We experimentally study the coherence time of a below-threshold Raman laser in which the gain medium is a gas of magneto-optically trapped atoms. The second-order optical coherence exhibits photon bunching with a correlation time which is varied by two orders of magnitude by controlling the gain. Results are in good agreement with a simple analytic model which suggests the effect is dominated by gain, rather than dispersion, in this system. Cavity ring-down measurements show the photon lifetime, related to the first-order coherence time, is also increased.
Coherent effects manifested in light scattering from cold, optically dense and disordered atomic systems are reviewed from a primarily theoretical point of view. Development of the basic theoretical tools is then elaborated through several physical atomic physics based processes which have been at least partly explored experimentally. These include illustrations drawn from the coherent backscattering effect, random lasing in atomic gases, quantum memories and light-atoms interface assisted by the light trapping mechanism. Current understanding and challenges associated with the transition to h…
We herein report a simultaneous frequency stabilization of two 780-nm external cavity diode lasers using a precision wavelength meter (WLM). The laser lock performance is characterized by the Allan deviation measurement in which we find $σ_{y}=10^{-12}$ at an averaging time of 1000 s. We also obtain spectral profiles through a heterodyne spectroscopy, identifying the contribution of white and flicker noises to the laser linewidth. The frequency drift of the WLM is measured to be about 2.0(4) MHz over 36 hours. Utilizing the two lasers as a cooling and repumping field, we demonstrate a magneto-…
We have observed the propagation of an approximately 35 ns long light pulse with a negative group velocity through a laser-cooled 85Rb atomic medium. The anomalous dispersion results from linear atom-light interaction, and is unrelated to long-lived ground state coherences often associated with fast light in atomic media. The observed negative group velocity (-c/360) in the Rb magneto-optical trap for a pulse attenuated by less than 50% is in good agreement with the value of dispersion measured independently by an RF heterodyne method. The spectral region of anomalous dispersion is between 15 …
The invention of lasers 60 years ago is one of the greatest breakthroughs in modern optics. Throughout the years, lasers have enabled major scientific and technological advancements, and have been exploited in numerous applications due to their advantages such as high brightness and high coherence. However, the high spatial coherence of laser illumination is not always desirable, as it can cause adverse artifacts such as speckle noise. To reduce the spatial coherence, novel laser cavity geometries and alternative feedback mechanisms have been developed. By tailoring the spatial and spectral pr…
We experimentally studied the spatial coherence of random laser emission from dye solutions containing nanoparticles. The spatial coherence, measured in a double-slit experiment, varied significantly with the density of scatterers and the size and shape of the excitation volume. A qualitative explanation is provided, illustrating the dramatic difference from the spatial coherence of a conventional laser. This work demonstrates that random lasers can be controlled to provide intense, spatially incoherent emission for applications in which spatial cross talk or speckle limit performance.
We demonstrate lasing into counter-propagating modes of a ring cavity using a gas of cold atoms as a gain medium. The laser operates under the usual conditions of magneto-optical trapping with no additional fields. We characterize the threshold behavior of the laser and measure the second-order optical coherence. The laser emission exhibits directional bistability, switching randomly between clockwise and counter-clockwise modes, and a tuneable nonreciprocity is observed as the atoms are displaced along the cavity axis.
Hybrid systems of cold atoms and optical cavities are promising systems for increasing the stability of laser oscillators used in quantum metrology and atomic clocks. In this paper we map out the atom-cavity dynamics in such a system and demonstrate limitations as well as robustness of the approach. We investigate the phase response of an ensemble of cold strontium-88 atoms inside an optical cavity for use as an error signal in laser frequency stabilization. With this system we realize a regime where the high atomic phase-shift limits the dynamical locking range. The limitation is caused by th…
We address the problem of achieving a random laser with a cloud of cold atoms, in which gain and scattering are provided by the same atoms. In this system, the elastic scattering cross-section is related to the complex atomic polarizability. As a consequence, the random laser threshold is expressed as a function of this polarizability, which can be fully determined by spectroscopic measurements. We apply this idea to experimentally evaluate the threshold of a random laser based on Raman gain between non-degenerate Zeeman states and find a critical optical thickness on the order of 200, which i…
We show that semiconductor Fano lasers strongly suppress dynamic instabilities induced by external optical feedback. A comparison with conventional Fabry-Perot lasers shows orders of magnitude improvement in feedback stability, and in many cases even total suppression of coherence collapse, which is of major importance for applications in integrated photonics. The laser dynamics are analysed using a generalisation of the Lang-Kobayashi model for semiconductor lasers with external feedback, and an analytical expression for the critical feedback level is derived.
