We present the first calculation of coherent backscattering with inelastic scattering by saturated atoms. We consider the scattering of a quasi-monochromatic laser pulse by two distant atoms in free space. By restricting ourselves to scattering of two photons, we employ a perturbative approach, valid up to second order in the incident laser intensity. The backscattering enhancement factor is found to be smaller than two (after excluding single scattering), indicating a loss of coherence between the doubly scattered light emitted by both atoms. Since the undetected photon carries information about the path of the detected photon, the coherence loss can be explained by a which-path argument, in analogy with a double-slit experiment.
We survey recent progress achieved in understanding the impact of inelastic processes on coherent backscattering of light from cold atoms that are saturated by a powerful laser field.
We present a nonperturbative treatment of coherent backscattering of intense laser light from cold atoms, and predict a nonvanishing backscattering signal even at very large intensities, due to the constructive (self-)interference of inelastically scattered photons.
We study theoretically inelastic spectrum of coherent backscattering of laser light by two atoms. For an intense laser field, there are frequency domains of not only constructive but also destructive (self-)interference of the inelastic photons. We interpret the emergent spectral features using the dressed states and considering coherent backscattering as a kind of the pump-probe experiment.
We investigate coherent backscattering of light by two harmonically trapped atoms in the light of quantitative quantum duality. Including recoil and Doppler shift close to an optical resonance, we calculate the interference visibility as well as the amount of which-path information, both for zero and finite temperature.
We give a detailed derivation of the master equation description of the coherent backscattering of laser light by cold atoms. In particular, our formalism accounts for the nonperturbative nonlinear response of the atoms when the injected intensity saturates the atomic transition. Explicit expressions are given for total and elastic backscattering intensities in the different polarization channels, for the simplest nontrivial multiple scattering scenario of intense laser light multiply scattering from two randomly placed atoms.
We demonstrate a strong coherent backward wave oscillation using forward propagating fields only. This is achieved by applying laser fields to an ultra-dispersive medium with proper chosen detunings to excite a molecular vibrational coherence that corresponds to a backward propagating wave. The physics then has much in common with propagation of ultra-slow light. Applications to coherent scattering and remote sensing are discussed.
Theoretical prediction of antilocalization of light in ultracold atomic gas samples, in the weak localization regime, is reported. Calculations and Monte-Carlo simulations show that, for selected spectral ranges in the vicinity of atomic 85Rb hyperfine transitions, quantum coherence in optical transitions through nondegenerate hyperfine levels in multiple light scattering generates destructive interference in otherwise reciprocal scattering paths. This effect leads to enhancement factors less than unity in a coherent backscattering geometry, and suggests the possibility of enhanced diffusion o…
We report a combined theoretical and experimental study of the spectral and polarization dependence of near resonant radiation coherently backscattered from an ultracold gas of 85Rb atoms. Measurements in an approximately 6 MHz range about the 5s^{2}S_{1/2}- 5p^{2}P_{3/2}, F=3 - F'=4 hyperfine transition are compared with simulations based on a realistic model of the experimental atomic density distribution. In the simulations, the influence of heating of the atoms in the vapor, magnetization of the vapor, finite spectral bandwidth, and other nonresonant hyperfine transitions are considered. G…
We present a diagrammatic derivation of the coherent backscattering spectrum from two two-level atoms using the pump-probe approach, wherein the multiple scattering signal is deduced from single-atom responses, and provide a physical interpretation of the single-atom building blocks.
We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering processes. Here, coherent backscattering can be formed by interference between {\em three} different scattering amplitudes. Consequently, if elastically scattered photons are filtered out from the photodetection signal by means of suitable frequency-selective detection, we find the nonlinear backscattering enhancement factor to exceed the linear barrier two.
We review experimental and theoretical studies of coherent backscattering of near resonant radiation from an ultracold atomic gas in the weak localization regime. Recent accomplishments in high resolution spectroscopy of atomic ensembles based on the coherent backscattering process are discussed. We also propose several new experimental schemes for time-dependent spectroscopy as applied to multiple scattering in the regime of weak localization.
