Thomas Wellens, Tobias Geiger, Vyacheslav Shatokhin, Andreas Buchleitner
We deduce the coherent backscattering signal from two distant laser-driven atoms using single-atom equations. In contrast to the standard master equation treatment, this new approach is suitable for the generalization to a large number of atomic scatterers.
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We present a diagrammatic derivation of the coherent backscattering spectrum from two two-level atoms using the pump-probe approach, wherein the multiple scattering signal is deduced from single-atom responses, and provide a physical interpretation of the single-atom building blocks.
The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic) potentials. A two electronic states model in the cesium dimer is used to analyse the effects of this strong coupling regime and to show specific results: i) acceleration of the ground state population to the inner zone due to a non-impulsive regime of coupling at short and intermediate interatomic distances; ii) formation of cold molecules in strongly bound level…
We have designed and implemented a straightforward method to deterministically measure the temperature of the selected segment of a cold atom ensemble, and we have also developed an upgrade in the form of nondestructive thermometry. The essence is to monitor the thermal expansion of the targeted cold atoms after labeling them through manipulating the internal states, and the nondestructive property relies upon the nearly lossless detection via driving a cycling transition. For cold atoms subject to isotropic laser cooling, this method has the unique capability of addressing only the atoms on t…
We study the dynamics of neutral cold atoms in an $L$-shaped crossed-beam optical waveguide formed by two perpendicular red-detuned lasers of different intensities and a blue-detuned laser at the corner. Complemented with a vibrational cooling process this setting works as a one-way device or "atom diode".
We use two-laser optical pumping on a continuous atomic fountain in order to prepare cold cesium atoms in the same quantum ground state. A first laser excites the F=4 ground state to pump the atoms toward F=3 while a second pi-polarized laser excites the F=3 -> F'=3 transition of the D2 line to produce Zeeman pumping toward m=0. To avoid trap states, we implement the first laser in a 2D optical lattice geometry, thereby creating polarization gradients. This configuration has the advantage of simultaneously producing Sisyphus cooling when the optical lattice laser is tuned between the F=4 -> F'…
We study the motion of a cold atom in a frequency-modulated standing laser wave. If the detuning between the atomic electronic transition and the field is large, the atom moves in a modulated optical potential demonstrating known classical nonlinear effects such as chaos and nonlinear resonances. If the atom-field detuning is small, then two optical potentials emerge in the system, and the atom performs Landau-Zener (LZ) tunnelings between them. It is a radically non-classical behavior. However, we show that classical nonlinear structures in system's phase space (KAM-tori and chaotic layers) s…
We present a nonperturbative treatment of coherent backscattering of intense laser light from cold atoms, and predict a nonvanishing backscattering signal even at very large intensities, due to the constructive (self-)interference of inelastically scattered photons.
We study the spectrum of density fluctuations in the ultra-cold gas of neutral atoms, confined in a magneto-optical trap. We determine the corresponding amplitude and spectra of laser light scattered by this medium. We derive an expression for the dynamical structure function, by using a test particle method. We propose to use the collective laser scattering as a diagnostic method for the microscopic properties of the ultra-cold matter. This will also allow us to check on the atomic correlations which are mediated by the collective mean field inside the gas.
Atom laser experiments with Bose-Einstein condensates (BECs) performed in ground-based laboratories feature a coherent and directed beam of atoms which is accelerated by gravity. In microgravity the situation is fundamentally different because the dynamics is entirely determined by the repulsive interaction between the atoms and not by the gravitational force. As a result, the output of a space atom laser is a spherical wave slowly expanding away from the initial BEC.We present a thorough theoretical study of this new source of matter waves based on rf outcoupling which exhibits an isotropic d…
We give a detailed derivation of the master equation description of the coherent backscattering of laser light by cold atoms. In particular, our formalism accounts for the nonperturbative nonlinear response of the atoms when the injected intensity saturates the atomic transition. Explicit expressions are given for total and elastic backscattering intensities in the different polarization channels, for the simplest nontrivial multiple scattering scenario of intense laser light multiply scattering from two randomly placed atoms.