The combination of ultra-cold atomic clouds with the light fields of optical cavities provides a powerful model system for the development of new types of laser cooling and for studying cooperative phenomena. These experiments critically depend on the precise tuning of an incident pump laser with respect to a cavity resonance. Here, we present a simple and reliable experimental tuning scheme based on a two-mode laser spectrometer. The scheme uses a first laser for probing higher-order transversal modes of the cavity having an intensity minimum near the cavity's optical axis, where the atoms ar…
An efficient method to tune the spatial coherence of a degenerate laser over a broad range with minimum variation in the total output power is presented. It is based on varying the diameter of a spatial filter inside the laser cavity. The number of lasing modes supported by the degenerate laser can be controlled from 1 to 320,000, with less than a 50% change in the total output power. We show that a degenerate laser designed for low spatial coherence can be used as an illumination source for speckle-free microscopy that is 9 orders of magnitude brighter than conventional thermal light.
We propose the novel combination of a laser guide and magnetic lens to transport a cold atomic cloud. We have modelled the loading and guiding of a launched cloud of cold atoms with the optical dipole force. We discuss the optimum strategy for loading typically 30% of the atoms from a MOT and guiding them vertically through 22cm. However, although the atoms are tightly confined transversely, thermal expansion in the propagation direction still results in a density loss of two orders of magnitude. By combining the laser guide with a single impulse from a magnetic lens we show one can actually i…
We report non-invasive detection of spin coherence in a collection of Raman-driven cold atoms using dispersive Faraday rotation fluctuation measurements, which opens up new possibilities of probing spin correlations in quantum gases and other similar systems. We demonstrate five orders of magnitude enhancement of the measured signal strength than the traditional spin noise spectroscopy with thermal atoms in equilibrium. Our observations are in good agreement with the comprehensive theoretical modeling of the driven atoms at various temperatures. The extracted spin relaxation rate of cold rubid…
The method of digital processing of laser radiation interference pattern with the digital microscope and original two-beam interferometer with the phase Bragg grating as the amplitude beam splitter for a quantitative determination of the spatial and temporary coherence module of radiation is described. The digital processing of the interference pattern images was carried out with known software algorithms. Principles and functionality of a measurement procedures are demonstrated on measuring of the radiation coherence of several gas, solid-state and diode lasers.
FDML lasers provide sweep rates in the MHz range at wide optical bandwidths, making them ideal sources for high speed OCT. Recently, at lower speed, ultralong-range swept-source OCT has been demonstrated1, 2 using a tunable vertical cavity surface emitting laser (VCSEL) and also using a Vernier-tunable laser. These sources provide relatively high sweep rates and meter range coherence lengths. In order to achieve similar coherence, we developed an extremely well dispersion compensated Fourier Domain Mode Locked (FDML) laser, running at 3.2 MHz sweep rate and 120 nm spectral bandwidth. We demons…
A compact and robust laser system, based on a frequency-doubled telecom laser, providing all the lasers needed for a rubidium cold atom interferometer using optical lattices is presented. Thanks to an optical switch at 1.5 μm and a dual-wavelength second harmonic generation system, only one laser amplifier is needed for all the laser system. Our system delivers at 780 nm a power of 900 mW with a detuning of 110 GHz for the optical lattice and a power of 650 mW with an adjustable detuning between 0 and -1 GHz for the laser cooling, the detection and the Raman transitions.
We design and fabricate an on-chip laser source that produces a directional beam with low spatial coherence. The lasing modes are based on the axial orbit in a stable cavity and have good directionality. To reduce the spatial coherence of emission, the number of transverse lasing modes is maximized by fine-tuning the cavity geometry. Decoherence is reached in a few nanoseconds. Such rapid decoherence will facilitate applications in ultrafast speckle-free full-field imaging.
