We show that the material dependencies of macroscopically quantized fields in linear media are not consistent with the classical electromagnetic boundary conditions. We then phenomenologically construct macroscopic quantized fields that satisfy quantum--classical correspondence with the result indicating that the canonical momentum in a linear medium is modified as a consequence of the reduced speed of light. We re-derive D'Alembert's principle and Lagrange's equations for an arbitrarily large region of space in which light signals travel slower than in the vacuum and show that the resulting modifications to Lagrangian dynamics, including the canonical momenta, repair the violation of the correspondence principle for macroscopically quantized fields.
We formulate macroscopic quantum electrodynamics for the most general linear, absorbing media. In particular, Onsager reciprocity is not assumed to hold. For media with a non-local response, the field quantisation is based on the conductivity tensor and the Green tensor for the electromagnetic field. For a local medium response, we introduce the permittivity, permeability and magnetoelectric susceptibilities to obtain an explicitly duality-invariant scheme. We find that duality invariance only holds as a continuous symmetry when non-reciprocal responses are allowed for.
We consider the interaction of atoms with the quantized electromagnetic field in the presence of materials with negative index of refraction. Spontaneous emission of an atom embedded in a negative index material is discussed. It is shown furthermore that the possibility of a vanishing optical path length between two spatially separated points provided by these materials can lead to complete suppression of spontaneous emission of an atom in front of a perfect mirror even if the distance between atom and mirror is large compared to the transition wavelength. Two atoms put in the focal points of …
The description of dispersion forces within the framework of macroscopic quantum electrodynamics in linear, dispersing, and absorbing media combines the benefits of approaches based on normal-mode techniques of standard quantum electrodynamics and methods based on linear response theory in a natural way. It renders generally valid expressions for both the forces between bodies and the forces on atoms in the presence of bodies, while showing very clearly the intimate relation between the different types of dispersion forces. By considering examples, the influence of various factors like form, s…
We develop fluctuational electrodynamics for media with nonlinear optical response. In a perturbative manner, we amend the stochastic Helmholtz equation to describe fluctuations in a nonlinear setting, in agreement with the fluctuation dissipation theorem, and identify the local (Rytov) current fluctuations. We show how the linear response (the solution of the scattering problem) of a collection of objects is found from the individual responses, as measured in isolation. As an example, we compute the Casimir force acting between nonlinear objects which approaches the result for linear optics f…
We address two issues in the quantum electrodynamical description of photonic media with some disorder, neglecting material dispersion. When choosing a gauge in which the static potential vanishes, the normal modes of the medium with disorder satisfy another transversality condition than the modes of the ideal medium. Our first result is an integral equation for optical modes such that all perturbation-theory solutions automatically satisfy the desired transversality condition. Secondly, when expanding the vector potential for the medium with disorder in terms of the normal modes of the ideal …
The quantization of optical fields in vacuum has been known for decades, but extending the field quantization to lossy and dispersive media in nonequilibrium conditions has proven to be complicated due to the position-dependent electric and magnetic responses of the media. In fact, consistent position-dependent quantum models for the photon number in resonant structures have only been formulated very recently and only for dielectric media. Here we present a general position-dependent quantized fluctuational electrodynamics (QFED) formalism that extends the consistent field quantization to desc…
