We study the loss of spatial coherence in the extended wave function of fullerenes due to collisions with background gases. From the gradual suppression of quantum interference with increasing gas pressure we are able to support quantitatively both the predictions of decoherence theory and our picture of the interaction process. We thus explore the practical limits of matter wave interferometry at finite gas pressures and estimate the required experimental vacuum conditions for interferometry with even larger objects.
A most simple theoretical argument is given in order to explain the quantitative estimate of the effect of collisional decoherence in matter-wave interferometry. The argument highlights the relevance of quantum and classical features in the description of the phenomenon, showing in particular the connection between the formula used for the experimental fit and the loss term in the classical linear Boltzmann equation.
The quantum state of motion of a large and rotating polar molecule can lose coherence through the collisions with gas atoms. We show how the associated quantum master equation for the center of mass can be expressed in terms of the orientationally averaged differential and total scattering cross sections, for which we provide approximate analytic expressions. The master equation is then utilized to quantify collisional decoherence in a interference experiment with polar molecules.
Recently there has been much interest in optomechanical devices for the production of macroscopic quantum states. Here we focus on a proposed scheme for achieving macroscopic superpositions via nested interferometry. We consider the effects of finite temperature on the superposition produced. We also investigate in detail the scheme's feasibility for probing various novel decoherence mechanisms.
We employ a continuous dynamical decoupling scheme to suppress the decoherence induced by elastic collisions of cold atoms. Using a continuous echo pulse we achieve a thirty-fold increase in the coherence time of Rb87 atoms trapped in a dipole trap. Coherence times of more than 100ms are demonstrated for an ensemble with an optical depth of 120.
We study the emergence and dynamics of pointer states in the motion of a quantum test particle affected by collisional decoherence. These environmentally distinguished states are shown to be exponentially localized solitonic wave functions which evolve according to the classical equations of motion. We explain their formation using the orthogonal unraveling of the master equation, and we demonstrate that the statistical weights of the arising mixture are given by projections of the initial state onto the pointer basis.
We re-derive the quantum master equation for the decoherence of a massive Brownian particle due to collisions with the lighter particles from a thermal environment. Our careful treatment avoids the occurrence of squares of Dirac delta functions. It leads to a decoherence rate which is smaller by a factor of 2 pi compared to previous findings. This result, which is in agreement with recent experiments, is confirmed by both a physical analysis of the problem and by a perturbative calculation in the weak coupling limit.
Stochastic backgrounds of gravitational waves are intrinsic fluctuations of spacetime which lead to an unavoidable decoherence mechanism. This mechanism manifests itself as a degradation of the contrast of quantum interferences. It defines an ultimate decoherence border for matter-wave interferometry using larger and larger molecules. We give a quantitative characterization of this border in terms of figures involving the gravitational environment as well as the sensitivity of the interferometer to gravitational waves. The known level of gravitational noise determines the maximal size of the m…
A two-slit interference of a massive particle in the presence of environment induced decoherence is theoretically analyzed using a fully quantum mechanical calculation. The Markovian Master equation, derived from coupling the particle to a harmonic-oscillator heat bath, is used to obtain exact solutions which show the existence of an interference. Interestingly, decoherence does not affect the pattern, but only leads to a reduction in the fringe visibility.
We study decoherence of the external degree of freedom of a tracer particle moving in a one dimensional dilute Boltzmann gas. We find that phase averaging is the dominant decoherence effect, rather than information exchange between tracer and gas particles. While a coherent superposition of two wave packets with different mean positions quickly turns into a mixed state, it is demonstrated that such superpositions of different momenta are robust to phase averaging, until the two wave packets acquire a different position due to the different velocity of each wave packet.
We study two different decoherence modes for entangled qubits by considering a Liouville - von Neumann master equation. Mode A is determined by projection operators onto the eigenstates of the Hamiltonian and mode B by projectors onto rotated states. We present solutions for general and for Bell diagonal states and calculate for the later the mixedness and the amount of entanglement given by the concurrence. We propose a realization of the decoherence modes within neutron interferometry by applying fluctuating magnetic fields. An experimental test of the Kraus operator decomposition describing…
A full treatment of decoherence and dephasing effects in BEC interferometry has been developed based on using quantum correlation functions for treating interferometric effects. The BEC is described via a phase space distribution functional of the Wigner type for the condensate modes and the positive P type for the non-condensate modes. Ito equations for stochastic condensate and non-condensate field functions replace the functional Fokker-Planck equation for the distribution functional and stochastic averages of field function products determine the quantum correlation functions.