We discuss a method to select the velocities of ultra-cold atoms with a modified Fabry-Perot type of device made of two effective barriers and a well created, respectively, by blue and red detuned lasers. The laser parameters may be used to select the peak and width of the transmitted velocity window. In particular, lowering the central well provides a peak arbitrarily close to zero velocity having a minimum but finite width. The low-energy atomic scattering off this laser device is parameterized and approximate formulae are found to describe and explain its behaviour.
The extreme miniaturization of a cold-atom interferometer accelerometer requires the development of novel technologies and architectures for the interferometer subsystems. Here we describe several component technologies and a laser system architecture to enable a path to such miniaturization. We developed a custom, compact titanium vacuum package containing a microfabricated grating chip for a tetrahedral grating magneto-optical trap (GMOT) using a single cooling beam. In addition, we designed a multi-channel photonic-integrated-circuit-compatible laser system implemented with a single seed la…
We consider light trapping in an amplifying medium consisting of cold alkali-metal atoms; the atomic gas plays a dual role as a scattering and as a gain medium. We perform Monte-Carlo simulations for the combined processes. In some configurations of the inhomogeneous distribution this leads to a point of instability behavior and a signature of random lasing in a cold atomic gas.
We report on the creation, observation and optimization of superposition states of cold atoms. In our experiments, rubidium atoms are prepared in a magneto-optical trap and later, after switching off the trapping fields, Faraday rotation of a weak probe beam is used to characterize atomic states prepared by application of appropriate light pulses and external magnetic fields. We discuss the signatures of polarization and alignment of atomic spin states and identify main factors responsible for deterioration of the atomic number and their coherence and present means for their optimization, like…
In the last 5 years, a novel field of physics and chemistry has developed in which cold trapped ions and ultracold atomic gases are brought into contact with each other. Combining ion traps with traps for neutral atoms yields a variety of new possibilities for research and experiments. These range from studies of cold atom-ion collisions and atom-ion chemistry to applications in quantum information science and condensed matter related research. In this article we give a brief introduction into this new field and describe some of the perspectives for its future development.
We have demonstrated an atom-optical lens, with the advantage of a small scale and flexible adjustment of the parameters, realized by a far red-detuned Gaussian laser beam perpendicular to the propagation direction of the cold atomic cloud. The one-dimensional transverse focusing effect of cold atomic clouds at the temperature order of 1 $μ$K freely falling through the atom-optical lens on the micron scale have been studied theoretically and then verified experimentally. It is found that theory and experiment are in good agreement.
We herein report a simultaneous frequency stabilization of two 780-nm external cavity diode lasers using a precision wavelength meter (WLM). The laser lock performance is characterized by the Allan deviation measurement in which we find $σ_{y}=10^{-12}$ at an averaging time of 1000 s. We also obtain spectral profiles through a heterodyne spectroscopy, identifying the contribution of white and flicker noises to the laser linewidth. The frequency drift of the WLM is measured to be about 2.0(4) MHz over 36 hours. Utilizing the two lasers as a cooling and repumping field, we demonstrate a magneto-…
The electric fields near the heterogeneous metal/dielectric surface of an atom chip were measured using cold atoms. The atomic sensitivity to electric fields was enhanced by exciting the atoms to Rydberg states that are 10^8 times more polarizable than the ground state. We attribute the measured fields to charging of the insulators between the atom chip wires. Surprisingly, it is observed that these fields may be dramatically lowered with appropriate voltage biasing, suggesting configurations for the future development of hybrid quantum systems.
