We investigate the implementation of a controlled-Z gate on a pair of Rydberg atoms in spatially separated dipole traps where the joint excitation of both atoms into the Rydberg level is strongly suppressed (the Rydberg blockade). We follow the adiabatic gate scheme of Jaksch et al. [1], where the pair of atoms are coherently excited using lasers, and apply it to the experimental setup outlined in Gaëtan et al. [2]. We apply optimisation to the experimental parameters to improve gate fidelity, and consider the impact of several experimental constraints on the gate success.
We consider the dynamics of intracavity electromagnetically induced transparency (EIT) in an ensemble of strongly interacting Rydberg atoms. By combining the advantage of variable cavity lifetimes with intracavity EIT and strongly interacting Rydberg dark-state polaritons, we show that such intracavity EIT system could exhibit very strong photon blockade effect.
The dipole blockade of multiple Rydberg excitations in mesoscopic atomic ensembles allows the implementation of various quantum information tasks using collective states of cold, trapped atoms. Precise coherent manipulations of the collective ground and single Rydberg excitation states of an atomic ensemble requires the knowledge of the number of atoms with small uncertainty. We present an efficient method to acquire such information by interrogating the atomic ensemble with resonant pulses while monitoring the resulting Rydberg excitations. We show that after several such steps accompanied by…
We propose an efficient method to filter out single atoms from trapped ensembles with unknown number of atoms. The method employs stimulated adiabatic passage to reversibly transfer a single atom to the Rydberg state which blocks subsequent Rydberg excitation of all the other atoms within the ensemble. This triggers the excitation of Rydberg blockaded atoms to short lived intermediate states and their subsequent decay to untrapped states. Using an auxiliary microwave field to carefully engineer the dissipation, we obtain a nearly deterministic single-atom source. Our method is applicable to sm…
We show that Jaynes-Cummings dynamics can be observed in mesoscopic atomic ensembles interacting with a classical electromagnetic field in the regime of Rydberg blockade, where the time dynamics of the average number of Rydberg excitations in mesoscopic ensembles displays collapses and revivals typical of this model. As the frequency of Rabi oscillations between collective states of Rydberg blockaded ensembles depends on the number of interacting atoms, for randomly loaded optical dipole traps we predict collapses and revivals of Rabi oscillations. We have studied the effects of finite interac…
Strongly Rydberg-blockaded two-level atoms form a Rydberg superatom, which is excited only to a collective symmetrical Dicke state. However, emerging often in the alkali-earth atoms, the spontaneous decay from the Rydberg state to an additional pooling state renders the ensemble no longer a closed superatom. Herein we present a computationally-efficient model to characterize the interaction between a fully Rydberg-blockaded ensemble of $N$ $Λ$-type three-level atoms and a strong probe light field in a coherent state. The model enables us to achieve a decomposition of the coupled dynamics in th…
By coupling a probe transition to a Rydberg state using electro-magnetically induced transparency (EIT) we map the strong dipole-dipole interactions onto an optical field. We characterize the resulting cooperative optical non-linearity as a function of probe strength and density. We show that the effect of dipole blockade cannot be described using a mean-field but requires an $N$-atom cooperative model. Good quantitative agreement is obtained for three atoms per blockade with the $n=60$ Rydberg state. We place an upper-limit on the dephasing rate of the blockade spheres of $<110$ kHz.
