Photons are natural carriers of quantum information due to their ease of distribution and long lifetime. This thesis concerns various related aspects of quantum information processing with single photons. Firstly, we demonstrate N-photon entanglement generation through a generalised N X N symmetric beam splitter known as the Bell multiport. A wide variety of 4-photon entangled states as well as the N-photon W-state can be generated with an unexpected non-monotonic decreasing probability of success with N. We also show how the same setup can be used to generate multiatom entanglement. A further study of multiports also leads us to a multiparticle generalisation of the Hong-Ou-Mandel dip which holds for all Bell multiports of even number of input ports. Next, we demonstrate a generalised linear optics based photon filter that has a constant success probability regardless of the number of photons involved. This filter has the highest reported success probability and is interferometrically robust. Finally, we demonstrate how repeat-until-success quantum computing can be performed with two distant nodes with unit success probability using only linear optics resource. We further show that using non-identical photon sources, robustness can still be achieved, an illustration of the nature and advantages of measurement-based quantum computation. A direct application to the same setup leads naturally to arbitrary multiphoton state generation on demand. Finally, we demonstrate how polarisation entanglement of photons can be detected from the emission of two atoms in a Young's double-slit type experiment without linear optics, resulting in both atoms being also maximally entangled.
We answer the question whether linear-optical processing of the states produced by one or multiple imperfect single-photon sources can improve the single-photon fidelity. This processing can include arbitrary interferometers, coherent states, feedforward, and conditioning on results of detections. We show that without introducing multiphoton components, the single-photon fraction in any of the single-mode states resulting from such processing cannot be made to exceed the efficiency of the best available photon source. If multiphoton components are allowed, the single-photon fidelity cannot be …
We demonstrate two key components for optical quantum information processing: a bright source of heralded single photons; and a bright source of entangled photon pairs. A pair of pump photons produces a correlated pair of photons at widely spaced wavelengths (583 nm and 900 nm), via a $χ^{(3)}$ four-wave mixing process. We demonstrate a non-classical interference between heralded photons from independent sources with a visibility of 95%, and an entangled photon pair source, with a fidelity of 89% with a Bell state.
We show that the two-photon transition rates of quantum dots coupled to nanocavities are enhanced by up to 8 orders of magnitude relative to quantum dots in bulk host. We then propose how to take advantage of this enhancement to implement coherent quantum dot excitation by two-photon absorption, entangled photon pair generation by two-photon spontaneous emission, and single-photon generation at telecommunication wavelengths by two-photon stimulated and spontaneous emission.
By virtue of a silicon high-Q photonic crystal nanocavity, we propose and examine theoretically interactions between a stationary electron spin qubit of a semiconductor nanocrystal and a flying photon qubit. Firstly, we introduce, derive and demonstrate for the first time the explicit conditions towards realization of a spin-photon two-qubit phase gate, and propose these interactions as a generalized quantum interface for quantum information processing. Secondly, we examine novel single-spin-induced reflections as direct evidence of intrinsic bare and dressed modes in our coupled nanocrystal-c…
Random nonlinear layered structures have been found to be a useful source of photon pairs with perfectly indistinguishable un-entangled photons emitted into a very narrow spectral range. Localization of the interacting optical fields typical for random structures gives relatively high photon-pair fluxes. Superposing photon-pair emission quantum paths at different emission angles, several kinds of two-photon states (including states with coincident frequencies) useful in quantum-information processing can easily be generated.