We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear refractive index) and the scattering events. Using a perturbative approach, the nonlinear effects arise from inelastic two-photon scattering processes. We present a detailed diagrammatic derivation of the elastic and inelastic components of the backscattering signal both for scalar and vectorial photons. Especially, we show that the coherent backscattering …
Coherent backscattering is a coherence effect in the propagation of waves through disordered media involving two or more scattering events. Here, we report on the observation of coherent backscattering from individual atoms and their mirror images. This system displays two important advantages: First, the effect can be observed at low optical densities, which allows to work in very dilute clouds or far from resonance. Second, due to the fact that the radiation of an atom interferes constructively with that of its own image, the phenomenon is much more robust to dephasing induced by strong satu…
We present a generalization of the diagrammatic pump-probe approach to coherent backscattering (CBS) of intense laser light for atoms with degenerate energy levels. We employ this approach for a characterization of the double scattering signal from optically pumped atoms with the transition $J_g\rightarrow J_e=J_g+1$ in the helicity preserving polarization channel. We show that, in the saturation regime, the internal degeneracy becomes manifest for atoms with $J_g\geq 1$, leading to a faster decrease of the CBS enhancement factor with increasing saturation parameter than in the non-degenerate …
We study the impact of double and triple scattering contributions on coherent backscattering of laser light from saturated isotropic atoms, in the helicity preserving polarization channel. Using the recently proposed diagrammatic pump-probe approach, we analytically derive single-atom spectral responses to a classical polychromatic driving field, combine them self-consistently to double and triple scattering processes, and numerically deduce the corresponding elastic and inelastic spectra, as well as the total backscattered intensities. We find that account of the triple scattering contributio…
Reciprocity is a universal principle that has a profound impact on many areas of physics. A fundamental phenomenon in condensed-matter physics, optical physics and acoustics, arising from reciprocity, is the constructive interference of quantum or classical waves which propagate along time-reversed paths in disordered media, leading to, for example, weak localization and metal-insulator transition. Previous studies have shown that such coherent effects are suppressed when reciprocity is broken. Here we show that by breaking reciprocity in a controlled manner, we can tune, rather than simply su…
In condensed matter systems, coherent backscattering and quantum interference in the presence of time-reversal symmetry lead to well-known phenomena such as weak localization (WL) and universal conductance fluctuations (UCF). Here we use multi-pass Landau-Zener transitions at the avoided crossing of a highly-coherent superconducting qubit to emulate these phenomena. The average and standard deviation of the qubit transition rate exhibit a dip and peak when the driving waveform is time-reversal symmetric, analogous to WL and UCF, respectively. The higher coherence of this qubit enabled the real…
In this theoretical paper, we investigate coherence properties of the near-resonant light scattered by two atoms exposed to a strong monochromatic field. To properly incorporate saturation effects, we use a quantum Langevin approach. In contrast to the standard optical Bloch equations, this method naturally provides the inelastic spectrum of the radiated light induced by the quantum electromagnetic vacuum fluctuations. However, to get the right spectral properties of the scattered light, it is essential to correctly describe the statistical properties of these vacuum fluctuations. Because of t…
We predict a generic manifestation of quantum interference in many-body bosonic systems resulting in a coherent enhancement of the average return probability in Fock space. This enhancement is both robust with respect to variations of external parameters and genuinely quantum insofar as it cannot be described within mean-field approaches. As a direct manifestation of the superposition principle in Fock space, it arises when many-body equilibration due to interactions sets in. Using a semiclassical approach based on interfering paths in Fock space, we calculate the magnitude of the backscatteri…
We consider the influence of a resonant control field on weak localization of light in ultracold atomic ensembles. Both steady-state and pulsed light excitation are considered. We show that the presence of a control field essentially changes the type of interference effects which occur under conditions of multiple scattering. For example, for some scattering polarization channels the presence of a control field can cause destructive interference through which the enhancement factor, normally considered to be greater than one, becomes less than one.
We present a detailed analytical and numerical analysis of the inelastic coherent backscattering spectrum of laser light incident on cold atoms. We identify frequency domains where the interference contribution can be positive \emph{as well as} negative -- or exhibits dispersive character. These distinctive features are explained by reciprocity arguments and dressed state two-photon scattering amplitudes.
