A quantum repeater at telecommunications wavelengths with long-lived atomic memory is proposed, and its critical elements are experimentally demonstrated using a cold atomic ensemble. Via atomic cascade emission, an entangled pair of 1530 nm and 780 nm photons is generated. The former is ideal for long-distance quantum communication, and the latter is naturally suited for mapping to a long-lived atomic memory. Together with our previous demonstration of photonic-to-atomic qubit conversion, both of the essential elements for the proposed telecommunications quantum repeater have now been realized.
We report experimental storage and retrieval of weak coherent states of light at telecommunication wavelengths using erbium ions doped into a solid. We use two photon echo based quantum storage protocols. The first one is based on controlled reversible inhomogeneous broadening (CRIB). It allows the retrieval of the light on demand by controlling the collective atomic coherence with an external electric field, via the linear Stark effect. We study how atoms in the excited state affect the signal to noise ratio of the CRIB memory. Additionally we show how CRIB can be used to modify the temporal …
The superradiant emission properties from an atomic ensemble with cascade level configuration is numerically simulated. The correlated spontaneous emissions (signal then idler fields) are purely stochastic processes which are initiated by quantum fluctuations. We utilize the positive-P phase space method to investigate the dynamics of the atoms and counter-propagating emissions. The light field intensities are calculated, and the signal-idler correlation function is studied for different optical depths of the atomic ensemble. Shorter correlation time scale for a denser atomic ensemble implies …
The ladder configuration of atomic levels provides a source for telecom photons (signal) from the upper atomic transition. \ For rubidium and cesium atoms, the signal field has the range around 1.3-1.5 $μ$m that can be coupled to an optical fiber and transmitted to a remote location. \ Cascade emission may result in pairs of photons, the signal entangled with the subsequently emitted infrared photon (idler) from the lower atomic transition.\ This correlated two-photon source is potentially useful in the (Duan-Lukin-Cirac-Zoller) DLCZ protocol for the quantum repeater.\ We implement the cascade…
We investigate superradiant cascade emissions from an atomic ensemble driven by two-color classical fields. The correlated pair of photons (signal and idler) is generated by adiabatically driving the system with large-detuned light fields via four-wave mixing. The signal photon from the upper transition of the diamond-type atomic levels is followed by the idler one which can be superradiant due to light-induced dipole-dipole interactions. We then calculate the cooperative Lamb shift (CLS) of the idler photon, which is a cumulative effect of interaction energy.We study its dependence on a cylin…
We investigate the spectral properties of the biphoton state from the cascade emissions of cold atomic ensembles, which composes of a telecommunication photon (signal) followed by an infrared one (idler) via four-wave mixing.\ With adiabatic conditions for Gaussian driving pulses of width $τ$, the spectrum of the biphoton state has the form of a Gaussian that conserves signal and idler photon energies within $\hbar/τ$ modulated by a Lorentzian with a superradiant linewidth.\ Multiplexing the atomic ensembles with frequency-shifted cascade emissions, we may manipulate and shape the spectrum of …
We characterize a source of photon pairs based on cascade decay in a cold Rb-87 ensemble. This source is particularly suited to generate of photons for interaction with Rb-87 based atomic systems. We experimentally investigate the dependence of pair generation rate, single photon heralding efficiency, and bandwidth as a function of the number of atoms, detuning and intensity of the pump beams. The observed power and detuning behaviors can be explained by the steady state solution of an established three-level model of an atom. Measurements presented here provide a useful insight on the optimiz…
Large-scale quantum networks will employ telecommunication-wavelength photons to exchange quantum information between remote measurement, storage, and processing nodes via fibre-optic channels. Quantum memories compatible with telecommunication-wavelength photons are a key element towards building such a quantum network. Here, we demonstrate the storage and retrieval of heralded 1532 nm-wavelength photons using a solid-state waveguide quantum memory. The heralded photons are derived from a photon-pair source that is based on parametric down-conversion, and our quantum memory is based on a 6 GH…
We report an experiment demonstrating quantum frequency conversion of weak light pulses compatible with atomic quantum memories to telecommunication wavelengths. We use a PPLN nonlinear waveguide to convert weak coherent states at the single photon level with a duration of 30ns from a wavelength of 780nm to 1552nm. We measure a maximal waveguide internal (external) conversion efficiency eta_int = 0.41 (eta_ext = 0.25), and we show that the signal to noise ratio (SNR) is good enough to reduce the input photon number below 1. In addition, we show that the noise generated by the pump beam in the …
