We review different attempts to show the decoherence process in double-slit-like experiments both for charged particles (electrons) and neutral particles with permanent dipole moments. Interference is studied when electrons or atomic systems are coupled to classical or quantum electromagnetic fields. The interaction between the particles and time-dependent fields induces a time-varying Aharonov phase. Averaging over the phase generates a suppression of fringe visibility in the interference pattern. We show that, for suitable experimental conditions, the loss of contrast for dipoles can be almost as large as the corresponding one for coherent electrons and therefore, be observed. We analyze different trajectories in order to show the dependence of the decoherence factor with the velocity of the particles.
We discuss matter wave experiments in a near-field interferometer and focus on dephasing phenomena due to inertial forces. Their presence may result in a significant reduction of the observed interference contrast, even though they do not lead to genuine decoherence. We provide quantitative estimates for the most important effects and demonstrate experimentally the strong influence of acoustic vibrations. Since the effects of inertial forces get increasingly important for the interferometry with more massive particles they have to be identified and compensated in future experiments.
Vibrations, electromagnetic oscillations and temperature drifts are among the main reasons for dephasing in matter-wave interferometry. Sophisticated interferometry experiments, e.g. with ions or heavy molecules, often require integration times of several minutes due to the low source intensity or the high velocity selection. Here we present a scheme to suppress the influence of such dephasing mechanisms - especially in the low-frequency regime - by analyzing temporal and spatial particle correlations available in modern detectors. Such correlations can reveal interference properties that woul…
High contrast matter-wave interferometry is essential in various fundamental quantum mechanical experiments as well as for technical applications. Thereby, contrast and sensitivity are typically reduced by decoherence and dephasing effects. While decoherence accounts for a general loss of quantum information in a system due to entanglement with the environment, dephasing is due to collective time-dependent external phase shifts, which can be related to temperature drifts, mechanical vibrations or electromagnetic oscillations. In contrast to decoherence, dephasing can in principle be reversed. …
We derive upper bounds on the quantum Fisher information in interferometry with $N$ subsystems, e.g. two-level atoms or Gaussian modes, in the presence of arbitrarily correlated Gaussian dephasing including independent and collective dephasing. The derived upper bound enables us to analyse the Fisher information asymptotic behaviour when $N\rightarrow\infty$. Dephasing introduces random phases to subsystems dynamics, which lowers the precision of estimating the phase difference $ϕ$ in an interferometer. The method presented uses Bayesian estimation of the random phases and eliminates dephasing…
Most matter-wave interferometry (MWI) schemes for quantum sensing are so far evaluated in ideal situations without noises. In this work, we provide assessments of generic multiqubit MWI schemes under Markovian dephasing noises. We find that for certain classes of the MWI schemes with scale factors that are nonlinearly dependent on the interrogation time, the optimal precision of maximally entangled probes \emph{decreases} with increasing the particle number $N$, for both independent and collective dephasing situations. This result challenges the conventional wisdom found in dephasing Ramsey-ty…
I analyze a metrological strategy for improving the precision of frequency estimation via Ramsey interferometry with strings of atoms in the presence of correlated dephasing. This strategy does not employ entangled states, but rather a product state which evolves into a stationary state under the influence of correlated dephasing. It is shown that by using this state an improvement in precision compared to standard Ramsey interferometry can be gained. This improvement is not an improvement in scaling, i.e. the estimation precision has the same scaling with the number of atoms as the standard q…
Interferometric signals are degraded by decoherence, which encompasses dephasing, mixing and any distinguishing which-path information. These three paradigmatic processes are fundamentally different, but, for coherent, single-photon and $N00N$-states, they degrade interferometric visibility in the very same way, which impedes the diagnosis of the cause for reduced visibility in a single experiment. We introduce a versatile formalism for many-boson interferometry based on double-sided Feynman diagrams, which we apply to a protocol for differential decoherence diagnosis: Twin-Fock states |N,N> w…
A Bose-Einstein "double-slit" interferometer has been recently realized experimentally by (Y. Shin et. al., Phys. Rev. Lett. 92 50405 (2004)). We analyze the interferometric steps by solving numerically the time-dependent Gross-Pitaevski equation in three-dimensional space. We focus on the adiabaticity time scales of the problem and on the creation of spurious collective excitations as a possible source of the strong dephasing observed experimentally. The role of quantum fluctuations is discussed.
