We consider the interaction of atoms with the quantized electromagnetic field in the presence of materials with negative index of refraction. Spontaneous emission of an atom embedded in a negative index material is discussed. It is shown furthermore that the possibility of a vanishing optical path length between two spatially separated points provided by these materials can lead to complete suppression of spontaneous emission of an atom in front of a perfect mirror even if the distance between atom and mirror is large compared to the transition wavelength. Two atoms put in the focal points of a lens formed by a parallel slab of ideal negative index material are shown to exhibit perfect sub- and superradiance. The maximum length scale in both cases is limited only by the propagation distance within the free-space radiative decay time. Limitations of the predicted effects arising from absorption, finite transversal extension and dispersion of the material are analyzed.
We discuss the recent proposal by Thommen and Mandel (Phys. Rev. Lett. {\bf 96}, 053601 (2006)) for electromagnetically induced negative refraction. Although the main conclusion of the paper -- the possibility to achieve negative refraction in an experimentally accessible atomic scheme -- remains valid, we show that the weak-excitation approximation used is invalid in the parameter regime studied and leads to quantitatively incorrect predictions. We show that negative refraction is always accompanied by absorption rather than by gain, and that the maximum value of the refraction-absorption rat…
We formulate macroscopic quantum electrodynamics for the most general linear, absorbing media. In particular, Onsager reciprocity is not assumed to hold. For media with a non-local response, the field quantisation is based on the conductivity tensor and the Green tensor for the electromagnetic field. For a local medium response, we introduce the permittivity, permeability and magnetoelectric susceptibilities to obtain an explicitly duality-invariant scheme. We find that duality invariance only holds as a continuous symmetry when non-reciprocal responses are allowed for.
Refractive index enhancement accompanied by vanishing absorption in a four-level atomic system interacting with two control and two probe fields in a regime of four-wave mixing (FWM) has been predicted and studied in the present work. We analyzed the maximal index enhancement in the four-level FWM system and gave index estimates for a real atomic gas of $^{40}$K, taking into account its multilevel structure and collisional and Doppler broadenings at large atomic densities. We also discussed how vanishing absorption with no nearby amplification can be realized in a two species system, consistin…
We give a microscopic derivation of the Clausius-Mossotti relations for a homogeneous and isotropic magneto-dielectric medium consisting of radiatively broadened atomic oscillators. To this end the diagram series of electromagnetic propagators is calculated exactly for an infinite bi-cubic lattice of dielectric and magnetic dipoles for a lattice constant small compared to the resonance wavelength $λ$. Modifications of transition frequencies and linewidth of the elementary oscillators are taken into account in a selfconsistent way by a proper incorporation of the singular self-interaction terms…
We show that the material dependencies of macroscopically quantized fields in linear media are not consistent with the classical electromagnetic boundary conditions. We then phenomenologically construct macroscopic quantized fields that satisfy quantum--classical correspondence with the result indicating that the canonical momentum in a linear medium is modified as a consequence of the reduced speed of light. We re-derive D'Alembert's principle and Lagrange's equations for an arbitrarily large region of space in which light signals travel slower than in the vacuum and show that the resulting m…
The description of dispersion forces within the framework of macroscopic quantum electrodynamics in linear, dispersing, and absorbing media combines the benefits of approaches based on normal-mode techniques of standard quantum electrodynamics and methods based on linear response theory in a natural way. It renders generally valid expressions for both the forces between bodies and the forces on atoms in the presence of bodies, while showing very clearly the intimate relation between the different types of dispersion forces. By considering examples, the influence of various factors like form, s…
We discuss the feasibility of negative refraction with reduced absorption in coherently driven atomic media. Coherent coupling of an electric and a magnetic dipole transition by laser fields induces magneto-electric cross-coupling and negative refraction at dipole densities which are considerably smaller than necessary to achieve a negative permeability. At the same time the absorption gets minimized due to destructive quantum interference and the ratio of negative refraction index to absorption becomes orders of magnitude larger than in systems without coherent cross-coupling. The proposed sc…