We theoretically investigate the spectral property of biphoton state from the cascade emissions from a Doppler-broadened atomic ensemble. This biphoton state is spontaneously created in the four-wave-mixing process. The upper transition of the emissions lies in telecom bandwidth, which prevails in fiber-based quantum communication for low-loss transmission. We obtain the spectral property in terms of superradiant decay rates of the lower transition, excitation pulse durations, and temperature of the medium. We quantify their frequency entanglement by Schmidt decomposition and find that more en…
In this thesis, we investigate the quantum mechanical interaction of light with matter in the form of a gas of ultracold atoms: the atomic ensemble. We present a theoretical analysis of two problems, which involve the interaction of quantized electromagnetic fields (called signal and idler) with the atomic ensemble (i) cascade two-photon emission in an atomic ladder configuration, and (ii) photon frequency conversion in an atomic diamond configuration. The motivation of these studies comes from potential applications in long-distance quantum communication where it is desirable to generate quan…
Quantum networks will enable a variety of applications, from secure communication and precision measurements to distributed quantum computing. Storing photonic qubits and controlling their frequency, bandwidth and retrieval time are important functionalities in future optical quantum networks. Here we demonstrate these functions using an ensemble of erbium ions in yttrium orthosilicate coupled to a silicon photonic resonator and controlled via on-chip electrodes. Light in the telecommunication C-band is stored, manipulated and retrieved using a dynamic atomic frequency comb protocol controlled…
The efficient storage and on-demand retrieval of quantum optical states that are compatible with the telecommunications C-band is a requirement for future terrestrial-based quantum optical networking. Spectrum in the C-band minimises optical fiber-propagation losses, and broad optical bandwidth facilitates high-speed networking protocols. Here we report on a telecommunication wavelength and bandwidth compatible quantum memory. Using the Off-Resonant Cascaded Absorption protocol in hot $^{87}$Rb vapour, we demonstrate a total memory efficiency of $20.90(1)\,\%$ with a Doppler-limited storage ti…
Quantum memories for light are important components for future long distance quantum networks. We present on-chip quantum storage of telecommunications band light at the single photon level in an ensemble of erbium-167 ions in an yttrium orthosilicate photonic crystal nanobeam resonator. Storage times of up to 10 $μ$s are demonstrated using an all-optical atomic frequency comb protocol in a dilution refrigerator under a magnetic field of 380 mT. We show this quantum storage platform to have high bandwidth, high fidelity, and multimode capacity, and we outline a path towards an efficient erbium…
Bell's theorem of 1965 is a proof that all realistic interpretations of quantum mechanics must be non-local. Bell's theorem consists of two parts: first a correlation inequality is derived that must be satisfied by all local realistic theories; second it is demonstrated that quantum mechanical probabilities violate this inequality in certain cases. In the case of ideal experiments, Bell's theorem has been proven. However, in the case of real experiments where polarizers and detectors are non-ideal, the theorem has not yet been proven since the proof always requires some arbitrary and {\em ad h…
The dynamics of a three-level atom in a cascade configuration with both transitions coupled to a single structured reservoir of quantized field modes is treated using Laplace transform methods applied to the coupled amplitude equations. Results are also obtained from master equations by two different approaches, that is, involving either pseudomodes or quasimodes. Two different types of reservoir are considered, namely a high-Q cavity and a photonic band-gap system, in which the respective reservoir structure functions involve Lorentzians. Non-resonant transitions are included in the model. In…
A correlation inequality is derived from local realism and a supplementary assumption. This inequality is violated by a factor of 1.5 in the case of real experiments, whereas previous inequalities such as Clauser-Horne-Shimony-Holt inequality of 1969 and Clauser-Horne inequality of 1974 are violated by a factor of $\sqrt 2$. Thus the magnitude of violation of this inequality is approximately 20.7% larger than the magnitude of violation of previous inequalities. Moreover, the present inequality can be used to test locality very simply because it requires the measurements of only two detection p…