Interferometric signals are degraded by decoherence, which encompasses dephasing, mixing and any distinguishing which-path information. These three paradigmatic processes are fundamentally different, but, for coherent, single-photon and $N00N$-states, they degrade interferometric visibility in the very same way, which impedes the diagnosis of the cause for reduced visibility in a single experiment. We introduce a versatile formalism for many-boson interferometry based on double-sided Feynman diagrams, which we apply to a protocol for differential decoherence diagnosis: Twin-Fock states |N,N> w…
We consider the collision model of Ziman {\em et al.} and study the robustness of $N$-qubit Greenberger-Horne-Zeilinger (GHZ), W, and linear cluster states. Our results show that $N$-qubit entanglement of GHZ states would be extremely fragile under collisional decoherence, and that of W states could be more robust than of linear cluster states. We indicate that the collision model of Ziman {\em et al.} could provide a physical mechanism to some known results in this area of investigations. More importantly, we show that it could give a clue as to how $N$-partite distillable entanglement would …
We analyze collisional decoherence of atoms or molecules prepared in a coherent superposition of nondegenerate internal states at ultralow temperatures and placed in an ultracold buffer gas. Our analysis is applicable for an arbitrary bath particle/tracer particle mass ratio. Both elastic and inelastic collisions contribute to decoherence. We obtain an expression relating the observable decoherence rate to pairwise scattering properties, specifically the low-temperature scattering amplitudes. We consider the dependence on the bath particle/tracer particle mass ratio for the case of light bath …
Collisions, even though they do not limit the lifetime of quantum information stored in ground state hyperfine coherences, may severely limit the fidelity for quantum memory when they happen during the write and read process. This imposes restrictions on the implementation of quantum processes in thermal vapor cells and their performance as a quantum memory. We study the effect of these collisions in our experiment.
We study the limitations for entanglement due to collisional decoherence in a Bose-Einstein condensate. Specifically we consider relative number squeezing between photons and atoms coupled out from a homogeneous condensate. We study the decay of excited quasiparticle modes due to collisions, in condensates of atoms with one or two internal degrees of freedom. The time evolution of these modes is determined in the linear response approximation to the deviation from equilibrium. We use Heisenberg-Langevin equations to derive equations of motion for the densities and higher correlation functions …
We analyze the coherence properties of polarized neutrons, after they have interacted with a magnetic field or a phase shifter undergoing different kinds of statistical fluctuations. We endeavor to probe the degree of disorder of the distribution of the phase shifts by means of the loss of quantum mechanical coherence of the neutron. We find that the notion of entropy of the shifts and that of decoherence of the neutron do not necessarily agree. In some cases the neutron wave function is more coherent, even though it has interacted with a more disordered medium.
Complex molecules are intriguing objects at the interface between quantum and classical phenomena. Compared to the electrons, neutrons, or atoms studied in earlier matter-wave experiments, they feature a much more complicated internal structure, but can still behave as quantum objects in their center-of-mass motion. Molecules may involve a large number of vibrational modes and highly excited rotational states, they can emit thermal photons, electrons, or even atoms, and they exhibit large cross sections for collisional interactions with residual background gases. This makes them ideal candidat…
We present expressions demonstrating that collisional decoherence of ultracold atoms or molecules in a coherent superposition of non-degenerate quantum states is suppressed when both the real and imaginary parts of the scattering lengths for the states in the coherent superposition are equal. We show that the rate of collisional decoherence can be enhanced or suppressed by varying an external magnetic field near a Feshbach resonance. For some resonances, the suppression is very dramatic. We propose a method for measuring the scattering length of ultracold particles in excited quantum states ex…
We analyse the effect of decoherence and noise on quantum Fourier transform interferometry, in which a boson sampling photonic network is used to measure optical phase gradients. This novel type of metrology is shown to be robust against phase decoherence. One can also measure gradients using lower order correlations without substantial degradation. Our results involve estimation of up to a 100 x 100 matrix permanent.
Most matter-wave interferometry (MWI) schemes for quantum sensing are so far evaluated in ideal situations without noises. In this work, we provide assessments of generic multiqubit MWI schemes under Markovian dephasing noises. We find that for certain classes of the MWI schemes with scale factors that are nonlinearly dependent on the interrogation time, the optimal precision of maximally entangled probes \emph{decreases} with increasing the particle number $N$, for both independent and collective dephasing situations. This result challenges the conventional wisdom found in dephasing Ramsey-ty…
Usually, decoherence is generated from the coupling with an outer environment. However, a macroscopic object generically possesses its own environment in itself, namely the complicated dynamics of internal degrees of freedom. We address a question: when and how the internal dynamics decohere interference of the center of mass motion of a macroscopic object. We will also show that weak localization of a macroscopic object in disordered potentials can be destroyed by such decoherence.
