We demonstrate broadband laser cooling of atomic ions in an rf trap using ultrafast pulses from a modelocked laser. The temperature of a single ion is measured by observing the size of a time-averaged image of the ion in the known harmonic trap potential. While the lowest observed temperature was only about 1 K, this method efficiently cools very hot atoms and can sufficiently localize trapped atoms to produce near diffraction-limited atomic images.
We demonstrate ultrafast coherent coupling between an atomic qubit stored in a single trapped cadmium ion and a photonic qubit represented by two resolved frequencies of a photon. Such ultrafast coupling is crucial for entangling networks of remotely-located trapped ions through photon interference, and is also a key component for realizing ultrafast quantum gates between Coulomb-coupled ions.
We report precision measurements of the excited state lifetime of the $5p$ $^2P_{1/2}$ and $5p$ $^2P_{3/2}$ levels of a single trapped Cd$^+$ ion. The ion is excited with picosecond laser pulses from a mode-locked laser and the distribution of arrival times of spontaneously emitted photons is recorded. The resulting lifetimes are 3.148 $\pm$ 0.011 ns and 2.647 $\pm$ 0.010 ns for $^2P_{1/2}$ and $^2P_{3/2}$ respectively. With a total uncertainty of under 0.4%, these are among the most precise measurements of any atomic state lifetimes to date.
We study a hybrid quantum system composed of an ion and an electric dipole. We show how a trapped ion can be used to measure the small electric field generated by a classical dipole. We discuss the application of this scheme to measure the electric dipole moment of cold polar molecules, whose internal state can be controlled with ultrafast laser pulses, by trapping them in the vicinity of a trapped ion.
We introduce the concept of a quantum pulse gate (QPG), a method for accessing the intrinsic broadband spectral mode structure of ultrafast quantum states of light. This mode structure can now be harnessed for applications in quantum information processing. We propose an implementation in a PPLN waveguide, based on spectrally engineered sum frequency generation (SFG). It allows us to pick well-defined spectral broadband modes from an ultrafast multi-mode state for interconversion to a broadband mode at another frequency. By pulse-shaping the bright SFG pump beam, different orthogonal broadband…
Atomic cadmium ions are loaded into radiofrequency ion traps by photoionization of atoms in a cadmium vapor with ultrafast laser pulses. The photoionization is driven through an intermediate atomic resonance with a frequency-quadrupled mode-locked Ti:Sapphire laser that produces pulses of either 100 fsec or 1 psec duration at a central wavelength of 229 nm. The large bandwidth of the pulses photoionizes all velocity classes of the Cd vapor, resulting in high loading efficiencies compared to previous ion trap loading techniques. Measured loading rates are compared with a simple theoretical mode…
We observe at record-high speed the nonclassical nature of ultra-broadband bi-photons, reducing the measurement time by four orders of magnitude compared to standard techniques of Hong-Ou-Mandel interference or sum-frequency generation. We measure the quantum state of the broadband bi-photons, amplitude and phase, with a pairwise "Mach-Zehnder" quantum interferometer, where bi-photons that are generated in one nonlinear crystal are enhanced (constructive interference) or diminished (destructive interference) in another crystal, depending on the bi-photon phase. We verify the quantum nature of …
We report a conceptually straightforward witness that isolates coherent electronic oscillations from their vibronic counterparts in nonlinear optical spectra of molecular aggregates: Coherent oscillations as a function of waiting time in broadband pump/broadband probe spectra correspond to coherent electronic oscillations. Oscillations in individual peaks of 2D electronic spectra do not necessarily yield this conclusion. Our witness is simpler to implement than quantum process tomography and potentially resolves a long-standing controversy on the character of oscillations in ultrafast spectra …
The absorption of a single photon that excites a quantum system from a low to a high energy level is an elementary process of light-matter interaction, and a route towards realizing pure single-photon absorption has both fundamental and practical implications in quantum technology. Due to nonlinear optical effects, however, the probability of pure single-photon absorption is usually very low, which is particularly pertinent in the case of strong ultrafast laser pulses with broad bandwidth. Here we demonstrate theoretically a counterintuitive coherent single-photon absorption scheme by eliminat…
We propose and experimentally demonstrate a scheme to generate optically-controlled delays based on off-resonant Raman absorption. Dispersion in a transparency window between two neighboring, optically-activated Raman absorption lines is used to reduce the group velocity of broadband 765 nm pulses. We implement this approach in a potassium titanyl phosphate (KTP) waveguide at room temperature, and demonstrate Raman-induced delays of up to 140 fs for a 650-fs duration, 1.8-THz bandwidth, signal pulse; the available delay-bandwidth product is $\approx1$. Our approach is applicable to single phot…
The advent of dispersion-engineered and highly nonlinear nanophotonics is expected to open up an all-optical path towards the strong-interaction regime of quantum optics by combining high transverse field confinement with ultra-short-pulse operation. Obtaining a full understanding of photon dynamics in such broadband devices, however, poses major challenges in the modeling and simulation of multimode non-Gaussian quantum physics, highlighting the need for sophisticated reduced models that facilitate efficient numerical study while providing useful physical insight. In this manuscript, we revie…