In this paper we report an experiment on the observation of the recoil-induced resonances (RIR) and electromagnetically induced absorption (EIA) of cold Rb87 atoms in diffuse light. The pump light of the RIR and the EIA comes from the diffuse light in an integrating sphere, which also serves the cooling light. The probe light beam is a weak laser split from the cooling laser in order to keep the cooling and probe lasers correlated. We measured the RIR and the EIA signal varying with the detuning of the diffuse laser light, and also measured the temperature of the cold atoms at the different de…
Combining topologically-protected chiral light transport and laser amplification gives rise to topological lasers, whose operation is immune to fabrication imperfections and defects, uncovering the role of topology in a novel nonlinear non-Hermitian regime. We study a topological laser based on the photonic Haldane model with selective pumping of chiral edge modes described by saturable gain. We investigate elementary excitations around the mean-field steady state and their consequences for the coherence properties. In particular, we show that the hybridization of chiral edge modes gives rise …
The spatial coherence of laser sources has limited their application to parallel imaging and projection due to coherent artifacts, such as speckle. In contrast, traditional incoherent light sources, such as thermal sources or light emitting diodes (LEDs), provide relatively low power per independent spatial mode. Here, we present a chip-scale, electrically-pumped semiconductor laser based on a novel design, demonstrating high power per mode with much lower spatial coherence than conventional laser sources. The laser resonator was fabricated with a chaotic, D-shaped cavity optimized to achieve …
We study quantum coherence of strongly interacting cold bosons in a double-well potential driven by a laser field. The system is initially in a Fock state and, for either with or without a static tilting field, evolves into the coherent states. The coherence is resonantly enhanced by the photon-assisted tunneling. For the tilted wells, it reveals a two-branch pattern which corresponds to the multiple photon absorption or emission, respectively.
Stochastically driven nonlinear processes limit the number of amplified modes in a natural system due to competitive mode interaction, which is accompanied by loss of coherence when increasing the complexity of system. Specifically, we find that modulation instability, which exhibits great fluctuations when it is spontaneously grown from noise in conservative systems, may possess a high degree of coherence in dissipative laser system with gain. Nonlinear mode interactions can be competitive or cooperative: adjusting the intracavity polarization state controls the process of loss of coherence. …
Full-field swept-source optical coherence tomography (FF-SS-OCT) and laser Doppler holography (LDH) are two holographic imaging techniques presenting unique capabilities for ophthalmology. We report on interlaced FF-SS-OCT and LDH imaging with a single instrument. Effectively, retinal blood flow and pulsation could be quasi-simultaneously monitored. This instrument holds potential for a wide scope of ophthalmic applications.
We realize a laser with a cloud of cold rubidium atoms as gain medium, placed in a low-finesse cavity. Three different regimes of laser emission are observed corresponding respectively to Mollow, Raman and Four Wave Mixing mechanisms. We measure an output power of up to 300 $μ$W and present the main properties of these different lasers in each regime.
Speckle is a wave interference phenomenon that has been studied in various fields, including optics, hydrodynamics and acoustics. Speckle patterns contain spectral information of the interfering waves, and of the scattering medium that generates the pattern. Here we study experimentally the speckle patterns generated by the light emitted by two types of semiconductor lasers: conventional laser diodes, where we induce low-coherence emission by optical feedback or by pump current modulation, and coupled nanolasers. In both cases we analyze the intensity statistics of the respective speckle patte…
We propose and demonstrate a method for measuring the time evolution of the off-diagonal elements $ρ_{n,n+k}(t)$ of the reduced density matrix obtained from the quantum theory of the laser. The decay rates of the off-diagonal matrix element $ρ_{n,n+k}(t)$ (k=2,3) are measured for the first time and compared with that of $ρ_{n,n+1}(t)$, which corresponds to the linewidth of the laser. The experimental results agree with the quantum theory of the laser.
