We analyzed the efficiency of coherent population trapping (CPT) in a superposition of the ground states of three-level atoms under the influence of the decoherence process induced by a broadband thermal field. We showed that in a single atom there is no perfect CPT when the atomic transitions are affected by the thermal field. The perfect CPT may occur when only one of the two atomic transitions is affected by the thermal field. In the case when both atomic transitions are affected by the thermal field, we demonstrated that regardless of the intensity of the thermal field the destructive effect on the CPT can be circumvented by the collective behavior of the atoms. An analytic expression was obtained for the populations of the upper atomic levels which can be considered as a measure of the level of thermal decoherence. The results show that the collective interaction between the atoms can significantly enhance the population trapping in that the population of the upper state decreases with increased number of atoms. The physical origin of this feature was explained by the semiclassical dressed atom model of the system. We introduced the concept of multiatom collective coherent population trapping by demonstrating the existence of collective (entangled) states whose storage capacity is larger than that of the equivalent states of independent atoms.
We experimentally demonstrate optical dipole trapping of a cloud of cold atoms by means of a dynamically coupled mode of a high-finesse cavity. We show that the trap requires a collective action of the atoms, i.e. a single atom would not be trapped under the same laser drive conditions. The atoms pull the frequency of the mode closer to resonance, thereby allowing the necessary light intensity for trapping into the cavity. The back-action of the atoms on the trapping light mode is also manifested by the non-exponential collapse of the trap.
We isolate a novel four-wave mixing process, enabled by Coherent Population Trapping (CPT), leading to efficient phase sensitive amplification. This process is permitted by the exploitation of two transitions starting from the same twofold degenerate ground state. One of the transitions is used for CPT, defining bright and dark states from which ultra intense four-wave mixing is obtained via the other transition. This leads to the measurement of a strong phase sensitive gain even for low optical densities and out-of-resonance excitation. The enhancement of four-wave mixing is interpreted in th…
We study phase-dependent fluctuations of the resonance fluorescence of a single $Λ$-type three-level atom in the regime near coherent population trapping, i.e., alongside the two-photon detuning condition. To this end, we employ the method of conditional homodyne detection (CHD) which considers squeezing in the weak driving regime, and extends to non-Gaussian fluctuations for saturating and strong fields. In this framework, and using estimated parameter settings of the resonance fluorescence of a single trapped $^{138} \mathrm{Ba}^{+}$ ion, the light scattered from the probe transitions is fou…
We propose a procedure to achieve a complete energy conversion between laser pulses carrying orbital angular momentum (OAM) in a cloud of cold atoms characterized by a double-Λatom-light coupling scheme. A pair of resonant spatially dependent control fields prepare atoms in a position-dependent coherent population trapping state, while a pair of much weaker vortex probe beams propagate in the coherently driven atomic medium. Using the adiabatic approximation we derive the propagation equations for the probe beams. We consider a situation where the second control field is absent at the entrance…
Coherent population trapping is a well-known quantum phenomenon in a driven $Λ$ system, with many applications across quantum optics. However, when a stochastic bath is present in addition to vacuum noise, the observed trapping is no longer perfect. Here we derive a time-convolutionless master equation describing the equilibration of the $Λ$ system in the presence of additional temporally correlated classical noise, with an unknown decay parameter. Our simulations show a one-to-one correspondence between the decay parameter and the depth of the characteristic dip in the photoluminescence spect…
Quantum computing with an inhomogeneously broadened ensemble of ions: Suppression of errors from detuning variations by specially adapted pulses and coherent population trapping
We consider a three-node fully connected network (Delta network) showing that a coherent population trapping phenomenon occurs, generalizing results for the Lambda network known to support a dark state. Transport in such structures provides signatures of detrapping, which can be triggered by external controls. In the presence of an environment it turns out to be sensitive to its Markovianity. Adiabatic modulation of the system's parameters may yield coherent population transfer, analogous to the stimulated Raman adiabatic passage phenomenon. Robustness of this protocol against non-adiabatic tr…
The coherent population trapping (CPT) effect is used for making compact atomic clocks. There are two types of CPT clocks: the one in which the Raman beams are applied continuously and the one in which two CPT pulses separated by a dark period are applied (Ramsey scheme). It is obvious that the technique of spin squeezing can only be applied to the Ramsey CPT clock to enhance the sensitivity. However, it is not apparent how to adapt to the CPT clock the protocols for the microwave clock using one-axis-twist squeezing (OATS), since the Ramsey CPT clock is not trivially equivalent to the Ramsey …
A novel protocol of interrogation based on coherent population trapping in an N-level scheme atomic system leads to dark resonances involving three different photons. An ensemble of several hundreds of radiofrequency-trapped ions is probed by three lasers simultaneously locked onto the same optical frequency comb, resulting in high-contrast spectral lines referenced to an atomic transition in the THz domain. We discuss the cause of uncertainties and limitations for this method and show that reaching a sub-kHz resolution is experimentally accessible via this interrogation protocole.
