Existence of self-similar, superposed pulse-train solutions of the nonlinear, coupled Maxwell-Schrödinger equations, with the frequencies controlled by the oscillator strengths of the transitions, is established. Some of these excitations are specific to the resonant media, with energy levels in the configurations of $Λ$ and $N$ and arise because of the interference effects of cnoidal waves, as evidenced from some recently discovered identities involving the Jacobian elliptic functions. Interestingly, these excitations also admit a dual interpretation as single pulse-trains, with widely different amplitudes, which can lead to substantially different field intensities and population densities in different atomic levels.
Using resonant interaction between atoms and the field in a high quality cavity, we show how to generate a superposition of many mesoscopic states of the field. We study the quasi-probability distributions and demonstrate the nonclassicality of the superposition in terms of the zeroes of the Q-function as well as the negativity of the Wigner function. We discuss the decoherence of the generated superposition state. We propose homodyne techniques of the type developed by Auffeves et al [Phys. Rev. Lett. 91, 230405 (2003)] to monitor the superposition of many mesoscopic states.
Nonlinear dynamics of establishment of electron-hole coherent superpositions states in graphene by multiphoton resonant excitation of interband transitions in laser fields is considered. The single-particle time dependent density matrix for such a quantized system is calculated in the multiphoton resonant approximation. The dependence of Rabi oscillations of Fermi-Dirac sea in graphene on the time, momentum, and photon number at multiphoton laser-excitation is analyzed.
We propose and analyze a scheme for "on demand" creation of coherent superposition of meta-stable states in a tripod-structured atom using frequency-chirped laser pulses. Negligible excitation of the atoms during the creation of the superposition states is a priority in our consideration. The underlying physics of the scheme is explained using the formalism of adiabatic states. By numerically solving master equation for the density matrix operator, we analyze the influence of the spontaneous decay and transverse relaxation on the efficiency of the creation of superposition states. We show that…
An interaction of electromagnetic field with a nanostructure composed of two quantum dots is studied theoretically. An effect of a resonant electron transfer between the localized low-lying states of quantum dots is predicted. A necessary condition for such an effect is the existence of an excited bound state whose energy lies close to the top of the barrier separating the quantum dots. This effect may be used to realize the reversible quantum logic gate NOT if the superposition of electron states in different quantum dots is viewed as the superposition of bits 0 and 1.
We present a simple approach allowing to obtain analytical expressions for laser pulses that can drive a two-level system in an arbitrarily chosen way. The proposed scheme relates every desired population-evolution path to a single resonant laser pulse. It allows to drive the system from any initial superposition of the two states to a final state having the desired distribution of the populations. We exemplify the scheme with a concrete example, where the system is driven from a non-stationary superposition of states to one of its eigenstates. We argue that the proposed approach may have inte…
We propose a scheme for creating atomic coherent superpositions via stimulated Raman adiabatic passage in a Lambda-type system where the final state has twofold levels. In the employ of a control field, the presence of double dark states leads to two arbitrary coherent superposition states with equal amplitude but inverse relative phase without the condition of multi-photon resonance. In particular, two orthogonal maximal coherent superposition states are created when the control field is resonant with the transition of the twofold levels. This scheme can also be extended to manifold Lambda-ty…
We propose measurement based conditional generation of superposition of motional states of nanomechanical resonator. We consider a two level quantum mechanical system coupled with nanomechanical resonator through phonon exchange. An interaction, which produces shifts in the state of nanomechanical resonator depending on the state of the qubit, is realized by driving qubit through two resonant lasers. The measurement of the state of quantum mechanical system produces superposition states of nanomechanical resonator. We show that the quantum interference between states in superposition may lead …
Well controlled nonlinear interactions between light field pulses and single atoms could be used to implement optical quantum information technologies based on qubits encoded in superpositions of coherent states of light. Here, we investigate the transformation of a coherent light field input at a single atom sufficiently far from resonance to limit the decoherence effects associated with random excitations of the atom. The conditions for suppressing multi-photon scattering to implement arbitrarily large shifts of the coherent light amplitude without decoherence are studied. It is shown that q…
In this chapter we review the use of semiconductor quantum dots as sources of quantum light. Principally, we focus on resonant two-photon excitation, which is a method that allows for on-demand generation of photon pairs. We explore the advantages of resonant excitation and present a number of measurements that were made in this excitation regime. In particular, we cover the following topics: photon statistics, coherent manipulation of the ground-excited state superposition, and generation of time-bin entangled photon pairs.