Magnetic resonance in an ensemble of laser-cooled trapped Rb atoms is excited using a micro- cantilever with a magnetic tip. The cantilever is mounted on a multi-layer chip designed to capture, cool, and magnetically transport cold atoms. The coupling is observed by measuring the loss from a magnetic trap as the oscillating cantilever induces Zeeman state transitions in the atoms. Interfacing cold atoms with mechanical devices could enable probing and manipulating atomic spins with nanometer spatial resolution and single-spin sensitivity, leading to new capabilities in quantum computation, qua…
Different laser devices working as ``atom diodes'' or ``one-way barriers'' for ultra-cold atoms have been proposed recently. They transmit ground state level atoms coming from one side, say from the left, but reflect them when they come from the other side. We combine a previous model, consisting of the stimulated Raman adiabatic passage (STIRAP) from the ground to an excited state and a state-selective mirror potential, with a localized quenching laser which produces spontaneous decay back to the ground state. This avoids backwards motion, provides more control of the decay process and theref…
Cold-atom interferometers commonly face systematic effects originating from the coupling between the trajectory of the atomic wave packet and the wave front of the laser beams driving the interferometer. Detrimental for the accuracy and the stability of such inertial sensors, these systematics are particularly enhanced in architectures based on spatially separated laser beams. Here we analyze the effect of a coupling between the relative alignment of two separated laser beams and the trajectory of the atomic wave packet in a four-light-pulse cold-atom gyroscope operated in fountain configurati…
The potential energy curves, permanent and transition dipole moments, and the static dipolar polarizability, of molecular ions composed of one alkali-metal atom and a Strontium ion are determined with a quantum chemistry approach. The molecular ions are treated as effective two-electron systems and are treated using effective core potentials including core polarization, large gaussian basis sets, and full configuration interaction. In the perspective of upcoming experiments aiming at merging cold atom and cold ion traps, possible paths for radiative charge exchange, photoassociation of a cold …
Coherent motion of cold atoms in a standing-wave field is interpreted as a propagation in two optical potentials. It is shown that the wave-packet dynamics can be either regular or chaotic with transitions between these potentials after passing field nodes. Manifestations of de Broglie-wave chaos are found in the behavior of the momentum and position probabilities and the Wigner function. The probability of those transitions depends on the ratio of the squared detuning to the Doppler shift and is large in that range of the parameters where the classical motion is shown to be chaotic.
A mixed system of cooled and trapped, ions and atoms, paves the way for ion assisted cold chemistry and novel many body studies. Due to the different individual trapping mechanisms, trapped atoms are significantly colder than trapped ions, therefore in the combined system, the strong binary ion$-$atom interaction results in heat flow from ions to atoms. Conversely, trapped ions can also get collisionally heated by the cold atoms, making the resulting equilibrium between ions and atoms intriguing. Here we experimentally demonstrate, Rubidium ions (Rb$^+$) cool in contact with magneto-optically …
The equations of motion for the molecular rotation are derived for vibrationally cold dimers that are polarized by off-resonant laser light. It is shown that, by eliminating electronic and vibrational degrees of freedom, a quantum master equation for the reduced rotational density operator can be obtained. The coherent rotational dynamics is caused by stimulated Raman transitions, whereas spontaneous Raman transitions lead to decoherence in the motion of the quantized angular momentum. As an example the molecular dynamics for the optical Kerr effect is chosen, revealing decoherence and heating…
We experimentally study the coherence time of a below-threshold Raman laser in which the gain medium is a gas of magneto-optically trapped atoms. The second-order optical coherence exhibits photon bunching with a correlation time which is varied by two orders of magnitude by controlling the gain. Results are in good agreement with a simple analytic model which suggests the effect is dominated by gain, rather than dispersion, in this system. Cavity ring-down measurements show the photon lifetime, related to the first-order coherence time, is also increased.
We report on the transverse laser cooling of a magnetically guided beam of ultra cold chromium atoms. Radial compression by a tapering of the guide is employed to adiabatically heat the beam. Inside the tapered section heat is extracted from the atom beam by a two-dimensional optical molasses perpendicular to it, resulting in a significant increase of atomic phase space density. A magnetic offset field is applied to prevent optical pumping to untrapped states. Our results demonstrate that by a suitable choice of the magnetic offset field, the cooling beam intensity and detuning, atom losses an…
We analyze the temporal response of the fluorescence light that is emitted from a dense gas of cold atoms driven by a laser. When the average interatomic distance is smaller than the wavelength of the photons scattered by the atoms, the system exhibits strong dipolar interactions and collective dissipation. We solve the exact dynamics of small systems with different geometries and show how these collective features are manifest in the scattered light properties such as the photon emission rate, the power spectrum and the second-order correlation function. By calculating these quantities beyond…
Threshold and frequency properties of a cold ytterbium laser
本文研究了冷镱原子在高精细度腔内的激光作用，重点分析了其激光阈值与频率特性，并与理论模型进行了比较。
We consider the process of cold emission of electrons from a metal in a strong low-frequency laser field. An expression is obtained for the electron spectrum with allowance for their rescattering at the metal surface as a result of an extension of the Fowler-Nordheim theory and modification of the Simplemen model. The numerically simulated features of the electron spectrum are similar to the ATI spectra for atoms and have the same form as the experimental surface emission dependencies for a metal.