A recent experiment on a 51-atom Rydberg blockaded chain observed anomalously long-lived temporal oscillations of local observables after quenching from an antiferromagnetic initial state. This coherence is surprising as the initial state should have thermalized rapidly to infinite temperature. In this article, we show that the experimental Hamiltonian exhibits non-thermal behavior across its entire many-body spectrum, with similar finite-size scaling properties as models proximate to integrable points. Moreover, we construct an explicit small local deformation of the Hamiltonian which enhance…
In a previous letter we studied the giant optical nonlinearities of a Rydberg atomic medium within an optical cavity, in the Schwinger-Keldysh formalism. In particular, we calculated the non-linear contributions to the spectrum of the light transmitted through the cavity. In this article we spell out the essential details of this calculation, and we show how it can be extended to higher input photon numbers, and higher order correlation functions. As a relevant example, we calculate and discuss the three-photon correlation function of the transmitted light, and discuss its physical significanc…
We observe and measure dispersive optical non-linearities in an ensemble of cold Rydberg atoms placed inside an optical cavity. The experimental results are in agreement with a simple model where the optical non-linearities are due to the progressive appearance of a Rydberg blockaded volume within the medium. The measurements allow a direct estimation of the "blockaded fraction" of atoms within the atomic ensemble.
Controlling strongly interacting many-body systems enables the creation of tailored quantum matter, with properties transcending those based solely on single particle physics. Atomic ensembles which are optically driven to a Rydberg state provide many examples of this, such as atom-atom entanglement, many-body Rabi oscillations, strong photon-photon interaction and spatial pair correlations. In its most basic form, Rydberg quantum matter consists of an isolated ensemble of strongly interacting atoms spatially confined to the blockade volume - a so-called superatom. Here we demonstrate the cont…
We study the quantum melting of quasi-one-dimensional lattice models in which the dominant energy scale is given by a repulsive dipolar interaction. By constructing an effective low-energy theory, we show that the melting of crystalline phases can occur into two distinct liquid phases, having the same algebraic decay of density-density correlations, but showing a different non-local correlation function expressing string order. We present possible experimental realizations using ultracold atoms and molecules, introducing an implementation based on resonantly driven Rydberg atoms that offers ad…
The Toffoli gate serving as a basic building block for reversible quantum computation, has manifested its great potentials in improving the error-tolerant rate in quantum communication. While current route to the creation of Toffoli gate requires implementing sequential single- and two-qubit gates, limited by longer operation time and lower average fidelity. We develop a new theoretical protocol to construct a universal $(n+1)$-qubit Toffoli gate sphere based on the Rydberg blockade mechanism, by constraining the behavior of one central target atom with $n$ surrounding control atoms. Its merit…
Due to the intrinsic strong blockaded interaction shifting the energy level of Rydberg state, the steady Rydberg probability may be substantially restrained to a low level, especially for atoms suffering from weak drivings. We report an exotic excitation facilitation using strong blockaded energy shifting the double excitation state, leading to the weakly-driven atom deterministically excited by a significantly improved fraction even at far off-resonant regimes. This phenomenon is attributed to the effective induction of a reduced detuning to the weakly-driven atom by optimizing parameters of …
Kinetically constrained cavity QED: from blockaded ferromagnetism to long-range quantum scars
