A natural approach to measure the time of arrival of an atom at a spatial region is to illuminate this region with a laser and detect the first fluorescence photons produced by the excitation of the atom and subsequent decay. We investigate the actual physical content of such a measurement in terms of atomic dynamical variables, taking into account the finite width of the laser beam. Different operation regimes are identified, in particular the ones in which the quantum current density may be obtained.
An operational arrival-time distribution is defined as the distribution of detection times of the first photons emitted by two level atoms in resonance with a perpendicular laser beam in a time of flight experiment. For ultracold Cesium atoms the simulations are in excellent agreement with the theoretical ideal time-of-arrival distribution of Kijowski.
We study the scattering of two-level atoms at narrow laser fields, modeled by a $δ$-shape intensity profile. The unique properties of these potentials allow us to give simple analytic solutions for one or two field zones. Several applications are studied: a single $δ$-laser may serve as a detector model for atom detection and arrival-time measurements, either by means of fluorescence or variations in occupation probabilities. We show that, in principle, this ideal detector can measure the particle density, the quantum mechanical flux, arrival time distributions or local kinetic energy densitie…
A recent approach to arrival times used the fluorescence of an atom entering a laser illuminated region and the resulting arrival-time distribution was close to the axiomatic distribution of Kijowski, but not exactly equal, neither in limiting cases nor after compensation of reflection losses by normalization on the level of expectation values. In this paper we employ a normalization on the level of operators, recently proposed in a slightly different context. We show that in this case the axiomatic arrival time distribution of Kijowski is recovered as a limiting case. In addition, it is shown…
For a quantum-mechanically spread-out particle we investigate a method for determining its arrival time at a specific location. The procedure is based on the emission of a first photon from a two-level system moving into a laser-illuminated region. The resulting temporal distribution is explicitly calculated for the one-dimensional case and compared with axiomatically proposed expressions. As a main result we show that by means of a deconvolution one obtains the well known quantum mechanical probability flux of the particle at the location as a limiting distribution.
Classical and quantum scattering of a non-Gaussian wave packet by a rectangular barrier is studied in terms of arrival times to a given detector location. A classical wave equation, proposed by N. Rosen [{\it{Am. J. Phys.}} {\bf 32} (1964) 377], is used to study the corresponding classical dynamics. Mean arrival times are then computed and compared for different values of initial wave packet parameters and barrier width. The agreement is improved in the large mass limit as one expects. A short comment on the possibility of generalization of Rosen's proposal to a two-body system is given. Diffe…
A semiclassical model supporting the destructive interference interpretation of zero-width resonances (ZWR) is extended to wavelengths inducing c_minus-type curve crossing situations in Na2 strong field dissociation. This opens the possibility to get critical couples of wavelengths lambda and field intensities I to reach ZWRs associated with the ground vibrationless level v = 0, that, contrary to other vibrational states (v > 0), is not attainable for the commonly referred c+-type crossings. The morphology of such ZWRs in the laser (I; lambda) parameter plane and their usefulness in filtration…
We model ideal arrival-time measurements for free quantum particles and for particles subject to an external interaction by means of a narrow and weak absorbing potential. This approach is related to the operational approach of measuring the first photon emitted from a two-level atom illuminated by a laser. By operator-normalizing the resulting time-of-arrival distribution, a distribution is obtained which for freely moving particles not only recovers the axiomatically derived distribution of Kijowski for states with purely positive momenta but is also applicable to general momentum components…
We discuss a method to select the velocities of ultra-cold atoms with a modified Fabry-Perot type of device made of two effective barriers and a well created, respectively, by blue and red detuned lasers. The laser parameters may be used to select the peak and width of the transmitted velocity window. In particular, lowering the central well provides a peak arbitrarily close to zero velocity having a minimum but finite width. The low-energy atomic scattering off this laser device is parameterized and approximate formulae are found to describe and explain its behaviour.