We sense the motion of a trapped atomic ion using a sequence of state-dependent ultrafast momentum kicks. We use this atom interferometer to characterize a nearly-pure quantum state with $n=1$ phonon and accurately measure thermal states ranging from near the zero-point energy to $\bar{n}\sim 10^4$, with the possibility of extending at least 100 times higher in energy. The complete energy range of this method spans from the ground state to far outside of the Lamb-Dicke regime, where atomic motion is greater than the optical wavelength. Apart from thermometry, these interferometric techniques a…
This paper reports on photoionisation loading based on ultrafast pulses of singly-ionised strontium ions in a linear Paul trap. We take advantage of an autoionising resonance of Sr neutral atoms to form Sr+ by two-photon absorption of femtosecond pulses at a wavelength of 431nm. We compare this technique to electron-bombardment ionisation and observe several advantages of photoionisation. It actually allows the loading of a pure Sr+ ion cloud in a low radio-frequency voltage amplitude regime. In these conditions up to 4x10^4 laser-cooled Sr+ ions were trapped.
We investigate the cavity excitation spectrum and the photon number distribution in a cavity QED system driven by a broadband squeezed vacuum. In an empty cavity, we show that only states with even number of photons can be measured under resonant condition since the squeezed vacuum consists of states with even number of photons only. When a single atom is trapped in the cavity, the strong coupling between the atom and cavity results in energy splittings of the system, and there exist two peaks in the cavity excitation spectrum at two-photon transition frequencies. At the central frequency, how…
The ability to control spins in semiconductors is important in a variety of fields including spintronics and quantum information processing. Due to the potentially fast dephasing times of spins in the solid state [1-3], spin control operating on the picosecond or faster timescale may be necessary. Such speeds, which are not possible to attain with standard electron spin resonance (ESR) techniques based on microwave sources, can be attained with broadband optical pulses. One promising ultrafast technique utilizes single broadband pulses detuned from resonance in a three-level Lambda system [4].…
Experimental realizations of two qubit entangling gates with trapped ions typically rely on addressing spectroscopically resolved motional sidebands, limiting gate speed to the secular frequency. Fast entangling gates using ultrafast pulsed lasers overcome this speed limit. This approach is based on state-dependent photon recoil kicks from a sequence of counter-propagating, resonant, ultrafast pulse pairs, which can allow sub-microsecond gate speeds. Here we demonstrate a key component of the ultrafast gate protocol, the coherent excitation of a 171Yb+ ion across the 2S1/2-2P1/2 transition wit…
Quantum systems with sublevel structures prevent full population inversion from one manifold of sublevels to the other using strong ultrafast resonant pulses. In this work we explain the mechanism by which this population transfer is blocked. We then develop a novel concept of geometric control, assuming full or partial coherent manipulation within the manifolds and show that by preparing specific coherent superpositions in the initial manifold, full population inversion or full population blockade, {\it i.e} laser-induced transparency, can be achieved. In particular, by parallel population tr…
We present an efficient scheme for the controlled generation of pure two-qubit states possessing {\em any} desired degree of entanglement and a {\em prescribed} symmetry in two cavity QED based systems, namely, cold trapped ions and flying atoms. This is achieved via on-resonance ion/atom-cavity couplings which are time-dependent and asymmetric, leading to a trapping vacuum state condition which does not arise for identical couplings. A duality in the role of the coupling ratio yields states with a given concurrence but opposing symmetries. The experimental feasibility of the proposed scheme i…
Trapped ions are a well-studied and promising system for the realization of a scalable quantum computer. Faster quantum gates would greatly improve the applicability of such a system and allow for greater flexibility in the number of calculation steps. In this paper we present a pulsed laser system, delivering picosecond pulses at a repetition rate of 5 GHz and resonant to the S$_{1/2}$ to P$_{3/2}$ transition in Ca$^+$ for coherent population transfer to implement fast phase gate operations. The optical pulse train is derived from a mode-locked, stabilized optical frequency comb and inherits …
The absorption of broadband photons in atomic ensembles requires either an effective broadening of the atomic transition linewidth, or an off-resonance Raman interaction. Here we propose a scheme for a quantum memory capable of storing and retrieving ultrafast photons in an ensemble of two-level atoms by using a propagation medium with a time-dependent refractive index generated from aligning an ensemble of gas-phase diatomic molecules. The refractive index dynamics generates an effective longitudinal inhomogeneous broadening of the two-level transition. We numerically demonstrate this scheme …
We demonstrate single qubit operations on a trapped atom hyperfine qubit using a single ultrafast pulse from a mode-locked laser. We shape the pulse from the laser and perform a pi rotation of the qubit in less than 50 ps with a population transfer exceeding 99% and negligible effects from spontaneous emission or ac Stark shifts. The gate time is significantly shorter than the period of atomic motion in the trap (Rabi frequency / trap frequency > 10000), demonstrating that this interaction takes place deep within the strong excitation regime.
