The strong evanescent field around ultra-thin unclad optical fibers bears a high potential for detecting, trapping, and manipulating cold atoms. Introducing such a fiber into a cold atom cloud, we investigate the interaction of a small number of cold Caesium atoms with the guided fiber mode and with the fiber surface. Using high resolution spectroscopy, we observe and analyze light-induced dipole forces, van der Waals interaction, and a significant enhancement of the spontaneous emission rate of the atoms. The latter can be assigned to the modification of the vacuum modes by the fiber.
We consider the effect of the long range dipole-dipole interaction on the excitation exchange dynamics of cold two-level atomic gase in the conditions where the size of the atomic cloud is large as compared to the wavelength of the dipole transition. We show that this interaction results in population redistribution across the atomic cloud and in specific spectra of the spontaneous photons emitted at different angles with respect to the direction of atomic polarization.
Tapered optical fibers with a nanofiber waist are versatile tools for interfacing light and matter. In this context, laser-cooled atoms trapped in the evanescent field surrounding the optical nanofiber are of particular interest: They exhibit both long ground-state coherence times and efficient coupling to fiber-guided fields. Here, we demonstrate electromagnetically induced transparency, slow light, and the storage of fiber-guided optical pulses in an ensemble of cold atoms trapped in a nanofiber-based optical lattice. We measure a slow-down of light pulses to group velocities of 50 m/s. More…
We theoretically investigate the interaction of a single quantum dipole with the modes of a fiber-coupled semiconductor waveguide. Through a combination of tight modal confinement and phase-matched evanescent coupling, we predict that approximately 70 % of the dipole's emission can be collected into a single mode optical fiber. Calculations further show that the dipole strongly modifies resonant light transmission through the system, with over an order of magnitude change possible for an appropriate choice of fiber-waveguide coupler geometry.
We investigate a two-way cascaded cavity QED system consisting of microtoroidal resonators coupled through an optical fiber. Each microtoroidal cavity supports two counter-propagating whispering-gallery modes coupled to single atoms through their evanescent fields. We focus on a pair of atom-microtoroid systems and compute the spectrum of spontaneous emission into the fiber with one atom initially excited. Explicit results are presented for strong-coupling and bad-cavity regimes, where the latter allows the effective atom-atom interaction to be controlled through the atom-cavity coupling and d…
We present an omnidirectional matter wave guide on an atom chip. The rotational symmetry of the guide is maintained by a combination of two current carrying wires and a bias field pointing perpendicular to the chip surface. We demonstrate guiding of thermal atoms around more than two complete turns along a spiral shaped 25mm long curved path (curve radii down to 200$μ$m) at various atom--surface distances (35-450$μ$m). An extension of the scheme for the guiding of Bose-Einstein condensates is outlined.
We report on a versatile, highly controllable hybrid cold Rydberg atom fiber interface, based on laser cooled atoms transported into a hollow core Kagomé crystal fiber. Our experiments are the first to demonstrate the feasibility of exciting cold Rydberg atoms inside a hollow core fiber and we study the influence of the fiber on Rydberg electromagnetically induced transparency (EIT) signals. Using a temporally resolved detection method to distinguish between excitation and loss, we observe two different regimes of the Rydberg excitations: one EIT regime and one regime dominated by atom loss. T…
We demonstrate theoretically that photon-photon attraction can be engineered in the continuum of scattering states for pairs of photons propagating in a hollow-core photonic crystal fiber filled with cold atoms. The atoms are regularly spaced in an optical lattice configuration and the photons are resonantly tuned to an internal atomic transition. We show that the hard-core repulsion resulting from saturation of the atomic transitions induces bunching in the photonic component of the collective atom-photon modes (polaritons). Bunching is obtained in a frequency range as large as tens of GHz, a…
We describe a simple scheme for the implementation and control of effective spin-spin interactions in self-assembled crystals of cold polar molecules. In our scheme spin states are encoded in two long-lived rotational states of the molecules and coupled via state dependent dipole-dipole forces to the lattice vibrations. We show that by choosing an appropriate time dependent modulation of the induced dipole moments the resulting phonon-mediated interactions compete with the direct dipole-dipole coupling and lead to long-range and tunable spin-spin interaction patterns. We illustrate how this te…
We model single photon nonlinearities resulting from the dipole-dipole interactions of cold polar molecules. We propose utilizing ``dark state polaritons'' to effectively couple photon and molecular states; through this framework, coherent control of the nonlinearity can be expressed and potentially used in an optical quantum computation architecture. Due to the dipole-dipole interaction the photons pick up a measurable nonlinear phase even in the single photon regime. A manifold of protected symmetric eigenstates is used as basis. Depending on the implementation, major sources of decoherence …
