We present a detailed analytical and numerical analysis of the inelastic coherent backscattering spectrum of laser light incident on cold atoms. We identify frequency domains where the interference contribution can be positive \emph{as well as} negative -- or exhibits dispersive character. These distinctive features are explained by reciprocity arguments and dressed state two-photon scattering amplitudes.
We report on the simultaneous observation, by delayed Bragg diffraction, of four- and six-wave mixing processes in a coherently prepared atomic ensemble consisting of cold cesium atoms. For each diffracted order, we observe different temporal pulse shapes and dependencies with the intensities of the exciting fields, evidencing the different mechanisms involved in each process. The various observations are well described by a simplified analytical theory, which considers the atomic system as an ensemble of three-level atoms in Λ configuration.
We present a scheme to obtain the coherently enhanced Raman scattering in atomic vapor which is induced by a spin wave initially written by a weak write laser. The enhancement of Raman scattering is dependent on the number and the spatial distribution of the flipped atoms generated by the weak write laser. Such an enhanced Raman scattering may have practical applications in quantum information, nonlinear optics and laser spectroscopy because of its simplicity.
We describe parametric down conversion process in a two-level atomic gas, where the atoms are in a superposition state of relevant energy levels. This superposition results in splitting of the phase matching condition into three different conditions. Another, more important, peculiarity of the system under discussion is the nonsaturability of amplification coefficients with increasing pump wave intensity, under "sideband" generation conditions.
We show deterministic generation of Werner states as a steady state of the collective decay dynamics of a pair of neutral atom coupled to a leaky cavity and strong coherent drive. We also show how the scheme can be extended to generate $2N$-particle analogue of the bipartite Werner states.
It has been shown in recent years that incoherent pumping through multiple atomic levels provides a mechanism for the production of highly anti-bunched light, and that as the number of incoherent steps is increased the light becomes increasingly regular. We show that in a resonance fluorescence situation, a multi-level atom may be multiply coherently driven so that the fluorescent light is highly anti-bunched. We show that as the number of coherently driven levels is increased, the spontaneous emissions may be made increasingly more regular. We present a systematic method for designing the lev…
Stochastic perturbation of two-level atoms strongly driven by a coherent light field is analyzed by the quantum trajectory method. A new method is developed for calculating the resonance fluorescence spectra from numerical simulations. It is shown that in the case of dominant incoherent perturbation, the stochastic noise can unexpectedly create phase correlation between the neighboring atomic dressed states. This phase correlation is responsible for quantum interference between the related transitions resulting in anomalous modifications of the resonance fluorescence spectra.
We demonstrate the existence of new nonclassical correlations in the radiation of two atoms, which are coherently driven by a continuous laser source. The photon-photon-correlations of the fluorescence light show a spatial interferene pattern not present in a classical treatment. A feature of the new phenomenon is, that bunched and antibunched light is emitted in different spatial directions. The calculations are performed analytically. It is pointed out, that the correlations are induced by state reduction due to the measurement process when the detection of the photons does not distinguish b…
A system of coherently-driven two-level atoms is analyzed in presence of two independent stochastic perturbations: one due to collisions and a second one due to phase fluctuations of the driving field. The behaviour of the quantum interference induced by the collisional noise is considered in detail. The quantum-trajectory method is utilized to reveal the phase correlations between the dressed states involved in the interfering transition channels. It is shown that the quantum interference induced by the collisional noise is remarkably robust against phase noise. This effect is due to the fact…
Analysis of the effects of decoherence on the radiative and squeezing properties of a coherently driven two-level atom trapped in a resonant cavity applying the corresponding master equation is presented. The atomic dynamics as well as the squeezing and statistical properties of the emitted radiation are investigated. It is found that the atom stays in the lower energy level more often at steady state irrespective of the strength of the coherent radiation and thermal fluctuations entering the cavity. Moreover, a strong external coherent radiation results the splitting of the line of the emissi…
Optical lattice loaded with cold atoms can exhibit a tunable photonic band gap for a weak probe field under the conditions of electromagnetically induced transparency. This system possesses a number of advantageous properties, including reduced relaxation of Raman coherence and the associated probe absorption, and simultaneous enhancement of the index modulation and the resulting reflectivity of the medium. This flexible system has a potential to serve as a testbed of various designs for the linear and nonlinear photonic band gap materials at a very low light level and can be employed for real…
We report the observation of small group velocities of order 90 meters per second, and large group delays of greater than 0.26 ms, in an optically dense hot rubidium gas (~360 K). Media of this kind yield strong nonlinear interactions between very weak optical fields, and very sharp spectral features. The result is in agreement with previous studies on nonlinear spectroscopy of dense coherent media.
