Quantum memories for light are important components for future long distance quantum networks. We present on-chip quantum storage of telecommunications band light at the single photon level in an ensemble of erbium-167 ions in an yttrium orthosilicate photonic crystal nanobeam resonator. Storage times of up to 10 $μ$s are demonstrated using an all-optical atomic frequency comb protocol in a dilution refrigerator under a magnetic field of 380 mT. We show this quantum storage platform to have high bandwidth, high fidelity, and multimode capacity, and we outline a path towards an efficient erbium-167 quantum memory for light.
We demonstrate heralded single photon generation in a CMOS-compatible silicon nanophotonic device. The strong modal confinement and slow group velocity provided by a coupled resonator optical waveguide (CROW) produced a large four-wave-mixing nonlinearity coefficient gamma_eff ~4100 W^-1 m^-1 at telecommunications wavelengths. Spontaneous four-wave-mixing using a degenerate pump beam at 1549.6 nm created photon pairs at 1529.5 nm and 1570.5 nm with a coincidence-to-accidental ratio exceeding 20. A photon correlation measurement of the signal (1529.5 nm) photons heralded by the detection of the…
Using a compact optically-pumped silicon nanophotonic chip consisting of coupled silicon microrings, we generate photon pairs in multiple pairs of wavelengths around 1.55 μm. The wavelengths are tunable over several nanometers, demonstrating the capability to generate wavelength division multiplexed photon pairs at freely-chosen telecommunications-band wavelengths.
Large-scale quantum networks will employ telecommunication-wavelength photons to exchange quantum information between remote measurement, storage, and processing nodes via fibre-optic channels. Quantum memories compatible with telecommunication-wavelength photons are a key element towards building such a quantum network. Here, we demonstrate the storage and retrieval of heralded 1532 nm-wavelength photons using a solid-state waveguide quantum memory. The heralded photons are derived from a photon-pair source that is based on parametric down-conversion, and our quantum memory is based on a 6 GH…
Hybrid quantum systems are essential for the realization of distributed quantum networks. In particular, piezo-mechanics operating at typical superconducting qubit frequencies features low thermal excitations, and offers an appealing platform to bridge superconducting quantum processors and optical telecommunication channels. However, integrating superconducting and optomechanical elements at cryogenic temperatures with sufficiently strong interactions remains a tremendous challenge. Here, we report an integrated superconducting cavity piezo-optomechanical platform where 10-GHz phonons are res…
Optical frequency conversion has applications ranging from tunable light sources to telecommunications-band interfaces for quantum information science. Here, we demonstrate efficient, low-noise frequency conversion on a nanophotonic chip through four-wave-mixing Bragg scattering in compact (footprint < 0.5 x 10^-4 cm^2) Si3N4 microring resonators. We investigate three frequency conversion configurations: (1) spectral translation over a few nanometers within the 980 nm band, (2) upconversion from 1550 nm to 980 nm, and (3) downconversion from 980 nm to 1550 nm. With conversion efficiencies rang…
The detection of individual photons is an inherently binary mechanism, revealing either their absence or presence while concealing their spectral information. For multi-color imaging techniques, such as single photon spectroscopy, fluorescence resonance energy transfer microscopy and fluorescence correlation spectroscopy, wavelength discrimination is essential and mandates spectral separation prior to detection. Here, we adopt an approach borrowed from quantum photonic integration to realize a compact and scalable waveguide-integrated single-photon spectrometer capable of parallel detection on…
The emergence of coherent quantum feedback control (CQFC) as a new paradigm for precise manipulation of dynamics of complex quantum systems has led to the development of efficient theoretical modeling and simulation tools and opened avenues for new practical implementations. This work explores the applicability of the integrated silicon photonics platform for implementing scalable CQFC networks. If proven successful, on-chip implementations of these networks would provide scalable and efficient nanophotonic components for autonomous quantum information processing devices and ultra-low-power op…