We describe statistical and coherence properties of the radiation from x-ray free electron lasers (XFEL). It is shown that the X-ray FEL radiation before saturation is described with gaussian statistics. Particularly important is the case of the optimized X-ray FEL, studied in detail. Applying similarity techniques to the results of numerical simulations allowed us to find universal scaling relations for the main characteristics of an X-ray FEL operating in the saturation regime: efficiency, coherence time and degree of transverse coherence. We find that with an appropriate normalization of th…
We address the problem of achieving an optical random laser with a cloud of cold atoms, in which gain and scattering are provided by the same atoms. The lasing threshold can be defined using the on-resonance optical thickness b0 as a single critical parameter. We predict the threshold quantitatively, as well as power and frequency of the emitted light, using two different light transport models and the atomic polarizability of a strongly-pumped two-level atom. We find a critical b0 on the order of 300, which is within reach of state-of-the-art cold-atom experiments. Interestingly, we find that…
Biologically inspired photonic structures are the key for technological advances and for miniaturized lasers. Here random lasers in dye-doped titania with the disordered structure of paper are proposed. Sharp electromagnetic resonances with unexpected broad spatial extension are reported. The modes interact and compete on wide length scales, enabling to control precisely the device performance by acting on the pumping
We develop a large scale quantum master equation approach to describe dynamical processes of practical open quantum systems driven by both coherent and stochastic interactions by including more than one thousand true states of the systems, motivated by the development of highly bright and fully coherent lasers in the X-ray wavelength regime. The method combines the processes of coherent dynamics induced by the X-ray laser and incoherent relaxations due to spontaneous emissions, Auger decays, and electronic collisions. As examples, theoretical investigation of {\it real} coherent dynamics of in…
We reported a detailed experimental study of the cold collision of Barium monofluoride (BaF) with buffer gas and the high-resolution spectroscopy relevant with direct laser cooling. BaF molecules are efficiently produced with laser ablation and buffer-gas cooled in a cryogenic apparatus. The laser cooling relevant transition $|X^2Σ, v=0, N=1\rangle$ to $|A^2Π, v'=0, J'=1/2\rangle$ is identified. The collision cross section with buffer gas is measured to be $1.4(7)\times10^{-14} cm^{-2}$, which is very suitable for buffer gas cooling. Both rotational and vibrational temperatures are effectively…
To quantify quantum optical coherence requires both the particle- and wave-natures of light. For an ideal laser beam [1,2,3], it can be thought of roughly as the number of photons emitted consecutively into the beam with the same phase. This number, $\mathfrak{C}$, can be much larger than $μ$, the number of photons in the laser itself. The limit on $\mathfrak{C}$ for an ideal laser was thought to be of order $μ^2$ [4,5]. Here, assuming nothing about the laser operation, only that it produces a beam with certain properties close to those of an ideal laser beam, and that it does not have externa…
Spatial coherence quantifies spatial field correlations over time, and is one of the fundamental properties of light. Here we investigate the spatial coherence of highly multimode lasers in the regime of short time scales. Counter intuitively, we show that in this regime, the temporal (longitudinal) modes play a crucial role in spatial coherence reduction. To evaluate the spatial coherence we measured the temporal dynamics of speckle fields generated by a highly multimode laser with over $10^5$ lasing spatial (transverse) modes, and examined the dependence of speckle contrast on the exposure t…
We present an optical trap for atoms that we have developed for precision spectroscopy measurements. Cold atoms are captured in a dark region of space inside a blue-detuned hollow laser beam formed by an axicon. We analyze the light potential in a ray optics picture and experimentally demonstrate trapping of laser-cooled metastable xenon atoms.
We present an all solid-state narrow line-width laser source emitting $670\,\mathrm{mW}$ output power at $671\,\mathrm{nm}$ delivered in a diffraction-limited beam. The \linebreak source is based on a fre-quency-doubled diode-end-linebreak pumped ring laser operating on the ${^4F}_{3/2} \rightarrow {^4I}_{13/2}$ transition in Nd:YVO$_4$. By using periodically-poled po-tassium titanyl phosphate (ppKTP) in an external build-up cavity, doubling efficiencies of up to 86% are obtained. Tunability of the source over $100\,\rm GHz$ is accomplished. We demonstrate the suitability of this robust freque…
A metasurface hologram combines fine spatial resolution and large viewing angles with a planar form factor and compact size. However, it suffers coherent artifacts originating from electromagnetic cross-talk between closely packed meta-atoms and fabrication defects of nanoscale features. Here, we introduce an efficient method to remove all artifacts by fine-tuning the spatial coherence of illumination. Our method is implemented with a degenerate cavity laser, which allows precise, continuous tuning of spatial coherence over a wide range with little variation in emission spectrum and total powe…
A general theoretical approach based on the results of statistical optics is used for the analysis of the transverse coherence properties of 3-rd generation synchrotron sources and x-ray free-electron lasers (XFEL). Correlation properties of the wavefields are calculated at different distances from an equivalent Gaussian Schell-model source. This model is used to describe coherence properties of the five meter undulator source at the synchrotron storage ring PETRA III. In the case of XFEL sources the decomposition of the statistical fields into a sum of independently propagating transverse mod…
A rapid and efficient method for generating laser beams with controlled intensity, phase and coherence distributions is presented. It is based on a degenerate cavity laser in which a digital phase-only spatial light modulator is incorporated. We show that a variety of unique and high-resolution shaped laser beams can be generated with either a low or a high spatial coherence. We also show that by controlling the phase, intensity and coherence distributions, a laser beam can be efficiently reshaped after propagation.
We demonstrate that the shift of the stop band position with increasing oblique angle in periodic structures results in a wide transverse exponential field distribution corresponding to strong angular confinement of the radiation. The beam expansion follows an effective diffusive equation depending only upon the spectral mode width. In the presence of gain, the beam cross section is limited only by the size of the gain area. As an example of an active periodic photonic medium, we calculate and measure laser emission from a dye-doped cholesteric liquid crystal film.