The cascade-emitted biphotons generated from the alkali metal atomic ensembles are an excellent entanglement resource which enables long-distance quantum communication. The communication of quantum information between distant locations can be realized by utilizing the low-loss telecom bandwidth in the upper transition of the cascaded photons in a fiber-based quantum network. Meanwhile, the infrared photon from the lower transition of this highly directional and frequency-correlated biphoton can be created under the four-wave mixing process and can be stored locally as a collective spin wave. H…
A hybrid interface of solid state single-photon sources and atomic quantum memories is a long sought-after goal in photonic quantum technologies. Here we demonstrate deterministic storage and retrieval of photons from a semiconductor quantum dot in an atomic ensemble quantum memory at telecommunications wavelengths. We store single photons from an InAs quantum dot in a high-bandwidth rubidium vapour based quantum memory, with a total internal memory efficiency of $(12.9 \pm 0.4) \%$. The signal-to-noise ratio of the retrieved photons is $18.2\pm 0.6$, limited only by detector dark counts. This…
We present a quantum repeater scheme that is based on individual erbium and europium ions. Erbium ions are attractive because they emit photons at telecommunication wavelength, while europium ions offer exceptional spin coherence for long-term storage. Entanglement between distant erbium ions is created by photon detection. The photon emission rate of each erbium ion is enhanced by a microcavity with high Purcell factor, as has recently been demonstrated. Entanglement is then transferred to nearby europium ions for storage. Gate operations between nearby ions are performed using dynamically co…
The distribution of quantum states over long distances is limited by photon loss. Straightforward amplification as in classical telecommunications is not an option in quantum communication because of the no-cloning theorem. This problem could be overcome by implementing quantum repeater protocols, which create long-distance entanglement from shorter-distance entanglement via entanglement swapping. Such protocols require the capacity to create entanglement in a heralded fashion, to store it in quantum memories, and to swap it. One attractive general strategy for realizing quantum repeaters is b…
We demonstrate laser frequency stabilization to excited state transitions using cascade electromagnetically induced transparency (EIT). Using a room temperature Rb vapor cell as a reference, we stabilize a first diode laser to the D2 transition and a second laser to a transition from the intermediate state to a Rydberg state with principal quantum number n=19 - 70. A combined laser linewidth of 280 kHz over a 0.1 ms time period is achieved. This method may be applied generally to any cascade system and allows laser stabilization to an atomic reference in the absence of strong optical transitio…
Interfacing fundamentally different quantum systems is key to build future hybrid quantum networks. Such heterogeneous networks offer superior capabilities compared to their homogeneous counterparts as they merge individual advantages of disparate quantum nodes in a single network architecture. However, only very few investigations on optical hybrid-interconnections have been carried out due to the high fundamental and technological challenges, which involve e.g. wavelength and bandwidth matching of the interfacing photons. Here we report the first optical quantum interconnection between two d…
We demonstrate the coherent transport of two-dimensional (2D) arrays of small ensembles of neutral atoms in a shift register architecture based on 2D arrays of microlenses. We show the scalability of the transport process by presenting the repeated hand-over of atoms from site to site. We prove the conservation of coherence during transport, reloading, and a full shift register cycle. This shows that the fundamental shift sequence can be cascaded and thus scaled to complex and versatile 2D architectures for atom-based quantum information processing, quantum simulation, and the investigation of…
Entanglement is the fundamental characteristic of quantum physics. Large experimental efforts are devoted to harness entanglement between various physical systems. In particular, entanglement between light and material systems is interesting due to their prospective roles as "flying" and stationary qubits in future quantum information technologies, such as quantum repeaters and quantum networks. Here we report the first demonstration of entanglement between a photon at telecommunication wavelength and a single collective atomic excitation stored in a crystal. One photon from an energy-time ent…
We propose a super-resolution quantum lithography scheme based on coherent population trapping in lambda-type atoms coupled to temporally-cascaded standing-wave driving fields. By realizing effective multiplication of optical intensity profiles on an atomic state density distribution, the scheme enables an arbitrarily high degree of resolution enhancement without modifying the atomic level structure of the photographic medium or the light source configuration. It is also shown that the visibility of the super-resolution patterns is preserved under a significant atomic state decoherence rate.