We demonstrate lasing into counter-propagating modes of a ring cavity using a gas of cold atoms as a gain medium. The laser operates under the usual conditions of magneto-optical trapping with no additional fields. We characterize the threshold behavior of the laser and measure the second-order optical coherence. The laser emission exhibits directional bistability, switching randomly between clockwise and counter-clockwise modes, and a tuneable nonreciprocity is observed as the atoms are displaced along the cavity axis.
We study photoionization of cold rubidium atoms in a strong infrared laser field using a magneto-optical trap (MOT) recoil ion momentum spectrometer. Three types of cold rubidium target are provided, operating in two-dimension (2D) MOT, 2D molasses, and 3D MOT with densities in the orders of $10^7$ atoms/cm$^3$, $10^8$ atoms/cm$^3$, and $10^9$ atoms/cm$^3$, respectively. The density profile and the temperature of 3D MOT are characterized using the absorption imaging and photoionization. The momentum distributions of Rb$^+$ created by absorption of two- or three-photon illuminate a dipole-like …
While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a significant challenge. We describe here a one-step method to generate entanglement in a dilute gas of cold polar molecules. For molecules in optical traps separated by a few micrometers, we show that maximally entangled states can be created using the strong off-resonant pulses that are routinely used in molecular alignment experiments. We show that the resulting a…
Quantum entanglement has been generated and verified in cold-atom experiments and used to make atom-interferometric measurements below the shot-noise limit. However, current state-of-the-art cold-atom devices exploit separable (i.e. unentangled) atomic states. This Perspective piece asks the question: can entanglement usefully improve cold-atom sensors, in the sense that it gives new sensing capabilities unachievable with current state-of-the-art devices? We briefly review the state-of-the-art in precision cold-atom sensing, focussing on clocks and inertial sensors, identifying the potential b…
We have demonstrated and modeled a simple and efficient method to transfer atoms from a first Magneto-Optical Trap (MOT) to a second one. Two independent setups, with cesium and rubidium atoms respectively, have shown that a high power and slightly diverging laser beam optimizes the transfer between the two traps when its frequency is red-detuned from the atomic transition. This pushing laser extracts a continuous beam of slow and cold atoms out of the first MOT and also provides a guiding to the second one through the dipolar force. In order to optimize the transfer efficiency, the dependence…
We study the spectra of emission of a system composed by an atom, tightly confined inside a high-finesse resonator, when the atom is driven by a laser and is at steady state of the cooling dynamics induced by laser and cavity field. In general, the spectrum of resonance fluorescence and the spectrum at the cavity output contain complementary information about the dynamics undergone by the system. In certain parameter regimes, quantum interference effects between the scattering processes induced by cavity and laser field lead to the selective suppression of features of the resonance fluorescenc…
This work reviews the topic of rotation sensing with compact cold atom interferometers. A representative set of compact free-falling cold atom gyroscopes is considered because, in different respects, they establish a rotation-measurement reference for cold guided-atom technologies. This review first discusses enabling technologies relevant to a set of key functional building blocks of an atom chip-based compact inertial sensor with cold guided atoms. These functionalities concern the accurate and reproducible positioning of atoms to initiate a measurement cycle, the coherent momentum transfer …
Towards a Twisted Atom Laser: Cold Atoms Released from Helical Optical Tube Potentials
本文研究冷原子从螺旋光管势释放后的量子动力学，揭示束缚几何结构可形成空间相干的结构化波包，为实现扭曲玻色-爱因斯坦凝聚体和定向原子激光奠定基础。
We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the strong dipolar exchange interaction between two rotation levels of the polar molecule and two Rydberg states. Such a controllable decay rate opens the way to optically pump the hyperfine levels of polar molecules and it enables the application of conventional laser cooling techniques for cooling polar molecules into quantum degeneracy.
