We report precision measurements of the excited state lifetime of the $5p$ $^2P_{1/2}$ and $5p$ $^2P_{3/2}$ levels of a single trapped Cd$^+$ ion. The ion is excited with picosecond laser pulses from a mode-locked laser and the distribution of arrival times of spontaneously emitted photons is recorded. The resulting lifetimes are 3.148 $\pm$ 0.011 ns and 2.647 $\pm$ 0.010 ns for $^2P_{1/2}$ and $^2P_{3/2}$ respectively. With a total uncertainty of under 0.4%, these are among the most precise measurements of any atomic state lifetimes to date.
We demonstrate broadband laser cooling of atomic ions in an rf trap using ultrafast pulses from a modelocked laser. The temperature of a single ion is measured by observing the size of a time-averaged image of the ion in the known harmonic trap potential. While the lowest observed temperature was only about 1 K, this method efficiently cools very hot atoms and can sufficiently localize trapped atoms to produce near diffraction-limited atomic images.
We demonstrate ultrafast coherent coupling between an atomic qubit stored in a single trapped cadmium ion and a photonic qubit represented by two resolved frequencies of a photon. Such ultrafast coupling is crucial for entangling networks of remotely-located trapped ions through photon interference, and is also a key component for realizing ultrafast quantum gates between Coulomb-coupled ions.
We study a hybrid quantum system composed of an ion and an electric dipole. We show how a trapped ion can be used to measure the small electric field generated by a classical dipole. We discuss the application of this scheme to measure the electric dipole moment of cold polar molecules, whose internal state can be controlled with ultrafast laser pulses, by trapping them in the vicinity of a trapped ion.
Atomic cadmium ions are loaded into radiofrequency ion traps by photoionization of atoms in a cadmium vapor with ultrafast laser pulses. The photoionization is driven through an intermediate atomic resonance with a frequency-quadrupled mode-locked Ti:Sapphire laser that produces pulses of either 100 fsec or 1 psec duration at a central wavelength of 229 nm. The large bandwidth of the pulses photoionizes all velocity classes of the Cd vapor, resulting in high loading efficiencies compared to previous ion trap loading techniques. Measured loading rates are compared with a simple theoretical mode…
We sense the motion of a trapped atomic ion using a sequence of state-dependent ultrafast momentum kicks. We use this atom interferometer to characterize a nearly-pure quantum state with $n=1$ phonon and accurately measure thermal states ranging from near the zero-point energy to $\bar{n}\sim 10^4$, with the possibility of extending at least 100 times higher in energy. The complete energy range of this method spans from the ground state to far outside of the Lamb-Dicke regime, where atomic motion is greater than the optical wavelength. Apart from thermometry, these interferometric techniques a…
This paper reports on photoionisation loading based on ultrafast pulses of singly-ionised strontium ions in a linear Paul trap. We take advantage of an autoionising resonance of Sr neutral atoms to form Sr+ by two-photon absorption of femtosecond pulses at a wavelength of 431nm. We compare this technique to electron-bombardment ionisation and observe several advantages of photoionisation. It actually allows the loading of a pure Sr+ ion cloud in a low radio-frequency voltage amplitude regime. In these conditions up to 4x10^4 laser-cooled Sr+ ions were trapped.
