We create entangled states of the spin and motion of a single $^{40}$Ca$^+$ ion in a linear ion trap. The motional part consists of coherent states of large separation and long coherence time. The states are created by driving the motion using counterpropagating laser beams. We theoretically study and experimentally observe the behaviour outside the Lamb-Dicke regime, where the trajectory in phase space is modified and the coherent states become squeezed. We directly observe the modification of the return time of the trajectory, and infer the squeezing. The mesoscopic entanglement is observed up to $Δα= 5.1$ with coherence time 170 microseconds and mean phonon excitation $\nbar = 16$.
A scheme for preparing Schrödinger cat (SC) states is proposed beyond the Lamb-Dicke limit in a Raman-$Λ$-type configuration. It is shown that SC states can be obtained more efficiently with our scheme than with the former ones.
First order Doppler effects are usually ignored in laser driven trapped ions when the recoil frequency is much smaller than the trapping frequency (Lamb-Dicke regime). This means that the central, carrier excitation band is supposed to be unaffected by vibronic transitions in which the vibrational number changes. While this is strictly true in the Lamb-Dicke limit (infinitely tight confinement), the vibronic transitions do play a role in the Lamb-Dicke regime. In this paper we quantify the asymptotic behaviour of their effect with respect to the Lamb-Dicke parameter. In particular, we give ana…
Based on the exact conditional quantum dynamics for a two-ion system, we propose an efficient {\it single-step} scheme for coherently manipulating quantum information of two trapped cold ions by using a pair of synchronous laser pulses. Neither the auxiliary atomic level nor the Lamb-Dicke approximation are needed.
A scheme to implement quantum logic gates by manipulating trapped ions through interaction with monochromatic external laser field and quantized cavity field, beyond the Lamb-Dicke regime, is presented. Characteristic times, for implementing ionic state transitions using non-resont laser pulse or quantized cavity field, shows a sharp decline for large Lamb-Dicke parameter value of $η_{L}=η_{c}=0.2$, and is seen to decrease further with increase in number of initial state vibrational quanta $m$.
We study laser cooling of two ions that are trapped in a harmonic potential and interact by Coulomb repulsion. Sideband cooling in the Lamb-Dicke regime is shown to work analogously to sideband cooling of a single ion. Outside the Lamb-Dicke regime, the incommensurable frequencies of the two vibrational modes result in a quasi-continuous energy spectrum that significantly alters the cooling dynamics. The cooling time decreases nonlinearly with the linewidth of the cooling transition, and the effect of trapping states which may slow down the cooling is considerably reduced. We show that cooling…
We investigate the dynamics of a cold trapped ion coupled to the quantized field inside a high-finesse cavity. We have used an approach for preparing the SC states of motion of ion. This approach, based on unitary transformating the Hamiltonian, allows its exact diagonalization without performing the Lamb-Dicke aproximation. We show that is possible to generate a SC states having rather simple initial state preparation, e.g., the vacuum sate for both cavity field and the ion motion.
Based on the conditional quantum dynamics of laser-ion interaction, we propose an efficient theoretical scheme to deterministically generate quantum pure states of a single trapped cold ion without performing the Lamb-Dicke approximation. An arbitrary quantum state can be created by using a series of classical laser beams with selected frequencies, initial phases and durations. As special examples, we further show how to create or approximate several typical macroscopic quantum states, such as the phase state and (even/odd) coherent states. Unlike previous schemes operated in the Lamb-Dicke re…
We propose a laser cooling scheme that allows to cool a single atom confined in a harmonic potential to the trap ground state $|0>$. The scheme assumes strong confinement, where the oscillation frequency in the trap is larger than the effective spontaneous decay width, but is not restricted to the Lamb-Dicke limit, i.e. the size of the trap ground state can be larger than the optical wavelength. This cooling scheme may be useful in the context of quantum computations with ions and Bose-Einstein condensation.