We develop fluctuational electrodynamics for media with nonlinear optical response. In a perturbative manner, we amend the stochastic Helmholtz equation to describe fluctuations in a nonlinear setting, in agreement with the fluctuation dissipation theorem, and identify the local (Rytov) current fluctuations. We show how the linear response (the solution of the scattering problem) of a collection of objects is found from the individual responses, as measured in isolation. As an example, we compute the Casimir force acting between nonlinear objects which approaches the result for linear optics f…
We address two issues in the quantum electrodynamical description of photonic media with some disorder, neglecting material dispersion. When choosing a gauge in which the static potential vanishes, the normal modes of the medium with disorder satisfy another transversality condition than the modes of the ideal medium. Our first result is an integral equation for optical modes such that all perturbation-theory solutions automatically satisfy the desired transversality condition. Secondly, when expanding the vector potential for the medium with disorder in terms of the normal modes of the ideal …
The quantization of optical fields in vacuum has been known for decades, but extending the field quantization to lossy and dispersive media in nonequilibrium conditions has proven to be complicated due to the position-dependent electric and magnetic responses of the media. In fact, consistent position-dependent quantum models for the photon number in resonant structures have only been formulated very recently and only for dielectric media. Here we present a general position-dependent quantized fluctuational electrodynamics (QFED) formalism that extends the consistent field quantization to desc…
We study different architectures for a photonic crystal in the microwave regime based on superconducting transmission lines interrupted by Josephson junctions, both in one and two dimensions. A study of the scattering properties of a single junction in the line shows that the junction behaves as a perfect mirror when the photon frequency matches the Josephson plasma frequency. We generalize our calculations to periodic arrangements of junctions, demonstrating that they can be used for tunable band engineering, forming what we call a quantum circuit crystal. Two applications are discussed in de…
We present a canonical quantization of macroscopic electrodynamics. The results apply to inhomogeneous media with a broad class of linear magneto-electric responses which are consistent with the Kramers-Kronig and Onsager relations. Through its ability to accommodate strong dispersion and loss, our theory provides a rigorous foundation for the study of quantum optical processes in structures incorporating metamaterials, provided these may be modeled as magneto-electric media. Previous canonical treatments of dielectric and magneto-dielectric media have expressed the electromagnetic field opera…
Fluctuational Quantum Electrodynamics of Dispersive Time-Varying Media
Universidad Autónoma de Madrid（马德里自治大学）；Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid（马德里自治大学凝聚态物理中心 (IFIMAC)）；Instituto Nicolás Cabrera (INC), Universidad Autónoma de Madrid（马德里自治大学尼古拉斯·卡布雷拉研究所 (INC)）
Which systems are ideal to obtain negative refraction with no absorption? Electromagnetically induced transparency (EIT) is a method to suppress absorption and make a material transparent to a field of a given frequency. Such a system has been discussed in [1]; however the main limitations for negative refraction introduced are the necessity of resonant electric and magnetic dipole transitions, and the necessity of very dense media. We suggest using frequency translators in a composite system that would provide negative refraction for a range of optical frequencies while attempting to overcome…
We consider a two-dimensional extension of the 1D waveguide quantum electrodynamics and investigate the nature of linear excitations in two-dimensional arrays of qubits coupled to networks of chiral waveguides. We show that the combined effects of chirality and long-range photon mediated qubit-qubit interactions lead to the emergence of the two-dimensional flat bands in the polaritonic spectrum, corresponding to slow strongly correlated light.
In this work we calculate the closed time path (CTP) generating functional for the electromagnetic (EM) field interacting with inhomogeneous anisotropic matter. For this purpose, we first find a general expression for the electromagnetic field's influence action from the interaction of the field with a composite environment consisting in the quantum polarization degrees of freedom in each point of space, at arbitrary temperatures, connected to thermal baths. Then, we evaluate the generating functional for the gauge field, in the temporal gauge, by implementing the Faddeev-Popov procedure. Fina…