This chapter reviews recent experiments on matter wave interferometry with large molecules. Starting from an elementary introduction to matter wave physics we discuss far-field diffraction and near-field interferometry with thermally excited many-body systems. We describe the constraints imposed by decoherence and dephasing effects, and present an outlook to the future challenges in macromolecule and cluster interferometry.
A full treatment of decoherence and dephasing effects in BEC interferometry has been developed based on using quantum correlation functions for treating interferometric effects. The BEC is described via a phase space distribution functional of the Wigner type for the condensate modes and the positive P type for the non-condensate modes. Ito equations for stochastic condensate and non-condensate field functions replace the functional Fokker-Planck equation for the distribution functional and stochastic averages of field function products determine the quantum correlation functions.
We present a detailed derivation of a model to study effects of self-gravitation from semi-classical gravity, described by the Schrödinger-Newton equation, employing spin superposition states in inhomogeneous magnetic fields, as proposed recently for experiments searching for gravity induced entanglement. Approximations for the experimentally relevant limits are discussed. Results suggest that spin interferometry could provide a more accessible route towards an experimental test of quantum aspects of gravity than both previous proposals to test semi-classical gravity and the observation of gra…
A new type of electron sources has emerged which permits to inject particles in a controllable manner, one at a time, into an electronic circuit. Such single electron sources make it possible to fully exploit the particles' quantum nature. We determine the single-particle coherence length from the decay of the Aharonov-Bohm oscillations as a function of the imbalance of a Mach-Zehnder interferometer connected to a single electron source. The single-particle coherence length is of particular importance as it is an intrinsic property of the source in contrast to the dephasing length.
We study Landau-Zener dynamics in a double quantum dot filled with two electrons, where the spin states can become correlated with charge states and the level velocity can be tuned in a time-dependent fashion. We show that a correct interpretation of experimental data is only possible when finite-time effects are taken into account. In addition, our formalism allows the study of partial adiabatic dynamics in the presence of phonon-mediated hyperfine relaxation and charge-noise-induced dephasing. Our findings demonstrate that charge noise severely impacts the visibility of Landau-Zener-Stückelb…
The loss of contrast in double-slit electron-diffraction due to dephasing and decoherence processes is studied. It is shown that the spatial correlation function of diffraction patterns can be used to distinguish between dephasing and decoherence. This establishes a measure of time-reversibility that does not require the determination of coherence terms of the density matrix, while von Neumann entropy, another measure of time-reversibility, does require coherence terms. This technique is exciting in view of the need to understand and control the detrimental experimental effects of contrast los…
We study the loss of spatial coherence in the extended wave function of fullerenes due to collisions with background gases. From the gradual suppression of quantum interference with increasing gas pressure we are able to support quantitatively both the predictions of decoherence theory and our picture of the interaction process. We thus explore the practical limits of matter wave interferometry at finite gas pressures and estimate the required experimental vacuum conditions for interferometry with even larger objects.
We report on a demonstration of Ramsey interferometry by three-dimensional motion with a trapped $^{171}Yb^+$ ion. We applied a momentum kick to the ion in a direction diagonal to the trap axes to initiate three-dimensional motion using a mode-locked pulse laser. The interference signal was analyzed theoretically to demonstrate three-dimensional matter-wave interference. This work paves the way to realizing matter-wave interferometry using trapped ions.
Landau-Zener-Stuckelberg interferometry has been extensively investigated in quantum two-level systems, with particular interests on artificial system such as superconducting flux qubits. With increasing the driving field amplitude, more energy levels will be involved into the quantum evolution, which results in population inversion and many interesting interference patterns. These interference patterns can be used to obtain the parameters characterizing the system and probe dephasing mechanisms of the qubit. Most recently, experiments have been extended to the regime with higher-frequency and…
Enhanced Dark Matter Quantum Sensing via Phase-Space Geometric Interferometry
International Center for Quantum-field Measurement Systems for Studies of the Universe and Particles (QUP, WPI), High Energy Accelerator Research Organization (KEK)（宇宙与粒子研究量子场测量系统国际中心（QUP，WPI），高能加速器研究机构（KEK））；Kavli IPMU (WPI), UTIAS, University of Tokyo（Kavli 宇宙起源研究所（WPI），东京大学宇宙线研究所（UTIAS））
Starting from an elementary model and refining it to take into account more realistic effects, we discuss the limitations and advantages of matter-wave interferometry in different configurations. We focus on the possibility to apply this approach to scenarios involving antimatter, such as positrons and positronium atoms. In particular, we investigate the Talbot-Lau interferometer with material gratings and discuss in details the results in view of the possible experimental verification.