We report on a quantitative measurement of the spatial coherence of electrons emitted from a sharp metal needle tip. We investigate the coherence in photoemission using near-ultraviolet laser triggering with a photon energy of 3.1 eV and compare it to DC-field emission. A carbon-nanotube is brought in close proximity to the emitter tip to act as an electrostatic biprism. From the resulting electron matter wave interference fringes we deduce an upper limit of the effective source radius both in laser-triggered and DC-field emission mode, which quantifies the spatial coherence of the emitted ele…
Conventional lasers make use of optical cavities to provide feedback to gain media. Conversely, mirrorless lasers can be built by using disordered structures to induce multiple scattering, which increases the effective path length in the gain medium and thus provides the necessary feedback. These so-called random lasers potentially offer a new and simple mean to address applications such as lighting. To date, they are all based on condensed-matter media. Interestingly, light or microwave amplification by stimulated emission occurs also naturally in stellar gases and planetary atmospheres. The …
Using a two-dipole model of an optical near-field of Scanning Near-field Optical Microscope tip, i. e. taking into account contributions of magnetic and electric dipoles, we propose and analyze a new type of 3D optical nanotrap found for certain relations between electric and magnetic dipoles. Electric field attains a minimum value in vacuum in the vicinity of the tip and hence such a trap is quite suitable for manipulations with cold atoms.
We present a comprehensive analysis of coherence properties of the radiation from X-ray free electron laser (XFEL). We consider practically important case when XFEL is optimized for maximum gain. Such an optimization allows to reduce significantly parameter space. Application of similarity techniques to the results of numerical simulations allows to present all output characteristics of the optimized XFEL as functions of the only parameter, ratio of the emittance to the radiation wavelength, $ \hatε = 2πε/λ$. Our studies show that optimum performance of the XFEL in terms of transverse coherenc…
Atoms can scatter light and they can also amplify it by stimulated emission. From this simple starting point, we examine the possibility of realizing a random laser in a cloud of laser-cooled atoms. The answer is not obvious as both processes (elastic scattering and stimulated emission) seem to exclude one another: pumping atoms to make them behave as amplifier reduces drastically their scattering cross-section. However, we show that even the simplest atom model allows the efficient combination of gain and scattering. Moreover, supplementary degrees of freedom that atoms offer allow the use of…
We perform a beat-frequency-resolved analysis for two-dimensional electronic spectroscopy using a high-speed and stable 2D electronic spectrometer and few-cycle visible laser pulses to disentangle the vibrational coherences in an artificial fluorescent protein. We develop a highly stable ultrashort light source that generates 5.3-fs visible pulses with a pulse energy of 4.7 uJ at a repetition rate of 10 kHz using multi-plate pulse compression and laser filamentation in a gas cell. The above-5.3-fs laser pulses together with a high-speed multichannel detector enable us to measure a series of 2D…
Single mode laser fields oscillate at frequencies well outside the realm of electronics, but their phase/frequency fluctuations fall into the radio frequency domain, where direct manipulation is possible. Electro-optic devices have sufficient bandwidth for controlling and tailoring the dynamics of a laser field down to sub-nanosecond time scales. Thus, a laser field can be arbitrarily reshaped and in particular its phase/frequency fluctuations can be in principle removed. In practice, the time evolution of a reference laser field can be cloned to replace the fluctuations of another laser field…
Coherence properties and wavelength of light sources are indispensable for optical coherence microscopy/tomography as they greatly influence the signal to noise ratio, axial resolution, and penetration depth of the system. In the present letter, we investigated the longitudinal spatial coherence properties of the pseudo-thermal light source (PTS) as a function of spot size at the diffuser plane, which is controlled by translating microscope objective lens towards or away from the diffuser plane. The axial resolution of PTS is found to be maximum ~ 13 microns for the beam spot size of 3.5 mm at…
The experimental characterization of the spatial and temporal coherence properties of the free-electron laser in Hamburg (FLASH) at a wavelength of 8.0 nm is presented. Double pinhole diffraction patterns of single femtosecond pulses focused to a size of about 10 microns by 10 microns were measured. A transverse coherence length of 6.2 microns in the horizontal and 8.7 microns in the vertical direction was determined from the most coherent pulses. Using a split and delay unit the coherence time of the pulses produced in the same operation conditions of FLASH was measured to be 1.75 fs. From ou…