Interest in lossless nonlinearities has focussed on the the dispersive properties of $Λ$ systems under conditions of electromagnetically induced transparency (EIT). We generalize the lambda system by introducing further degenerate states to realize a `Chain $ Λ$' atom where multiple coupling of the probe field significantly enhances the intensity dependent dispersion without compromising the EIT condition.
A broadband squeezed vacuum photon field is characterized by a complex squeezing function. We show that by controlling the wavelength dependence of its phase it is possible to change the dynamics of the atomic polarization interacting with the squeezed vacuum. Such a phase modulation effectively produces a finite range temporal interaction kernel between the two quadratures of the atomic polarization yielding the change in the decay rates as well as the appearance of additional oscillation frequencies. We show that decay rates slower than the spontaneous decay rate can be achieved even for a s…
Simultaneous strong coherent pumping of the two transitions of a V-level atom with very differentdecay rates has been predicted to create almost perfect inversion on the narrower transition. Usingthe example of the blue and red transitions in Strontium we show that for suitable operatingconditions the corresponding resonant gain can be used to continuously operate a laser on thenarrow transition. In particular, for a strong detuning of the pump field with respect to the narrowtransition, coherent laser emission occurs close to the bare atomic transition frequency exhibitingonly a negligible co…
We propose a procedure to achieve a complete energy conversion between laser pulses carrying orbital angular momentum (OAM) in a cloud of cold atoms characterized by a double-Λatom-light coupling scheme. A pair of resonant spatially dependent control fields prepare atoms in a position-dependent coherent population trapping state, while a pair of much weaker vortex probe beams propagate in the coherently driven atomic medium. Using the adiabatic approximation we derive the propagation equations for the probe beams. We consider a situation where the second control field is absent at the entrance…
The collective behavior of ensembles of atoms has been studied in-depth since the seminal paper of Dicke [R. H. Dicke, Phys. Rev. 93, 99 (1954)], where he demonstrated that a group of emitters in collective states is able to radiate with increased intensity and modified decay rates in particular directions, a phenomenon which he called superradiance. Here, we show that the fundamental setup of two atoms coupled to a single-mode cavity can be distinctly exceeding the free-space superradiant behavior, a phenomenon which we call hyperradiance. The effect is accompanied by strong quantum fluctuati…
We study the interaction of a weak probe field, having two orthogonally polarized components, with an optically dense medium of four-level atoms in a tripod configuration. In the presence of a coherent driving laser, electromagnetically induced transparency is attained in the medium, dramatically enhancing its linear as well as nonlinear dispersion while simultaneously suppressing the probe field absorption. We present the semiclassical and fully quantum analysis of the system. We propose an experimentally feasible setup that can induce large Faraday rotation of the probe field polarization an…
A detailed derivation of the master equation of the cavity radiation of a coherently prepared $Y$-shaped four-level correlated emission laser is presented. The outline of the procedures that can be employed in analytically solving the stochastic differential equations and the rate equations of various correlations are also provided. It is shown that coherently preparing the atoms in the upper two energy levels and the lower, initially, can lead to a genuine continuous variable tripartite entanglement. Moreover, preparing the atoms in the coherent superposition, other than the possible maximum …
We report a combined theoretical and experimental study of the spectral and polarization dependence of near resonant radiation coherently backscattered from an ultracold gas of 85Rb atoms. Measurements in an approximately 6 MHz range about the 5s^{2}S_{1/2}- 5p^{2}P_{3/2}, F=3 - F'=4 hyperfine transition are compared with simulations based on a realistic model of the experimental atomic density distribution. In the simulations, the influence of heating of the atoms in the vapor, magnetization of the vapor, finite spectral bandwidth, and other nonresonant hyperfine transitions are considered. G…