Quantum metrology is the science that aims to achieve precision measurements by making use of quantum principles. Attribute to the well-developed techniques of manipulating and detecting cold atoms, cold atomic systems provide an excellent platform for implementing precision quantum metrology. In this chapter, we review the general procedures of quantum metrology and some experimental progresses in quantum metrology with cold atoms. Firstly, we give the general framework of quantum metrology and the calculation of quantum Fisher information, which is the core of quantum parameter estimation. T…
We report on the observation of strong transmission line shape alterations in a cold-atom hollow-core fiber interface. We show that this can lead to a significant overestimation of the assigned resonant optical depth for high atom densities. By modeling light beam propagation in an inhomogeneous dispersive medium, we attribute the observations to micro lensing in the atomic ensemble in combination with the mode selection of the atom-fiber interface. The approach is confirmed by studies of Rydberg EIT line shapes.
An advanced apparatus for the integration of nanophotonics and cold atoms
研究提出一种结合 nanophotonics 与 cold atoms 的新装置，能将单原子光镊阵列输运至光子晶体波导附近，实现了两者的有效集成。
This paper considers the analogy between the force exerted on cold atoms when they interact with a highly twisted tightly focused laser beam and the forces exerted on a charged dielectric particle inside a uniform electric field when we perform the Millikan's experiment. In the later case the particle experiences its weight, a force due to the electric field which is arranged in the opposite direction of the weight, and a drag force due to the air proportional and opposite to the velocity of the particle. The force due to the electric field is "quantised" since the charge of the particle is al…
We report on the design and characterization of a cold atom source for strontium (Sr) based on a two-dimensional magneto-optical trap (MOT) that is directly loaded from the atom jet of a dispenser. We characterize the atom flux of the source by measuring the loading rate of a three-dimensional MOT. We find loading rates of up to $10^{8}$ atoms per second. The setup is compact, easy to construct, and has low power consumption. It addresses the long standing challenge of reducing the complexity of cold beam sources for Sr, which is relevant for optical atomic clocks and quantum simulation and co…
Optical transport of cold atoms to quantum degeneracy
利用移动光学晶格实现冷原子快速传输至量子简并态，效率超60%，产生40%凝聚分数的简并气体，用于量子传感与计算。
We report the first implementation of a Gauss sum factorization algorithm by an internal state Ramsey interferometer using cold atoms. A sequence of appropriately designed light pulses interacts with an ensemble of cold rubidium atoms. The final population in the involved atomic levels determines a Gauss sum. With this technique we factor the number N=263193.
Using the transfer matrix method, we numerically compute the precise position of the mobility edge of atoms exposed to a laser speckle potential, and study its dependence vs. the disorder strength and correlation function. Our results deviate significantly from previous theoretical estimates using an approximate self-consistent approach of localization. In particular we find that the position of the mobility edge in blue-detuned speckles is much lower than in the red-detuned counterpart, pointing out the crucial role played by the asymmetric on-site distribution of speckle patterns.
Cold atoms from a magneto-optic trap have been used as a nonlinear medium in a nearly resonant cavity. Squeezing in a probe beam passing through the cavity was demonstrated. The measured noise reduction is 40% for free atoms and 20% for weakly trapped atoms.
We show that the adiabatic motion of ultra-cold, multi-level atoms in spatially varying laser fields can give rise to effective non-Abelian gauge fields if degenerate adiabatic eigenstates of the atom-laser interaction exist. A pair of such degenerate dark states emerges e.g. if laser fields couple three internal states of an atom to a fourth common one under pairwise two--photon-resonance conditions. For this so-called tripod scheme we derive general conditions for truly non-Abelian gauge potentials and discuss special examples. In particular we show that using orthogonal laser beams with orb…
We show that giant quasi-bound diatomic complexes, whose size is typically hundreds of nm, can be formed by intra-cavity cold diatom photoassociation or photodissociation in the strong atom-cavity coupling regime.