We study the lifetime of an atom trapped in an optical vertical lattice in proximity of a massive surface using a complex scaling approach. We analyze how the presence of the surface modifies the known lifetimes of Wannier-Stark states associated to Landau-Zener tunnelling. We also investigate how the existence of a hypothetical short-distance deviation from Newton's gravitational law could affect these lifetimes. Our study is relevant in order to discuss the feasibility of any atomic- interferometry experiment performed near a surface. Finally, the difficulties encountered in applying the com…
We propose a method to investigate the vibrational dynamics of single polyatomic molecular ions confined in a Paul trap. Quantum logic techniques are employed to detect the recoil of single photon absorption events in the molecule via a co-trapped atomic ion. In particular, the recoil is mapped onto the electronic state of the atom which can be read out with high fidelity. This recoil detection serves as the basis for a pump-probe scheme to investigate ultrafast molecular dynamics, such as intra-molecular vibrational redistribution. The total recoil from the interaction with a sequence of ultr…
Experimental realizations of two qubit entangling gates with trapped ions typically rely on addressing spectroscopically resolved motional sidebands, limiting gate speed to the secular frequency. Fast entangling gates using ultrafast pulsed lasers overcome this speed limit. This approach is based on state-dependent photon recoil kicks from a sequence of counter-propagating, resonant, ultrafast pulse pairs, which can allow sub-microsecond gate speeds. Here we demonstrate a key component of the ultrafast gate protocol, the coherent excitation of a 171Yb+ ion across the 2S1/2-2P1/2 transition wit…
We study the electromagnetic coupling and concomitant heating of a particle in a miniaturized trap close to a solid surface. Two dominant heating mechanisms are identified: proximity fields generated by thermally excited currents in the absorbing solid and time-dependent image potentials due to elastic surface distortions (Rayleigh phonons). Estimates for the lifetime of the trap ground state are given. Ions are particularly sensitive to electric proximity fields: for a silver substrate, we find a lifetime below one second at distances closer than some ten micrometer to the surface. Neutral at…
Trapped ions are a well-studied and promising system for the realization of a scalable quantum computer. Faster quantum gates would greatly improve the applicability of such a system and allow for greater flexibility in the number of calculation steps. In this paper we present a pulsed laser system, delivering picosecond pulses at a repetition rate of 5 GHz and resonant to the S$_{1/2}$ to P$_{3/2}$ transition in Ca$^+$ for coherent population transfer to implement fast phase gate operations. The optical pulse train is derived from a mode-locked, stabilized optical frequency comb and inherits …
We demonstrate single qubit operations on a trapped atom hyperfine qubit using a single ultrafast pulse from a mode-locked laser. We shape the pulse from the laser and perform a pi rotation of the qubit in less than 50 ps with a population transfer exceeding 99% and negligible effects from spontaneous emission or ac Stark shifts. The gate time is significantly shorter than the period of atomic motion in the trap (Rabi frequency / trap frequency > 10000), demonstrating that this interaction takes place deep within the strong excitation regime.
Amplitude noise which inflicts a random two qubit term is one of the main obstacles preventing the implementation of a high fidelity two-body gate below the fault tolerance threshold. This noise is difficult to refocus as any refocusing technique could only tackle noise with frequency below the operation rate. Since the two qubit gate speed is normally the slowest rate in the system, it constitutes the last bottleneck towards an implementation of a gate below the fault tolerant threshold. Here we propose to use composite pulses as a dynamical decoupling approach, in order to reduce two qubit g…
Neutral atom qubits with Rydberg-mediated interactions are a leading platform for developing large-scale coherent quantum systems. In the majority of experiments to date, the Rydberg states are not trapped by the same potential that confines ground state atoms, resulting in atom loss and constraints on the achievable interaction time. In this work, we demonstrate that the Rydberg states of an alkaline earth atom, ytterbium, can be stably trapped by the same red-detuned optical tweezer that also confines the ground state, by leveraging the polarizability of the Yb$^+$ ion core. Using the previo…
Qubit state detection is an important part of a quantum computation. As number of qubits in a quantum register increases, it is necessary to maintain high fidelity detection to accurately measure the multi-qubit state. Here we present experimental demonstration of high-fidelity detection of a multi-qubit trapped ion register with average single qubit detection error of 4.2(1.5) ppm and a 4-qubit state detection error of 17(2) ppm, limited by the decay lifetime of the qubit, using a novel single-photon-sensitive camera with fast data collection, excellent temporal and spatial resolution, and lo…
We demonstrate quantum entanglement of two trapped atomic ion qubits using a sequence of ultrafast laser pulses. Unlike previous demonstrations of entanglement mediated by the Coulomb interaction, this scheme does not require confinement to the Lamb-Dicke regime and can be less sensitive to ambient noise due to its speed. To elucidate the physics of an ultrafast phase gate, we generate a high entanglement rate using just 10 pulses, each of $\sim20$ ps duration, and demonstrate an entangled Bell-state with $(76\pm1)$% fidelity. These results pave the way for entanglement operations within a lar…
Purcell effect predicts that spontaneous radiation is not an intrinsic property of matter, but is affected by the environment in which it is located, and is the result of the interaction of matter and field. Purcell effect can be inferred from Fermi Gold rule through strict quantum electrodynamics (QED), and through it can achieve the enhancement or suppression of radiation. We suggest that, in principle, the Purcell effect can be detected at the percentage level of neutron decay in experiments with trapped ultra-cold neutrons. As a test of our claim, we propose a currently achievable experime…
We present a precise measurement of the lifetime of the 6p 2P_1/2 excited state of a single trapped ytterbium ion (Yb+). A time-correlated single-photon counting technique is used, where ultrafast pulses excite the ion and the emitted photons are coupled into a single-mode optical fiber. By performing the measurement on a single atom with fast excitation and excellent spatial filtering, we are able to eliminate common systematics. The lifetime of the 6p 2P_1/2 state is measured to be 8.12 +/- 0.02 ns.