Photonic quantum information processing schemes, such as linear optics quantum computing, and other experiments relying on single-photon interference, inherently require complete photon indistinguishability to enable the desired photonic interactions to take place. Mode-mismatch is the dominant cause of photon distinguishability in optical circuits. Here we study the effects of photon wave-packet shape on tolerance against the effects of mode-mismatch in linear optical circuits, and show that Gaussian distributed photons with large bandwidth are optimal. The result is general and holds for arb…
Information processing with light is ubiquitous, from communication, metrology and imaging to computing. When we consider light as a quantum mechanical object, new ways of information processing become possible. In this review I give an overview how quantum information processing can be implemented with single photons, and what hurdles still need to be overcome to implement the various applications in practice. I will place special emphasis on the quantum mechanical properties of light that make it different from classical light, and how these properties relate to quantum information processin…
Characterising the input-output photon-number distribution of an unknown optical quantum channel is an important task for many applications in quantum information processing. Ideally, this would require deterministic photon-number sources and photon-number-resolving detectors, but these technologies are still work-in-progress. In this work, we propose a general method to rigorously bound the input-output photon number distribution of an unknown optical channel using standard optical devices such as coherent light sources and non-photon-number-resolving detectors/homodyne detectors. To demonstr…
In the last two decades, many quantum optics experiments have demonstrated small-scale quantum information processing applications with several photons. Beyond such proof-of-principle demonstrations, efficient preparation of large, but definite, numbers of photons is of great importance for further scaling up and speeding up photonic quantum information processing. Typical single-photon generation techniques based on nonlinear parametric processes face challenges of probabilistic generation. Here we demonstrate efficient synchronization of photons from multiple nonlinear parametric heralded si…
We analyze the problem of increasing the efficiency of single-photon sources or single-rail photonic qubits via linear optical processing and destructive conditional measurements. In contrast to previous work we allow for the use of coherent states and do not limit to photon-counting measurements. We conjecture that it is not possible to increase the efficiency, prove this conjecture for several important special cases, and provide extensive numerical results for the general case.
We experimentally demonstrate a bright pulsed source of correlated photon pairs at 1550 nm telecom band by pumping 300 m dispersion shifted fiber with a 4 ps pulse train. We investigate the coherence property of the source by measuring the second order intensity correlation function $g^{(2)}$ of individual signal (idler) photons. A preliminary Hong-Ou-Mandel type two-photon interference experiment with two such sources confirms the high temporal and spatial coherence of the source. The source is suitable for multi-photon quantum interference of independent sources, required in quantum informat…
Multi-photon states are widely applied in quantum information technology. By the methods presented in this paper, the structure of a multi-photon state in the form of multiple single photon qubit product can be mapped to a single photon qudit, which could also be in separable product with other photons. This makes the possible manipulation of such multi-photon states in the way of processing single photon states. The optical realization of unknown qubit discrimination [B. He, J. A. Bergou, and Y.-H. Ren, Phys. Rev. A 76, 032301 (2007)] is simplified with the transformation methods. Another app…
Both cavity QED and photons are promising candidates for quantum information processing. We consider a combination of both candidates with a single photon going through spatially separate cavities to entangle the atomic qubits, based on the input-output process of the cavities. We present a general expression for the input-output process regarding the low-Q cavity confining a single atom, which works in a wide range of parameters. Focusing on low-Q cavity case, we propose some schemes for quantum information processing with Faraday rotation using single photons, which is much different from th…
A fundamental element of quantum information processing with photonic qubits is the nonclassical quantum interference between two photons when they bunch together via the Hong-Ou-Mandel (HOM) effect. Ultimately, many such pure photons must be processed in complex interferometric networks, and for this it is essential to synchronize the arrival times of the flying photons preserving their purity. Here we demonstrate for the first time the HOM interference of two heralded, pure optical photons synchronized through two independent quantum memories. Controlled storage times up to 1.8 microseconds …
How to implement multi-qubit gates is an important problem in quantum information processing. Based on cross phase modulation, we present an approach to realizing a family of multi-qubit gates that deterministically operate on single photons as the qubits. A general $n$-qubit unitary operation is a typical example of these gates. The approach greatly relax the requirement on the resources, such as the ancilla photons and coherent beams, as well as the number of operations on the qubits. The improvement in this framework may facilitate large scale quantum information processing.
We study distinguishing information in the context of quantum interference involving more than one parametric downconversion (PDC) source and in the context of polarization-entangled photon pairs based on PDC. We arrive at specific design criteria for two-photon sources so that when used as part of complex optical systems, such as photon-based quantum information processing schemes, distinguishing information between the photons is eliminated guaranteeing high visibility interference. We propose practical techniques which lead to suitably engineered two-photon states that can be realistically …
We investigate the use of integrated, microfabricated photonic-atomic junctions for quantum information processing applications. The coupling between atoms and light is enhanced by using microscopic optics without the need for cavity enhancement. Qubits that are collectively encoded in hyperfine states of small ensembles of optically trapped atoms, coupled via the Rydberg blockade mechanism, seem a particularly promising implementation. Fast and high-fidelity gate operations, efficient readout, long coherence times and large numbers of qubits are all possible.