We describe a simple experimental technique which allows us to store a small and deterministic number of neutral atoms in an optical dipole trap. The desired atom number is prepared in a magneto-optical trap overlapped with a single focused Nd:YAG laser beam. Dipole trap loading efficiency of 100 % and storage times of about one minute have been achieved. We have also prepared atoms in a certain hyperfine state and demonstrated the feasibility of a state-selective detection via resonance fluorescence at the level of a few neutral atoms. A spin relaxation time of the polarized sample of $4.2\pm…
We show that it is possible to simulate an anyon by a trapped atom which possesses an induced electric dipole moment in the background of electromagnetic fields with a specific configuration. The electromagnetic fields we applied contain a magnetic and two electric fields. We find that when the atom is cooled down to the limit of the negligibly small kinetic energy, the atom behaves like an anyon because its angular momentum takes fractional values. The fractional part of the angular momentum is determined by both the magnetic and one of the electric fields. Roles two electromagnetic fields pl…
We experimentally demonstrate a ring geometry all-fiber cavity system for cavity quantum electrodynamics with an ensemble of cold atoms. The fiber cavity contains a nanofiber section which mediates atom-light interactions through an evanescent field. We observe well-resolved, vacuum Rabi splitting of the cavity transmission spectrum in the weak driving limit due to a collective enhancement of the coupling rate by the ensemble of atoms within the evanescent field, and we present a simple theoretical model to describe this. In addition, we demonstrate a method to control and stabilize the resona…
We report on the observation of strong transmission line shape alterations in a cold-atom hollow-core fiber interface. We show that this can lead to a significant overestimation of the assigned resonant optical depth for high atom densities. By modeling light beam propagation in an inhomogeneous dispersive medium, we attribute the observations to micro lensing in the atomic ensemble in combination with the mode selection of the atom-fiber interface. The approach is confirmed by studies of Rydberg EIT line shapes.
We report on an efficient and highly controlled cold atom hollow-core fiber interface, suitable for quantum simulation, information, and sensing. The main focus of this manuscript is a detailed study on transporting cold atoms into the fiber using an optical conveyor belt. We discuss how we can precisely control the spatial, thermal, and temporal distribution of the atoms by, e.g., varying the speed at which the atoms are transported or adjusting the depth of the transport potential according to the atomic position. We characterize the transport of atoms to the fiber tip for these different pa…
We demonstrate the first guiding of cold atoms through a 88 mm long piece of photonic band gap fiber. The guiding potential is created by a far-off resonance dipole trap propagating inside the fiber with a hollow core of 12 mu m. We load the fiber from a dark spot 85-Rb magneto optical trap and observe a peak flux of more than 10^5 atoms/s at a velocity of 1.5 m/s. With an additional reservoir optical dipole trap, a constant atomic flux of 1.5 10^4 atoms/s is sustained for more than 150\,ms. These results open up interesting possibilities to study nonlinear light-matter interaction in a nearly…
We develop a one-step scheme for generating multiparticle entangled states between two cold atomic clouds in distant cavities coupled by an optical fiber. We show that, through suitably choosing the intensities and detunings of the fields and precisely tuning the time evolution of the system, multiparticle entanglement between the separated atomic clouds can be engineered deterministically, in which quantum manipulations are insensitive to the states of the cavity and losses of the fiber. The experimental feasibility of this scheme is analyzed based on recent experimental advances in the reali…
To manipulate cold atoms in spatially constrained quantum engineering platforms, we developed a lensless optical system with a $\sim$1 $μ$m resolution and a transverse size of only 225 $μ$m. We use a multimode optical fiber with a high numerical aperture, which directly guides light inside the ultra-high-vacuum system. Spatial light modulators allow us to generate control beams at the in-vacuum fiber end by digital optical phase conjugation. As a demonstration, we use this system to optically transport cold atoms towards the in-vacuum fiber end, to load them in optical microtraps and to re-coo…
We developed an ultra-compact high-resolution imaging system for cold atoms. Its only in-vacuum element is a multimode optical fiber with a diameter of $230\,μ$m, which simultaneously collects light and guides it out of the vacuum chamber. External adaptive optics allow us to image cold Rb atoms with a $\sim 1\,μ$m resolution over a $100 \times 100\,μ$m$^2$ field of view. These optics can be easily rearranged to switch between fast absorption imaging and high-sensitivity fluorescence imaging. This system is particularly suited for hybrid quantum engineering platforms where cold atoms are combi…
We study the emergence of collective scattering in the presence of dipole-dipole interactions when we illuminate a cold cloud of rubidium atoms with a near-resonant and weak intensity laser. The size of the atomic sample is comparable to the wavelength of light. When we gradually increase the atom number from 1 to 450, we observe a broadening of the line, a small red shift and, consistently with these, a strong suppression of the scattered light with respect to the noninteracting atom case. Numerical simulations, which include the internal atomic level structure, agree with the data.