Electromagnetically induced transparency (EIT) is an optical phenomenon which allows a drastic modification of the optical properties of an atomic system by applying a control field. It has been largely studied in the last decades and nowadays we can find a huge number of experimental and theoretical related studies. Recently a similar phenomenon was also shown in quantum dot molecules (QDM) , where the control field is replaced by the tunneling rate between quantum dots. Our results show that in the EIT regime, the optical properties of QDM and the atomic system are identical. However, here w…
Coherent control of quantum systems has far-reaching implications in quantum engineering. In this context, coherent population trapping (CPT) involving dark resonances has played a prominent role, leading to a wealth of major applications including laser cooling of atoms and molecules, optical magnetometry, light storage and highly precise atomic clocks. Extending CPT methods to individual solid-state quantum systems has been only achieved in cryogenic environments for electron spin impurities and superconducting circuits. Here, we demonstrate efficient CPT of a single nuclear spin in a room t…
We propose and theoretically analyze the use of coherent population trapping of a single diamond nitrogen vacancy (NV) center for continuous real-time sensing. The formation of the dark state in coherent population trapping prevents optical emissions from the NV center. Fluctuating magnetic fields, however, can kick the NV center out of the dark state, leading to a sequence of single-photon emissions. A time series of the photon counts detected can be used for magnetic field estimations, even when the average photon count per update time interval is much smaller than 1. For a theoretical demon…
We analyze the properties of a pulsed Coherent Population Trapping protocol that uses a controlled decay from the excited state in a $Λ$-level scheme. We study this problem analytically and numerically and find regimes where narrow transmission, absorption, or fluorescence spectral lines occur. We then look for optimal frequency measurements using these spectral features by computing the Allan deviation in the presence of ground state decoherence and show that the protocol is on a par with Ramsey-CPT. We discuss possible implementations with ensembles of alkali atoms and single ions and demons…
Optical spin rotations and cycling transitions for measurement are normally incompatible in quantum dots, presenting a fundamental problem for quantum information applications. Here we show that for a hole spin this problem can be addressed using a trion with one hole in an excited orbital, where strong spin-orbit interaction tilts the spin. Then, a particular trion triplet forms a double $Λ$ system, even in a Faraday magnetic field, which we use to demonstrate fast hole spin initialization and coherent population trapping. The lowest trion transitions still strongly preserve spin, thus combin…
Magnetically induced coherent population trapping has been studied in a single trapped laser cooled ion. The magnetic field dependent narrow spectral feature is found to be an useful tool in determining the null point of magnetic field at the ion position. In particular, we use a double lambda scheme that allows us to measure the null magnetic field point limited by the detector shot noise. We analyzed the system theoretically and found certain long lived bright states as the dark state is generated under steady state condition.
Hybrid spin-optomechanical quantum systems offer high flexibility, integrability and applicability for quantum science and technology. Particularly, on-chip surface acoustic waves (SAWs) can efficiently drive spin transitions in the ground states (GSs) of atomic-scale, color centre qubits, which are forbidden in case of the more frequently used electromagnetic fields. Here, we demonstrate that strain-induced spin interactions within their optically excited state (ES) can exceed by two orders of magnitude the ones within the GS. This gives rise to novel physical phenomena, such as the acoustica…
Quantum interference is a natural consequence of wave-particle duality in quantum mechanics, and is widely observed at the atomic scale. One interesting manifestation of quantum interference is coherent population trapping (CPT), first proposed in three-level driven atomic systems and observed in quantum optical experiments. Here, we demonstrate CPT in a gate-defined semiconductor double quantum dot (DQD), with some unique twists as compared to the atomic systems. Specifically, we observe CPT in both driven and non-driven situations. We further show that CPT in a driven DQD could be used to ge…
Analysis of the frequency shift in coherent population trapping resonance's dynamic continuous-wave spectroscopy at the phase-jump modulation and its comparison with the conventional approach
P. N. Lebedev Physical Institute of the Russian Academy of Sciences（俄罗斯科学院列别杰夫物理研究所）