Advances in quantum photonics have shown that chip-scale quantum devices are translating from the realm of basic research to applied technologies. Recent developments in integrated photonic circuits and single photon detectors indicate that the bottleneck for fidelity in quantum photonic processes will ultimately lie with the photon sources. We present and demonstrate a silicon nanophotonic chip capable of emitting telecommunication band photon pairs that exhibit the highest raw degree of time-energy entanglement from a micro/nanoscale source, to date. Biphotons are generated through cavity-en…
Quantum networks will enable a variety of applications, from secure communication and precision measurements to distributed quantum computing. Storing photonic qubits and controlling their frequency, bandwidth and retrieval time are important functionalities in future optical quantum networks. Here we demonstrate these functions using an ensemble of erbium ions in yttrium orthosilicate coupled to a silicon photonic resonator and controlled via on-chip electrodes. Light in the telecommunication C-band is stored, manipulated and retrieved using a dynamic atomic frequency comb protocol controlled…
We report experimental storage and retrieval of weak coherent states of light at telecommunication wavelengths using erbium ions doped into a solid. We use two photon echo based quantum storage protocols. The first one is based on controlled reversible inhomogeneous broadening (CRIB). It allows the retrieval of the light on demand by controlling the collective atomic coherence with an external electric field, via the linear Stark effect. We study how atoms in the excited state affect the signal to noise ratio of the CRIB memory. Additionally we show how CRIB can be used to modify the temporal …
We present a quantum repeater scheme that is based on individual erbium and europium ions. Erbium ions are attractive because they emit photons at telecommunication wavelength, while europium ions offer exceptional spin coherence for long-term storage. Entanglement between distant erbium ions is created by photon detection. The photon emission rate of each erbium ion is enhanced by a microcavity with high Purcell factor, as has recently been demonstrated. Entanglement is then transferred to nearby europium ions for storage. Gate operations between nearby ions are performed using dynamically co…
Wavelengths in the telecommunication window (~1.25-1.65 microns) are ideal for quantum communication due to low transmission loss in fiber networks. To realize quantum networks operating at these wavelengths, long-lived quantum memories that couple to telecom-band photons with high efficiency need to be developed. We propose coupling neutral ytterbium atoms, which have a strong telecom-wavelength transition, to a silicon photonic crystal cavity. Specifically, we consider the 3P0-3D1 transition in neutral 171Yb to interface its long-lived nuclear spin in the metastable 3P0 'clock' state with a …
Quantum networks require functional nodes consisting of stationary registers with the capability of high-fidelity quantum processing and storage, which efficiently interface with photons propagating in an optical fiber. We report a significant step towards realization of such nodes using a diamond nanocavity with an embedded silicon-vacancy (SiV) color center and a proximal nuclear spin. Specifically, we show that efficient SiV-cavity coupling (with cooperativity $C >30$) provides a nearly-deterministic interface between photons and the electron spin memory, featuring coherence times exceeding…
Optical waveguides in the form of glass fibers are the backbone of global telecommunication networks. In such optical fibers, the light is guided over long distances by continuous total internal reflection which occurs at the interface between the fiber core with a higher refractive index and the lower index cladding. Although this mechanism ensures that no light escapes from the waveguide, it gives rise to an evanescent field in the cladding. While this field is protected from interacting with the environment in standard optical fibers, it is routinely employed in air- or vacuum-clad fibers i…
We study the bandwidth and multiplexing capacity of an erbium-doped optical memory for quantum storage purposes. We concentrate on the protocol ROSE (Revival of a Silenced Echo) because it has the largest potential multiplexing capacity. Our analysis is applicable to other protocols that involve strong optical excitation. We show that the memory performance is limited by instantaneous spectral diffusion and we describe how this effect can be minimised to achieve optimal performance.
