Imaging of surface adsorbed molecules is investigated as a novel detection method for matter wave interferometry with fluorescent particles. Mechanically magnified fluorescence imaging turns out to be an excellent tool for recording quantum interference patterns. It has a good sensitivity and yields patterns of high visibility. The spatial resolution of this technique is only determined by the Talbot gratings and can exceed the optical resolution limit by an order of magnitude. A unique advantage of this approach is its scalability: for certain classes of nano-sized objects, the detection sensitivity will even increase significantly with increasing size of the particle.
Time-reversal Interferometry Using Cat States with Scalable Entangling Resources
DEVCOM Army Research Laboratory（美国国防部陆军研究实验室）；MIT-Harvard Center for Ultracold Atoms and Research Laboratory of Electronics, Massachusetts Institute of Technology（麻省理工学院哈佛超冷原子中心及电子研究实验室）；Department of Applied Physics, Stanford University（斯坦福大学应用物理系）；Department of Physics, University of Connecticut（康涅狄格大学物理系）；Institute of Quantum Physics and Center for Integrated Quantum Science and Technology (IQST), Ulm University（乌尔姆大学量子物理研究所及集成量子科学与技术中心）
We study the loss of spatial coherence in the extended wave function of fullerenes due to collisions with background gases. From the gradual suppression of quantum interference with increasing gas pressure we are able to support quantitatively both the predictions of decoherence theory and our picture of the interaction process. We thus explore the practical limits of matter wave interferometry at finite gas pressures and estimate the required experimental vacuum conditions for interferometry with even larger objects.
Starting from an elementary model and refining it to take into account more realistic effects, we discuss the limitations and advantages of matter-wave interferometry in different configurations. We focus on the possibility to apply this approach to scenarios involving antimatter, such as positrons and positronium atoms. In particular, we investigate the Talbot-Lau interferometer with material gratings and discuss in details the results in view of the possible experimental verification.
We investigated the estimation of an unknown Gaussian process (containing displacement, squeezing and phase-shift) applied to a matter system. The state of the matter system is not directly measured; instead, we measure an optical mode which interacts with the system. We propose an interferometric setup exploiting a beam-splitter-type of light-matter interaction with homodyne detectors and two methods of estimation. We demonstrate the superiority of the interferometric setup over alternative non-interferometric schemes. Importantly, we show that even limited coupling strength and a noisy matte…
Stochastic backgrounds of gravitational waves are intrinsic fluctuations of spacetime which lead to an unavoidable decoherence mechanism. This mechanism manifests itself as a degradation of the contrast of quantum interferences. It defines an ultimate decoherence border for matter-wave interferometry using larger and larger molecules. We give a quantitative characterization of this border in terms of figures involving the gravitational environment as well as the sensitivity of the interferometer to gravitational waves. The known level of gravitational noise determines the maximal size of the m…
We discuss modern developments in quantum optics with organic molecules, clusters and nanoparticles -- in particular recent realizations of near-field matter-wave interferometry. A unified theoretical description in phase space allows us to describe quantum interferometry in position space and in the time domain on an equal footing. In order to establish matter-wave interferometers as a universal tool, which can accept and address a variety of nanoparticles, we elaborate on new quantum optical elements, such as diffraction gratings made of matter and light, as well as their absorptive and disp…
Matter-wave interferometry is a direct test of the quantum superposition principle for massive systems, and of collapse models. Here we show that the bounds placed by matter-wave interferometry depend weakly on the details of the collapse mechanism. Specifically, we compute the bounds on the CSL model and its variants, provided by the the KDTL interferometry experiment of Arndt's group [Phys. Chem. Chem. Phys., 2013, 15, 14696-14700], which currently holds the record of largest mass in interferometry. We also show that the CSL family of models emerges naturally by considering a minimal set of …
We extend the theory of matter-wave interferometry of point-like particles to non-spherical objects by taking the orientational degrees of freedom into account. In particular, we derive the grating transformation operator, that maps the impinging state onto the outgoing state, for a general, orientation-dependent interaction potential between the grating and the molecule. The grating operator is then worked out for the diffraction of symmetric top molecules from standing light waves, and the resulting interference pattern is calculated in the near-field. This allows us to identify a signature …
We establish a rigorous quantitative connection between (i) the interferometric duality relation for which-way information and fringe visibility and (ii) Heisenberg's uncertainty relation for position and modular momentum. We apply our theory to atom interferometry, wherein spontaneously emitted photons provide which way information, and unambiguously resolve the challenge posed by the metamaterial `perfect lens' to complementarity and to the Heisenberg-Bohr interpretation of the Heisenberg microscope thought experiment.
