficiency, but strong…
Neutral atom array serves as an ideal platform to study the quantum logic gates, where intense efforts have been devoted to improve the two-qubit gate fidelity. We report our recent findings in constructing a different type of two-qubit controlled-PHASE quantum gate protocol with neutral atoms enabled by Rydberg blockade, which aims at both robustness and high-fidelity. It relies upon modulated driving pulse with specially tailored smooth waveform to gain appropriate phase accumulations for quantum gates. The major features include finishing gate operation within a single pulse, not necessaril…
We study the photoionization and autoionization of Helium atom subject to ultrashort laser pulses by using a Feshbach formalism in the time domain. We solve the time-dependent Schrödinger equation in terms of a configuration interaction (CI) spectral method, in which the total wavefunction is expanded with configurations defined within bound-like ($\mathcal{Q}$) and scattering-like ($\mathcal{P}$) halfspaces. The method allowsone to provide accurate descriptions of both the atomic structure (energy positions and widths) and the photodynamics. We illustrate our approach by i) calculating the ti…
Fiber guided optical signal propagating in a Erbium doped nonlinear resonant medium is known to produce cleaner solitonic pulse, described by the self induced transparency (SIT) coupled to nonlinear Schroedinger equation. We discover two new possibilities hidden in its integrable structure, for amplification and control of the optical pulse. Using the variable soliton width permitted by the integrability of this model, the broadening pulse can be regulated by adjusting the initial population inversion of the opant atoms. The effect can be enhanced by another innovative application of its const…