The propagation of polarized photons in optical media can be effectively modeled by means of quantum dynamical semigroups. These generalized time evolutions consistently describe phenomena leading to loss of phase coherence and dissipation originating from the interaction with a large, external environment. High sensitive experiments in the laboratory can provide stringent bounds on the fundamental energy scale that characterizes these non-standard effects.
The decoherence of a two-state tunneling molecule, such as a chiral molecule or ammonia, due to collisions with a buffer gas is analyzed in terms of a succession of quantum states of the molecule satisfying the conditions for a consistent family of histories. With $\hbar ω$ the separation in energy of the levels in the isolated molecule and $γ$ a decoherence rate proportional to the rate of collisions, we find for $γ\gg ω$ (strong decoherence) a consistent family in which the molecule flips randomly back and forth between the left- and right-handed chiral states in a stationary Markov process.…
Hypothetical models have been proposed in which explicit collapse mechanisms prevent the superposition principle to hold at large scales. In particular, the model introduced by Ellis and co-workers [Phys. Lett. B ${\bf 221}$, 113 (1989)] suggests that quantum gravity might be responsible for the collapse of the wavefunction of massive objects in spatial superpositions. We here consider a recent experiment reporting on interferometry with atoms delocalized over half a meter for timescale of a second [Nature ${\bf 528}$, 530 (2015)] and show that the corresponding data strongly bound quantum gra…
The eigenstate decoherence hypothesis (EDH) asserts that each individual eigenstate of a large closed system is locally classical-like. We test this hypothesis for a heavy particle interacting with a gas of light particles. This system is paradigmatic for studies of the quantum-to-classical transition: The reduced state of the heavy particle is widely believed to rapidly loose any nonclassical features due to the interaction with the gas. Yet, we find numerical evidence that the EDH is violated: certain eigenstates of this model are manifestly non-classical. Only the weak version of EDH referr…
We present a scheme for achieving macroscopic quantum superpositions in optomechanical systems by using single photon postselection and detecting them with nested interferometers. This method relieves many of the challenges associated with previous optical schemes for measuring macroscopic superpositions, and only requires the devices to be in the weak coupling regime. It requires only small improvements on currently achievable device parameters, and allows observation of decoherence on a timescale unconstrained by the system's optical decay time. Prospects for observing novel decoherence mech…
Non-classical states of light find applications in enhancing the performance of optical interferometric experiments, with notable example of gravitational wave-detectors. Still, the presence of decoherence hinders significantly the performance of quantum-enhanced protocols. In this review, we summarize the developments of quantum metrology with particular focus on optical interferometry and derive fundamental bounds on achievable quantum-enhanced precision in optical interferometry taking into account the most relevant decoherence processes including: phase diffusion, losses and imperfect inte…
High contrast matter-wave interferometry is essential in various fundamental quantum mechanical experiments as well as for technical applications. Thereby, contrast and sensitivity are typically reduced by decoherence and dephasing effects. While decoherence accounts for a general loss of quantum information in a system due to entanglement with the environment, dephasing is due to collective time-dependent external phase shifts, which can be related to temperature drifts, mechanical vibrations or electromagnetic oscillations. In contrast to decoherence, dephasing can in principle be reversed. …
We discuss the coherent splitting and recombining of a nanoparticle in a mesoscopic "closed-loop" Stern-Gerlach interferometer in which the observable is the spin of a single impurity embedded in the particle. This spin, when interacting with a pulsed magnetic gradient, generates the force on the particle. We calculate the internal decoherence which arises as the displaced impurity excites internal degrees of freedom (phonons) that may provide Welcher Weg information and preclude interference. We estimate the constraints this decoherence channel puts on future interference experiments with mas…
We show that when the Hornberger--Sipe calculation of collisional decoherence is carried out with the squared delta function a delta of energy instead of a delta of the absolute value of momentum, following a method introduced by Diósi, the corrected formula for the decoherence rate is simply obtained. The results of Hornberger and Sipe and of Diósi are shown to be in agreement. As an independent cross-check, we calculate the mean squared coordinate diffusion of a hard sphere implied by the corrected decoherence master equation, and show that it agrees precisely with the same quantity as calcu…
Perfect single-crystal neutron interferometers are adversely sensitive to environmental disturbances, particularly mechanical vibrations. The sensitivity to vibrations results from the slow velocity of thermal neutrons and the long measurement time that are encountered in a typical experiment. Consequently, to achieve a good interference solutions for reducing vibration other than those normally used in optical experiments must be explored. Here we introduce a geometry for a neutron interferometer that is less sensitive to low-frequency vibrations. This design may be compared with both dynamic…
We examine the emergence of objectivity via quantum Darwinism through the use of a collision model, i.e. where the dynamics is modeled through sequences of unitary interactions between the system and the individual constituents of the environment, termed "ancillas". By exploiting versatility of this framework, we show that one can transition from a "Darwinistic" to an "encoding" environment by simply tuning their interaction. Furthermore we establish that in order for a setting to exhibit quantum Darwinism we require a mutual decoherence to occur between the system and environmental ancillas, …
We examine interferometric measurements of the topological charge of (non-Abelian) anyons. The target's topological charge is measured from its effect on the interference of probe particles sent through the interferometer. We find that superpositions of distinct anyonic charges a and a' in the target decohere (exponentially in the number of probes particles used) when the probes have nontrivial monodromy with the charges that may be fused with a to give a'.