Quantum electrodynamics under conditions of distinguishability of interacting matter entities, and of controlled actions and back-actions between them, is considered. Such "mesoscopic quantum electrodynamics" is shown to share its dynamical structure with the classical stochastic electrodynamics. In formal terms, we demonstrate that all general relations of the mesoscopic quantum electrodynamics may be recast in a form lacking Planck's constant. Mesoscopic quantum electrodynamics is therefore subject to "doing quantum electrodynamics while thinking classically," allowing one to substitute esse…
We present a canonical quantization of macroscopic electrodynamics. The results apply to inhomogeneous media with a broad class of linear magneto-electric responses which are consistent with the Kramers-Kronig and Onsager relations. Through its ability to accommodate strong dispersion and loss, our theory provides a rigorous foundation for the study of quantum optical processes in structures incorporating metamaterials, provided these may be modeled as magneto-electric media. Previous canonical treatments of dielectric and magneto-dielectric media have expressed the electromagnetic field opera…
The canonical quantization of macroscopic electromagnetism was recently presented in New J. Phys. 12 (2010) 123008. This theory is here used to derive the Casimir effect, by considering the special case of thermal and zero-point fields. The stress-energy-momentum tensor of the canonical theory follows from Noether's theorem, and its electromagnetic part in thermal equilibrium gives the Casimir energy density and stress tensor. The results hold for arbitrary inhomogeneous magnetodielectrics and are obtained from a rigorous quantization of electromagnetism in dispersive, dissipative media. Conti…
Here, a comprehensive theory of the couplings between a nanocavity and exciton complexes in a quantum dot is developed, which successfully predicts the spectral triplet in the strong coupling regime that has been observed in several experiments but is unexpected according to conventional cavity quantum electrodynamics. The quantum anti-Zeno effect is found to play an essential role in the appearance of the central peak in the triplet under a low-excitation regime. The effect of hyperfine interactions is also discussed, which results in the cavity-mediated mixing of bright and dark exciton stat…
Fluctuational Quantum Electrodynamics of Dispersive Time-Varying Media
Universidad Autónoma de Madrid（马德里自治大学）；Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid（马德里自治大学凝聚态物理中心 (IFIMAC)）；Instituto Nicolás Cabrera (INC), Universidad Autónoma de Madrid（马德里自治大学尼古拉斯·卡布雷拉研究所 (INC)）
Resonance energy transfer between chiral molecules can be used to discriminate between different enantiomers. The transfer rate between chiral molecules consists of a non-discriminatory and discriminatory parts. We derive these two rate contributions in the framework of macroscopic quantum electrodynamics. We show that their ratio is usually larger in the retarded regime or far-zone of large separation distances and that the degree of discrimination can be modified when considering a surrounding medium. We highlight the importance of local field effects onto the degree of discrimination and pr…
Fast and High Excitation Transport in Waveguide Quantum Electrodynamics
Institute of Atomic and Molecular Sciences, Academia Sinica（原子分子科学研究所，中央研究院）；Molecular Science and Technology Program, Taiwan International Graduate Program, Academia Sinica（分子科学与技术项目，台湾国际研究生计划，中央研究院）；Department of Physics, National Central University（物理系，中央大学）；Department of Physics and Center for Theoretical Physics, National Taiwan University（物理系与理论物理中心，国立台湾大学）；Center for Quantum Science and Engineering, National Taiwan University（量子科学与工程中心，国立台湾大学）；Physics Division, National Center for Theoretical Sciences（物理组，国家理论科学中心）
Microscopic theory of exciton-polariton model involving multiple molecules: Macroscopic quantum electrodynamics formulation and essence of direct intermolecular interactions
National Taiwan University（国立台湾大学）；Institute of Atomic and Molecular Sciences, Academia Sinica（中央研究院原子与分子科学研究所）；Physics Division, National Center for Theoretical Sciences（国家理论科学中心物理部）
The local-field renormalization of the spontaneous emission rate in a dielectric is explicitly obtained from a fully microscopic quantum-electrodynamical, many-body derivation of Langevin-Bloch operator equations for two-level atoms embedded in an absorptive and dispersive, linear dielectric host. We find that the dielectric local-field enhancement of the spontaneous emission rate is smaller than indicated by previous studies.
