Theoretical prediction of antilocalization of light in ultracold atomic gas samples, in the weak localization regime, is reported. Calculations and Monte-Carlo simulations show that, for selected spectral ranges in the vicinity of atomic 85Rb hyperfine transitions, quantum coherence in optical transitions through nondegenerate hyperfine levels in multiple light scattering generates destructive interference in otherwise reciprocal scattering paths. This effect leads to enhancement factors less than unity in a coherent backscattering geometry, and suggests the possibility of enhanced diffusion of light in ultracold atomic vapors.
The paper discusses the Berry phase influence on the weak localization phenomenon at the adiabatic backscattering of ultrarelativistic particles in a random medium. We demonstrate that bosons that pass along a certain closed path in opposite directions come back always in phase (an example: the backscattering enhancement of electromagnetic waves), whereas fermions come exactly in antiphase. This produces a "complete weak antilocalization" of ultrarelativistic fermions: the backscattering field intensity vanishes.
We report a combined theoretical and experimental study of the spectral and polarization dependence of near resonant radiation coherently backscattered from an ultracold gas of 85Rb atoms. Measurements in an approximately 6 MHz range about the 5s^{2}S_{1/2}- 5p^{2}P_{3/2}, F=3 - F'=4 hyperfine transition are compared with simulations based on a realistic model of the experimental atomic density distribution. In the simulations, the influence of heating of the atoms in the vapor, magnetization of the vapor, finite spectral bandwidth, and other nonresonant hyperfine transitions are considered. G…
We review experimental and theoretical studies of coherent backscattering of near resonant radiation from an ultracold atomic gas in the weak localization regime. Recent accomplishments in high resolution spectroscopy of atomic ensembles based on the coherent backscattering process are discussed. We also propose several new experimental schemes for time-dependent spectroscopy as applied to multiple scattering in the regime of weak localization.
We give a detailed derivation of the master equation description of the coherent backscattering of laser light by cold atoms. In particular, our formalism accounts for the nonperturbative nonlinear response of the atoms when the injected intensity saturates the atomic transition. Explicit expressions are given for total and elastic backscattering intensities in the different polarization channels, for the simplest nontrivial multiple scattering scenario of intense laser light multiply scattering from two randomly placed atoms.
We study coherent backscattering of a quasi-monochromatic laser by a dilute gas of cold two-level atoms. We consider the perturbative regime of weak intensities, where nonlinear effects arise from {\em inelastic} two-photon scattering processes. Here, coherent backscattering can be formed by interference between {\em three} different scattering amplitudes. Consequently, if elastically scattered photons are filtered out from the photodetection signal by means of suitable frequency-selective detection, we find the nonlinear backscattering enhancement factor to exceed the linear barrier two.
We study coherent backscattering of a monochromatic laser by a dilute gas of cold two-level atoms in the weakly nonlinear regime. The nonlinear response of the atoms results in a modification of both the average field propagation (nonlinear refractive index) and the scattering events. Using a perturbative approach, the nonlinear effects arise from inelastic two-photon scattering processes. We present a detailed diagrammatic derivation of the elastic and inelastic components of the backscattering signal both for scalar and vectorial photons. Especially, we show that the coherent backscattering …
In this theoretical paper, we investigate coherence properties of the near-resonant light scattered by two atoms exposed to a strong monochromatic field. To properly incorporate saturation effects, we use a quantum Langevin approach. In contrast to the standard optical Bloch equations, this method naturally provides the inelastic spectrum of the radiated light induced by the quantum electromagnetic vacuum fluctuations. However, to get the right spectral properties of the scattered light, it is essential to correctly describe the statistical properties of these vacuum fluctuations. Because of t…
We observe the buildup of a frequency-shifted reverse light field in a unidirectionally pumped high-$Q$ optical ring cavity serving as a dipole trap for cold atoms. This effect is enhanced and a steady state is reached, if via an optical molasses an additional friction force is applied to the atoms. We observe the displacement of the atoms accelerated by momentum transfer in the backscattering process and interpret our observations in terms of the collective atomic recoil laser. Numerical simulations are in good agreement with the experimental results.