Experimental observation of the decoherence of macroscopic objects is of fundamental importance to the study of quantum collapse models and the quantum to classical transition. Optomechanics is a promising field for the study of such models because of its fine control and readout of mechanical motion. Nevertheless, it is challenging to monitor a mechanical superposition state for long enough to investigate this transition. We present a scheme for entangling two mechanical resonators in spatial superposition states such that all quantum information is stored in the mechanical resonators. The sc…
This chapter reviews recent experiments on matter wave interferometry with large molecules. Starting from an elementary introduction to matter wave physics we discuss far-field diffraction and near-field interferometry with thermally excited many-body systems. We describe the constraints imposed by decoherence and dephasing effects, and present an outlook to the future challenges in macromolecule and cluster interferometry.
Path-Degenerate Quantum Interferometry for Loss Resilience in Gravitational-Wave Detectors
Universität Hamburg（汉堡大学）；Russian Quantum Center, Skolkovo IC（俄罗斯量子中心，斯科尔科沃创新中心）；Faculty of Physics, M V Lomonosov Moscow State University（莫斯科国立大学物理学院）
We propose to test the theory of continuous spontaneous localization (CSL) in an all-optical time-domain Talbot-Lau interferometer for clusters with masses exceeding 1000000 amu. By assessing the relevant environmental decoherence mechanisms, as well as the growing size of the particles relative to the grating fringes, we argue that it will be feasible to test the quantum superposition principle in a mass range excluded by recent estimates of the CSL effect.
We discuss matter wave experiments in a near-field interferometer and focus on dephasing phenomena due to inertial forces. Their presence may result in a significant reduction of the observed interference contrast, even though they do not lead to genuine decoherence. We provide quantitative estimates for the most important effects and demonstrate experimentally the strong influence of acoustic vibrations. Since the effects of inertial forces get increasingly important for the interferometry with more massive particles they have to be identified and compensated in future experiments.
In this paper, we present a brief overview of atom interferometry. This field of research has developed very rapidly since 1991. Atom and light wave interferometers present some similarities but there are very important differences in the tools used to manipulate these two types of waves. Moreover, the sensitivity of atomic waves and light waves to their environment is very different. Atom interferometry has already been used for a large variety of studies: measurements of atomic properties and of inertial effects (accelerations and rotations), new access to some fundamental constants, observa…
To investigate the possibility that intrinsic gravitational decoherence can be theoretically demonstrated within canonical quantum gravity, we develop a model of a self-gravitating interferometer. We search for evidence in the resulting interference pattern that would indicate coherence is fundamentally limited due to general relativistic effects. To eliminate the occurence of gravitational waves, we work in spherical symmetry, and construct the "beam" of the interferometer out of WKB states for an infinitesimally thin shell of matter. For internal consistency, we encode information about the …
We propose an experiment to observe interference of a single electron as it is transported along two parallel quasi-one-dimensional channels trapped in a single minimum of a travelling periodic electric field. The experimental device is a modification of the surface acoustic wave (SAW) based quantum processor. Interference is achieved by creating a superposition of spatial wavefunctions between the two channels and inducing a relative phase shift via either a transverse electric field or a magnetic field. The interference can be used to estimate the decoherence time of an electron in this type…
Coherent electrons coupled to the quantized electromagnetic field undergo decoherence which can be viewed as due either to fluctuations of the Aharonov-Bohm phase or to photon emission. When the electromagnetic field is in a squeezed vacuum state, it is possible for this decoherence to be reduced, leading to the phenomenon of recoherence. This recoherence effect requires electrons which are emitted at selected times during the cycle of the excited mode of the electromagnetic field. We show that there are bounds on the degree of recoherence which are analogous to quantum inequality restriction …
We present a theoretical framework to describe the effects of decoherence on matter waves in Talbot-Lau interferometry. Using a Wigner description of the stationary beam the loss of interference contrast can be calculated in closed form. The formulation includes both the decohering coupling to the environment and the coherent interaction with the grating walls. It facilitates the quantitative distinction of genuine quantum interference from the expectations of classical mechanics. We provide realistic microscopic descriptions of the experimentally relevant interactions in terms of the bulk pro…
We identify the dominant collisional decoherence mechanism which serves to stabilize and super-select the configuration states of chiral molecules. A high-energy description of this effect is compared to the results of the exact molecular scattering problem, obtained by solving the coupled-channel equations. It allows to predict the experimental conditions for observing the collisional suppression of the tunneling dynamics between the left-handed and the right-handed configuration of D2S2 molecules.