We present a new method to obtain the first-order temporal correlation function, $g^{(1)} (τ)$, of the light scattered by an assembly of point-like quantum scatterers, or equivalently its spectral power distribution. This new method is based on the mirror-assisted backscattering interferometric setup. The contrast of its angular fringes was already linked in the past to the convolution of $g^{(1)} (τ)$ for different Rabi frequencies taking into account the incoming spatial intensity profile of the probe beam, but we show here that by simply adding a half waveplate to the interferometer in a sp…
We consider a relaxation of a single mode of the quantized field in a presence of one- and two-photon absorption and emission processes. Exact stationary solutions of the master equation for the diagonal elements of the density matrix in the Fock basis are found in the case of completely saturated two-photon emission. If two-photon processes dominate over single-photon ones, the stationary state is a mixture of phase averaged even and odd coherent states.
We theoretically study the out-of-equilibrium dynamics in momentum space of a weakly interacting disordered Bose gas launched with a finite velocity. In the absence of interactions, coherent multiple scattering gives rise to a background of diffusive particles, on top of which a coherent backscattering interference emerges. We revisit this scenario in the presence of interactions, using a diagrammatic quantum transport theory. We find that the dynamics is governed by coupled kinetic equations describing the thermalization of the diffusive and coherent components of the gas. This phenomenon lea…
We outline the non-perturbative theory of multiple scattering of resonant, intense laser light off a dilute cloud of cold atoms. A combination of master equation and diagrammatic techniques allows, for the first time, a quantitative description of nonlinear diffusive transport as well as of coherent backscattering of the injected electromagnetic field, notwithstanding the exponential growth of Hilbert space with the number of atomic scatterers. As an exemplary application, we monitor the laser light's intensity profile within the medium, the spectrum of the backscattered light and the coherent…
Since the work of Anderson on localization, interference effects for the propagation of a wave in the presence of disorder have been extensively studied, as exemplified in coherent backscattering (CBS) of light. In the multiple scattering of light by a disordered sample of thermal atoms, interference effects are usually washed out by the fast atomic motion. This is no longer true for cold atoms where CBS has recently been observed. However, the internal structure of the atoms strongly influences the interference properties. In this paper, we consider light scattering by an atomic dipole transi…
Wave-particle duality finds a natural application for electrons or light propagating in disordered media where coherent corrections to transport are given by two-wave interference. For scatterers with internal degrees of freedom, these corrections are observed to be much smaller than would be expected for structureless scatterers. By examining the basic example of the scattering of one photon by two spin-1/2 atoms--a case-study for coherent backscattering--we demonstrate that the loss of interference strength is associated with which-path information stored by the scattering atoms.
This paper analyzes coherent backscattering of intense laser light by two randomly placed distant atoms. Starting from the general two-atom master equation, we analytically derive the elastic and inelastic background and interference components of the double scattering spectrum. By expressing the final results in terms of single-atom observables, the two-atom problem is shown to be equivalent to a description in terms of single atoms under bichromatic driving.
We deduce the coherent backscattering signal from two distant laser-driven atoms using single-atom equations. In contrast to the standard master equation treatment, this new approach is suitable for the generalization to a large number of atomic scatterers.
The reflectionless coherent light transport in the coupled resonator array is investigated in the presence of intra-resonator intermodal coupling between the clockwise and counterclockwise modes, which plays a constructive role for modulating the light flow rather than inducing the unwanted backscattering. The interplay between the intra-resonator intermodal coupling and the inter-resonator couplings enables the coherent resonant transmission (CRT) of the properly superposed injection constituted by the clockwise and counterclockwise modes. The superposition coefficients of the initial excitat…
By using the coherent backscattering interference effect, we investigate experimentally and theoretically how coherent transport of light inside a cold atomic vapour is affected by the residual motion of atomic scatterers. As the temperature of the atomic cloud increases, the interference contrast dramatically decreases emphazising the role of motion-induced decoherence for resonant scatterers even in the sub-Doppler regime of temperature. We derive analytical expressions for the corresponding coherence time.