We study nonlinear optical effects in the laser excitation of Rydberg states. $5S_{1/2}$ and $5P_{3/2}$ levels of $^{85}$Rb are strongly coupled by a strong laser field and probed by a weak laser tuned to the $5P_{3/2} - 44D$ Rydberg resonance. We observe high contrast Autler-Townes spectra which are dependent on the pump polarization, intensity and detuning. The observed behavior agrees with calculations, which include the effect of optical pumping.
Low-order quantum resonances manifested by directed currents have been realized with cold atoms. Here we show that by increasing the strength of an experimentally achievable delta-kicking ratchet potential, quantum resonances of a very high order may naturally emerge and can induce larger ratchet currents than low-order resonances, with the underlying classical limit being fully chaotic. The results offer a means of controlling quantum transport of cold atoms.
The strong evanescent field around ultra-thin unclad optical fibers bears a high potential for detecting, trapping, and manipulating cold atoms. Introducing such a fiber into a cold atom cloud, we investigate the interaction of a small number of cold Caesium atoms with the guided fiber mode and with the fiber surface. Using high resolution spectroscopy, we observe and analyze light-induced dipole forces, van der Waals interaction, and a significant enhancement of the spontaneous emission rate of the atoms. The latter can be assigned to the modification of the vacuum modes by the fiber.
A scheme is proposed for engineering two-mode squeezed states of two separated cold atomic clouds positioned near the surface of a superconducting stripline resonator. Based on the coherent magnetic coupling between the atomic spins and a stripline resonator mode, the desired two-mode squeezed state can be produced via precisely control on the dynamics of the system. This scheme may be used to realize scalable on-chip quantum networks with cold atoms coupling to stripline resonators.
We show that and how ultra-cold atoms in an accelerated two-band lattice are a controlled realization of Landau--Zener--Stückelberg interferometry.
Semiunitary transformation is applied to discuss supersymmetrization of cold Rydberg atoms. In the limit of vanishing kinetic energy the lowest angular momentum of the supersymmetric cold Rydberg atom is $3\hbar/2$. A possible experimental verification is suggested.
We demonstrate experimentally that a cloud of cold atoms with a size comparable to the wavelength of light can induce large group delays on a laser pulse when the laser is tightly focused on it and is close to an atomic resonance. Delays as large as -10 ns are observed, corresponding to "superluminal" propagation with negative group velocities as low as -300 m/s. Strikingly, this large delay is associated with a moderate extinction owing to the very small size of the cloud and to the light-induced interactions between atoms. It implies that a large phase shift is imprinted on the continuous la…
Atom interferometers are a useful tool for precision measurements of fundamental physical phenomena, ranging from local gravitational field strength to the atomic fine structure constant. In such experiments, it is desirable to implement a high momentum transfer "beam-splitter," which may be achieved by inducing quantum resonance in a finite-temperature laser-driven atomic gas. We use Monte Carlo simulations to investigate these quantum resonances in the regime where the gas receives laser pulses of finite duration, and demonstrate that an $ε$-classical model for the dynamics of the gas atoms …
We investigate theoretically the slow group velocity of a pulse probe laser propagating through a cold sample and interacting with atoms in a three-level $Λ$ configuration having losses towards external states. The EIT phenomenon produces very small group velocities for the probe pulse in presence of a strong coupling field even in presence of the population losses, as in an open three-level system. The group velocity and the transmission of the pulses are examined numerically as functions of several parameters, the adiabatic transfer, the loss rate, the modification of the atomic velocity pro…
A new approach to the measurement of gravitational fields with an equilibrium ensemble of ultra-cold alkali atoms confined in a cell of volume $V$ is investigated. The proposed model of the gravitational sensor is based on a variation of the density profile of the ensemble due to changing of the gravitational field. For measurement the atomic density variations of the ensemble the electromagnetically induced transparency method is used.
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