Institute of Physics, Johannes Gutenberg University Mainz（约翰内斯·古腾堡大学美因茨物理研究所）；Department of Physics, University of Konstanz（康斯坦茨大学物理系）；ICFO—Institut de Ciències Fotòniques, The Barcelona Institute of Science and Technology（巴塞罗那科技学院光子科学研究所）；ICREA—Institució Catalana de Recerca i Estudis Avançats（加泰罗尼亚高级研究学院）；Max-Planck-Institut für Quantenoptik（马克斯·普朗克量子光学研究所）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）；Fakultät für Physik, Ludwig-Maximilians-Universität（路德维希-马克西米利安大学物理学院）；Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）；Department of Physics, The State University of New York at Buffalo（纽约州立大学布法罗分校物理系）
We present a fast and Quasideterministic protocol for the production of single ions and electrons from a cloud of laser cooled atoms. The approach is based on a two-step process where first a single Rydberg atom is photo-excited from a dipole-blockade configuration and subsequently ionized by an electric field pulse. We theoretically describe these excitation-ionization cycles via dynamical quantum maps and observe a rich behavior of the ionization dynamics as a function of laser Rabi frequency, pulse duration and particle number. Our results show that a fast sequential heralded production of …
Recent atomic physics experiments and numerical works have reported complementary signatures of the emergence of a topological quantum spin liquid in models with blockade interactions. However, the specific mechanism stabilizing such a phase remains unclear. Here, we introduce an exact relation between an Ising-Higgs lattice gauge theory on the kagome lattice and blockaded models on Ruby lattices. This relation elucidates the origin of previously observed topological spin liquids by directly linking the latter to a deconfined phase of a solvable gauge theory. By means of exact diagonalization …
We present an entanglement scheme for Rydberg atoms using the van der Waals interaction phase induced by Ramsey-type pulsed interactions. This scheme realizes not only controlled phase operations between atoms at a distance larger than Rydberg blockade distance, but also various counter-intuitive entanglement examples, including two-atom entanglement in the presence of a closer third atom and $W$-state generation for partially-blockaded three atoms. Experimental realization is conducted with single rubidium atoms loaded in an array of optical tweezer dipole traps, to demonstrate the proposed e…
We demonstrate a new versatile building block for optical quantum technologies, based on an intracavity Rydberg-blockaded atomic ensemble acting as a single two-level superatom. We coherently control its state and optically detect it in a single shot with a $95\%$ efficiency. Crucially, we demonstrate a superatom-state-dependent $π$ phase rotation on the light reflected from the cavity. Together with the state manipulation and detection, it is a key ingredient for implementing deterministic photonic entangling gates and for generating highly non-classical light states.
We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is conditioned on the rotational state of the polar molecules, allowing for realization of a CNOT quantum gate between the molecules and the atom. Subsequent readout of the atomic fluorescence results in a non-destructive measurement of the rotational state. We study the interaction between a 1D array of polar molecules and an array or a cloud of atoms in a Rydberg su…
Rydberg blockaded gate is a fundamental ingredient for scalable quantum computation with neutral Rydberg atoms. However the fidelity of such a gate is intrinsically limited by a blockade error coming from a Rydberg level shift that forbids its extensive use. Based on a dark-state adiabatic passage, we develop a novel protocol for realizing a two-atom blockade-error-free quantum gate in a hybrid system with simultaneous van der Waals (vdWsI) and resonant dipole-dipole interactions (DDI). The basic idea relies on converting the roles of two interactions, which is, the DDI serves as one time-depe…
Scheme to prepare three-dimensional entangled state between a pair of Rydberg atoms is proposed via dissipative dynamics and Electromagnetic Induced Transparency (EIT) associated with the single-atom dark state. The prepared entangled state is the dark state of the whole system. The schemes are feasible no matter the system initially in arbitrary purity or mixed states and do not have accurate requirements on evolution time. In contrast to most of the former Rydberg-atombased dissipative schemes, the Rydberg-Rydberg interaction (RRI) strength do not need to satisfy a certain relation with lase…