We investigated the estimation of an unknown Gaussian process (containing displacement, squeezing and phase-shift) applied to a matter system. The state of the matter system is not directly measured; instead, we measure an optical mode which interacts with the system. We propose an interferometric setup exploiting a beam-splitter-type of light-matter interaction with homodyne detectors and two methods of estimation. We demonstrate the superiority of the interferometric setup over alternative non-interferometric schemes. Importantly, we show that even limited coupling strength and a noisy matte…
Stochastic backgrounds of gravitational waves are intrinsic fluctuations of spacetime which lead to an unavoidable decoherence mechanism. This mechanism manifests itself as a degradation of the contrast of quantum interferences. It defines an ultimate decoherence border for matter-wave interferometry using larger and larger molecules. We give a quantitative characterization of this border in terms of figures involving the gravitational environment as well as the sensitivity of the interferometer to gravitational waves. The known level of gravitational noise determines the maximal size of the m…
We discuss modern developments in quantum optics with organic molecules, clusters and nanoparticles -- in particular recent realizations of near-field matter-wave interferometry. A unified theoretical description in phase space allows us to describe quantum interferometry in position space and in the time domain on an equal footing. In order to establish matter-wave interferometers as a universal tool, which can accept and address a variety of nanoparticles, we elaborate on new quantum optical elements, such as diffraction gratings made of matter and light, as well as their absorptive and disp…
In this comment, we agree with the formulas derived in Refs. [1,2] but show that the results are not due to "interference between spatially separated states of the center of mass of a mesoscopic harmonic oscillator".
Matter-wave interferometry is a direct test of the quantum superposition principle for massive systems, and of collapse models. Here we show that the bounds placed by matter-wave interferometry depend weakly on the details of the collapse mechanism. Specifically, we compute the bounds on the CSL model and its variants, provided by the the KDTL interferometry experiment of Arndt's group [Phys. Chem. Chem. Phys., 2013, 15, 14696-14700], which currently holds the record of largest mass in interferometry. We also show that the CSL family of models emerges naturally by considering a minimal set of …
We extend the theory of matter-wave interferometry of point-like particles to non-spherical objects by taking the orientational degrees of freedom into account. In particular, we derive the grating transformation operator, that maps the impinging state onto the outgoing state, for a general, orientation-dependent interaction potential between the grating and the molecule. The grating operator is then worked out for the diffraction of symmetric top molecules from standing light waves, and the resulting interference pattern is calculated in the near-field. This allows us to identify a signature …
We establish a rigorous quantitative connection between (i) the interferometric duality relation for which-way information and fringe visibility and (ii) Heisenberg's uncertainty relation for position and modular momentum. We apply our theory to atom interferometry, wherein spontaneously emitted photons provide which way information, and unambiguously resolve the challenge posed by the metamaterial `perfect lens' to complementarity and to the Heisenberg-Bohr interpretation of the Heisenberg microscope thought experiment.
Interferometers with single particles are susceptible for dephasing perturbations from the environment, such as electromagnetic oscillations or mechanical vibrations. On the one hand, this limits sensitive quantum phase measurements as it reduces the interference contrast. On the other hand, it enables single-particle interferometers to be used as sensitive sensors for electromagnetic and mechanical perturbations. Recently, it was demonstrated experimentally, that a second-order correlation analysis can decrease the shielding and damping requirements significantly. Thereby, the relevant matter…
Attosecond Path Qubits in High-Harmonic Generation: Classical Dephasing and Trace-Out Decoherence
Guangdong Technion - Israel Institute of Technology（广东以色列理工学院）；Technion – Israel Institute of Technology（以色列理工学院）；Eastern Institute of Technology（东方理工大学）
The superposition principle is one of the bizarre predictions of quantum mechanics. Nevertheless, it has been experimentally verified using electrons, photons, atoms, and molecules. In this article, using a $20~$nm levitated ferromagnetic FePt nanoparticle, an exotic all optical spin polarization technique and the matter-wave interferometry, we show that a mesoscopic spatial Schrodinger cat can be created. Additionally, we argue that the maximum spatial separation between the delocalized wavepackets can be $25~μm$ and is significantly larger than the object itself.