We consider transfer of optical vortices between laser pulses carrying orbital angular momentum (OAM) in a cloud of cold atoms characterized by the $Λ$ configuration of the atom-light coupling. The atoms are initially prepared in a coherent superposition of the lower levels, creating a so-called phaseonium medium. If a single vortex beam initially acts on one transition of the $Λ$ scheme, an extra laser beam is subsequently generated with the same vorticity as that of the incident vortex beam. The absorption of the incident probe beam takes place mostly at the beginning of the atomic medium wi…
In this tutorial we provide a short review of attosecond pulse characterization techniques and a pedagogical account of a recently proposed method called Pulse Analysis by Delayed Absorption (PANDA) [Pabst and Dahlström, Phys. Rev. A, 94, 13411 (2016)]. We discuss possible implementations of PANDA in alkali atoms using either principal quantum number wave packets or spin-orbit wave packets. The main merit of the PANDA method is that it can be used as a pulse characterization method that is free from atomic latency effects, such as scattering phase shifts and long-lived atomic resonances. Final…
The efficiency of an ensemble-based optical quantum memory depends critically on the strength of the atom-light coupling. An optical cavity is an effective method to enhance atom-light coupling strength, with the drawback that cavities can be difficult to integrate into a memory setup. In this work we show coherent enhancement of atom-light coupling via an interference effect. The light to be absorbed into the atomic ensemble is split and used to drive the atoms from opposite ends of the ensemble. We compare this method theoretically to a cavity enhanced scheme and present experimental results…
We report a detailed investigation on the generation of pulse pairs during the readout of a coherence grating stored in a cold atomic ensemble. The pulse shapes and the split of the retrieved energy between the two pulses are studied as a function of the relative intensities of the two reading fields, and a minimum is observed for the total retrieved energy. We introduce a simplified analytical theory for the process, considering a three-level atomic system, which explains all the most striking experimental features.
Adiabatic preparation of a fractional quantum Hall fluid by coherently pumping atoms from a Bose-Einstein condensate
Pitaevskii BEC Center, INO-CNR and Dipartimento di Fisica, Università di Trento（皮塔耶夫斯基玻色-爱因斯坦凝聚中心，意大利国家研究委员会物质研究所和特伦托大学物理系）；Department of Physics, TU Dortmund University（多特蒙德大学物理系）；Technische Universität Berlin, Institut für Physik und Astronomie（柏林工业大学物理与天文学研究所）
Several sequential operations are usually needed for implementing controlled quantum gates and generating entanglement between a pair of quantum bits. Based on the conditional quantum dynamics for a two-ion system beyond the Lamb-Dicke limit, here we propose a theoretical scheme for manipulating two-qubit quantum information, i.e., implementing a universal two-qubit quantum gate and generating a two-qubit entangled state, by using a pair of simultaneous laser pulses. Neither the Lamb-Dicke approximation nor the auxiliary atomic level are required. The experimental realizability of this simple …
We propose a method to study the quantum nonlinearity and observe the multiphoton transitions in a multiatom CQED system. We show that by inducing simultaneously destructive quantum interference for the single-photon and two-photon excitations in the CQED system, it is possible to observe the direct three-photon excitation of the higher-order ladder states of the CQED system. We report an experiment with cold Rb atoms confined in an optical cavity and demonstrate such interference control of the multi-photon excitations of the CQED system. The observed nonlinear excitation of the CQED ladder s…
Recent experiments [K. R. Brown, et al., Nature 471, 196 (2011); and M. Harlander, et al., Nature 471, 200 (2011)] have demonstrated the coherent manipulations on the external vibrations of two ions, confined individually in the separated ion traps. Using these recently developed techniques, we propose here an approach to realize the coherent operations, e.g., the universal quantum gates, between the separated ion-trap qubits encoded by two internal atomic states of the trapped ions. Our proposal operates beyond the usual Lamb-Dicke limits, and could be applied to the scalable ion traps couple…
Coherently displaced harmonic oscillator number states of a harmonically bound ion can be coupled to two internal states of the ion by a laser-induced motional sideband interaction. The internal states can subsequently be read out in a projective measurement via state-dependent fluorescence, with near-unit fidelity. This leads to a rich set of line shapes when recording the internal-state excitation probability after a sideband excitation, as a function of the frequency detuning of the displacement drive with respect to the ion's motional frequency. We precisely characterize the coherent displ…