We report on experiments demonstrating the reversible mapping of heralded single photons to long lived collective optical atomic excitations stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely non-degenerate narrow-band ($\approx 2\,\mathrm{MHz}$) photon-pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr$^{3+}$ transition. The signal photons are stored and retrieved using the atomic frequency comb pr…
Superradiant lasers based on atomic ensembles exhibiting ultra-narrow optical transitions can emit light of unprecedented spectral purity and may serve as active atomic clocks. We consider two frequency-detuned active atomic clocks, which are coupled in a cascaded setup, i.e. as master & slave lasers, and study the synchronization of the slave to the master clock. In a setup where both atomic ensembles are coupled to a common cavity mode such synchronization phenomena have been predicted by Xu et al. [Phys. Rev. Lett. 113, 154101 (2014)] and experimentally observed by Weiner et al. [arXiv:1503…
Quantum repeaters based on heralded entanglement require quantum nodes that are able to generate multimode quantum correlations between memories and telecommunication photons. The communication rate scales linearly with the number of modes, yet highly multimode quantum storage remains challenging. In this work, we demonstrate an atomic frequency comb quantum memory with a time-domain mode capacity of 1250 modes and a bandwidth of 100 MHz, to our knowledge the largest number of modes stored in the quantum regime. The memory is based on a $Y_{2}SiO_{5}$ crystal doped with $^{171}Yb^{3+}$ ions, w…
Non-classical multi-photon and number states attracts many people because of their wide applications in fundamental quantum mechanics tests, quantum metrology and quantum computation, therefore it is a longstanding aim to generate such states experimentally. Here, we prepare photon triplets by using the spontaneously Raman scattering process in a hot atomic ensemble cascaded by the spontaneous parametric down conversion process in a periodical poled nonlinear waveguide, the strong temporal correlations of these three photons are observed. Our experiment represents the first combination of the …
Multipartite entanglement plays an important role in quantum information processing and quantum metrology. Here, the dressing-energy-level-cascaded (DELC) four-wave mixing (FWM) processes are proposed to generate all-optical controlled multipartite entanglement within a single device. The entanglement characteristics of the produced states of light are characterized by applying the Duan criterion and the positivity under partial transposition criterion. Moreover, by using an internal dressing field to modulate atomic coherence, multiple quantum coherent channels of FWM are simultaneously const…
Bright, entangled multiphoton sources based on atom photon interactions are an essential requirement in the realization of several quantum information and quantum computation schemes based on photonic quantum systems. Here, we experimentally demonstrate a four photon polarization entangled GHZ state obtained from Doppler broadened atomic ensembles of 87Rb atoms. Owing to collective two photon coherence in the Doppler broadened cascade-type atomic system, our setup enables the generation of robust four photon GHZ states with a fidelity of 0.82 and a measured four photon average coincidence rate…
Interference effects in quantum transitions, giving rise to amplification without inversion, optical transparency and to enhancements in nonlinear optical frequency conversions are considered. Review of the relevant early theoretical and experimental results is given. The role of relaxation processes, spontaneous cascade of polarizations, local field effects, Doppler-broadening, as well as specific features of the interference in the spectral continuum are discussed.