We derive analytic solution for pulsed frequency conversion based on electromagnetically induced transparency (EIT) or maximum coherence in resonant atomic vapors. In particular drive-field and coherence depletion are taken into account. The solutions are obtained with the help of an Hamiltonian approach which in the adiabatic limit allows to reduce the full set of Maxwell-Bloch equations to simple canonical equations of Hamiltonian mechanics for the field variables. Adiabatic integrals of motion can be obtained and general expressions for the spatio-temporal evolution of field intensities der…
The resonant interaction between x-ray photons and nuclei is one of the most exciting subjects of the burgeoning field of x-ray quantum optics. A resourceful platform used so far are thin-film x-ray cavities with embedded layers or Mössbauer nuclei such as $^{57}\mathrm{Fe}$. A new quantum optical model based on the classical electromagnetic Green's function is developed to investigate theoretically the nuclear response inside the x-ray cavity. The model is versatile and provides an intuitive picture about the influence of the cavity structure on the resulting spectra. We test its predictive p…
We study the quantum dynamics of a two-level system driven by a pulse that starts near-resonant for small amplitudes, yielding nonadiabatic evolution, and induces an adiabatic evolution for larger amplitudes. This problem is analyzed in terms of lifting of degeneracy for rising amplitudes. It is solved exactly for the case of linear and exponential rising. Approximate solutions are given in the case of power law rising. This allows us to determine approximative formulas for the lineshape of resonant excitation by various forms of pulses such as truncated trig-pulses. We also analyze and explai…
An efficient technique to produce a periodic sequence of ultrashort pulses of recoilless gamma-radiation via its transmission through the optically thick vibrating resonant absorber was demonstrated recently [Nature, 508, 80 (2014)]. In this work we extend the theoretical analysis to the case of a set of multiple absorbers. We consider an analytical model describing the control of spectral content of a frequency modulated gamma-radiation by selective correction of amplitudes and initial phases of some spectral components, using, respectively, the resonant absorption or dispersion of nuclei. On…
We consider the influence of the near dipole-dipole interaction, underlying the local field, on the dynamics of two-level and V-type three-level atoms exposed to cw-laser radiation. The dipole-dipole interaction between the V-type three-level atoms is shown to give rise to the Poincaré-Andronov-Hopf bifurcation in steady-state solution of the equations of motion. As a result, the populations of the energy levels periodically vary in time. In the framework of the two-level model, dynamical instabilities are proved to be impossible.
Resonant optical pumping in dense atomic media is discussed, where the absorption length is less than the smallest characteristic dimension of the sample. It is shown that reabsorption and multiple scattering of spontaneous photons (radiation trapping) can substantially slow down the rate of optical pumping. A very slow relaxation out of the target state of the pump process is then sufficient to make optical pumping impossible. As model systems an inhomogeneously and a radiatively broadened 3-level system resonantly driven with a strong broad-band pump field are considered.
Two dimensional materials are becoming increasingly popular as a platform for studies of quantum phenomena and for the production of prototype quantum technologies. Quantum emitters in 2D materials can host two level systems that can act as qubits for quantum information processing. Here, we characterize the behavior of position-controlled quantum emitters in hexagonal boron nitride at cryogenic temperatures. Over two dozen sites, we observe an ultra-narrow distribution of the zero phonon line at ~436 nm, together with strong linearly polarized emission. We employ resonant excitation to charac…
We demonstrate an efficient nonlinear process in which Stokes and anti-Stokes components are generated spontaneously in a Raman-like, near resonant media driven by low power counter-propagating fields. Oscillation of this kind does not require optical cavity and can be viewed as a spontaneous formation of atomic coherence grating.
Light propagation in disordered media is a fundamental and important problem in optics and photonics. In particular, engineering light-matter interaction in disordered cold atomic ensembles is one of the central topics in modern quantum and atomic optics. The collective response of dense atomic gases under light excitation, which crucially depends on the spatial distribution of atoms and the geometry of the ensemble, has important impacts on quantum technologies like quantum sensors, atomic clocks and quantum information storage. Here we analyze near-resonant light transmission in two-dimensio…
The ability to coherently couple arbitrary harmonic oscillators in a fully-controlled way is an important tool to process quantum information. Coupling between quantum harmonic oscillators has previously been demonstrated in several physical systems by use of a two-level system as a mediating element. Direct interaction at the quantum level has only recently been realized by use of resonant coupling between trapped ions. Here we implement a tunable direct coupling between the microwave harmonics of a superconducting resonator by use of parametric frequency conversion. We accomplish this by cou…
We consider adiabatic interaction of five-level atomic systems and their media with four short laser pulses under the condition of all two-photon detunings being zero. We derive analytical expressions for eigenvalues of the system's Hamiltonian and determine conditions of adiabaticity for both the atom and the medium. We analyse, in detail, the system's behaviour when the eigenvalue with non-vanishing energy is realized. As distinct from the usual dark state of a five-level system (corresponding to zero eigenvalue), which is a superposition of three states, in our case the superposition of fou…
Coherent nonlinear multi-pulse processes, nonlinear waves and echo effects in resonant media are the topical problems of modern optics and important tools of coherent spectroscopy and quantum information science. We generalize the McCall-Hahn area theorem to the formation of an arbitrary photon echo generated during the multi-pulse excitation of the optically dense resonant media. The derived theorem made it possible to reveal the nonlinear mechanism of generation and evolution of the photon echo signals inside the media after a two-pulse excitation. We find that a series of self-reviving echo…
