We have studied electromagnetically induced transparency (EIT) in diatomic cesium molecules in a vapor cell by using tunable diode lasers. We have observed a sub-natural Lambda-resonance in an absorption molecular band at different cesium vapor pressures. The width of the EIT resonance shows a linear dependence on cesium vapor pressure. Narrow Lambda-resonances in molecules can be used as frequency references for femtosecond laser frequency combs.
We report on the observation of enhanced four-wave mixing via crossover resonance in a Doppler broadened cesium vapor. Using a single laser frequency, a resonant parametric process in a double-$Λ$ level configuration is directly excited for a specific velocity class. We investigate this process in different saturation regimes and demonstrate the possibility of generating intensity correlation and anti-correlation between the probe and conjugate beams. A simple theoretical model is developed that accounts qualitatively well to the observed results.
Using a nondegenerate four-wave mixing process based on a double-$Λ$ scheme in hot cesium vapor, we generate quantum correlated twin beams with a maximum intensity-difference squeezing of 6.5 dB. The substantially improved squeezing can be mainly attributed to very good frequency and phase-difference stability between the pump and probe beams in our experiment. Intensity-difference squeezing can be observed within a wide experimental parameter range, which guarantees its robust generation. Since this scheme produces multi-spatial-mode twin beams at the Cs $D_{1}$ line, it is of interest for ex…
Slow light of an amplitude modulated Gaussian (AMG) pulse in cesium vapor is demonstrated and studied, as an appropriate amplitude modulation to a single pulse can expand its spectrum and thus increase the utilization efficiency of the bandwidth of a slow light system. In a single-$Λ$ type electromagnetically induced transparency (EIT) system, the slowed AMG pulse experiences severe distortion, mainly owing to the frequency dependent transmission of medium. Additionally, due to its spectral distribution, the frequency dependent dispersion of the medium causes simultaneous slow and fast light o…
The ability to store large amounts of photonic quantum states is regarded as substantial for future optical quantum computation and communication technologies. However, research for multiplexed quantum memories has been focused on systems that show good performance only after an elaborate preparation of the storage media. This makes it generally more difficult to apply outside a laboratory environment. In this work, we demonstrate a multiplexed random-access memory to store up to four optical pulses using electromagnetically induced transparency in warm cesium vapor. Using a Λ-System on the hy…
Quantum-enhanced measurements represent the path towards the best measurement precision allowed by the laws of quantum mechanics. Known protocols usually rely on the preparation of entangled states and promise high or even optimal precision, but fall short in real-word applications because of the difficulty to generate entangled states and to protect them against decoherence. Here, we refrain from the preparation of entangled states but supplement the integrable parameter-encoding dynamics by non-linear kicks driving the system in the dynamical regime of quantum chaos. We show that large impro…
Using a nondegenerate four-wave mixing (FWM) process based on a double-Λ scheme in hot cesium vapor, we demonstrate a compact diode-laser-pumped quantum light source for the generation of quantum correlated twin beams with a maximum squeezing of 6.5 dB. The squeezing is observed at a Fourier frequency in the audio band down to 0.7 kHz which, to the best of our knowledge, is the first observation of sub-kilohertz intensity-difference squeezing in an atomic system so far. A phase-matching condition is also investigated in our system, which confirms the spatial-multi-mode characteristics of the F…
Single photons from solid-state quantum emitters are playing a crucial role in the development of photonic quantum technologies. Higher order states, such as N-photon Fock-states allow for applications e.g. in quantum-enhanced sensing. In this study, we utilize the dispersion of a hot cesium vapor at the D1 lines to realize a temporal delay for one and two-photon Fock-states as a result of the slow-light effect. Single photons are generated on-demand from an InGaAs quantum dot, while their quantum interference at a beam splitter is used to generate a two-photon Fockstate. We verify the success…
We report on the storage of light via the phenomenon of Coherent Population Oscillation (CPO) in an atomic cesium vapor at room temperature. In the experiment the optical information of a probe field is stored in the CPO of two ground states of a Lambda three-level system formed by the Zeeman sublevels of the hyperfine transition F = 3 - F' = 2 of cesium D2 line. We show directly that this CPO based memory is very insensitive to stray magnetic field inhomogeneities and presents a lifetime which is mainly limited only by atomic motion. A theoretical simulation of the measured spectra was also d…
We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S1/2 ground state to nP3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet (UV) laser,and Rydberg excitation spectra are obtained by transmission enhancement of a probe beam resonant to Cs 6S1/2, F = 4 - 6P3/2, F' = 5 transition as partial population on F = 4 ground state are transferred to Rydberg state .Analysis reveals that the observed spectra are velocity-selective spectroscopy of Rydberg state, from which the amplitude and lin…
Thanks to the atomic coherence in coupling laser driven atomic system, sub-Doppler absorption has been observed in Doppler-broadened cesium vapor cell via the /Lambda-type three-level scheme. The linewidth of the sub-Doppler absorption peak become narrower while the frequency detuning of coupling laser increases. The results are in agreement with the theoretical prediction by G. Vemuri et al.[PRA,Vol.53(1996) p.2842].