The theory of linear quantum measurement has been developed for analysing the sensitivities of experimental devices that measure extremely weak signals, such as gravitational waves. It has successfully contributed to the theoretical understanding of laser interferometer gravitational-wave detectors (used by LIGO, VIRGO and KaGRA) and helped many important experimental upgrades. In this work, we establish a linear quantum measurement theory for another kind of measurement device--- matter wave interferometers, which has been widely discussed as an important platform for many high-precision expe…
A two-slit interference of a massive particle in the presence of environment induced decoherence is theoretically analyzed using a fully quantum mechanical calculation. The Markovian Master equation, derived from coupling the particle to a harmonic-oscillator heat bath, is used to obtain exact solutions which show the existence of an interference. Interestingly, decoherence does not affect the pattern, but only leads to a reduction in the fringe visibility.
We propose to test the theory of continuous spontaneous localization (CSL) in an all-optical time-domain Talbot-Lau interferometer for clusters with masses exceeding 1000000 amu. By assessing the relevant environmental decoherence mechanisms, as well as the growing size of the particles relative to the grating fringes, we argue that it will be feasible to test the quantum superposition principle in a mass range excluded by recent estimates of the CSL effect.
Matter-wave interferometry of ultra-cold atoms with attractive interactions is studied at the full many-body level. First, we study how a coherent light-pulse applied to an initially-condensed solitonic system splits it into two matter-waves. The split system looses its coherence and develops correlations with time, and inevitably becomes fragmented due to inter-particle attractions. Next, we show that by re-colliding the sub-clouds constituting the split density together, along with a simultaneous application of the same laser-pulse, one creates three matter-waves propagating with different m…
Quantum superposition is central to quantum theory but challenges our concepts of reality and spacetime when applied to macroscopic objects like Schrödinger's cat. For that reason, it has been a long-standing question whether quantum physics remains valid unmodified even for truly macroscopic objects. By now, the predictions of quantum theory have been confirmed via matter-wave interferometry for massive objects up to $10^4\,$ atomic mass units (amu). The rapid development of new technologies promises to soon allow tests of quantum theory for significantly higher test masses by using novel tec…
The study of molecular physics using ultracold gases has provided a unique probe into the fundamental properties of nature and offers new tools for quantum technologies. In this article we outline how the use of a space environment to study ultracold molecular physics opens opportunities for 1) exploring ultra-low energy regimes of molecular physics with high efficiency, 2) providing a toolbox of capabilities for fundamental physics, and 3) enabling new classes of matter-wave interferometers with applications in precision measurement for fundamental and many-body physics.
We study the quantum dynamics of a two-mode Bose-Einstein condensate in a time-dependent symmetric double-well potential using analytical and numerical methods. The effects of internal degrees of freedom on the visibility of interference fringes during a stage of ballistic expansion are investigated varying particle number, nonlinear interaction sign and strength as well as tunneling coupling. Expressions for the phase resolution are derived and the possible enhancement due to squeezing is discussed. In particular, the role of the superfluid - Mott insulator cross-over and its analog for attra…
This chapter reviews recent experiments on matter wave interferometry with large molecules. Starting from an elementary introduction to matter wave physics we discuss far-field diffraction and near-field interferometry with thermally excited many-body systems. We describe the constraints imposed by decoherence and dephasing effects, and present an outlook to the future challenges in macromolecule and cluster interferometry.