We present a robust quantum optimal control framework for implementing fast entangling gates on ion-trap quantum processors. The framework leverages tailored laser pulses to drive the multiple vibrational sidebands of the ions to create phonon-mediated entangling gates and, unlike the state of the art, requires neither weak-coupling Lamb-Dicke approximation nor perturbation treatment. With the application of gradient-based optimal control, it enables finding amplitude- and phase-modulated laser control protocols that work beyond the Lamb-Dicke regime, promising gate speed at the order of micro…
We propose a simple scheme for implementing quantum logic gates with a string of two-level trapped cold ions outside the Lamb-Dicke limit. Two internal states of each ion are used as one computational qubit (CQ) and the collective vibration of ions acts as the information bus, i.e., bus qubit (BQ). Using the quantum dynamics for the laser-ion interaction as described by a generalized Jaynes-Cummings model, we show that quantum entanglement between any one CQ and the BQ can be coherently manipulated by applying classical laser beams. As a result, universal quantum gates, i.e. the one-qubit rota…
In the dissipative quantum dynamics of a mesoscopic aggregate of excited two level systems (atoms) coupled to a single resonance mode of a cavity, two physical phenomena associated with superradiance appear. A pronounced emission peak on short time scales is related to the known superradiant burst of excited atoms cooperatively radiating into free space. It is followed by relaxation to a stationary state of the composite system such that for sufficiently large atom-field coupling a strongly correlated state emerges. The crossover to this state can be interpreted as the precursor of the transit…
Cavity-mediated cooling has the potential to become one of the most efficient techniques to cool molecular species down to very low temperatures. In this paper we analyse cavity cooling with single-laser driving for relatively large cavity decay rates kappa and relatively large phonon frequencies nu. It is shown that cavity cooling and ordinary laser cooling are essentially the same within the validity range of the Lamb-Dicke approximation. This is done by deriving a closed set of rate equations and calculating the corresponding stationary state phonon number and cooling rate. For example, whe…
For certain {\it specific} (or {\it"magic"}) Lamb-Dicke (LD) parameters, Monroe {\it et al} showed [Phys. Rev. {\bf A 55}, R2489 (1997)] that a two-qubit quantum operation, between the external and internal degrees of freedom of a single trapped ion, could be implemented by applying a single carrier laser pulse. Here, we further show that, such a two-qubit operation (which is equivalent to the standard CNOT gate, only apart from certain phase factors) could also be significantly-well realized for {\it arbitrarily} selected LD parameters. Instead of the so-called "$π$-pulses" used in the previo…
A simple alternative scheme for implementing quantum gates with a single trapped cold two-level ion beyond the Lamb-Dicke (LD) limit is proposed. Basing on the quantum dynamics for the laser-ion interaction described by a generalized Jaynes-Cummings model, one can introduce two kinds of elementary quantum operations i.e., the simple rotation on the bare atomic state, generated by applying a resonant pulse, and the joint operation on the internal and external degrees of the ion, performed by using an off-resonant pulse. Several typical quantum gates, including Hadamard gate, controlled-Z and co…
Kibble--Zurek Scaling in the Dicke Model at Mesoscopic Scales
Institute for Advanced Study, Tsinghua University（清华大学高等研究院）；Beijing Key Laboratory of Cold Atom Quantum Computation, Tsinghua University（清华大学冷原子量子计算北京市重点实验室）
We investigate the dynamics of cavity cooling of a single ion beyond the Lamb-Dicke regime and demonstrate a cooling limit of approximately 50% of the Doppler temperature using a high finesse cavity for the first time. We also study the statistical properties of the ion-cavity emission and present a model that maps the phonon states to the photon states. With this model, we explain the super-Poissonian photon distribution observed in our experiments and propose a method to estimate the ion temperature in a real-time manner based on the statistical behavior of the photon emission from the cavit…
We apply wave packet methods to study an ion-trap system in the strong excitation regime imposing neither the rotating wave nor the Lamb-Dicke approximations. By this approach we show the existence of states with restricted phase space evolution, as a genuine consequence of quantum interference between wave packet fractions. A particular instance of such a state oscillates between maximal entanglement and pure disentanglement between the constitute subsystems. The characteristic crossover time is very rapid making them suitable for state preparations of EPR or Schrodinger cat states. Over long…