A Rydberg atom array coupled to a high-cooperativity optical cavity
University of California, Berkeley（加州大学伯克利分校）；Challenge Institute for Quantum Computation, University of California, Berkeley（加州大学伯克利分校量子计算挑战研究所）；Columbia University（哥伦比亚大学）；Oratomic
Rydberg-atom quantum simulators are of keen interest because of their possibilities towards high-dimensional qubit architectures. Here we report three-dimensional conformation spectra of quantum-Ising Hamiltonian systems with programmed qubit connections. With a Rydberg-atom quantum simulator, various connected graphs, in which vertices and edges represent atoms and blockaded couplings, respectively, are constructed in two or three-dimensional space and their eigenenergies are probed during their topological transformations. Star, complete, cyclic, and diamond graphs, and their geometric inter…
Fault-tolerant implementation of quantum gates is one of preconditions for realizing quantum computation. The platform of Rydberg atoms is one of the most promising candidates for achieving quantum computation. We propose to implement a controlled-$Z$ gate on Rydberg atoms where an amplitude-modulated field is employed to induce Rydberg antiblockade. Gate robustness against the fluctuations in the Rydberg-Rydberg interaction can be largely enhanced by adjusting amplitude-modulated field. Furthermore, we introduce a Landau-Zener-Stückelberg transition on the target atom so as to improve the gat…
We investigate the dynamical Casimir effect and its detection with Rydberg atoms. The photons are created in a resonant cavity with a plasma mirror of a semiconductor slab which is irradiated by periodic laser pulses. The canonical Hamiltonian is derived for the creation and annihilation operators showing the explicit time-variation in the couplings, which originates from the external configuration such as a nonstationary plasma mirror. The number of created photons is evaluated as squeezing from the Heisenberg equations with the Hamiltonian. Then, the detection of the photons as the atomic ex…
In this paperwe propose two theoretical schemes for implementation of quantum phase gates by engineering the phase-sensitive dark state of two atoms subjected to Rydberg-Rydberg interaction. Combining the conventional adiabatic techniques and currently developed approaches of phase control, a feasible proposal for implementation of a geometric phase gate is presented, where the conditional phase shift (Berry phase) is achieved by adiabatically and cyclically changing the parameters of the driving fields. Here we find that the geometric phase acquired is related to the way how the relative phas…
We theoretically investigate the manipulation of the motional states of trapped ground-state atoms using Rydberg dressing via nonresonant laser fields. The forces resulting from Rydberg-state interaction between dressed neighboring atoms in an array of microtraps or an optical lattice can strongly couple their motion. We show that intensity modulation of the dressing field allows to squeeze the relative motion of a pair of atoms and generate non-classical mechanical states. Extending this pairwise scheme to one-dimensional chains provides flexible control over the mechanical degrees of freedom…
Controlled phase (CPHASE) gates can in principle be realized with trapped neutral atoms by making use of the Rydberg blockade. Achieving the ultra-high fidelities required for quantum computation with such Rydberg gates is however compromised by experimental inaccuracies in pulse amplitudes and timings, as well as by stray fields that cause fluctuations of the Rydberg levels. We report here a comparative study of analytic and numerical pulse sequences for the Rydberg CPHASE gate that specifically examines the robustness of the gate fidelity with respect to such experimental perturbations. Anal…
We analyze excitation of two ground state atoms to a double Rydberg state by a two-photon chirped optical pulse in the regime of adiabatic rapid passage. For intermediate Rydberg-Rydberg interaction strengths, relevant for atoms separated by $\sim$ten $μ$m, adiabatic excitation can be achieved at experimentally feasible Rabi frequencies and chirp rates of the pulses, resulting in high transfer efficiencies. We also study the adiabatic transfer between ground and Rydberg states as a means to realize a controlled phase gate between atomic qubits.