High contrast matter-wave interferometry is essential in various fundamental quantum mechanical experiments as well as for technical applications. Thereby, contrast and sensitivity are typically reduced by decoherence and dephasing effects. While decoherence accounts for a general loss of quantum information in a system due to entanglement with the environment, dephasing is due to collective time-dependent external phase shifts, which can be related to temperature drifts, mechanical vibrations or electromagnetic oscillations. In contrast to decoherence, dephasing can in principle be reversed. …
We report on a demonstration of Ramsey interferometry by three-dimensional motion with a trapped $^{171}Yb^+$ ion. We applied a momentum kick to the ion in a direction diagonal to the trap axes to initiate three-dimensional motion using a mode-locked pulse laser. The interference signal was analyzed theoretically to demonstrate three-dimensional matter-wave interference. This work paves the way to realizing matter-wave interferometry using trapped ions.
We assess the most macroscopic matter-wave experiments to date as to the extent to which they probe the quantum-classical boundary by demonstrating interference of heavy molecules and cold atomic ensembles. To this end, we consider a rigorous Bayesian test protocol for a parametrized set of hypothetical modifications of quantum theory, including well-studied spontaneous collapse models, that destroy superpositions and reinstate macrorealism. The range of modification parameters ruled out by the measurement events quantifies the macroscopicity of a quantum experiment, while the shape of the pos…
We show how the interference between spatially separated states of the center of mass (COM) of a mesoscopic harmonic oscillator can be evidenced by coupling it to a spin and performing solely spin manipulations and measurements (Ramsey Interferometry). We propose to use an optically levitated diamond bead containing an NV center spin. The nano-scale size of the bead makes the motional decoherence due to levitation negligible. The form of the spin-motion coupling ensures that the scheme works for thermal states so that moderate feedback cooling suffices. No separate control or observation of th…
In this comment, we agree with the formulas derived in Refs. [1,2] but show that the results are not due to "interference between spatially separated states of the center of mass of a mesoscopic harmonic oscillator".
Most matter-wave interferometry (MWI) schemes for quantum sensing are so far evaluated in ideal situations without noises. In this work, we provide assessments of generic multiqubit MWI schemes under Markovian dephasing noises. We find that for certain classes of the MWI schemes with scale factors that are nonlinearly dependent on the interrogation time, the optimal precision of maximally entangled probes \emph{decreases} with increasing the particle number $N$, for both independent and collective dephasing situations. This result challenges the conventional wisdom found in dephasing Ramsey-ty…
We present a simple derivation of the interference pattern in matter-wave interferometry as predicted by a class of master equations, by using the density matrix formalism. We apply the obtained formulae to the most relevant collapse models, namely the Ghirardi-Rimini-Weber (GRW) model, the continuous spontaneous localization (CSL) model together with its dissipative (dCSL) and non-markovian generalizations (cCSL), the quantum mechanics with universal position localization (QMUPL) and the Diósi-Penrose (DP) model. We discuss the separability of the collapse models dynamics along the 3 spatial …
The superposition principle is one of the bizarre predictions of quantum mechanics. Nevertheless, it has been experimentally verified using electrons, photons, atoms, and molecules. In this article, using a $20~$nm levitated ferromagnetic FePt nanoparticle, an exotic all optical spin polarization technique and the matter-wave interferometry, we show that a mesoscopic spatial Schrodinger cat can be created. Additionally, we argue that the maximum spatial separation between the delocalized wavepackets can be $25~μm$ and is significantly larger than the object itself.