We numerically investigate the properties of speckle patterns formed by nonlinear point scatterers. We show that, in the weak localization regime, dynamical instability appears, eventually leading to chaotic behavior of the system. Analysing the statistical properties of the instability thresholds for different values of the system size and disorder strength, a scaling law is emphasized. The later is also found to govern the smallest decay rate of the linear system, putting thus forward the crucial importance of interference effects. This is also underlined by the fact that coherent backscatte…
We show that the phase sensitivity $Δθ$ of a Mach-Zehnder interferometer fed by a coherent state in one input port and squeezed-vacuum in the other one is i) independent from the true value of the phase shift and ii) can reach the Heisenberg limit $Δθ\sim 1/N_T$, where $N_T$ is the average number of particles of the input states. We also show that the Cramer-Rao lower bound, $Δθ\propto 1/ \sqrt{|α|^2 e^{2r} + \sinh^2r}$, can be saturated for arbitrary values of the squeezing parameter $r$ and the amplitude of the coherent mode $|α|$ by a Bayesian phase inference protocol.
We compare two different models of transport of light in a disordered system with a spherical Gaussian distribution of scatterers. A coupled dipole model, keeping into account all interference effects, is compared to an incoherent model, using a random walk of particles. Besides the well known coherent backscattering effect and a well pronounced forward lobe, the incoherent model reproduces extremely well all scattering features. In an experiment with cold atoms, we use the momentum recoil imparted on the center of mass of the sample as a partial probe of the light scattering properties. We fi…
Starting from a microscopic theory for atomic scatterers, we describe the scattering of light by a single atom and study the coherent propagation of light in a cold atomic cloud in the presence of a magnetic field B in the mesoscopic regime. Non-pertubative expressions in B are given for the magneto-optical effects and optical anisotropy. We then consider the multiple scattering regime and address the fate of the coherent backscattering (CBS) effect. We show that, for atoms with nonzero spin in their ground state, the CBS interference contrast can be increased compared to its value when B=0, a…
We study coherent backscattering of intense laser light from three immobile two-level atoms using the master equation approach. The master equation is solved analytically, and the triple scattering spectrum is expressed in quadratures. We show that this solution can be obtained via a self-consistent combination of single-atom spectral responses, and is equivalent to the solution following from the diagrammatic pump-probe approach. We deduce the general expressions for single-atom building blocks which can be used in simulations of multiple inelastic scattering of laser light in the bulk atomic…
Coherent effects manifested in light scattering from cold, optically dense and disordered atomic systems are reviewed from a primarily theoretical point of view. Development of the basic theoretical tools is then elaborated through several physical atomic physics based processes which have been at least partly explored experimentally. These include illustrations drawn from the coherent backscattering effect, random lasing in atomic gases, quantum memories and light-atoms interface assisted by the light trapping mechanism. Current understanding and challenges associated with the transition to h…
As recently discovered [PRL ${\bf 109}$ 190601(2012)], Anderson localization in a bulk disordered system triggers the emergence of a coherent forward scattering (CFS) peak in momentum space, which twins the well-known coherent backscattering (CBS) peak observed in weak localization experiments. Going beyond the perturbative regime, we address here the long-time dynamics of the CFS peak in a 1D random system and we relate this novel interference effect to the statistical properties of the eigenfunctions and eigenspectrum of the corresponding random Hamiltonian. Our numerical results show that t…
Coherent backscattering is a multiple scattering interference effect which enhances the diffuse reflection off a disordered sample in the backward direction. Classically, the enhanced intensity is twice the average background under well chosen experimental conditions. We show how the quantum internal structure of atomic scatterers leads to a significantly smaller enhancement. Theoretical results for double scattering in the weak localization regime are presented which confirm recent experimental observations.
The interference contrast observed in coherent backscattering by cold atoms is drastically reduced with respect to classical disordered media. We study the impact of the degeneracy of the resonant atomic dipole transition on multiple scattering of polarised photons. An analytical treatment allows to derive the diffusion coefficient and depolarisation times for the average light intensity, and dephasing times for the weak localisation corrections. The calculated CBS signals reproduce the experimental results.