The nitrogen-vacancy (N-V) center in diamond is a widely-used platform for quantum information processing and metrology. The electron-spin state of N-V center could be initialized and readout optically, and manipulated by resonate microwave fields. In this work, we analyze the dependence of electron-spin initialization on widths of laser pulses. We build a numerical model to simulate this process and verify the simulation results in experiment. Both simulations and experiments reveal a fact that shorter laser pulses are helpful to the electron-spin polarization. We therefore propose to use ext…
We propose a laser cooling concept for the translational motion of molecules which does not require repeated spontaneous emission by each molecule. The cooling works by repetition of three main steps: velocity selection of a narrow momentum width, deceleration of velocity selected molecules and accumulation of the decelerated molecules by an irreversible process, namely by single spontaneous emission. We develop a cooling model which enables analytical description of the transient populations and entropies for the total molecular system, the center of mass degree of freedom and the internal de…
We have studied electromagnetically induced transparency (EIT) in diatomic cesium molecules in a vapor cell by using tunable diode lasers. We have observed a sub-natural Lambda-resonance in an absorption molecular band at different cesium vapor pressures. The width of the EIT resonance shows a linear dependence on cesium vapor pressure. Narrow Lambda-resonances in molecules can be used as frequency references for femtosecond laser frequency combs.
We report precision measurements of the excited state lifetime of the $5p$ $^2P_{1/2}$ and $5p$ $^2P_{3/2}$ levels of a single trapped Cd$^+$ ion. The ion is excited with picosecond laser pulses from a mode-locked laser and the distribution of arrival times of spontaneously emitted photons is recorded. The resulting lifetimes are 3.148 $\pm$ 0.011 ns and 2.647 $\pm$ 0.010 ns for $^2P_{1/2}$ and $^2P_{3/2}$ respectively. With a total uncertainty of under 0.4%, these are among the most precise measurements of any atomic state lifetimes to date.
In molecular photodissociation, some specific combinations of laser parameters (wavelength and intensity) lead to unexpected Zero-Width Resonances (ZWR), with in principle infinite lifetimes. Their interest in inducing basic quenching mechanisms have recently been devised in the laser control of vibrational cooling through filtration strategies [O. Atabek et al., Phys. Rev. A87, 031403(R) (2013)]. A full quantum adiabatic control theory based on the adiabatic Floquet Hamiltonian is developed to show how a laser pulse could be envelop-shaped and frequency-chirped so as to protect a given initia…
We demonstrate the fabrication of micron-wide tungsten silicide superconducting nanowire single-photon detectors on a silicon substrate using laser lithography. We show saturated internal detection efficiencies with wire widths from 0.59$μ$m to 1.43$μ$m under illumination at 1550nm. We demonstrate both straight wires, as well as meandered structures. Single-photon sensitivity is shown in devices up to 4mm in length. Laser-lithographically written devices allow for fast and easy structuring of large areas while maintaining a saturated internal efficiency for wire width around 1$μ$m.
A detailed rate-equation-based model is developed to study carrier transport effects on optical and electrical characteristics of the Multiple Quantum Well Heterojunction Bipolar Transistor Laser in time-domain. Simulation results extracted using numerical techniques in small-signal regime predict significant enhancement in device optical bandwidth when multiple quantum wells are used. Cavity length and base width are also modified to optimize the optoelectronic performances of the device. An optical bandwidth of \approx 60GHz is achieved in the case of 5 quantum wells each of 70A widths and a…
An analytical approach to quantum mechanical wave packet dynamics of laser-driven particles is presented. The time-dependent Schroedinger equation is solved for an electron exposed to a linearly polarized plane wave of arbitrary shape. The calculation goes beyond the dipole approximation, such that magnetic field effects like wave packet shearing are included. Analytical expressions for the time-dependent widths of the wave packet and its orientation are established. These allow for a simple understanding of the wave packet dynamics.
We present a scheme for robust and efficient projection measurement of a qubit consisting of the two magnetic sublevels in the electronic ground state of alkali earth metal ions. The scheme is based on two stimulated Raman adiabatic passages (STIRAP) involving four partially coherent laser fields. We show how the efficiency depends on experimentally relevant parameters: Rabi frequencies, pulse widths, laser linewidths, one- and two-photon detunings, residual laser power, laser polarization and ion motion.