Hybrid spin-mechanical systems have great potentials in sensing, macroscopic quantum mechanics, and quantum information science. In order to induce strong coupling between an electron spin and the center-of-mass motion of a mechanical oscillator, a large magnetic gradient is usually required, which is difficult to achieve. Here we show that strong coupling between the electron spin of a nitrogen-vacancy (NV) center and the torsional vibration of an optically levitated nanodiamond can be achieved in a uniform magnetic field. Thanks to the uniform magnetic field, multiple spins can strongly coup…
Matter-wave interferometry provides a remarkably sensitive tool for probing minute forces and, potentially, the foundations of quantum physics by making use of interference between spatially separated matter waves. Furthering this development requires ever-increasing stability of the interferometer, typically achieved by improving its physical isolation from the environment. Here we introduce as an alternative strategy the concept of dynamical decoupling applied to spatial degrees of freedom of massive objects. We show that the superposed matter waves can be driven along paths in space that re…
Matter-wave interference experiments enable us to study matter at its most basic, quantum level and form the basis of high-precision sensors for applications such as inertial and gravitational field sensing. Success in both of these pursuits requires the development of atom-optical elements that can manipulate matter waves at the same time as preserving their coherence and phase. Here, we present an integrated interferometer based on a simple, coherent matter-wave beam splitter constructed on an atom chip. Through the use of radio-frequency-induced adiabatic double-well potentials, we demonstr…
The advantages of light and matter-wave Sagnac interferometers -- large area on one hand and high rotational sensitivity per unit area on the other -- can be combined utilizing ultra-slow light in cold atomic gases. While a group-velocity reduction alone does not affect the Sagnac phase shift, the associated momentum transfer from light to atoms generates a coherent matter-wave component which gives rise to a substantially enhanced rotational signal. It is shown that matter-wave sensitivity in a large-area interferometer can be achieved if an optically dense vapor at sub-recoil temperatures is…
Paths of particles, emitted from distributed sources and passing out through slits of two gratings, $G_{0}$ and $G_{1}$, up to detectors, have been computed in details by the path integral method. The slits are represented by Gaussian functions that simulate fuzzy edges of the slits. Waves of matter be computed by this method show perfect interference patterns both between the gratings and behind the second grating. Coherent and noncoherent the distributed particle sources reproducing the interference patterns are discussed in details. Paraxial approximation stems from the wave function when r…
Extending the range of quantum interferometry to a wider class of composite nanoparticles requires new tools to diffract matter waves. Recently, pulsed photoionization light gratings have demonstrated their suitability for high mass matter-wave physics. Here we extend quantum interference experiments to a new class of particles by introducing photofragmentation beam splitters into time-domain matter-wave interferometry. Photofragmentation gratings can act on objects as different as van der Waals clusters and biomolecules which are thermally unstable and often resilient to single-photon ionizat…
Usually, decoherence is generated from the coupling with an outer environment. However, a macroscopic object generically possesses its own environment in itself, namely the complicated dynamics of internal degrees of freedom. We address a question: when and how the internal dynamics decohere interference of the center of mass motion of a macroscopic object. We will also show that weak localization of a macroscopic object in disordered potentials can be destroyed by such decoherence.
We discuss a novel application of matter wave interferometry to characterize the scalar optical polarizability of molecules at 532 nm. The interferometer presented here consists of two material absorptive gratings and one central optical phase grating. The interaction of the molecules with the standing light wave is determined by the optical dipole force and is therefore directly dependent on the molecular polarizability at the wavelength of the diffracting laser light. By comparing the observed matter-wave interference contrast with a theoretical model for several intensities of the standing …
We propose a mechanism to use nonlinearity arising from inter-particle interactions to significantly enhance rotation sensitivity of matter-wave interferometers. The method relies on modifying Sagnac interferometers by introducing a weak circular lattice potential that couples modes with opposite orbital angular momenta (OAM). The primary observable comprises of the modal population distributions measured at particular times. This provides an alternate mechanism for rotation sensing that requires substantially smaller ring size, even in the linear non-interacting regime. Nonlinearity can impro…
There has been considerable recent interest in the mean-field dynamics of various atom-interferometry schemes designed for precision sensing. In the field of quantum metrology, the standard tools for evaluating metrological sensitivity are the classical- and quantum-Fisher information. In this letter, we show how these tools can be adapted to evaluate the sensitivity when the behaviour is dominated by mean-field dynamics. As an example, we compare the behaviour of four recent theoretical proposals for gyroscopes based on matterwaves interference in toroidally trapped geometries. We show that w…
This paper descrives the first experimental evidence of antimatter-wave interference, a process at the heart of Quantum Physics and its interpretation. For the case of ordinary matter particles, interference phenomena have been observed in a variety of cases, ranging to electrons up to complex molecules. Here I present the first demonstration of single-positrons quantum interference.