The capture of a moving atom by a non-dissipative trap, such as an optical dipole trap, requires the removal of the excessive kinetic energy of the atom. In this article we develop a mechanism to harvest ultra cold atoms from a guided atom beam into an optical dipole trap by removing their directed kinetic energy. We propose a continuous loading scheme where this is accomplished via deceleration by a magnetic potential barrier followed by optical pumping to the energetically lowest Zeeman sublevel. We theoretically investigate the application of this scheme to the transfer of ultra cold chromi…
We present a novel technique for measuring the characteristics of a magneto-optical trap for cold atoms by monitoring the spontaneous emission from trapped atoms coupled into the guided mode of a tapered optical nanofiber. We show that the nanofiber is highly sensitive to very small numbers of atoms close to its surface. The size and shape of the MOT, determined by translating the cold atom cloud across the tapered fiber, is in excellent agreement with measurements obtained using the conventional method of fluorescence imaging using a CCD camera. The coupling of atomic fluorescence into the ta…
We review here the studies performed about interactions in an assembly of cold Rydberg atoms. We focus more specially the review on the dipole-dipole interactions and on the effect of the dipole blockade in the laser Rydberg excitation, which offers attractive possibilities for quantum engineering. We present first the various interactions between Rydberg atoms. The laser Rydberg excitation of such an assembly is then described with the introduction of the dipole blockade phenomenon. We report recent experiments performed in this subject by starting with the case of a pair of atoms allowing th…
We theoretically investigate the process of coupling cold atoms into the core of a hollow-core photonic-crystal optical fiber using a blue-detuned Laguerre-Gaussian beam. In contrast to the use of a red-detuned Gaussian beam to couple the atoms, the blue-detuned hollow-beam can confine cold atoms to the darkest regions of the beam thereby minimizing shifts in the internal states and making the guide highly robust to heating effects. This single optical beam is used as both a funnel and guide to maximize the number of atoms into the fiber. In the proposed experiment, Rb atoms are loaded into a …
Results of numerical Monte Carlo simulations for the Stark-tuned Förster resonance and dipole blockade between two to five cold rubidium Rydberg atoms in various spatial configurations are presented. The effects of the atoms' spatial uncertainties on the resonance amplitude and spectra are investigated. The feasibility of observing coherent Rabi-like population oscillations at a Förster resonance between two cold Rydberg atoms is analyzed. Spectra and the fidelity of the Rydberg dipole blockade are calculated for various experimental conditions, including nonzero detuning from the Förster reso…
We show that microwave spectroscopy of a dense Rydberg gas trapped on a superconducting atom chip in the dipole blockade regime reveals directly the dipole-dipole many-body interaction energy spectrum. We use this method to investigate the expansion of the Rydberg cloud under the effect of repulsive van der Waals forces and the breakdown of the frozen gas approximation. This study opens a promising route for quantum simulation of many-body systems and quantum information transport in chains of strongly interacting Rydberg atoms.
We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the strong dipolar exchange interaction between two rotation levels of the polar molecule and two Rydberg states. Such a controllable decay rate opens the way to optically pump the hyperfine levels of polar molecules and it enables the application of conventional laser cooling techniques for cooling polar molecules into quantum degeneracy.