Motivated by a recent prediction to engineer the dispersion relation of a waveguide constructed from atomic components [arXiv:2104.08121], we explore the possibility to create directional transport in an open, collective quantum system. The optical response of the atomic waveguide is characterized through a scattering-matrix formalism built upon theories of photoelectric detection that allows us to find the required conditions for directional mode-to-mode transmission to occur and be measured in an experimental setting. We find that directional waveguides allow for an efficient outcoupling of …
We outline the non-perturbative theory of multiple scattering of resonant, intense laser light off a dilute cloud of cold atoms. A combination of master equation and diagrammatic techniques allows, for the first time, a quantitative description of nonlinear diffusive transport as well as of coherent backscattering of the injected electromagnetic field, notwithstanding the exponential growth of Hilbert space with the number of atomic scatterers. As an exemplary application, we monitor the laser light's intensity profile within the medium, the spectrum of the backscattered light and the coherent…
We study the impact of double and triple scattering contributions on coherent backscattering of laser light from saturated isotropic atoms, in the helicity preserving polarization channel. Using the recently proposed diagrammatic pump-probe approach, we analytically derive single-atom spectral responses to a classical polychromatic driving field, combine them self-consistently to double and triple scattering processes, and numerically deduce the corresponding elastic and inelastic spectra, as well as the total backscattered intensities. We find that account of the triple scattering contributio…
Since the work of Anderson on localization, interference effects for the propagation of a wave in the presence of disorder have been extensively studied, as exemplified in coherent backscattering (CBS) of light. In the multiple scattering of light by a disordered sample of thermal atoms, interference effects are usually washed out by the fast atomic motion. This is no longer true for cold atoms where CBS has recently been observed. However, the internal structure of the atoms strongly influences the interference properties. In this paper, we consider light scattering by an atomic dipole transi…
We consider the influence of a resonant control field on weak localization of light in ultracold atomic ensembles. Both steady-state and pulsed light excitation are considered. We show that the presence of a control field essentially changes the type of interference effects which occur under conditions of multiple scattering. For example, for some scattering polarization channels the presence of a control field can cause destructive interference through which the enhancement factor, normally considered to be greater than one, becomes less than one.
By using the coherent backscattering interference effect, we investigate experimentally and theoretically how coherent transport of light inside a cold atomic vapour is affected by the residual motion of atomic scatterers. As the temperature of the atomic cloud increases, the interference contrast dramatically decreases emphazising the role of motion-induced decoherence for resonant scatterers even in the sub-Doppler regime of temperature. We derive analytical expressions for the corresponding coherence time.
We theoretically explore the possibility to detect weak localization of light in a hot atomic vapor, where one usually expects the fast thermal motion of the atoms to destroy any interference in multiple scattering. To this end, we compute the coherent backscattering peak, assuming high temperature and taking into account the quantum level structure of the atomic scatterers. It is found that the decoherence due to thermal motion can be partially counterbalanced by working at large laser detuning and using small atomic cells with an elongated geometry. Under these conditions, our estimates sugg…
We deduce the coherent backscattering signal from two distant laser-driven atoms using single-atom equations. In contrast to the standard master equation treatment, this new approach is suitable for the generalization to a large number of atomic scatterers.
Coherent effects manifested in light scattering from cold, optically dense and disordered atomic systems are reviewed from a primarily theoretical point of view. Development of the basic theoretical tools is then elaborated through several physical atomic physics based processes which have been at least partly explored experimentally. These include illustrations drawn from the coherent backscattering effect, random lasing in atomic gases, quantum memories and light-atoms interface assisted by the light trapping mechanism. Current understanding and challenges associated with the transition to h…
Starting from a microscopic theory for atomic scatterers, we describe the scattering of light by a single atom and study the coherent propagation of light in a cold atomic cloud in the presence of a magnetic field B in the mesoscopic regime. Non-pertubative expressions in B are given for the magneto-optical effects and optical anisotropy. We then consider the multiple scattering regime and address the fate of the coherent backscattering (CBS) effect. We show that, for atoms with nonzero spin in their ground state, the CBS interference contrast can be increased compared to its value when B=0, a…
We study coherent backscattering of intense laser light from three immobile two-level atoms using the master equation approach. The master equation is solved analytically, and the triple scattering spectrum is expressed in quadratures. We show that this solution can be obtained via a self-consistent combination of single-atom spectral responses, and is equivalent to the solution following from the diagrammatic pump-probe approach. We deduce the general expressions for single-atom building blocks which can be used in simulations of multiple inelastic scattering of laser light in the bulk atomic…
Coherent backscattering is a multiple scattering interference effect which enhances the diffuse reflection off a disordered sample in the backward direction. Classically, the enhanced intensity is twice the average background under well chosen experimental conditions. We show how the quantum internal structure of atomic scatterers leads to a significantly smaller enhancement. Theoretical results for double scattering in the weak localization regime are presented which confirm recent experimental observations.
The interference contrast observed in coherent backscattering by cold atoms is drastically reduced with respect to classical disordered media. We study the impact of the degeneracy of the resonant atomic dipole transition on multiple scattering of polarised photons. An analytical treatment allows to derive the diffusion coefficient and depolarisation times for the average light intensity, and dephasing times for the weak localisation corrections. The calculated CBS signals reproduce the experimental results.