Photonic crystals provide an extremely powerful toolset for manipulation of optical dispersion and density of states, and have thus been employed for applications from photon generation to quantum sensing with NVs and atoms. The unique control afforded by these media make them a beautiful, if unexplored, playground for strong coupling quantum electrodynamics, where a single, highly nonlinear emitter hybridizes with the band structure of the crystal. In this work we demonstrate that such hybridization can create localized cavity modes that live within the photonic band-gap, whose localization a…
This paper aims to present an elaborate view on the motivation and realization of the idea to extend Maxwell's electrodynamics to Extended Electrodynamics in a reasonable and appropriate way in order to make it possible to describe electromagnetic (3+1)-soliton-like objects in vacuum and in the presence of continuous media (external fields), exchanging energy-momentum with the electromagnetic field.
The electromagnetic vacuum is known to have energy. It has been recently argued that the quantum vacuum can possess momentum, that adds up to the momentum of matter. This ``Casimir momentum'' is closely related to the Casimir effect, in which case energy is exchanged. In previous theory it was treated semi-classically. We present a non-relativistic quantum theory for the linear momentum of electromagnetic zero-point fluctuations, considering an harmonic oscillator subject to crossed, quasi-static magnetic and electric and coupled to the quantum vacuum. We derive a contribution of the quantum v…
Within the framework of macroscopic quantum electrodynamics, general expressions for the Casimir force acting on linearly and causally responding magnetodielectric bodies that can be embedded in another linear and causal magnetodielectric medium are derived. Consistency with microscopic harmonic-oscillator models of the matter is shown. The theory is applied to planar structures and proper generalizations of Casimir's and Lifshitz-type formulas are given.
We consider a two-dimensional extension of the 1D waveguide quantum electrodynamics and investigate the nature of linear excitations in two-dimensional arrays of qubits coupled to networks of chiral waveguides. We show that the combined effects of chirality and long-range photon mediated qubit-qubit interactions lead to the emergence of the two-dimensional flat bands in the polaritonic spectrum, corresponding to slow strongly correlated light.
In this work we calculate the closed time path (CTP) generating functional for the electromagnetic (EM) field interacting with inhomogeneous anisotropic matter. For this purpose, we first find a general expression for the electromagnetic field's influence action from the interaction of the field with a composite environment consisting in the quantum polarization degrees of freedom in each point of space, at arbitrary temperatures, connected to thermal baths. Then, we evaluate the generating functional for the gauge field, in the temporal gauge, by implementing the Faddeev-Popov procedure. Fina…
In this work we establish a density-functional reformulation of coupled matter-photon problems subject to general external electromagnetic fields and charge currents. We first show that for static minimally-coupled matter-photon systems an external electromagnetic field is equivalent to an external charge current. We employ this to show that scalar external potentials and transversal external charge currents are in a one-to-one correspondence to the expectation values of the charge density and the vector-potential of the correlated matter-photon ground state. This allows to establish a Maxwell…
One of the most striking predictions of quantum electrodynamics is that vacuum fluctuations of the electromagnetic field can lead to spontaneous emission of atoms as well as photon-mediated interactions among them. Since these processes strongly depend on the nature of the photonic bath, a current burgeoning field is the study of their modification in the presence of photons with non-trivial energy dispersions, e.g., the ones confined in photonic crystals. A remarkable example is the case of isotropic Dirac-photons, which has been recently shown to lead to non-exponential spontaneous emission …
We propose a novel quantum electrodynamics (QED) platform where quantum emitters interact with a Hofstadter-ladder waveguide. We demonstrate several intriguing phenomena stemming from the exotic dispersion relation and vacuum mode properties led by the effective spin-orbit coupling, which have no analog in other QED setups. First, by assuming emitter's frequency to be resonant with the lower band, we find that the spontaneous emission is chiral with most photonic field decaying unidirectionally. Both numerical and analytical results indicate that the Hofstadter-ladder waveguide can be engineer…