Amplitude noise which inflicts a random two qubit term is one of the main obstacles preventing the implementation of a high fidelity two-body gate below the fault tolerance threshold. This noise is difficult to refocus as any refocusing technique could only tackle noise with frequency below the operation rate. Since the two qubit gate speed is normally the slowest rate in the system, it constitutes the last bottleneck towards an implementation of a gate below the fault tolerant threshold. Here we propose to use composite pulses as a dynamical decoupling approach, in order to reduce two qubit g…
We demonstrate quantum entanglement of two trapped atomic ion qubits using a sequence of ultrafast laser pulses. Unlike previous demonstrations of entanglement mediated by the Coulomb interaction, this scheme does not require confinement to the Lamb-Dicke regime and can be less sensitive to ambient noise due to its speed. To elucidate the physics of an ultrafast phase gate, we generate a high entanglement rate using just 10 pulses, each of $\sim20$ ps duration, and demonstrate an entangled Bell-state with $(76\pm1)$% fidelity. These results pave the way for entanglement operations within a lar…
We measure the sensitivity of a broadband atomic magnetometer using quantum non-demolition spin measurements. A cold, dipole-trapped sample of rubidium atoms provides a long-lived spin system in a non-magnetic environment, and is probed non-destructively by paramagnetic Faraday rotation. The calibration procedure employs a known reference state, the maximum-entropy or 'thermal' spin state and quantitative imaging-based atom counting to identify electronic, quantum, and technical noise in both the probe and spin system. The measurement achieves sensitivity 2.8 dB better than the projection nois…
Mesoscopic quantum superpositions, or Schrödinger cat states, are widely studied for fundamental investigations of quantum measurement and decoherence as well as applications in sensing and quantum information science. The generation and maintenance of such states relies upon a balance between efficient external coherent control of the system and sufficient isolation from the environment. Here we create a variety of cat states of a single trapped atom's motion in a harmonic oscillator using ultrafast laser pulses. These pulses produce high fidelity impulsive forces that separate the atom into …
Motion of an atomic ensemble trapped into a deep optical lattice is considered. We propose a novel approach to construct an atomic ratchet by superimposing two additional lattices whose amplitudes are small and subjected to broadband modulation. The broadband modulation is modeled by means of harmonic noise. Directed atomic transport occurs with the properly chosen phase shift between the signals modulating the amplitudes of the additional lattices. It is shown that efficiency of the ratchet depends non-monotonously on the parameter determining the spectral width of modulating signals.
We propose a long-lived and rapidly accessible quantum memory unit, for which the operational Hilbert space is spanned by states involving the two macroscopically occupied hyperfine levels of a miscible binary atomic Bose-Einstein condensate and the Rydberg state of a single atom. It is shown that an arbitrary qubit state, initially prepared using a flux qubit, can be rapidly transferred to and from the trapped atomic ensemble in approximately 10 ns and with a large fidelity of 97%, via an effective two-photon process using an external laser for the transition to the Rydberg level. The achieva…
Pulsed lasers offer significant advantages over CW lasers in the coherent control of qubits. Here we review the theoretical and experimental aspects of controlling the internal and external states of individual trapped atoms with pulse trains. Two distinct regimes of laser intensity are identified. When the pulses are sufficiently weak that the Rabi frequency $Ω$ is much smaller than the trap frequency $\otrap$, sideband transitions can be addressed and atom-atom entanglement can be accomplished in much the same way as with CW lasers. By contrast, if the pulses are very strong ($Ω\gg \otrap$),…