The theory of linear quantum measurement has been developed for analysing the sensitivities of experimental devices that measure extremely weak signals, such as gravitational waves. It has successfully contributed to the theoretical understanding of laser interferometer gravitational-wave detectors (used by LIGO, VIRGO and KaGRA) and helped many important experimental upgrades. In this work, we establish a linear quantum measurement theory for another kind of measurement device--- matter wave interferometers, which has been widely discussed as an important platform for many high-precision expe…
We consider a large class of Ramsey interferometry protocols which are enhanced by squeezing and un-squeezing operations before and after a phase signal is imprinted on the collective spin of $N$ particles. We report an analytical optimization for any given particle number and strengths of (un-)squeezing. These results can be applied even when experimentally relevant decoherence processes during the squeezing and un-squeezing interactions are included. Noise between the two interactions is however not considered in this work. This provides a generalized characterization of squeezing echo proto…
We discuss the dephasing induced by the internal classical chaotic motion in the absence of any external environment. To this end a new extension of fidelity for mixed states is introduced, which we name {\it allegiance}. Such quantity directly accounts for quantum interference and is measurable in a Ramsey interferometry experiment. We show that in the semiclassical limit the decay of the allegiance is exactly expressed, due to the dephasing, in terms of an appropriate classical correlation function. Our results are derived analytically for the case of a nonlinear driven oscillator and then n…
Matter-wave interferometry is a highly sensitive tool to measure small perturbations in a quantum system. This property allows the creation of precision sensors for dephasing mechanisms such as mechanical vibrations. They are a challenge for phase measurements under perturbing conditions that cannot be perfectly decoupled from the interferometer, e.g. for mobile interferometric devices or vibrations with a broad frequency range. Here, we demonstrate a method based on second-order correlation theory in combination with Fourier analysis, to use an electron interferometer as a sensor that precise…
Imaging of surface adsorbed molecules is investigated as a novel detection method for matter wave interferometry with fluorescent particles. Mechanically magnified fluorescence imaging turns out to be an excellent tool for recording quantum interference patterns. It has a good sensitivity and yields patterns of high visibility. The spatial resolution of this technique is only determined by the Talbot gratings and can exceed the optical resolution limit by an order of magnitude. A unique advantage of this approach is its scalability: for certain classes of nano-sized objects, the detection sens…
Extending the range of quantum interferometry to a wider class of composite nanoparticles requires new tools to diffract matter waves. Recently, pulsed photoionization light gratings have demonstrated their suitability for high mass matter-wave physics. Here we extend quantum interference experiments to a new class of particles by introducing photofragmentation beam splitters into time-domain matter-wave interferometry. Photofragmentation gratings can act on objects as different as van der Waals clusters and biomolecules which are thermally unstable and often resilient to single-photon ionizat…
A two-slit interference of a massive particle in the presence of environment induced decoherence is theoretically analyzed using a fully quantum mechanical calculation. The Markovian Master equation, derived from coupling the particle to a harmonic-oscillator heat bath, is used to obtain exact solutions which show the existence of an interference. Interestingly, decoherence does not affect the pattern, but only leads to a reduction in the fringe visibility.
We propose to test the theory of continuous spontaneous localization (CSL) in an all-optical time-domain Talbot-Lau interferometer for clusters with masses exceeding 1000000 amu. By assessing the relevant environmental decoherence mechanisms, as well as the growing size of the particles relative to the grating fringes, we argue that it will be feasible to test the quantum superposition principle in a mass range excluded by recent estimates of the CSL effect.
Matter-wave interferometry of ultra-cold atoms with attractive interactions is studied at the full many-body level. First, we study how a coherent light-pulse applied to an initially-condensed solitonic system splits it into two matter-waves. The split system looses its coherence and develops correlations with time, and inevitably becomes fragmented due to inter-particle attractions. Next, we show that by re-colliding the sub-clouds constituting the split density together, along with a simultaneous application of the same laser-pulse, one creates three matter-waves propagating with different m…
Quantum superposition is central to quantum theory but challenges our concepts of reality and spacetime when applied to macroscopic objects like Schrödinger's cat. For that reason, it has been a long-standing question whether quantum physics remains valid unmodified even for truly macroscopic objects. By now, the predictions of quantum theory have been confirmed via matter-wave interferometry for massive objects up to $10^4\,$ atomic mass units (amu). The rapid development of new technologies promises to soon allow tests of quantum theory for significantly higher test masses by using novel tec…
Usually, decoherence is generated from the coupling with an outer environment. However, a macroscopic object generically possesses its own environment in itself, namely the complicated dynamics of internal degrees of freedom. We address a question: when and how the internal dynamics decohere interference of the center of mass motion of a macroscopic object. We will also show that weak localization of a macroscopic object in disordered potentials can be destroyed by such decoherence.