We introduce multiplexed atom-cavity quantum electrodynamics with an atomic ensemble coupled to a single optical cavity mode. Multiple Raman dressing beams establish cavity-coupled spin-wave excitations with distinctive spatial profiles. Experimentally, we demonstrate the concept by observing spin-wave vacuum Rabi splittings, selective superradiance, and interference in the cavity-mediated interactions of two spin waves. We highlight that the current experimental configuration allows rapid, interchangeable cavity-coupling to 4 profiles with an overlap parameter of less than 10%, enough to demo…
We investigate a hybrid quantum system consisting of spatially separated resonant exchange qubits, defined in three-electron semiconductor triple quantum dots, that are coupled via a superconducting transmission line resonator. Drawing on methods from circuit quantum electrodynamics and Hartmann-Hahn double resonance techniques, we analyze three specific approaches for implementing resonator-mediated two-qubit entangling gates in both dispersive and resonant regimes of interaction. We calculate entangling gate fidelities as well as the rate of relaxation via phonons for resonant exchange qubit…
Macroscopic Quantum Electrodynamics with Gain: Modified Fluctuations and Their Consequences
RIKEN Centre for Advanced Photonics, RIKEN（RIKEN先进光子学中心）；Instituto Superior Técnico—University of Lisbon and Instituto de Telecomunicações（里斯本高等理工学院与电信研究所）；The Blackett Laboratory, Imperial College London（帝国理工学院布莱克特实验室）
By means of quantum mechanics and quantum electrodynamics applied to coupled harmonic Drude oscillators, we study the interaction between two neutral atoms or molecules subject to a uniform static electric field. Our focus is to understand the interplay between leading contributions to field-induced electrostatics/polarization and dispersion interactions, as considered within the employed Drude model for both non-retarded and retarded regimes. For the first case, we present an exact solution for two coupled oscillators obtained by diagonalizing the corresponding quantum-mechanical Hamiltonian …
Quantum description of mulitiparticle nano-systems is studied in a hot and dense electromagnetic medium. We use renormalization techniques of quantum field theory to show that the electromagnetic properties like electric permittivity and magnetic permeability depend on the temperature and density of the media. Casimir force also depends upon the physical properties of the medium and becomes a function of these parameters within the nano-systems. We discuss the effect of the Casimir force on the nanosystems in terms of temperature and density of the system. We present carbon nanotubes and biomo…
We build up a consistent theory of quantum electrodynamics in the presence of macroscopic polarizable media. We use the Huttner-Barnett model of a dispersive and absorbing dielectric medium and formulate the theory in terms of interacting quantum fields. We integrate out the damped polaritons by using diagrammatic techniques and find an exact expression for the displacement field (photon) propagator in the presence of a dispersive and absorbing dielectric half-space. This opens a new route to traceable perturbative calculations of the same kind as in free-space quantum electrodynamics. As a wo…
A major challenge in quantum optics and quantum information technology is to enhance the interaction between single photons and single quantum emitters. Highly engineered optical cavities are generally implemented requiring nanoscale fabrication precision. We demonstrate a fundamentally different approach in which disorder is used as a resource rather than a nuisance. We generate strongly confined Anderson-localized cavity modes by deliberately adding disorder to photonic crystal waveguides. The emission rate of a semiconductor quantum dot embedded in the waveguide is enhanced by a factor of 1…
Quantum correlations between distant particles remain enigmatic since the birth of quantum mechanics. Here we predict a novel kind of bound quantum state in the simplest one-dimensional setup of two interacting particles in a box. Paradoxically, two entangled particles become localized at the opposite edges of the box even though their interactions at large distance should seemingly play no role. Such states could be realized in the waveguide quantum electrodynamics platform, where an array of superconducting qubits or cold atoms is coupled to a waveguide. We demonstrate how long-range wavegui…
We study cavity quantum electrodynamics of Bose-condensed atoms that are subjected to continuous monitoring of the light leaking out of the cavity. Due to a given detection record of each stochastic realization, individual runs spontaneously break the symmetry of the spatial profile of the atom cloud and this symmetry can be restored by considering ensemble averages over many realizations. We show that the cavity optomechanical excitations of the condensate can be engineered to target specific collective modes. This is achieved by exploiting the spatial structure and symmetries of the collecti…