Photonic quantum technologies represent a promising platform for several applications, ranging from long-distance communications to the simulation of complex phenomena. Indeed, the advantages offered by single photons do make them the candidate of choice for carrying quantum information in a broad variety of areas with a versatile approach. Furthermore, recent technological advances are now enabling first concrete applications of photonic quantum information processing. The goal of this manuscript is to provide the reader with a comprehensive review of the state of the art in this active field…
We show that pairs of atoms optically excited to the Rydberg states can strongly interact with each other via effective long-range dipole-dipole or van der Waals interactions mediated by their non-resonant coupling to a common microwave field mode of a superconducting coplanar waveguide cavity. These cavity mediated interactions can be employed to generate single photons and to realize in a scalable configuration a universal phase gate between pairs of single photon pulses propagating or stored in atomic ensembles in the regime of electromagnetically induced transparency.
Multi-photon interference is at the heart of photonic quantum technologies. Arrays of integrated cavities can support bright sources of single-photons with high purity and small footprint, but the inevitable spectral distinguishability between photons generated from non-identical cavities is an obstacle to scaling. In principle, this problem can be alleviated by measuring photons with high timing resolution, which erases spectral information through the time-energy uncertainty relation. Here, we experimentally demonstrate that detection can be implemented with a temporal resolution sufficient …
Quantum technologies are the next big revolution in information technologies, computing, communication security, sensing as well as metrology. What do you use to explore all these fascinating applications when you work in Optics? Photons of course. In this review, we discuss the different available single photon source technologies, compare and contrast them in terms of applicability and properties, discuss state of the art and conclude that the future is indeed bright!
The Visible Light Photon Counter (VLPC) features high quantum efficiency and low pulse height dispersion. These properties make it ideal for efficient photon number state detection. The ability to perform efficient photon number state detection is important in many quantum information processing applications, including recent proposals for performing quantum computation with linear optical elements. In this paper we investigate the unique capabilities of the VLPC. The efficiency of the detector and cryogenic system is measured at 543nm wavelengths to be 85%. A picosecond pulsed laser is then u…
Integrated optics is an engineering solution proposed for exquisite control of photonic quantum information. Here we use silicon photonics and the linear combination of quantum operators scheme to realise a fully programmable two-qubit quantum processor. The device is fabricated with readily available CMOS based processing and comprises four nonlinear photon-sources, four filters, eighty-two beam splitters and fifty-eight individually addressable phase shifters. To demonstrate performance, we programmed the device to implement ninety-eight various two-qubit unitary operations (with average qua…
The mapping of photonic states to collective excitations of atomic ensembles is a powerful tool which finds a useful application in the realization of quantum memories and quantum repeaters. In this work we show that cold atoms in optical lattices can be used to perform an entangling unitary operation on the transferred atomic excitations. After the release of the quantum atomic state, our protocol results in a deterministic two qubit gate for photons. The proposed scheme is feasible with current experimental techniques and robust against the dominant sources of noise.
Decoherence-free states protect quantum information from collective noise, the predominant cause of decoherence in current implementations of quantum communication and computation. Here we demonstrate that spontaneous parametric down-conversion can be used to generate four-photon states which enable the encoding of one qubit in a decoherence-free subspace. The immunity against noise is verified by quantum state tomography of the encoded qubit. We show that particular states of the encoded qubit can be distinguished by local measurements on the four photons only.