We employ a quantum defect theory framework to provide a detailed analysis of the interplay between a magnetic Feshbach resonance and a shape resonance in cold collisions of ultracold $\rm ^{87}Rb$ atoms as captured in recent experiments using a laser-based collider [Phys. Rev. Research 3, 033209 (2021)]. By exerting control over a parameter space spanned by both collision energy and magnetic field, the width of a Feshbach resonance can be tuned over several orders of magnitude. We apply a quantum defect theory specialized for ultracold atomic collisions to fully describe of the experimental o…
A typical implementation of BB84 protocol for quantum communication uses four laser diodes for transmitting weak coherent pulses, which may not have the same characteristics. We have characterized these lasers for mismatch in various parameters such as spectral width, pulse width, spatial mode, peak wavelength, polarization and their arrival times at the receiver. This information is utilized to calculate possible information leakage through side channel attacks by evaluating mutual information between source and eavesdropper. Based on our experimental observations of cross correlation between…
Measurement-device-independent quantum key distribution (MDI-QKD) is immune to all security loopholes on detection. Previous experiments on MDI-QKD required spatially separated signal lasers and complicated stabilization systems. In this paper, we perform a proof-of-principle experimental demonstration of plug-and-play MDI-QKD over an asymmetric channel setting with a single signal laser, in which the whole system is automatically stabilized in spectrum, polarization, arrival time and phase reference. Both the signal laser and the single-photon detectors are in the possession of a common serve…
Three-photon laser excitation of Rydberg states by three different laser beams can be arranged in a star-like geometry that simultaneously eliminates the recoil effect and Doppler broadening. Our analytical and numerical calculations for a particular laser excitation scheme 5S_{1/2}->5P_{3/2}->6S_{1/2}->nP in Rb atoms have shown that compared to the one- and two-photon laser excitation this approach provides much narrower line width and longer coherence time for both cold atom samples and hot vapors, if the intermediate one-photon resonances of the three-photon transition are detuned by more t…
The first detection of a quantum particle on a graph has been shown to depend sensitively on the sampling time τ . Here we use the recently introduced quantum renewal equation to investigate the statistics of first detection on an infinite line, using a tight-binding lattice Hamiltonian with nearest- neighbor hops. Universal features of the first detection probability are uncovered and simple limiting cases are analyzed. These include the small τ limit and the power law decay with attempt number of the detection probability over which quantum oscillations are superimposed. When the sampling ti…
We theoretically study the focusing of a quasi-continuous atom laser beam of rubidium-85 ($^{85}$Rb). A two-sate model analysis based on the Gross-Pitaevskii equation is used which comprises the effects of two-body atom-atom interactions and three-body recombination losses. Utilizing optical focusing potentials such as harmonic potentials, the essential factors such as the width, peak density and atom loss rate of the focused atom laser beam profile are investigated. Our analysis predicts that using an atom laser offers a dramatic improvement in resolution of up to $8$ nm.
We use a probabilistic method to describe the effect of laser noise on the laser-atom interaction, in the case that the atom is a two level system without spontaneous emission. The stochastic differential equation for the laser-atom interaction is analyzed in the sense of perturbation approach, and we construct a stochastic process corresponding to the time evolution of the atom's wave function, whose extra randomness is induced by the laser noise. It also provides the layout of a theory for the possible experiment of measuring the laser line width by driving a narrow atomic transition.
Some optical experiments provide the easiest way to test quantum mechanical predictions. Such a situation applies to a laser beam traversing a dielectric structure. The dielectric structure mir- roring quantum mechanical potentials. The simplest of these, studied in this paper, involves a single dielectric block. We exhibit both by analytic and numerical calculations explicit examples of total coherence and total incoherence phenomena. Which case appears depends upon the angle of incidence of the laser beam and/or the dimensions of beam vs block width. Unlike our previ- ous studies our calcula…