Lattice quantum electrodynamics of a molecular emitter in a topological gap
Univ. Lille, CNRS, UMR 8523 – PhLAM – Physique des Lasers Atomes et Molécules（里尔大学）；University of Würzburg（维尔茨堡大学）；National Institute of Optics (CNR-INO)（国家光学研究所）；European Laboratory for Non-Linear Spectroscopy (LENS)（欧洲非线性光谱学实验室）；Institute of Physics, Czech Academy of Sciences（捷克科学院物理研究所）
Mainly on nano-scale, but maybe not exclusively, it can be imagined a spontaneous charge disjunction inside certain media due to the fluctuations, collisions, wall effects, radiation or/and other presently unknown interactions. The repulsive Casimir-Lifshitz force may be also a good candidate as a source of this kind of phenomenon. To cover this assumption mathematically an additional term should appear in the Maxwell equations. As a consequence of this term, similar Klein-Gordon equations with a negative mass term will be obtained for the electric and magnetic fields. These equations may have…
The duality symmetry between electricity and magnetism hidden in classical Maxwell equations suggests the existence of dual charges, which have usually been interpreted as magnetic charges and have not been observed in experiments. In quantum electrodynamics (QED), both the electric and magnetic fields have been unified into one gauge field, which makes this symmetry inconspicuous. Here, we recheck the duality symmetry of QED by introducing a dual gauge field and a dual symmetric Lagrangian. Within the framework of gauge-field theory, we show that the electric-magnetic duality symmetry cannot …
The generation and control of quantum states of light constitute fundamental tasks in cavity quantum electrodynamics (QED). The superconducting realization of cavity QED, circuit QED, enables on-chip microwave photonics, where superconducting qubits control and measure individual photon states. A long-standing issue in cavity QED is the coherent transfer of photons between two or more resonators. Here, we use circuit QED to implement a three-resonator architecture on a single chip, where the resonators are interconnected by two superconducting phase qubits. We use this circuit to shuffle one- …
Masers, the microwave analogue of lasers, promise to deliver ultra-low noise amplification of microwave signals for use in medical MRI imaging and deep-space communication. Research on masers in modern times was rekindled thanks to the discovery of gain media that were operable at room-temperature, eschewing bulky cryogenics that hindered their use. However, besides the two known materials of pentacene doped in para-terphenyl and negatively-charged nitrogen-vacancy defects in diamond, there has been scarce progress in the search for completely new room-temperature gain media. Here we show the …
The search for a quantum theory of gravity has led to the discovery of quantum many-body systems that are dual to gravitational models with quantum properties. The perhaps most famous of these systems is the Sachdev-Ye-Kitaev (SYK) model. It features maximal scrambling of quantum information, and opens a potential inroad to experimentally investigating aspects of quantum gravity. A scalable laboratory realisation of this model, however, remains outstanding. Here, we propose a feasible implementation of the SYK model in cavity quantum electrodynamics platforms. Through detailed analytical and n…
Any quantum-confined electronic system coupled to the electromagnetic continuum is subject to radiative decay and renormalization of its energy levels. When coupled to a cavity, these quantities can be strongly modified with respect to their values in vacuum. Generally, this modification can be accurately captured by including only the closest resonant mode of the cavity. In the circuit quantum electrodynamics architecture, where the coupling strengths can be substantial, it is however found that the radiative decay rates are strongly influenced by far off-resonant modes. A multimode calculati…
The parity-preserving $U(1)\times U(1)$ massless QED$_3$ is proposed as a pristine graphene-like planar quantum electrodynamics model. The spectrum content, the degrees of freedom, spin, masses and charges of the quasiparticles (electron-polaron, hole-polaron, photon and Néel quasiparticles) which emerge from the model are discussed. The four-fold broken degeneracy of the Landau levels, similar as the one experimentally observed in pristine graphene submitted to high applied external magnetic fields, is obtained. Furthermore, the model exhibits zero-energy Landau level indicating a kind of ano…