We report continuous Raman sideband cooling (CRSC) of a long ion chain to the motional ground state beyond the Lamb-Dicke (LD) regime. By driving multiple sideband transitions simultaneously, we show that nearly all axial modes of a 24-ion chain are cooled to the ground state, with an LD parameter as large as $η= 1.3$, spanning a frequency bandwidth of 4 MHz. Compared to traditional ground-state cooling methods such as pulsed sideband cooling or electromagnetic-induced-transparency (EIT) cooling, our method offers two key advantages: robustness to timing errors; and an ultra-wide bandwidth unl…
We present the results of simulations of optical sideband cooling of atomic ions in a trap with a shallow potential well. In such traps, an ion cannot be Doppler cooled near to the Lamb-Dicke regime ($η^2(2n+1) \ll 1$). Outside the Lamb-Dicke regime, the sideband cooling dynamics are altered by the existence of various Fock states where the cooling becomes very slow. A calcium ion trapped in our Penning trap realises such a situation, hence single stage cooling is inefficient to prepare the ion in the motional ground state. For these systems, it is necessary to study the cooling dynamics in de…
We study the counterpart to the multi-photon down conversion in the quantised motion of a trapped atom. The Lamb-Dicke approximation leads to a divergence of the mean motional excitation in a finite interaction time for k-quantum down conversions with k>=3, analogous to the situation in the parametric approximation of nonlinear optics. We show that, in contrast to the Lamb-Dicke approximation, the correct treatment of the overlap of the atomic center-of-mass wave function and the driving laser waves leads to a proper dynamics without any divergence problem. That is, the wavy nature of both mat…
Sympathetic cooling of trapped ions has been established as a powerful technique for manipulation of non-laser-coolable ions (Raizen1992,Waki1992,Bowe1999,Barrett2003). For molecular ions, it promises vastly enhanced spectroscopic resolution and accuracy. However, this potential remains untapped so far, with the best resolution achieved being not better than $5\times10^{-8}$ fractionally, due to residual Doppler broadening being present in ion clusters even at the lowest achievable translational temperatures (Bressel2012). Here we introduce a general and accessible approach that enables Dopple…
We propose and demonstrate a scheme for strongly radially confining a single neutral atom in a bichromatic far-off resonance optical dipole trap(BFORT) . BFORT is composed of a blue-detuned Laguerre-Gaussian $LG^1_ 0$ beam and a red-detuned Gaussian beam. The trapping radial dimension of a single atom trapped in the Gaussian FORT can be greatly compressed by imposing a blue-detuned Laguerre-Gaussian $LG^1_ 0$ beam with moderate potential depth. By modulating the potential depth of the Gaussian FORT we observed that the resonant and parametric excitation of the oscillatory motion of a single at…
We propose a fast and efficient technique to create classes of highly entangled states of trapped ions, such as arbitrary Dicke states and superpositions of them, e.g. NOON states. The ions are initialized in the phonon ground state and are addressed globally with a composite pulse that is resonant with the first motional sideband. The technique operates on comparatively short time scales, as resonant interactions allow one to use the minimum laser pulse area. The number of single pulses from the composite sequence is equal to the number of ions, thus the implementation complexity grows only l…
We have investigated the efficiency of pulsed Raman sideband cooling in the presence of multiple decay and excitation channels. By applying sum rules we identify parameter regimes in which multiple scattering of photons can be described by an effective wave vector. Using this method we determine the rate of heating caused by optical pumping inside and outside the Lamb-Dicke regime. On this basis we discuss also the efficiency of a recently proposed scheme for ground-state cooling outside the Lamb-Dicke regime [G. Morigi, J.I. Cirac, M. Lewenstein, and P. Zoller, Europhys. Lett. {\bf 39}, 13 (1…
Implementations of solid state quantum optics provide us with devices where qubits are placed at fixed positions in photonic or plasmonic one dimensional waveguides. We show that solely by controlling the position of the qubits and with the help of a coherent driving, collective spontaneous decay may be engineered to yield an entangled mesoscopic steady-state. Our scheme relies on the realization of pure superradiant Dicke models by a destructive interference that cancels dipole-dipole interactions in one-dimension.