We propose the implementation of a light source, which can deterministically generate a rich variety of multi-mode quantum states. The desired states are encoded in the collective population of different ground hyperfine states of an atomic ensemble and converted to multi-mode photonic states by excitation to optically excited levels followed by cooperative spontaneous emission. Among our examples of applications, we demonstrate how two-photon entangled states can be prepared and implemented in a protocol for reference frame free quantum key distribution and how one-dimensional as well as high…
Among the objectives toward large-scale quantum computation is the quantum interconnect: a device which uses photons to interface qubits that otherwise could not interact. However, current approaches require photons indistinguishable in frequency---a major challenge for systems experiencing different local environments or of different physical compositions altogether. Here we develop an entirely new platform which actually exploits such frequency mismatch for processing quantum information. Labeled "spectral linear optical quantum computation" (spectral LOQC), our protocol offers favorable lin…
We compare effects of decoherence and detection inefficiency on entangled coherent states (ECSs) and entangled photon pairs (EPPs), both of which are known to be particularly useful for quantum information processing (QIP). When decoherence effects caused by photon losses are heavy, the ECSs outperform the EPPs as quantum channels for teleportation both in fidelities and in success probabilities. On the other hand, when inefficient detectors are used, the teleportation scheme using the ECSs suffers undetected errors that result in the degradation of fidelity, while this is not the case for the…
Lecture Notes of the Les Houches Summer School 2003 on Quantum entanglement and information processing to be published as P. Zoller, J. I. Cirac, Luming Duan and J. J. Garcia-Ripoll, in "Quantum entanglement and information processing", Proceedings of the Les Houches Summer School, Session 79, edited by D. Est{è}ve, J.M. Raimond and J. Dalibard (Elsevier, Amsterdam, 2004). This is an updated although shortened version of J. I. Cirac, L. M. Duan, and P. Zoller, in "Quantum optical implementation of quantum information processing", Proceedings of the International School of Physics "Enrico Fermi…
Recirculating Quantum Photonic Networks for Fast Deterministic Quantum Information Processing
DTU Electro, Technical University of Denmark(丹麦技术大学电气工程系);NanoPhoton - Center for Nanophotonics, Technical University of Denmark(丹麦技术大学纳米光子学中心);Department of Electrical Engineering and Computer Science, Massachusetts Institute of Technology(麻省理工学院电气工程和计算机科学系)
We propose a Bell measurement scheme by employing a logical qubit in Greenberger-Horne-Zeilinger (GHZ) entanglement with an arbitrary number of photons. Remarkably, the success probability of the Bell measurement as well as teleportation of the GHZ entanglement can be made arbitrarily high using only linear optics elements and photon on-off measurements as the number of photons increases. Our scheme outperforms previous proposals using single photon qubits when comparing the success probabilities in terms of the average photon usages. It has another important advantage for experimental feasibi…
We develop an experimental scheme based on a continuous-wave (cw) laser for generating arbitrary superpositions of photon number states. In this experiment, we successfully generate superposition states of zero to three photons, namely advanced versions of superpositions of two and three coherent states. They are fully compatible with developed quantum teleportation and measurement-based quantum operations with cw lasers. Due to achieved high detection efficiency, we observe, without any loss correction, multiple areas of negativity of Wigner function, which confirm strongly nonclassical natur…
We demonstrate polarization-entanglement for non-degenerate and degenerate photon-pairs generated through Kerr-nonlinearity in a nano-scale silicon-on-insulator(SOI) waveguide. We use a compact counter propagating configuration to create two-photon polarization-entangled state, |H>|H> + |V>|V>. We observe two-photon interference with visibility > 91% and > 80% for non-degenerate and degenerate photon-pairs, respectively. The experimental structure can be implemented on optical chips as an integrated source of entangled photons for future quantum computer and communication applications.