Photon-based quantum information processing promises new technologies including optical quantum computing, quantum cryptography, and distributed quantum networks. Polarization-encoded photons at telecommunication wavelengths provide a compelling platform for practical realization of these technologies. However, despite important success towards building elementary components compatible with this platform, including sources of entangled photons, efficient single photon detectors, and on-chip quantum circuits, a missing element has been atomic quantum memory that directly allows for reversible m…
We study in this paper the efficiency of different two-photon states of light to induce the simultaneous excitation of two atoms of different kinds when the sum of the energies of the two photons matches the sum of the energies of the two atomic transitions, while no photons are resonant with each individual transition. We find that entangled two-photon states produced by an atomic cascade are indeed capable of enhancing by a large factor the simultaneous excitation probability as compared to uncorrelated photons, as predicted some years ago by Muthukrishnan et al, but that several non-entangl…
Laser cooling is theoretically investigated in a cascade three-level scheme, where the excited state of a laser-driven transition is coupled by a second laser to a top, more stable level, as for alkali-earth atoms. The second laser action modifies the atomic scattering cross section and produces temperatures lower than those reached by Doppler cooling on the lower transition. When multiphoton processes due to the second laser are relevant, an electromagnetic induced transparency modifies the absorption of the first laser, and the final temperature is controlled by the second laser parameters. …
Long-lived population storage in optically pumped levels of rare-earth ions doped into solids, referred to as persistent spectral hole burning, is of significant fundamental and technological interest. However, the demonstration of deep and persistent holes in rare-earth ion doped amorphous hosts, e.g. glasses, has remained an open challenge since many decades -- a fact that motivates our work towards a better understanding of the interaction between impurities and vibrational modes in glasses. Here we report the first observation and detailed characterization of such holes in an erbium-doped …
Multi-color entangled states of light including low-loss optical fiber transmission and atomic resonance frequencies are essential resources for future quantum information network. We present the experimental achievement on the three-color entanglement generation at 852 nm, 1550 nm and 1440 nm wavelengths for optical continuous variables. The entanglement generation system consists of two cascaded non-degenerated optical parametric oscillators (NOPOs). The flexible selectivity of nonlinear crystals in the two NOPOs and the tunable property of NOPO provide large freedom for the frequency select…
Long distance quantum communication is one of the prime goals in the field of quantum information science. With information encoded in the quantum state of photons, existing telecommunication fiber networks can be effectively used as a transport medium. To achieve this goal, a source of robust entangled single photon pairs is required. While time-bin entanglement offers the required robustness, currently used parametric down-conversion sources have limited performance due to multi-pair contributions. We report the realization of a source of single time-bin entangled photon pairs utilizing the …
We theoretically study the quantum-coherence-enhanced subradiance in a chiral-coupled atomic chain with nonreciprocal decay channels. The collective radiation in this one-dimensional (1D) nanophotonics system results from the resonant dipole-dipole interactions (RDDI) in 1D reservoirs, which allow infinite-range couplings between atoms. When single photon interacts with part of the atomic chain from a side excitation, the subradiant decay can be further reduced when highly correlated states are initially excited. The excitation plateau in the decay process can emerge due to the ordered populat…
We propose an extreme test of quantum theory using astrophysical black holes and entangled photons from atomic cascades. The identification of a cascade emission close to a black-hole event horizon would allow us to observe photons entangled with partners that have fallen behind the horizon. The experiment involves testing the characteristic cos^2(theta) modulation of photon transmission through a pair of polarisers at relative angle theta (Malus' law). For single photons, Malus' law is a remarkable feature of quantum theory: it is equivalent to expectation additivity for incompatible observab…