We study light-assisted collisions in an ensemble containing a small number (~3) of cold Rb87 atoms trapped in a microscopic dipole trap. Using our ability to operate with one atom exactly in the trap, we measure the one-body heating rate associated to a near-resonant laser excitation, and we use this measurement to extract the two-body loss rate associated to light-assisted collisions when a few atoms are present in the trap. Our measurements indicate that the two-body loss rate can reach surprisingly large values beta>10^{-8} cm^{3}.s^{-1} and varies rapidly with the trap depth and the param…
An integrated optical dipole trap uses two-color (red and blue-detuned) traveling evanescent wave fields for trapping cold neutral atoms. To achieve longitudinal confinement, we propose using an integrated optical waveguide coupler, which provides a potential gradient along the beam propagation direction sufficient to confine atoms. This integrated optical dipole trap can support an atomic ensemble with a large optical depth due to its small mode area. Its quasi-TE0 waveguide mode has an advantage over the HE11 mode of a nanofiber, with little inhomogeneous Zeeman broadening at the trapping re…
The dipole blockade of Rydberg excitations is a hallmark of the strong interactions between atoms in these high-lying quantum states. One of the consequences of the dipole blockade is the suppression of fluctuations in the counting statistics of Rydberg excitations, of which some evidence has been found in previous experiments. Here we present experimental results on the dynamics and the counting statistics of Rydberg excitations of ultra-cold Rubidium atoms both on and off resonance, which exhibit sub- and super-Poissonian counting statistics, respectively. We compare our results with numeric…
We analyze the temporal response of the fluorescence light that is emitted from a dense gas of cold atoms driven by a laser. When the average interatomic distance is smaller than the wavelength of the photons scattered by the atoms, the system exhibits strong dipolar interactions and collective dissipation. We solve the exact dynamics of small systems with different geometries and show how these collective features are manifest in the scattered light properties such as the photon emission rate, the power spectrum and the second-order correlation function. By calculating these quantities beyond…
We study the coupling of internal electronic excitations to vibrational modes of the external motion of ultracold atoms in an optical lattice. For different ground and excited state potentials the on-site coupling of excitations and vibrations term renormalizes the effective electronic transition energy, which appears e.g. in clock transitions. In addition in the Mott state with filling factor one, the dipole-dipole coupling between neighbouring sites includes emission and absorption of vibrational quanta. Such processes create a significant mechanism for excitation of vibrations leading to mo…
We discuss the implementation of quantum gate operations in a self-assembled dipolar crystal of polar molecules. Here qubits are encoded in long-lived spin states of the molecular ground state and stabilized against collisions by repulsive dipole-dipole interactions. To overcome the single site addressability problem in this high density crystalline phase, we describe a new approach for implementing controlled single and two-qubit operations based on resonantly enhanced spin-spin interactions mediated by a localized phonon mode. This local mode is created at a specified lattice position with t…
The transversely confined propagating modes of an optical fiber mediate virtually infinite range energy exchanges among atoms placed within their field, which adds to the inherent free space dipole-dipole coupling. Typically, the single atom free space decay rate largely surpasses the emission rate into the guided fiber modes. However, scaling up the atom number as well as the system size amounts to entering a collective emission regime, where fiber-induced superradiant spontaneous emission dominates over free space decay. We numerically study this super- and subradiant decay of highly excited…
While the Rydberg-blockade regime provides the natural setting for creating $W$-type entanglement with cold neutral atoms, it is demonstrated here that a scalable entanglement resource of this type can even be obtained under completely different physical circumstances. To be more precise, a special instance of twisted $W$ states -- namely, $π$-twisted ones -- can be engineered in one-dimensional arrays of cold neutral atoms with Rydberg-dressed resonant dipole-dipole interaction. In particular, it is shown here that this is possible even when a (dressed) Rydberg excitation is coupled to the mo…
We report the confinement of large clouds of ultra-cold 85-Rb atoms in a standing-wave dipole trap formed by the two counter-propagating modes of a high-Q ring-cavity. Studying the properties of this trap we demonstrate loading of higher-order transverse cavity modes and excite recoil-induced resonances.
We present a brief overview of the transport of quantum light across a one-dimensional waveguide which is integrated with a periodic string of quantum-scale dipoles. We demonstrate a scheme to implement transparency by suitably tuning the atomic frequencies without applying a coupling field and bring out the pronounced non-reciprocity of this optical device. The fiber-mediated interaction between integrated dipoles allows one to achieve both dispersive and dissipative couplings, level repulsion and attraction, and enhanced sensing capabilities. All these ideas can be translated to a wide varie…
We present our results on the experiments with cold Rb Rydberg atoms in a magneto-optical trap (MOT). Characteristic features of our experiment were the excitation of Rydberg atoms in a small volume within the cold atom cloud and sorting of the measured signals and spectra over the number of registered Rydberg atoms. We have measured the effective lifetime of the Rydberg state 37P, as well as its polarizability in a weak electric field. The results are in good agreement with the theoretical calculations. We have shown that localization of the small excitation volume around the zero-magnetic-fi…
We demonstrate a cooperative optical non-linearity caused by dipolar interactions between Rydberg atoms in an ultra-cold atomic ensemble. By coupling a probe transition to the Rydberg state we map the strong dipole-dipole interactions between Rydberg pairs onto the optical field. We characterize the non-linearity as a function of electric field and density, and demonstrate the enhancement of the optical non-linearity due to cooperativity.