Physics and information are intimately connected, and the ultimate information processing devices will be those that harness the principles of quantum mechanics. Many physical systems have been identified as candidates for quantum information processing, but none of them are immune from errors. The challenge remains to find a path from the experiments of today to a reliable and scalable quantum computer. Here, we develop an architecture based on a simple module comprising an optical cavity containing a single negatively-charged nitrogen vacancy centre in diamond. Modules are connected by photo…
Triggered single-photon sources produce the vacuum state with non-negligible probability, but produce a much smaller multiphoton component. It is therefore reasonable to approximate the output of these photon sources as a mixture of the vacuum and single-photon states. We show that it is impossible to increase the probability for a single photon using linear optics and photodetection on fewer than four modes. This impossibility is due to the incoherence of the inputs; if the inputs were pure-state superpositions, it would be possible to obtain a perfect single-photon output. In the more genera…
Photons have been a flagship system for studying quantum mechanics, advancing quantum information science, and developing quantum technologies. Quantum entanglement, teleportation, quantum key distribution and early quantum computing demonstrations were pioneered in this technology because photons represent a naturally mobile and low-noise system with quantum-limited detection readily available. The quantum states of individual photons can be manipulated with very high precision using interferometry, an experimental staple that has been under continuous development since the 19th century. The …
We present a scheme for scalable quantum information processing (QIP) with atomic ensembles and flying photons. Using the Rydberg blockade, we encode the qubits in the collective atomic states, which could be manipulated fast and easily due to the enhanced interaction, in comparison to the single-atom case. We demonstrate that our proposed gating could be applied to generation of two-dimensional cluster states for measurement-based quantum computation. Moreover, the atomic ensembles also function as quantum repeaters useful for long distance quantum state transfer. We show the possibility of o…
We implement the squeezing operation as a genuine quantum gate, deterministically and reversibly acting `online' upon an input state no longer restricted to the set of Gaussian states. More specifically, by applying an efficient and robust squeezing operation for the first time to non-Gaussian states, we demonstrate a two-way conversion between a particle-like single-photon state and a wave-like superposition of coherent states. Our squeezing gate is reliable enough to preserve the negativities of the corresponding Wigner functions. This demonstration represents an important and necessary step…
Uniting Quantum Processing Nodes of Cavity-coupled Ions with Rare-earth Quantum Repeaters Using Single-photon Pulse Shaping Based on Atomic Frequency Comb
The quantum state of a single photon stands among the most fundamental and intriguing manifestations of quantum physics. At the same time single photons and pairs of single photons are important building blocks in the fields of linear optical based quantum computation and quantum repeater infrastructure. These fields possess enormous potential and much scientific and technological progress has been made in developing individual components, like quantum memories and photon sources using various physical implementations. However, further progress suffers from the lack of compatibility between th…
Photonic processors are pivotal for both quantum and classical information processing tasks using light. In particular, linear optical quantum information processing requires both largescale and low-loss programmable photonic processors. In this paper, we report the demonstration of the largest universal quantum photonic processor to date: a low-loss, 12-mode fully tunable linear interferometer with all-to-all coupling based on stoichiometric silicon nitride waveguides.
Many promising schemes for quantum information processing (QIP) rely on few-photon interference effects. In these proposals, the photons are treated as being indistinguishable particles. However, single photon sources are typically subject to variation from device to device. Thus the photons emitted from different sources will not be perfectly identical, and there will be some variation in their frequencies. Here, we analyse the effect of this frequency mismatch on QIP schemes. As examples, we consider the distributed QIP protocol proposed by Barrett and Kok, and Hong-Ou-Mandel interference wh…
We describe how strong resonant interactions in multimode optomechanical systems can be used to induce controlled nonlinear couplings between single photons and phonons. Combined with linear mapping schemes between photons and phonons, these techniques provide a universal building block for various classical and quantum information processing applications. Our approach is especially suited for nano-optomechanical devices, where strong optomechanical interactions on a single photon level are within experimental reach.
Device-independent quantum key distribution provides security even when the equipment used to communicate over the quantum channel is largely uncharacterized. An experimental demonstration of device-independent quantum key distribution is however challenging. A central obstacle in photonic implementations is that the global detection efficiency, i.e., the probability that the signals sent over the quantum channel are successfully received, must be above a certain threshold. We here propose a method to significantly relax this threshold, while maintaining provable device-independent security. T…
We report the experimental demonstration of four-photon quantum interference using telecom-wavelength photons. Realization of multi-photon quantum interference is essential to linear optics quantum information processing and measurement-based quantum computing. We have developed a source that efficiently emits photon pairs in a pure spectrotemporal mode at a telecom wavelength region, and have demonstrated the quantum interference exhibiting the reduced fringe intervals that correspond to the reduced de Broglie wavelength of up to the four photon `NOON' state. Our result should open a path to …
Hyperentanglement is a promising resource in quantum information processing with its high capacity character, defined as the entanglement in multiple degrees of freedom (DOFs) of a quantum system, such as polarization, spatial-mode, orbit-angular-momentum, time-bin and frequency DOFs of photons. Recently, hyperentanglement attracts much attention as all the multiple DOFs can be used to carry information in quantum information processing fully. In this review, we present an overview of the progress achieved so far in the field of hyperentanglement in photon systems and some of its important app…
Entanglement is an essential resource in current experimental implementations for quantum information processing. We review a class of experiments exploiting photonic entanglement, ranging from one-way quantum computing over quantum communication complexity to long-distance quantum communication. We then propose a set of feasible experiments that will underline the advantages of photonic entanglement for quantum information processing.