We demonstrate experimentally the storage and retrieval of weak coherent light fields at telecommunication wavelengths in a solid. Light pulses at the single photon level are stored for a time up to 600 ns in an Erbium-doped Y$_2$SiO$_5$ crystal at 2.6 K and retrieved on demand. The memory is based on photon echoes with controlled reversible inhomogeneous broadening, which is realized here for the first time at the single photon level. This is implemented with an external field gradient using the linear Stark effect. This experiment demonstrates the feasibility of a solid state quantum memory …
Photon pair sources are fundamental building blocks for quantum entanglement and quantum communication. Recent studies in silicon photonics have documented promising characteristics for photon pair sources within the telecommunications band, including sub-milliwatt optical pump power, high spectral brightness, and high photon purity. However, most quantum systems suitable for local operations, such as storage and computation, support optical transitions in the visible or short near-infrared bands. In comparison to telecommunications wavelengths, the significantly higher optical attenuation in …
Photonic molecules are composed of two or more optical resonators, arranged such that some of the modes of each resonator are coupled to those of the other. Such structures have been used for emulating the behaviour of two-level systems, lasing, and on-demand optical storage and retrieval. Coupled resonators have also been used for dispersion engineering of integrated devices, enhancing their performance for nonlinear optical applications. Delicate engineering of such integrated nonlinear structures is required for developing scalable sources of non-classical light to be deployed in quantum in…
Entanglement is the fundamental characteristic of quantum physics. Large experimental efforts are devoted to harness entanglement between various physical systems. In particular, entanglement between light and material systems is interesting due to their prospective roles as "flying" and stationary qubits in future quantum information technologies, such as quantum repeaters and quantum networks. Here we report the first demonstration of entanglement between a photon at telecommunication wavelength and a single collective atomic excitation stored in a crystal. One photon from an energy-time ent…
The ability to transduce non-classical states of light from one wavelength to another is a requirement for integrating disparate quantum systems that take advantage of telecommunications-band photons for optical fiber transmission of quantum information and near-visible, stationary systems for manipulation and storage. In addition, transducing a single-photon source at 1.3 μm to visible wavelengths for detection would be integral to linear optical quantum computation due to the challenges of detection in the near-infrared. Recently, transduction at single-photon power levels has been accomplis…
The efficient storage and on-demand retrieval of quantum optical states that are compatible with the telecommunications C-band is a requirement for future terrestrial-based quantum optical networking. Spectrum in the C-band minimises optical fiber-propagation losses, and broad optical bandwidth facilitates high-speed networking protocols. Here we report on a telecommunication wavelength and bandwidth compatible quantum memory. Using the Off-Resonant Cascaded Absorption protocol in hot $^{87}$Rb vapour, we demonstrate a total memory efficiency of $20.90(1)\,\%$ with a Doppler-limited storage ti…
PbS quantum dots are promising active emitters for use with high-quality Si nanophotonic devices in the telecommunications-band. Measurements of low quantum dot densities are limited both because of low fluorescence levels and the challenges of single photon detection at these wavelengths. Here, we report on methods using a fiber taper waveguide to efficiently extract PbS quantum dot photoluminescence. Temperature dependent ensemble measurements reveal an increase in emitted photons concomitant with an increase in excited-state lifetime from 58.9 ns at 293 K to 657 ns at 40 K. Measurements are…
Long-lived population storage in optically pumped levels of rare-earth ions doped into solids, referred to as persistent spectral hole burning, is of significant fundamental and technological interest. However, the demonstration of deep and persistent holes in rare-earth ion doped amorphous hosts, e.g. glasses, has remained an open challenge since many decades -- a fact that motivates our work towards a better understanding of the interaction between impurities and vibrational modes in glasses. Here we report the first observation and detailed characterization of such holes in an erbium-doped …
The deployment of a fully-fledged quantum internet poses the challenge of finding adequate building-blocks for entanglement distribution between remote quantum nodes. An ideal system would combine propagation in optical fibres with quantum memories for light, leveraging on the existing communication network while featuring the scalability required to extend to network sizes. Here we demonstrate a fiber-integrated quantum memory entangled with a photon at telecommunication wavelength. The storage device is based on a fiber-pigtailed laser written waveguide in a rare-earth doped solid and allows…