We have developed a torsion balance to detect the rotation of a cell containing spin-polarized gaseous atoms to study angular momentum transfer from gaseous atoms to solid. A cesium vapor cell was hung from a thin wire in a vacuum chamber, and irradiated from the bottom with circularly polarized light tuned to the $D_2$ transition to polarize cesium atoms in the cell. By varying the light helicity at the resonance frequency of the torsion balance, we induced forced rotational oscillation of the cell and detected radiation torque exerted on the cesium vapor cell through the cesium atoms inside.…
Ultralow-power diode-laser radiation is employed to induce photodesorption of cesium from a partially transparent thin-film cesium adsorbate on a solid surface. Using resonant Raman spectroscopy, we demonstrate that this photodesorption process enables an accurate local optical control of the density of dimer molecules in alkali-metal vapors.
We study the excitation redistribution from cesium $7\mathrm{P}_{1/2}$ or $7\mathrm{P}_{3/2}$ to neighboring energy levels by Black Body Radiation (BBR) and inter atomic collisions using pump-probe spectroscopy inside a vapor cell. At low vapor densities we measure redistribution of the initial, velocity-selected, atomic excitation by BBR. This preserves the selected atomic velocities allowing us to perform high resolution spectroscopy of the $\mathrm{6D\rightarrow 7F}$ transitions. This transfer mechanism could also be used to perform sub-Doppler spectroscopy of the cesium highly-excited $\ma…
The measurement of Cesium (Cs) 7D5/2 excited state's hyperfine splitting intervals and hyperfine-interaction constants has been experimentally investigated based on ladder-type (852 nm + 698 nm) three-level Cs system (6S1/2 - 6P3/2 - 7D5/2) with room-temperature Cs atomic vapor cell. By scanning the 698-nm coupling laser's frequency, the Doppler-free high-resolution electromagnetically-induced transparency (EIT) assisted double-resonance optical pumping (DROP) spectra have been demonstrated via transmission enhancement of the locked 852-nm probe laser. The EIT-assisted DROP spectra are employe…
We have experimentally observed switching between photon-photon correlations (bunching) and anti-correlations (anti-bunching) between two orthogonally polarized laser beams in an EIT configuration in Rb vapor. The bunching and anti-bunching sswitching occurs at a specific magnetic field strength.
We report slowed propagation and storage and retrieval of thermal light in warm rubidium vapor using the effect of electromagnetically-induced transparency (EIT). We first demonstrate slowed-propagation of the probe thermal light beam through an EIT medium by measuring the second-order correlation function of the light field using the Hanbury-Brown$-$Twiss interferometer. We also report an experimental study on the effect of the EIT slow-light medium on the temporal coherence of thermal light. Finally, we demonstrate the storage and retrieval of thermal light beam in the EIT medium. The direct…
Electromagnetically induced transparency (EIT) is observed in gaseous 4He at room temperature. Ultra-narrow (less than 10 kHz) EIT windows are obtained for the first time for purely electronic spins in the presence of Doppler broadening. The positive role of collisions is emphasized through measurements of the power dependence of the EIT resonance. Measurement of slow light opens up possible ways to applications.