In a cavity quantum electrodynamics (QED) system, where atoms coherently interact with photons in a cavity, the eigenstates of the system are the superposition states of atoms and cavity photons, the so-called dressed states of atoms. When two cavities are connected by an optical fiber with negligible loss, the coherent coupling between the cavities gives rise to photonic normal modes. One of these normal modes is the fiber-dark mode, in which photons are delocalized in the two distant cavities. Here we demonstrate the setting of coupled-cavities QED, where two nanofiber cavity-QED systems are…
We consider the near-resonant interaction between a single atom and a focused light mode, where a single atom localized at the focus of a lens can scatter a significant fraction of light. Complementary to previous experiments on extinction and phase shift effects of a single atom, we report here on the measurement of coherently backscattered light. The strength of the observed effect suggests combining strong focusing with the well-established methods of cavity QED. We consider theoretically a nearly concentric cavity, which should allow for a strongly focused optical mode. Simple estimates sh…
The long-range dipole-dipole interaction can create delocalized states due to the exchange of excitation between Rydberg atoms. We show that even in a random gas many of the single-exciton eigenstates are surprisingly delocalized, composed of roughly one quarter of the participating atoms. We identify two different types of eigenstates: one which stems from strongly-interacting clusters, resulting in localized states, and one which extends over large delocalized networks of atoms. These two types of states can be excited and distinguished by appropriately tuned microwave pulses, and their rela…
With quantum interference of two-path spontaneous emissions, we propose a novel scheme to coherently control the atom--photon momentum entanglement through atomic internal coherence. A novel phenomenon called ``momentum phase entanglement'' is reported, and we found, under certain conditions, that more controllable entangled state can be produced with super--high degree of entanglement.
Two light pulses propagating with ultra-slow group velocities in a coherently prepared atomic gas exhibit dissipation-free nonlinear coupling of an unprecedented strength. This enables a single-photon pulse to coherently control or manipulate the quantum state of the other. Processes of this kind result in generation of entangled states of radiation field and open up new prospectives for quantum information processing.
We study the impact of double and triple scattering contributions on coherent backscattering of laser light from saturated isotropic atoms, in the helicity preserving polarization channel. Using the recently proposed diagrammatic pump-probe approach, we analytically derive single-atom spectral responses to a classical polychromatic driving field, combine them self-consistently to double and triple scattering processes, and numerically deduce the corresponding elastic and inelastic spectra, as well as the total backscattered intensities. We find that account of the triple scattering contributio…
We outline the non-perturbative theory of multiple scattering of resonant, intense laser light off a dilute cloud of cold atoms. A combination of master equation and diagrammatic techniques allows, for the first time, a quantitative description of nonlinear diffusive transport as well as of coherent backscattering of the injected electromagnetic field, notwithstanding the exponential growth of Hilbert space with the number of atomic scatterers. As an exemplary application, we monitor the laser light's intensity profile within the medium, the spectrum of the backscattered light and the coherent…
Three level atom optics (TLAO) is introduced as a simple, efficient and robust method to coherently manipulate and transport neutral atoms. The tunneling interaction among three trapped states allows to realize the spatial analog of the stimulated Raman adiabatic passage (STIRAP), coherent population trapping (CPT), and electromagnetically induced transparency (EIT) techniques. We investigate a particular implementation in optical microtrap arrays and show that under realistic parameters the coherent manipulation and transfer of neutral atoms among dipole traps could be realized in the millise…
We consider N identical two-level atoms coupled to an optical cavity, which is coherently driven by an external field. In the limit of small atomic excitation, the reflection and transmission coefficients for both fields and intensities are calculated analytically. In addition, the frequency content of the cavity field and hence also the emission spectrum of the cavity is determined. It is discussed in particular how individual collisional dephasing and common atomic energy-level fluctuations prevent the cavity field from being in a coherent state, which in turn affects the outgoing fields.