We studied optical coherence properties of the 1.53 $μ$m telecommunication transition in an Er$^{3+}$-doped silicate optical fiber through spectral holeburning and photon echoes. We find decoherence times of up to 3.8 $μ$s at a magnetic field of 2.2 Tesla and a temperature of 150 mK. A strong magnetic-field dependent optical dephasing was observed and is believed to arise from an interaction between the electronic Er$^{3+}$ spin and the magnetic moment of tunneling modes in the glass. Furthermore, we observed fine-structure in the Erbium holeburning spectrum originating from superhyperfine int…
A hybrid interface of solid state single-photon sources and atomic quantum memories is a long sought-after goal in photonic quantum technologies. Here we demonstrate deterministic storage and retrieval of photons from a semiconductor quantum dot in an atomic ensemble quantum memory at telecommunications wavelengths. We store single photons from an InAs quantum dot in a high-bandwidth rubidium vapour based quantum memory, with a total internal memory efficiency of $(12.9 \pm 0.4) \%$. The signal-to-noise ratio of the retrieved photons is $18.2\pm 0.6$, limited only by detector dark counts. This…
We report on experiments demonstrating the reversible mapping of heralded single photons to long lived collective optical atomic excitations stored in a Pr$^{3+}$:Y$_2$SiO$_5$ crystal. A cavity-enhanced spontaneous down-conversion source is employed to produce widely non-degenerate narrow-band ($\approx 2\,\mathrm{MHz}$) photon-pairs. The idler photons, whose frequency is compatible with telecommunication optical fibers, are used to herald the creation of the signal photons, compatible with the Pr$^{3+}$ transition. The signal photons are stored and retrieved using the atomic frequency comb pr…
In a quantum network, coherent emitters can be entangled over large distances using photonic channels. In solid-state devices, the required efficient light-emitter interface can be implemented by confining the light in nanophotonic structures. However, fluctuating charges and magnetic moments at the nearby interface then lead to spectral instability of the emitters. Here we avoid this limitation when enhancing the photon emission up to 70(12)-fold using a Fabry-Perot resonator with an embedded 19 micrometer thin crystalline membrane, in which we observe around 100 individual erbium emitters. I…
Two photons can simultaneously share entanglement between several degrees of freedom such as polarization, energy-time, spatial mode and orbital angular momentum. This resource is known as hyperentanglement, and it has been shown to be an important tool for optical quantum information processing. Here we demonstrate the quantum storage and retrieval of photonic hyperentanglement in a solid-state quantum memory. A pair of photons entangled in polarization and energy-time is generated such that one photon is stored in the quantum memory, while the other photon has a telecommunication wavelength …
Ensembles of solid-state optical emitters enable broadband quantum storage and transduction of photonic qubits, with applications in high-rate optical quantum networks for secure communications, global time-keeping, and interconnecting future quantum computers. To realize coherent quantum information transfer using ensembles, spin rephasing techniques are currently used to mitigate fast decoherence resulting from inhomogeneous broadening. Here we use a dense ensemble of neodymium rare-earth ions strongly coupled to a nanophotonic resonator to demonstrate that decoherence of a single photon exc…
Quantum memories for light will be essential elements in future long-range quantum communication networks. These memories operate by reversibly mapping the quantum state of light onto the quantum transitions of a material system. For networks, the quantum coherence times of these transitions must be long compared to the network transmission times, approximately 100 ms for a global communication network. Due to a lack of a suitable storage material, a quantum memory that operates in the 1550 nm optical fiber communication band with a storage time greater than 1 us has not been demonstrated. Her…
Photon-based quantum information processing promises new technologies including optical quantum computing, quantum cryptography, and distributed quantum networks. Polarization-encoded photons at telecommunication wavelengths provide a compelling platform for practical realization of these technologies. However, despite important success towards building elementary components compatible with this platform, including sources of entangled photons, efficient single photon detectors, and on-chip quantum circuits, a missing element has been atomic quantum memory that directly allows for reversible m…
The ability to transmit quantum states over long distances is a fundamental requirement of the quantum internet and is reliant upon quantum repeaters. Quantum repeaters involve entangled photon sources that emit and deliver photonic entangled states at high rates and quantum memories that can temporarily store quantum states. Improvement of the entanglement distribution rate is essential for quantum repeaters, and multiplexing is expected to be a breakthrough. However, limited studies exist on multiplexed photon sources and their coupling with a multiplexed quantum memory. Here, we demonstrate…