We observed squeezed vacuum light at 795 nm in 87Rb vapor via resonant polarization self-rotation, and report noise sidebands suppression of ~1 dB below shot noise level spanning from acoustic (30 kHz) to MHz frequencies. This is the first demonstration of sub-MHz quadrature vacuum squeezing in atomic systems. The spectral range of observed squeezing matches well typical bandwidths of electromagnetically induced transparency (EIT) resonances, making this simple technique for generation of optical fields with non-classical statistics at atomic transitions wavelengths attractive for EIT-based qu…
We present preliminary results from an experimental study of slow light in anti-relaxation-coated Rb vapor cells, and describe the construction and testing of such cells. The slow ground state decoherence rate allowed by coated cell walls leads to a dual-structured electromagnetically induced transparency (EIT) spectrum with a very narrow (<100 Hz) transparency peak on top of a broad pedestal. Such dual-structure EIT permits optical probe pulses to propagate with greatly reduced group velocity on two time scales. We discuss ongoing efforts to optimize the pulse delay in such coated cell system…
We report characterization of electromagnetically induced transparency (EIT) resonances in the D1 line of Rb-87 under various experimental conditions. The dependence of the EIT linewidth on the power of the pump field was investigated, at various temperatures, for the ground states of the lambda-system associated with different hyperfine levels of the atomic 5S_1/2 state as well as magnetic sublevels of the same hyperfine level. Strictly linear behavior was observed in all cases. A theoretical analysis of our results shows that dephasing in the ground state is the main source of decoherence, w…
We have observed CW lasing without inversion in a gas of hot rubidium atoms in an optical cavity under conditions of electromagnetically-induced transparency (EIT). The medium is pumped coherently and resonantly by a single ``coupling'' beam which also produces EIT in the lasing transition. The steady-state intensity exhibits thresholds as a function of the atomic density and the strength of the coupling beam. A theoretical model for an effective three-level lambda system indicates that gain without inversion is possible in this system if the two ground states are coupled by depolarizing colli…
We systematically studied the temporal profile of biphotons, i.e., pairs of time-correlated single photons, generated from a hot atomic vapor via the spontaneous four-wave mixing process. The measured temporal width of biphoton wave packet or two-photon correlation function against the coupling power was varied from about 70 to 580 ns. We derived an analytical expression of the biphoton's spectral profile in the Doppler-broadened medium. The analytical expression reveals that the spectral profile is mainly determined by the effect of electromagnetically induced transparency (EIT), and behaves …
We observe transformation of the electromagnetically induced transparency (EIT) resonance into the absorption resonance in a $Λ$ interaction configuration in a cell filled with $^{87}$Rb and a buffer gas. This transformation occurs as a one-photon detuning of the coupling fields is varied from the atomic transition. No such absorption resonance is found in the absence of a buffer gas. The width of the absorption resonance is several times smaller than the width of the EIT resonance, and the changes of absorption near these resonances are about the same. Similar absorption resonances are detect…
We provide an exact analytic description of decelerating, stopping and re-accelerating optical solitons in atomic media. By virtue of this solution we describe in detail how spatially localized optical memory bits can be written down, read and moved along the atomic medium in a prescribed manner. Dynamical control over the solitons is realized via a background laser field whose intensity controls the velocity of the slow light in a similar way as in the linear theory of electromagnetically induced transparency (EIT). We solve the nonlinear model when the controlling field and the solitons inte…
Level-crossing (LC) resonances in a buffer-gas-filled cesium vapor cell are studied under counterpropagating pump and probe light waves with opposite circular polarizations. The waves excite the D$_1$-line ground-state level $F_g$$=\,$$4$, while a transverse magnetic field (${\rm B}_x$$\perp$${\rm k}$) is scanned around zero to observe the resonance of electromagnetically induced absorption (EIA). It is shown that adding the pump light wave significantly improves the properties of the resonances in comparison with the commonly used scheme with a single light wave. As far as a small vapor cell …
We propose a ``channelization'' architecture to achieve wide-band electromagnetically induced transparency (EIT) and ultra-slow light propagation in atomic Rb-87 vapors. EIT and slow light are achieved by shining a strong, resonant ``pump'' laser on the atomic medium, which allows slow and unattenuated propagation of a weaker ``signal'' beam, but only when a two-photon resonance condition is satisfied. Our wideband architecture is accomplished by dispersing a wideband signal spatially, transverse to the propagation direction, prior to entering the atomic cell. When particular Zeeman sub-levels…
Metal atoms in solid and liquid helium-4 have attracted some interest either as a way to keep the atoms in a weakly perturbing matrix, or using them as a probe for the helium host medium. Laser sputtering with nanosecond pulsed lasers is the most often used method for atom production, resulting however in a substantial perturbation of the matrix. We show that a much weaker perturbation can be obtained by using femtosecond laser pulses with energy as low as 10 $μ$J. As an unexpected benefit, the atomic density produced is much higher.
Dicke narrowing is a phenomena that dramatically reduces the Doppler width of spectral lines, due to frequent velocity-changing collisions. A similar phenomena occurs for electromagnetically induced transparency (EIT) resonances, and facilitates ultra-narrow spectral features in room-temperature vapor. We directly measure the Dicke-like narrowing by studying EIT line-shapes as a function of the angle between the pump and the probe beams. The measurements are in good agreement with an analytic theory with no fit parameters. The results show that Dicke narrowing can increase substantially the to…
We experimentally and theoretically study two different tripod configurations using metastable helium ($^4$He*), with the probe field polarization perpendicular and parallel to the quantization axis, defined by an applied weak magnetic field. In the first case, the two dark resonances interact incoherently and merge together into a single EIT peak with increasing coupling power. In the second case, we observe destructive interference between the two dark resonances inducing an extra absorption peak at the line center.