In spontaneous parametric down conversion (SPDC) based quantum information processing (QIP) experiments, there is a tradeoff between the coincide count rates (i.e. the pumping power of the SPDC), which limits the rate of the protocol, and the visibility of the quantum interference, which limits the quality of the protocol. This tradeoff is mainly caused by the multi-photon pair emissions from the SPDCs. In theory, the problem is how to model the experiments without truncating these multi-photon emissions while including practical imperfections. In this paper, we establish a method to theoretic…
Observables of quantum systems can posses either a discrete or a continuous spectrum. For example, upon measurements of the photon number of a light state, discrete outcomes will result whereas measurements of the light's quadrature amplitudes result in continuous outcomes. If one uses the continuous degree of freedom of a quantum system either for encoding, processing or detecting information, one enters the field of continuous variable (CV) quantum information processing. In this paper we review the basic principles of CV quantum information processing with main focus on recent developments …
Generations of technologies with fundamentally new information processing capabilities will emerge if microscopic physical systems can be controlled to encode, transmit, and process quantum information, at scale and with high fidelity. In the decade after its 2008 inception, the technology of integrated quantum photonics enabled the generation, processing, and detection of quantum states of light, at a steadily increasing scale and level of complexity. Using both established and advanced fabrication techniques, the field progressed from the demonstrations of fixed circuits comprising few compo…
We introduce a scheme to perform quantum-information processing that is based on a hybrid spin-photon qubit encoding. The proposed qubits consist of spin-ensembles coherently coupled to microwave photons in coplanar waveguide resonators. The quantum gates are performed solely by shifting the resonance frequencies of the resonators on a ns timescale. An additional cavity containing a Cooper-pair box is exploited as an auxiliary degree of freedom to implement two-qubit gates. The generality of the scheme allows its potential implementation with a wide class of spin systems.
We report the experimental resource-efficient implementation of the variational quantum eigensolver (VQE) using four-dimensional photonic quantum states of single-photons. The four-dimensional quantum states are implemented by utilizing polarization and path degrees of freedom of a single-photon. Our photonic VQE is equipped with the quantum error mitigation (QEM) protocol that efficiently reduces the effects of Pauli noise in the quantum processing unit. We apply our photonic VQE to estimate the ground state energy of He--H$^{+}$ cation. The simulation and experimental results demonstrate tha…
Large scale quantum information processing requires stable and long-lived quantum memories. Here, using atom-photon entanglement, we propose an experimentally feasible scheme to realize decoherence-free quantum memory with atomic ensembles, and show one of its applications, remote transfer of unknown quantum state, based on laser manipulation of atomic ensembles, photonic state operation through optical elements, and single-photon detection with moderate efficiency. The scheme, with inherent fault-tolerance to the practical noise and imperfections, allows one to retrieve the information in the…
We present a detailed analysis of the Bell measurement scheme proposed in [Phys. Rev. Lett. 114, 113603 (2015)] based on a logical qubit using Greenberger-Horne-Zeilinger (GHZ) entanglement of photons. The success probability of the proposed Bell measurement can be made arbitrarily high using only linear optics as the number of photons in a logical qubit increases. We compare our scheme with all the other proposals, using single-photon qubits, coherent-state qubits or hybrid qubits, suggested to enhance the efficiency of the Bell measurement. As a remarkable advantage, our scheme requires only…