Using a consistent quantum-mechanical treatment for the electromagnetic radiation, we theoretically investigate the magnetic spin-flip scatterings of a neutral two-level atom trapped in the vicinity of a superconducting body. We derive a simple scaling law for the corresponding spin-flip lifetime for such an atom trapped near a superconducting thick slab. For temperatures below the superconducting transition temperature T_c, the lifetime is found to be enhanced by several orders of magnitude in comparison to the case of a normal conducting slab. At zero temperature the spin-flip lifetime is gi…
We propose a long-lived and rapidly accessible quantum memory unit, for which the operational Hilbert space is spanned by states involving the two macroscopically occupied hyperfine levels of a miscible binary atomic Bose-Einstein condensate and the Rydberg state of a single atom. It is shown that an arbitrary qubit state, initially prepared using a flux qubit, can be rapidly transferred to and from the trapped atomic ensemble in approximately 10 ns and with a large fidelity of 97%, via an effective two-photon process using an external laser for the transition to the Rydberg level. The achieva…
Recent advances in attosecond physics provide access to the correlated motion of valence and core electrons on their intrinsic timescales. For valence excitations, processes related to the electron spin are usually driven by nuclear motion. For core-excited states, where the core hole has a nonzero angular momentum, spin-orbit coupling is strong enough to drive spin-flips on a much shorter time scale. Here, unprecedented short spin-crossover driven by spin-orbit coupling is demonstrated for L-edge (2p$\rightarrow$3d) excited states of a prototypical Fe(II) complex. It occurs on a time scale, w…
Pulsed lasers offer significant advantages over CW lasers in the coherent control of qubits. Here we review the theoretical and experimental aspects of controlling the internal and external states of individual trapped atoms with pulse trains. Two distinct regimes of laser intensity are identified. When the pulses are sufficiently weak that the Rabi frequency $Ω$ is much smaller than the trap frequency $\otrap$, sideband transitions can be addressed and atom-atom entanglement can be accomplished in much the same way as with CW lasers. By contrast, if the pulses are very strong ($Ω\gg \otrap$),…
We experimentally study the real-time susceptibility of trapped-ion quantum systems to small doses of ionizing radiation. We expose an ion-trap apparatus to a variety of $α$, $β$, and $γ$ sources and measure the resulting changes in trapped-ion qubit lifetimes, coherence times, gate fidelities, and motional heating rates. We found no quantifiable degradation of ion trap performance in the presence of low-dose radiation sources for any of the measurements performed. This finding is encouraging for the long-term prospects of using ion-based quantum information systems in extreme environments, in…
Ultrafast emission rates obtained from quantum emitters coupled to plasmonic nanoantennas have recently opened fundamentally new possibilities in quantum information and sensing applications. Plasmonic nanoantennas greatly improve the brightness of quantum emitters by dramatically shortening their fluorescence lifetimes. Gap plasmonic nanocavities that support strongly confined modes are of particular interest for such applications. We demonstrate single-photon emission from nitrogen-vacancy (NV) centers in nanodiamonds coupled to nanosized gap plasmonic cavities with internal mode volumes abo…
The requirement for optical-electrical-optical conversion of signals in optical technologies is often one of the majors bottleneck in terms of speed and energy consumption. The use of dressed photons (also called polaritons), that allows for intrinsic sizable interactions, could significantly improve the performances of optical integrated elements such as switches or optical gates. In this work we demonstrate the ultrafast switch of a laser coupled into a polaritonic waveguide triggered by an optical pulse resonant with the same dispersion but at a lower energy. Our experiments show two effect…
Viscosity is an important property of out-of-equilibrium systems such as active biological materials and driven non-Newtonian fluids, and for fields ranging from biomaterials to geology, energy technologies and medicine. However, noninvasive viscosity measurements typically require integration times of seconds. Here we demonstrate a four orders-of-magnitude improvement in speed, down to twenty microseconds, with uncertainty dominated by fundamental thermal noise for the first time. We achieve this using the instantaneous velocity of a trapped particle in an optical tweezer. To resolve the inst…