Optical interferometry has been a long-standing setup for characterization of quantum states of light. Both the linear and the nonlinear interferences can provide information about the light statistics an underlying detail of the light-matter interactions. Here we demonstrate how interferometric detection of nonlinear spectroscopic signals may be used to improve the measurement accuracy of matter susceptibilities. Light-matter interactions change the photon statistics of quantum light, which are encoded in the field correlation functions. Application is made to the Hong-Ou-Mandel two-photon in…
We define a quantum witness for high-mass matter-wave interferometers that allows us to test fundamental assumptions of macroscopic realism. We propose an experimental realisation using absorptive laser gratings and show that such systems can strongly violate a macrorealistic quantum-witness equality. The measurement of the witness can therefore provide clear evidence of physics beyond macrorealism for macromolecules and nanoparticles.
Vibrations, electromagnetic oscillations and temperature drifts are among the main reasons for dephasing in matter-wave interferometry. Sophisticated interferometry experiments, e.g. with ions or heavy molecules, often require integration times of several minutes due to the low source intensity or the high velocity selection. Here we present a scheme to suppress the influence of such dephasing mechanisms - especially in the low-frequency regime - by analyzing temporal and spatial particle correlations available in modern detectors. Such correlations can reveal interference properties that woul…
We demonstrate a method to generate spatially homogeneous entangled, spin-squeezed states of atoms appropriate for maintaining a large amount of squeezing even after release into the arm of a matter-wave interferometer or other free space quantum sensor. Using an effective intracavity dipole trap, we allow atoms to move along the cavity axis and time average their coupling to the standing wave used to generate entanglement via collective measurements, demonstrating 11(1) dB of directly observed spin squeezing. Our results show that time averaging in collective measurements can greatly reduce t…
Many different formalisms exist for computing the phase of a matter-wave interferometer. However, it can be challenging to develop physical intuition about what a particular interferometer is actually measuring or about whether a given classical measurement provides equivalent information. Here we investigate the physical content of the interferometer phase through a series of thought experiments. In low-order potentials, a matter-wave interferometer with a single internal state provides the same information as a sum of position measurements of a classical test object. In high-order potentials…
The Schrodinger-Newton equation has frequently been studied as a nonlinear modification of the Schrodinger equation incorporating gravitational self-interaction. However, there is no evidence yet as to whether nature actually behaves this way. This work investigates a possible way to experimentally test gravitational self-interaction. The effect of self-gravity on interference of massive particles is studied by numerically solving the Schrodinger-Newton equation for a particle passing through a double-slit. The results show that the presence of gravitational self-interaction has an effect on t…
If the structure of spacetime is discrete, then Lorentz symmetry should only be an approximation, valid at long length scales. At finite lattice spacings there will be small corrections to the Dirac evolution that could in principle be experimentally detected. In particular, the lattice structure should be reflected in a modification of the free-particle dispersion relation. We show that these can produce a surprisingly large phase shift between the two arms of an asymmetrical interferometer. This method could be employed to test any model that predicts a direction-dependent dispersion relatio…
Enhanced Dark Matter Quantum Sensing via Phase-Space Geometric Interferometry
International Center for Quantum-field Measurement Systems for Studies of the Universe and Particles (QUP, WPI), High Energy Accelerator Research Organization (KEK)（宇宙与粒子研究量子场测量系统国际中心（QUP，WPI），高能加速器研究机构（KEK））；Kavli IPMU (WPI), UTIAS, University of Tokyo（Kavli 宇宙起源研究所（WPI），东京大学宇宙线研究所（UTIAS））
Since the first atom interferometry experiments in 1991, measurements of rotation through the Sagnac effect in open-area atom interferometers has been studied. These studies have demonstrated very high sensitivity which can compete with state-of-the-art optical Sagnac interferometers. Since the early 2000s, these developments have been motivated by possible applications in inertial guidance and geophysics. Most matter-wave interferometers that have been investigated since then are based on two-photon Raman transitions for the manipulation of atomic wave packets. Results from the two most studi…
We discuss matter wave experiments in a near-field interferometer and focus on dephasing phenomena due to inertial forces. Their presence may result in a significant reduction of the observed interference contrast, even though they do not lead to genuine decoherence. We provide quantitative estimates for the most important effects and demonstrate experimentally the strong influence of acoustic vibrations. Since the effects of inertial forces get increasingly important for the interferometry with more massive particles they have to be identified and compensated in future experiments.