In this paper the possibility of generating nonlinear coherent states of the radiation field in a micromaser is explored. It is shown that these states can be provided in a lossless micromaser cavity under the weak Jaynes-Cummings interaction with intensity-dependent coupling of large number of individually injected two-level atoms in a coherent superposition of the upper and lower states. In particular, we show that the so-called nonlinear squeezed vacuum and nonlinear squeezed first excited states, as well as the even and odd nonlinear coherent states can be generated in the presence of two-…
Calibrating the strength of the light-matter interaction is an important experimental task in quantum information and quantum state engineering protocols. The strength of the off-resonant light-matter interaction in multi-atom spin oscillators can be characterized by the coupling rate $Γ_\text{S}$. Here we utilize the Coherently Induced Faraday Rotation (CIFAR) signal for determining the coupling rate. The method is suited for both continuous and pulsed readout of the spin oscillator, relying only on applying a known polarization modulation to the probe laser beam and detecting a known optical…
We discuss methods for coherently controlling mesoscopic atomic ensembles where the number of atoms varies randomly from one experimental run to the next. The proposed schemes are based on adiabatic passage and Rydberg blockade and can be used for implementation of a scalable quantum register formed by an array of randomly loaded optical dipole traps.
We investigate the implementation of a controlled-Z gate on a pair of Rydberg atoms in spatially separated dipole traps where the joint excitation of both atoms into the Rydberg level is strongly suppressed (the Rydberg blockade). We follow the adiabatic gate scheme of Jaksch et al. [1], where the pair of atoms are coherently excited using lasers, and apply it to the experimental setup outlined in Gaëtan et al. [2]. We apply optimisation to the experimental parameters to improve gate fidelity, and consider the impact of several experimental constraints on the gate success.
The orbital angular momentum (OAM) from a laser beam can be coherently transferred to a Bose-Einstein condensate in a ring trap, in quantized units of $\hbar$. The light-matter coupling allows for the superradiant transfer of the atoms between the discrete OAM states. Tuning the ring parameters and winding number of the pump light, specific angular momentum states can be populated. This in turn allows control of the emission to generate light with OAM different from that of the pump, as the atomic ring imprints its contribution on the scattered light.