We discuss continuous observation of the momentum of a single atom by employing the high velocity sensitivity of the index of refraction in a driven $Λ$-system based on electromagnetically induced transparency (EIT). In the ideal limit of unit collection efficiency this provides a quantum limited measurement with minimal backaction on the atomic motion. A feedback loop, which drives the atom with a force proportional to measured signal, provides a cooling mechanism for the atomic motion. We derive the master equation which describes the feedback cooling and show that in the Lamb-Dicke limit th…
We propose a scalable design of entangling quantum gates for large ion crystals with the following desirable features: 1) The gate design is universal and applicable for large ion crystals of arbitrary sizes; 2) The gate has no speed limitation and can work outside of the Lamb-Dicke region; 3) The gate operates by driving from either continuous-wave or pulsed laser beams; 4) The gate is insensitive to slow variation of the laser optical phase and works under a thermal state for the ions' motion; 5) The intrinsic gate infidelity can be reduced to a level well below the threshold for fault-toler…
Trapped ion in the Lamb-Dicke regime with the Lamb-Dicke parameter $η\ll1$ can be cooled down to its motional ground state using sideband cooling. Standard sideband cooling works in the weak sideband coupling limit, where the sideband coupling strength is small compared to the natural linewidth $γ$ of the internal excited state, with a cooling rate much less than $γ$. Here we consider cooling schemes in the strong sideband coupling regime, where the sideband coupling strength is comparable or even greater than $γ$. We derive analytic expressions for the cooling rate and the average occupation …
A review of coherent and collective quantum optical effects like superradiance and coherent population trapping in mesoscopic systems is presented. Various new physical realizations of these phenomena are discussed, with a focus on their role for electronic transport and quantum dissipation in coupled nano-scale systems like quantum dots. A number of theoretical tools such as Master equations, polaron transformations, correlation functions, or level statistics are used to describe recent work on dissipative charge qubits (double quantum dots), the Dicke effect, phonon cavities, single oscillat…
We present an effective method of coherent state superposition (cat state) generation using single trapped ion in a Paul trap. The method is experimentally feasible for coherent states with amplitude $α\le 2$ using available technology. It works both in and beyond the Lamb-Dicke regime.
Using the exact eigenstates of the inhomogeneous Dicke model obtained by numerically solving the Bethe equations, we study the decay of bosonic excitations due to the coupling of the mode to an ensemble of two-level (spin 1/2) systems. We compare the quantum time-evolution of the bosonic mode population with the mean field description which, for a few bosons agree up to a relatively long Ehrenfest time. We demonstrate that additional excitations lead to a dramatic shortening of the period of validity of the mean field analysis. However, even in the limit where the number of bosons equal the nu…
We show that in the trapped ion-laser interaction all the regimes may be considered analytically. We may solve not only for different laser intensities, but also away from resonance and from the Lamb-Dicke regime. It is found a dispersive Hamiltonian for the high intensity regime, that, being diagonal, its evolution operator may be easily calculated.
The Raman interaction of a trapped ultracold ion with two travelling wave lasers is studied analytically with series solutions, in the absence of the rotating wave approximation (RWA) and the restriction of both the Lamb-Dicke limit and the weak excitation regime. The comparison is made between our solutions and those under the RWA to demonstrate the validity region of the RWA. As a practical example, the preparation of Schrödinger-cat states with our solutions is proposed beyond the weak excitation regime.
Recent experiments [K. R. Brown, et al., Nature 471, 196 (2011); and M. Harlander, et al., Nature 471, 200 (2011)] have demonstrated the coherent manipulations on the external vibrations of two ions, confined individually in the separated ion traps. Using these recently developed techniques, we propose here an approach to realize the coherent operations, e.g., the universal quantum gates, between the separated ion-trap qubits encoded by two internal atomic states of the trapped ions. Our proposal operates beyond the usual Lamb-Dicke limits, and could be applied to the scalable ion traps couple…
A method for gaining information about the phonon-number moments and the generalized nonlinear and linear quadratures in the motion of trapped ions (in particular, position and momentum) is proposed, valid inside and outside the Lamb-Dicke regime. It is based on the measurement of first time derivatives of electronic populations, evaluated at the motion-probe interaction time t=0. In contrast to other state-reconstruction proposals, based on measuring Rabi oscillations or dispersive interactions, the present scheme can be performed resonantly at infinitesimal short motion-probe interaction tim…
In this contribution we investigate the interaction of a single ion in a trap with laser beams. Our approach, based on unitary transformating the Hamiltonian, allows its exact diagonalization without performing the Lamb-Dicke approximation. We obtain a transformed Jaynes-Cummings type Hamiltonian, and we demonstrate the existence of super-revivals in that system.