We demonstrate ladder-type electromagnetically induced transparency (EIT) using an optical nanofiber suspended in a warm rubidium vapor. The signal and control fields are both guided along the nanofiber, which enables strong nonlinear interactions with the surrounding atoms at relatively low powers. Transit-time broadening is found to be a significant EIT decoherence mechanism in this tightly-confined waveguiding geometry. Nonetheless, we observe significant EIT and controlled polarization rotation using control-field powers of only a few microWatts in this relatively robust warm-atom nanofibe…
We observe a narrow, isolated, two-photon absorption resonance in Rb for large one-photon detuning in the presence of a buffer gas. In the absence of buffer gas, a standard Lambda configuration of two laser frequencies gives rise to electromagnetically induced transparency (EIT) for all values of one-photon detuning throughout the inhomogeneously (Doppler) broadened line. However, when a buffer gas is added and the one-photon detuning is comparable to or greater than the Doppler width, an absorption resonance appears instead of the usual EIT resonance. We also observe large negative group dela…
This tutorial introduces the theoretical and experimental basics of Electromagnetically Induced Transparency (EIT) in thermal alkali vapors. We first introduce a brief phenomenological description of EIT in simple three-level systems of stationary atoms and derive analytical expressions for optical transmission and dispersion under EIT conditions. Then we focus on how the thermal motion of atoms affects various parameters of the EIT system. Specifically, we analyze the Doppler broadening of optical transitions, ballistic versus diffusive atomic motion in a limited-volume interaction region, an…
With our all-atomic squeezing and filtering setup, we demonstrate control over the noise amplitudes and manipulation of the frequency-dependent squeezing angle of a squeezed vacuum quantum state by passing it through an atomic medium with electromagnetically induced transparency (EIT). We generate low sideband frequency squeezed vacuum using the polarization self-rotation effect in a hot Rb vapor cell, and input it into a second atomic vapor subject to EIT conditions. We use the frequency-dependent absorption of the EIT window to demonstrate an example of squeeze amplitude attenuation and sque…
We report here the first observation of electromagnetically induced transparency (EIT) in $^{20}$Ne. The power broadening of the EIT linewidth is measured as a function of neon pressure and RF excitation power. Doppler effects on the EIT broadening are found even at low pressures and low intensities, where the linewidth should be governed only by homogeneous effects.
We have detected and analyzed narrow, high contrast coherent population trapping resonances, which appear in transmission of the probe monochromatic light beam under action of the counterpropagating two-frequency laser radiation, on example of the nonclosed three level Λ-system formed by spectral components of the Doppler broadened D2 line of cesium atoms (in the cell with the rarefied Cs vapor). These nontrivial resonances are determined directly by the trapped atomic population on the definite lower level of the Λ-system and may be used in atomic frequency standards, sensitive magnetometers …
We present a spectral analysis of Rydberg atoms in strong microwave fields using electromagnetically induced transparency (EIT) as an all-optical readout. The measured spectroscopic response enables optical, atom-based electric field measurements of high-power microwaves. In our experiments, microwaves are irradiated into a room-temperature rubidium vapor cell. The microwaves are tuned near the two-photon 65D-66D Rydberg transition and reach an electric field strength of 230V/m, about 20% of the microwave ionization threshold of these atoms. A Floquet treatment is used to model the Rydberg lev…
We study electromagnetically induced transparency (EIT) in a heated potassium vapor cell, using a simple optical setup with a single free-running diode laser and an acousto-optic modulator. Despite the fact that the Doppler width is comparable to the ground state hyperfine splitting, transparency windows with deeply sub-natural line widths and large group indices are obtained. A longitudinal magnetic field is used to split the EIT feature and induce magnetooptical anisotropy. Using the beat note between co-propagating coupling and probe beams, we perform a heterodyne measurement of the circula…
A comprehensive study of three-photon electromagnetically-induced transparency (EIT) and absorption (EIA) on the rubidium cascade $5S_{1/2} \rightarrow 5P_{3/2}$ (laser wavelength 780~nm), $5P_{3/2} \rightarrow 5D_{5/2}$ (776~nm), and $5D_{5/2}\rightarrow 28F_{7/2}$ (1260~nm) is performed. The 780-nm probe and 776-nm dressing beams are counter-aligned through a Rb room-temperature vapor cell, and the 1260-nm coupler beam is co- or counter-aligned with the probe beam. Several cases of EIT and EIA, measured over a range of detunings of the 776-nm beam, are studied. The observed phenomena are mod…