Symmetric ensembles of neutral atoms interacting via the Rydberg blockade are well-described by the Jaynes-Cummings Hamiltonian. We use this framework to study the problem of generating arbitrary superpositions of Dicke states of hyperfine qubits in such ensembles. The combination of the symmetric Rydberg blockade and microwaves that drive the qubits with a time-dependent phase is sufficient to make these ensembles completely controllable, in the sense that one can generate an arbitrary unitary transformation on the system. We apply this to the problem of state mapping. With currently feasible…
We propose a hybrid optomechanical quantum system consisting of a moving membrane strongly coupled to an ensemble of N atoms with a Rydberg state. Due to the strong van-der-Waals interaction between the atoms, the ensemble forms an effective two-level system, a Rydberg superatom, with a collectively enhanced atom-light coupling. Using this superatom imposed collective enhancement strong coupling between membrane and superatom is feasible for parameters within the range of current experiments. The quantum interface to couple the membrane and the superatom can be a pumped single mode cavity, or …
Significant efforts are being directed towards developing a quantum annealer capable of solving combinatorial optimization problems. The challenges are Hamiltonian programming and large-scale implementations. Here we report quantum annealing demonstration of Ising Hamiltonians programmed with up to $N=22$ spins mapped on various Cayley tree graphs. Experiments are performed with a Rydberg-atom quantum simulator, in which rubidium single atoms are arranged in three dimensional space in such a way that their Rydberg atoms and blockaded strong couplings respectively represent the nodes and edges …
Universal quantum gates and quantum error correction~(QEC) lie in the heart of quantum information science. Large-scale quantum computing depends on a universal set of quantum gates, in which some gates may be easily carried out, while others are hard with a certain physical system. There is a unique three-qubit quantum gate called the Deutsch gate~[$\mathbb{D}(θ)$], from which alone a circuit can be constructed so that any feasible quantum computing is attainable. As far as we know, however, $\mathbb{D}(θ)$ has not been demonstrated. Here we design an easily realizable $\mathbb{D}(θ)$ by usin…
We propose a robust localization of the highly-excited Rydberg atoms, interacting with doughnut-shaped optical vortices. Compared with the earlier standing-wave (SW)-based localization methods, a vortex beam can provide an ultrahigh-precision two-dimensional localization solely in the zero-intensity center, within a confined excitation region down to the nanometer scale. We show that the presence of the Rydberg-Rydberg interaction permits counter-intuitively much stronger confinement towards a high spatial resolution when it is partially compensated by a suitable detuning. In addition, applyin…
Based on the PXP model adapted for Rydberg-blockaded chains, we investigate dynamics of topological domain walls between different quantum many-body scar states of $\mathbb{Z}_2$ symmetry. It is found that, the domain walls not only possess oscillating features of scars but also manifest longstanding bipartite entanglement with exactly unchanged flip-flop phase difference, suggesting their potential as quantum information resource. A periodically driven field is exerted and the high-frequency drive gives rise to a phase transition from prethermalization to Floquet localization. In order to inv…
Optimized EIT-Based Multi-Target CNOT^k Gates in Heteronuclear Rydberg Atom Arrays
School of Physics, Beihang University（北京航空航天大学物理学院）；State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics, Wuhan Institute of Physics and Mathematics, Innovation Academy for Precision Measurement Science and Technology, Chinese Academy of Sciences（中国科学院精密测量科学与技术创新研究院武汉物理与数学研究所磁共振与原子分子物理国家重点实验室）
We discuss a method for scaling a neutral atom Rydberg gate quantum processor to a large number of qubits. Limits are derived showing that the number of qubits that can be directly connected by entangling gates with errors at the $10^{-3}$ level using long range Rydberg interactions between sites in an optical lattice, without mechanical motion or swap chains, is about 500 in two dimensions and 7500 in three dimensions. A scaling factor of 60 at a smaller number of sites can be obtained using collective register encoding in the hyperfine ground states of the rare earth atom Holmium. We present…
The spin-wave (SW) NOON state is an $N$-particle Fock state with two atomic spin-wave modes maximally entangled. Attributed to the property that the phase is sensitive to collective atomic motion, the SW NOON state can be utilized as a novel atomic interferometer and has promising application in quantum enhanced measurement. In this paper we propose an efficient protocol to deterministically produce the atomic SW NOON state by employing Rydberg blockade. Possible errors in practical manipulations are analyzed. A feasible experimental scheme is suggested. Our scheme is far more efficient than t…
We develop a scheme for deterministic generation of an entangled state between two atoms on different Rydberg states via a chirped adiabatic passage, which directly connects the initial ground and target entangled states and also does not request the normally needed blockade effect. The occupancy of intermediate states suffers from a strong reduction via two pulses with proper time-dependent detunings and the electromagnetically induced transparency condition. By solving the analytical expressions of eigenvalues and eigenstates of a two-atom system, we investigate the optimal parameters for gu…