The study of molecular physics using ultracold gases has provided a unique probe into the fundamental properties of nature and offers new tools for quantum technologies. In this article we outline how the use of a space environment to study ultracold molecular physics opens opportunities for 1) exploring ultra-low energy regimes of molecular physics with high efficiency, 2) providing a toolbox of capabilities for fundamental physics, and 3) enabling new classes of matter-wave interferometers with applications in precision measurement for fundamental and many-body physics.
We study the quantum dynamics of a two-mode Bose-Einstein condensate in a time-dependent symmetric double-well potential using analytical and numerical methods. The effects of internal degrees of freedom on the visibility of interference fringes during a stage of ballistic expansion are investigated varying particle number, nonlinear interaction sign and strength as well as tunneling coupling. Expressions for the phase resolution are derived and the possible enhancement due to squeezing is discussed. In particular, the role of the superfluid - Mott insulator cross-over and its analog for attra…
In this paper we study entropy production and transport of heat and matter in an 1D bipartite fermionic chain. Moreover, we input a phenomenological dephasing noise in order to show its effect on the dynamics of the system. Specially, it is shown the importance of such noise in the emergence of the entropy production. For the fluxes, analytical solutions are obtained using both Boltzmann and Fermi-Dirac distribuition. Finally, we show that a particular fluctuation theorem for energy and matter exchange is obeyed even in the presence of such noise.
We propose a mechanism to use nonlinearity arising from inter-particle interactions to significantly enhance rotation sensitivity of matter-wave interferometers. The method relies on modifying Sagnac interferometers by introducing a weak circular lattice potential that couples modes with opposite orbital angular momenta (OAM). The primary observable comprises of the modal population distributions measured at particular times. This provides an alternate mechanism for rotation sensing that requires substantially smaller ring size, even in the linear non-interacting regime. Nonlinearity can impro…
The quantum world distinguishes itself from the classical world by being governed by probability amplitudes rather than probabilities. On a single-particle level, quantum phases can be manipulated leading to observable interference patterns that can be used as a probe e.g. in matter wave microscopy. But the quantum world bears even more fascinating effects when it comes to the interplay between more than one particle. Correlations between quantum particles such as entanglement can be exploited to speed up computational algorithms or enable secure cryptography. Here, we propose and numerically …
We assess the most macroscopic matter-wave experiments to date as to the extent to which they probe the quantum-classical boundary by demonstrating interference of heavy molecules and cold atomic ensembles. To this end, we consider a rigorous Bayesian test protocol for a parametrized set of hypothetical modifications of quantum theory, including well-studied spontaneous collapse models, that destroy superpositions and reinstate macrorealism. The range of modification parameters ruled out by the measurement events quantifies the macroscopicity of a quantum experiment, while the shape of the pos…
There has been considerable recent interest in the mean-field dynamics of various atom-interferometry schemes designed for precision sensing. In the field of quantum metrology, the standard tools for evaluating metrological sensitivity are the classical- and quantum-Fisher information. In this letter, we show how these tools can be adapted to evaluate the sensitivity when the behaviour is dominated by mean-field dynamics. As an example, we compare the behaviour of four recent theoretical proposals for gyroscopes based on matterwaves interference in toroidally trapped geometries. We show that w…
Quantum annealing is explored as a resource for quantum information beyond solution of classical combinatorial problems. Envisaged as a generator of robust interferometric probes, we examine a Hamiltonian of $N>> 1$ uniformly-coupled spins subject to a transverse magnetic field. The discrete many-body problem is mapped onto dynamics of a single one-dimensional particle in a continuous potential. This reveals all the qualitative features of the ground state beyond typical mean-field or large classical spin models. It illustrates explicitly a graceful warping from an entangled unimodal to bi-mod…
Optical interferometry has been a long-standing setup for characterization of quantum states of light. Both the linear and the nonlinear interferences can provide information about the light statistics an underlying detail of the light-matter interactions. Here we demonstrate how interferometric detection of nonlinear spectroscopic signals may be used to improve the measurement accuracy of matter susceptibilities. Light-matter interactions change the photon statistics of quantum light, which are encoded in the field correlation functions. Application is made to the Hong-Ou-Mandel two-photon in…