The problem of on-demand generation of entanglement between single-atom qubits via a common photonic channel is examined within the framework of optical interferometry. As expected, for a Mach-Zehnder interferometer with coherent laser beam as input, a high-finesse optical cavity is required to overcome sensitivity to spontaneous emission. We show, however, that with a twin-Fock input, useful entanglement can in principle be created without cavity-enhancement. Both approaches require single-photon resolving detectors, and best results would be obtained by combining both cavity-feedback and twi…
We study in detail a peculiar configuration of the Talbot-Lau matter wave interferometer, characterised by unequal distances between the two diffraction gratings and the observation plane. We refer to this apparatus as the "asymmetric Talbot-Lau setup". Particular attention is given to its capabilities as an inertial sensor for particle and atomic beams, also in comparison with the classical moiré deflectometer. The present analysis is motivated by possible experimental applications in the context of antimatter wave interferometry, including the measurement of the gravitational acceleration of…
Bose-Einstein condensates (BECs) in free fall constitute a promising source for space-borne matter-wave interferometry. Indeed, BECs enjoy a slowly expanding wave function, display a large spatial coherence and can be engineered and probed by optical techniques. On a sounding rocket, we explore matter-wave fringes of multiple spinor components of a BEC released in free fall employing light-pulses to drive Bragg processes and induce phase imprinting. The prevailing microgravity played a crucial role in the observation of these interferences which not only reveal the spatial coherence of the con…
We investigate the influence of thermally activated internal molecular dynamics on the phase shifts of matter waves inside a molecule interferometer. While de Broglie physics generally describes only the center-of-mass motion of a quantum object, our experiment demonstrates that the translational quantum phase is sensitive to dynamic conformational state changes inside the diffracted molecules. The structural flexibility of tailor-made hot organic particles is sufficient to admit a mixture of strongly fluctuating dipole moments. These modify the electric susceptibility and through this the qua…
Matter-wave interferometry with solids is highly susceptible to minute fluctuations of environmental fields, including gravitational effects from distant sources. Hence, experiments require a degree of shielding that is extraordinarily challenging to achieve in realistic terrestrial or even space-based set-ups. Here, we design protocols that exploit the spatial correlations that are inherent in perturbations due to distant sources to reduce significantly their impact on the visibility of interference patterns. We show that interference patterns that are robust to such type of noise can be enco…
A new generation of atomic sensors using ultra-narrow optical clock transitions and composite pulses are pushing quantum engineering control to a very high level of precision for applied and fundamental physics. Here, we propose a new version of Ramsey-Bordé interferometry introducing arbitrary composite laser pulses with tailored pulse duration, Rabi field, detuning and phase-steps. We explore quantum metrology below the $10^{-18}$ level of fractional accuracy by a fine tuning control of light excitation parameters protecting ultra-narrow optical clock transitions against residual light-shift…