Coherent transport of atoms trapped in an optical lattice can be controlled by microwave-induced spin flips that correlate with site-to-site hopping. We study the controllability of homogeneous one-dimensional systems of noninteracting atoms in the absence of site addressability. Given these restrictions, we construct a deterministic protocol to map an initially localized Wannier state to a wave packet that that is coherently distributed over n sites. This is extended to analytic solutions for arbitrary unitary maps given homogenous systems and in the presence of time-dependent uniform forces.…
We study the coherent quantum evolution of a closed and driven mesoscopic chain of two-level systems that interact via the van-der-Waals interaction in their excited state. The Hamiltonian consists of a part corresponding to a classical lattice gas and an off-diagonal driving term without classical counterpart. We show that in a certain parameter range the latter leads to a thermalization of the system with respect to observables of the classical lattice gas such as the interaction energy and particle number distribution. We investigate the evolution of the system into this thermal state and d…
We analytically show that probabilistic amplification of a weak coherent state stored inside an atomic medium can be achieved via detection of coherently scattered photons. We show that this is because of collective excitations created among atoms in the ensemble. We describe the physics of the amplification and identify the failure events, which occur during the amplification process. The amplification is realized by coherently mapping a weak coherent state in an ensemble of $Λ$-level atoms followed by detection of multiple Raman scattered photons, conditionally projecting the coherent state …
We show how two circular polarization components of a linearly polarized pulse, propagating through a coherently driven dilute atomic vapor, can be well resolved in time domain by weak measurement. Slower group velocity of one of the components due to electromagnetically induced transparency leads to a differential group delay between the two components. For low number density, this delay may not be large enough to temporally resolve the two components. We show how this can be enhanced in terms of mean time of arrival of the output pulse through a post-selected polarizer. We demonstrate the id…
Atoms in a sub-wavelength lattices have remarkable optical properties that have become of high scientific and technological significance. Here, we show how the coupling of light to more than a single atomic array can expand these perspectives into the domain of quantum nonlinear optics. While a single array transmits and reflects light in a largely linear fashion, the combination of two arrays is found to induce strong photon-photon interactions that can convert an incoming classical beam into highly antibunched light. Such quantum metasurfaces open up new possibilities for coherently generati…
We suggest a combined atomic/molecular system for quantum computation, which takes advantage of highly developed techniques to control atoms and recent experimental progress in manipulation of ultracold molecules. We show that two atoms of different species in a given site, {\it e.g.}, in an optical lattice, could be used for qubit encoding, initialization and readout, with one atom carrying the qubit, the other enabling a gate. In particular, we describe how a two-qubit phase gate can be realized by transferring a pair of atoms into the ground rovibrational state of a polar molecule with a la…
We study the tunneling of a two-level atom in a double well potential while the atom is coupled to a single electromagnetic field mode of a cavity. The coupling between internal and external degrees of freedom, due to the mechanical effect on the atom from photon emission into the cavity mode, can dramatically change the tunneling behavior. We predict that in general the tunneling process becomes quasiperiodic. In a certain regime of parameters a collapse and revival of the tunneling occurs. Accessing the internal degrees of freedom of the atom with a laser allows to coherently manipulate the …
For a transition $F_e=0\leftrightarrow F_g=1$ driven by a linearly polarized light and probed by a circularly light, quantum coherence effects are investigated. Due to the coherence between the drive Rabi frequency and Zeeman splitting, electromagnetically induced transparency, electromagnetically induced absorption, and the transition from positive to negative dispersion are obtained, as well as the populations coherently oscillating in a wide spectral region. At the zero pump-probe detuning, the subluminal and superluminal light propagation is predicted. Finally, coherent population trapping…
We study the resonance fluorescence from a coherently driven four-level atom in the Y-type configuration. The effects of quantum interference induced by spontaneous emission on the fluorescence properties of the atom are investigated. It is found that the quantum interference resulting from cascade emission decays of the atom leads to a splitting of resonances in the excited level populations calculated as a function of light detuning. For some parameters, interference assisted enhancement of inner sidebands and narrowing of central peaks may also occur in the fluorescence spectrum. We present…
Efficient excitation of a single two-level system usually requires that the driving field is at the same frequency as the atomic transition. However, the scattered laser light in solid-state implementations can dominate over the single photons, imposing an outstanding challenge to perfect single-photon sources. Here, we propose a background-free method using a phase-locked dichromatic electromagnetic field with no spectral overlap with the optical transition for a coherent control of a two-level system, and we demonstrate this method experimentally with a single quantum dot embedded in a micro…
We demonstrate finite range binding potentials between pairs of Rydberg atoms interacting with each other via attractive and repulsive van der Waals potentials and driven by a microwave field. We show that, using destructive quantum interference to cancel single-atom Rydberg excitation, the Rydberg-dimer states can be selectively and coherently populated from the two-atom ground state. This can be used to realize a two-qubit interaction gate which is not susceptible to mechanical forces between the atoms and is therefore immune to motional decoherence.