The present paper outlines a basic theoretical treatment of decoherence and dephasing effects in interferometry based on single component BEC in double potential wells, where two condensate modes may be involved. Results for both two mode condensates and the simpler single mode condensate case are presented. A hybrid phase space distribution functional method is used where the condensate modes are described via a truncated Wigner representation, and the basically unoccupied non-condensate modes are described via a positive P representation. The Hamiltonian for the system is described in terms …
Matter-wave interferometry performed with massive objects elucidates their wave nature and thus tests the quantum superposition principle at large scales. Whereas standard quantum theory places no limit on particle size, alternative, yet untested theories---conceived to explain the apparent quantum to classical transition---forbid macroscopic superpositions. Here we propose an interferometer with a levitated, optically cooled, and then free-falling silicon nanoparticle in the mass range of one million atomic mass units, delocalized over more than 150 nm. The scheme employs the near-field Talbo…
We show how the interference between spatially separated states of the center of mass (COM) of a mesoscopic harmonic oscillator can be evidenced by coupling it to a spin and performing solely spin manipulations and measurements (Ramsey Interferometry). We propose to use an optically levitated diamond bead containing an NV center spin. The nano-scale size of the bead makes the motional decoherence due to levitation negligible. The form of the spin-motion coupling ensures that the scheme works for thermal states so that moderate feedback cooling suffices. No separate control or observation of th…
We review different attempts to show the decoherence process in double-slit-like experiments both for charged particles (electrons) and neutral particles with permanent dipole moments. Interference is studied when electrons or atomic systems are coupled to classical or quantum electromagnetic fields. The interaction between the particles and time-dependent fields induces a time-varying Aharonov phase. Averaging over the phase generates a suppression of fringe visibility in the interference pattern. We show that, for suitable experimental conditions, the loss of contrast for dipoles can be almo…
The quantum measurement problem still finds no consensus. Nonlocal interferometry provides an unprecedented experimental probe by entangling two photons in the "measurement state" (MS). The experiments show that each photon "measures" the other; the resulting entanglement decoheres both photons; decoherence collapses both photons to unpredictable but definite outcomes; and the two-photon MS continues evolving coherently. Thus, contrary to common opinion, when a two-part system is in the MS, the outcomes actually observed at both subsystems are definite. Although standard quantum physics postul…
Although various pieces of indirect evidence about the nature of dark matter have been collected, its direct detection has eluded experimental searches despite extensive effort. If the mass of dark matter is below 1 MeV, it is essentially imperceptible to conventional detection methods because negligible energy is transferred to nuclei during collisions. Here I propose directly detecting dark matter through the quantum decoherence it causes rather than its classical effects such as recoil or ionization. I show that quantum spatial superpositions are sensitive to low-mass dark matter that is in…
We demonstrate that memory in an $N$-qubit system subjected to decoherence, is a potential resource for the slow-down of the entanglement decay. We show that this effect can be used to retain the sub shot-noise sensitivity of the parameter estimation in quantum interferometry. We calculate quantum Fisher information, which sets the ultimate bound for the precision of the estimation. We also derive the sensitivity of such a noisy interferometer, when the phase is either estimated from the measurements of the population imbalance or from the one-body density.
We study how macroscopic superpositions of coherent states produced by the nondissipative dynamics of binary mixtures of ultracold atoms are affected by atom losses. We identify different decoherence scenarios for symmetric or asymmetric loss rates and interaction energies in the two modes. In the symmetric case the quantum coherence in the superposition is lost after a single loss event. By tuning appropriately the energies we show that the superposition can be protected, leading to quantum correlations useful for atom interferometry even after many loss events.