An optical-fibre-integrated buffer for packet-switched quantum networks
Linköpings Universitet（林雪平大学）；RISE-Research Institutes of Sweden（瑞研所）；Universidad de Concepción（康塞普西翁大学）；Millennium Institute for Research in Optics（光学研究千年研究所）
A device being a pinnacle of development of an optical quantum memory should combine the capabilities of storage, inter-communication and processing of stored information. In particular, the ability to capture a train of optical pulses, interfere them in an arbitrary way and finally perform on-demand release would in a loose sense realize an optical analogue of a Turing Machine. Here we demonstrate the operation of an optical quantum memory being able to store optical pulses in the form of collective spin-wave excitations in a multi-dimensional wavevector space. During storage, we perform comp…
Processing and distributing quantum information using photons through fibre-optic or free-space links is essential for building future quantum networks. The scalability needed for such networks can be achieved by employing photonic quantum states that are multiplexed into time and/or frequency, and light-matter interfaces that are able to store and process such states with large time-bandwidth product and multimode capacities. Despite important progress in developing such devices, the demonstration of these capabilities using non-classical light remains challenging. Employing the atomic freque…
Entanglement distribution and quantum storage of more than 8000 modes over a metropolitan network
University of Geneva（日内瓦大学）；Aalto University（阿尔托大学）；Chimie ParisTech, PSL University, CNRS, Institut de Recherche de Chimie Paris（巴黎高等化学学院，PSL大学，法国国家科学研究中心，巴黎化学研究 institute）
Hybrid quantum information devices that combine disparate physical systems interacting through photons offer the promise of combining low-loss telecommunications wavelength transmission with high fidelity visible wavelength storage and manipulation. The realization of such systems requires control over the waveform of single photons to achieve spectral and temporal matching. Here, we experimentally demonstrate the simultaneous wavelength translation and amplitude modulation of single photons generated by a quantum dot emitting near 1300 nm with an exponentially-decaying waveform (lifetime $\ap…
A central goal within quantum optics is to realize efficient interactions between photons and atoms. A fundamental limit in nearly all applications based on such systems arises from spontaneous emission, in which photons are absorbed by atoms and then re-scattered into undesired channels. In typical treatments of atomic ensembles, it is assumed that this re-scattering occurs independently, and at a rate given by a single isolated atom, which in turn gives rise to standard limits of fidelity in applications such as quantum memories or quantum gates. However, this assumption can be violated. In …
We theoretically study the quantum-coherence-enhanced subradiance in a chiral-coupled atomic chain with nonreciprocal decay channels. The collective radiation in this one-dimensional (1D) nanophotonics system results from the resonant dipole-dipole interactions (RDDI) in 1D reservoirs, which allow infinite-range couplings between atoms. When single photon interacts with part of the atomic chain from a side excitation, the subradiant decay can be further reduced when highly correlated states are initially excited. The excitation plateau in the decay process can emerge due to the ordered populat…
Entanglement between photons at telecommunication wavelengths and long-lived quantum memories is one of the fundamental requirements of long-distance quantum communication. Quantum memories featuring on-demand read-out and multimode operation are additional precious assets that will benefit the communication rate. In this work we report the first demonstration of entanglement between a telecom photon and a collective spin excitation in a multimode solid-state quantum memory. Photon pairs are generated through widely non-degenerate parametric down-conversion, featuring energy-time entanglement …
Entangling quantum systems with different characteristics through the exchange of photons is a prerequisite for building future quantum networks. Proving the presence of entanglement between quantum memories for light working at different wavelengths furthers this goal. Here, we report on a series of experiments with a thulium-doped crystal, serving as a quantum memory for 794 nm photons, an erbium-doped fibre, serving as a quantum memory for telecommunication-wavelength photons at 1535 nm, and a source of photon pairs created via spontaneous parametric down-conversion. Characterizing the phot…
Future quantum networks will enable the distribution of entanglement between distant locations and allow applications in quantum communication, quantum sensing and distributed quantum computation. At the core of this network lies the ability of generating and storing entanglement at remote, interconnected quantum nodes. While remote physical systems of various nature have been successfully entangled, none of these realisations encompassed all of the requirements for network operation, such as telecom-compatibility and multimode operation. Here we report the demonstration of heralded entangleme…