We have observed resonant energy transfer between cold Rydberg atoms in spatially separated cylinders. Resonant dipole-dipole coupling excites the 49s atoms in one cylinder to the 49p state while the 41d atoms in the second cylinder are transferred down to the 42p state. We have measured the production of the 49p state as a function of separation of the cylinders (0 - 80 um) and the interaction time (0 - 25 us). In addition we measured the width of the electric field resonances. A full many-body quantum calculation reproduces the main features of the experiments.
In this article, the atom excitation suppression is studied in two ways. The first way of exploring the excitation suppression is by an external DC electric field. The second way is to study the excitation suppression caused by electric field generated by free charges, which are created by ionizing atoms. This suppression is called Coulomb blockade. Here the Coulomb forces are created by ions through ionizing atoms by a UV laser. The theory shows that the interaction, which causes the suppression, is primarily caused by charge-dipole interactions. Here the charge is the ion, and the dipole is …
We calculate the optical potentials, i.e. the light shifts, of the ground and excited states of atomic cesium in a two-color evanescent field around a subwavelength-diameter fiber. We show that the light shifts of the $6S_{1/2}\leftrightarrow 6P_{3/2}$ transitions can be minimized by tuning one trapping light to around 934.5 nm in wavelength (central red-detuned magic wavelength) and the other light to around 685.5 nm in wavelength (central blue-detuned magic wavelength). The simultaneous use of the red- and blue-detuned magic wavelengths allows state-insensitive two-color trapping and guiding…
We study the behavior of a single laser-driven trapped ion inside a microscopic optical Fabry-Perot cavity. In particular, we demonstrate a fiber Fabry-Perot cavity operating on the principal $S_{1/2}\to P_{1/2}$ electric dipole transition of an Yb$^+$ ion at $369\,$nm with an atom-ion coupling strength of $g=2π\times 67(1)\,$MHz. We employ the cavity to study the generation of single photons and observe cavity-induced back-action in the Purcell-enhanced emission of photons. Tuning of the amplitude and phase of the back-action allows us to enhance or suppress the total rate of photoemission fr…
We report enhanced transmission in measurements of the spectral dependence of forward light scattering by a high-density and cold ensemble of 87Rb atoms. This phenomenon, which is a result of dipole-dipole interaction induced cooperative light scattering in the atomic sample, implies a significant departure from the traditional density dependence of the transmitted light as embodied in the Beer-Lambert Law. Absolute values of the density-dependent forward light scattering cross-section are extracted from the measurements.
Speckle-based feedback control of optical dipole trap axial waist position
Russian Quantum Center（俄罗斯量子中心）；Moscow Institute of Physics and Technology（莫斯科物理技术学院）；National Research Nuclear University MEPhI（国立核研究大学MEPhI）；PN Lebedev Institute RAS（P.N.列别捷夫物理研究所）
We have observed Stueckelberg oscillations in the dipole-dipole interaction between Rydberg atoms with an externally applied radio-frequency field. The oscillating RF field brings the interaction between cold Rydberg atoms in two separated volumes into resonance. We observe multi-photon transitions when varying the amplitude of the RF-field and the static electric field offset. The angular momentum states we use show a quadratic Stark shift, which leads to a fundamentally different behavior than linearly shifting states. Both cases are studied theoretically using the Floquet approach and are c…
Cold atoms in highly excited Rydberg states are promising candidates to implement quantum logic gates of a quantum computer via long-range dipole-dipole interaction. Two-qubit gates require a controlled interaction of only two close Rydberg atoms. We report on the first spectroscopic observation of the resonant dipole-dipole interaction between two cold rubidium Rydberg atoms confined in a small laser excitation volume. The interaction strength was controlled by fine-tuning of the Rydberg levels into a Forster resonance using the Stark effect. The observed resonance line shapes are in good agr…
Understanding decoherence in cryogenically-cooled rare-earth-ion doped glass fibers is of fundamental interest and a prerequisite for applications of these material in quantum information applications. Here we study the coherence properties in a weakly doped erbium silica glass fiber motivated by our recent observation of efficient and long-lived Zeeman sublevel storage in this material and by its potential for applications at telecommunication wavelengths. We analyze photon echo decays as well as the potential mechanisms of spectral diffusion that can be caused by coupling with dynamic disord…