We present a second-order perturbative analysis of the model describing a two-level trapped ion interacting with a traveling laser field, in the Lamb-Dicke regime. Unlike the customary approach, based on the interaction picture and the rotating wave approximation, we reduce the original Hamiltonian to a time-independent model, unitarily equivalent to a spin-boson model, which features a form well suited to apply the perturbation theory. We determine the first and second-order corrections of eigenstates and eigenvalues. By varying the interaction parameters we identify four regimes characterize…
We give a detailed description of the implementation of a Molmer-Sorensen gate entangling two Ca+ ions using a bichromatic laser beam near-resonant with a quadrupole transition. By amplitude pulse shaping and compensation of AC-Stark shifts we achieve a fast gate operation without compromising the error rate. Subjecting different input states to concatenations of up to 21 individual gate operations reveals Bell state fidelities above 0.80. In principle, the entangling gate does not require ground state cooling of the ions as long as the Lamb-Dicke criterion is fulfilled. We present the first e…
Quantum communication over long distances relies on the ability to create entanglement between two remote quantum nodes. Recent proposals aiming at experimental realization propose a hybrid quantum repeater setup where two distant material qubits are entangled by light-matter interaction. Motivated by these developments, we investigate possible decoherence effects originating from the centre- of-mass motion of the spatially well separated trapped qubits. Within the Lamb-Dicke regime we use photon exchange involving coherent states of the radiation field to entangle the two material qubits. Opt…
We study the quantum dynamics of an ion confined in a radiofrequency trap in interaction with either a Bose or spin-polarized Fermi gas. To this end, we derive quantum optical master equations in the limit of weak coupling and the Lamb-Dicke approximations. For the bosonic bath, we also include the so-called "Lamb-shift" correction to the ion trap due to the coupling to the quantum gas as well as the extended Fröhlich interaction within the Bogolyubov approximation that have been not considered in previous studies. We calculate the ion kinetic energy for various atom-ion scattering lengths as …
We sense the motion of a trapped atomic ion using a sequence of state-dependent ultrafast momentum kicks. We use this atom interferometer to characterize a nearly-pure quantum state with $n=1$ phonon and accurately measure thermal states ranging from near the zero-point energy to $\bar{n}\sim 10^4$, with the possibility of extending at least 100 times higher in energy. The complete energy range of this method spans from the ground state to far outside of the Lamb-Dicke regime, where atomic motion is greater than the optical wavelength. Apart from thermometry, these interferometric techniques a…
We present a family of generalized unitary transformations that simplifies the Hamiltonian for a harmonically trapped two level atom (or ion) interacting with a plane wave laser field. Novel near resonant single as well as double vibrational phonon dynamical regimes are found. The validity condition of the often used motional rotating wave approximation (MRWA) is examined both numerically and analytically. Large errors are found within typical regimes of MRWA with respect to the motional degrees of freedom. The effects of MRWA in trapped ion systems are shown to be opposite to that of the rota…
Pulsed lasers offer significant advantages over CW lasers in the coherent control of qubits. Here we review the theoretical and experimental aspects of controlling the internal and external states of individual trapped atoms with pulse trains. Two distinct regimes of laser intensity are identified. When the pulses are sufficiently weak that the Rabi frequency $Ω$ is much smaller than the trap frequency $\otrap$, sideband transitions can be addressed and atom-atom entanglement can be accomplished in much the same way as with CW lasers. By contrast, if the pulses are very strong ($Ω\gg \otrap$),…
